The classical limit of quantum mechanics is discussed for closed quantum systems in terms of observational aspects. Initially, the failure of the limit h->0 is explicitly demonstrated in a model of two quantum mechanically interacting oscillators by showing that neither quantum expectations reduce to Newtonian trajectories nor entanglement vanishes. This result suggests that the quantum-to-classical transition occurs only at an approximative level, which is regulated by the low accuracy of the measurements. In order to verify the consistence of these ideas we take into account the experimental resolution of physical measurements by introducing a discretized formulation for the quantum structure of wave functions. As a result, in the low-resolution limit the quasi-determinism is recovered and hence the quantum-to-classical transition is shown to occur adequately. Other puzzling problems, such as the classical limit of quantum superpositions and nonlocal correlations, are naturally address as well.
We propose a general argument to show that if a physical system can mediate locally the generation of entanglement between two quantum systems, then it itself must be non-classical. Remarkably, we do not assume any classical or quantum formalism to describe the mediating physical system: our result follows from general information-theoretic principles, drawn from the recently proposed constructor theory of information. This argument provides the indispensable theoretical basis for recently proposed tests of non-classicality in gravity, based on witnessing gravitationally-induced entanglement i…
Niels Bohr famously insisted on the indispensability of what he termed "classical concepts." In the context of the decoherence program, on the other hand, it has become fashionable to talk about the "dynamical emergence of classicality" from the quantum formalism alone. Does this mean that decoherence challenges Bohr's dictum -- for example, that classical concepts do not need to be assumed but can be derived? In this paper, we'll try to shed some light down the murky waters where formalism and philosophy mingle. To begin, we'll clarify the notion of classicality in the decoherence description…
The origin of non-classicality in physical systems and its connection to distinctly quantum features such as entanglement and coherence is a central question in quantum physics. This work analyses this question theoretically and experimentally, linking quantitatively non-classicality with quantum coherence. On the theoretical front, we show when the coherence of an observable is linearly related to the degree of violation of the Kolmogorov condition, which quantifies the deviation from any classical (non-invasive) explanation of the multi-time statistics. Experimentally, we probe this connecti…
We introduce a model for a two configurations system, and we study the transition from quantum to classical behaviour. We first consider the effect of the interaction with the environment as an external noise and we show that it produces decoherence and suppression of tunnelling. These features are widely accepted as definition of classicality, while we believe that classicality implies that quantum delocalized states spontaneously evolve into localized ones. We than show that this evolution take place only when both noise and non linearity in the equations are present.
We investigate signatures of non-classicality in quantum states, in particular, those involved in the DQC1 model of mixed-state quantum computation [Phys. Rev. Lett. 81, 5672 (1998)]. To do so, we consider two known non-classicality criteria. The first quantifies disturbance of a quantum state under locally noneffective unitary operations (LNU), which are local unitaries acting invariantly on a subsystem. The second quantifies measurement induced disturbance (MID) in the eigenbasis of the reduced density matrices. We study the role of both figures of non-classicality in the exponential speedup…
Modern quantum information theory provides new tools for investigating the decoherence-induced "classicality" of open quantum systems. Recent observation that almost all quantum states bear non-classical correlations [A. Ferraro {\it et al}, Phys. Rev. A {\bf 81}, 052318 (2010)] distinguishes the zero-discord classicality essentially as a pathology of the Markovian bipartite-systems realm. Nevertheless, we formally construct such a classical model and its variant that represents a matter-of-principle formal proof, i.e. a sufficient condition for the, otherwise not obvious, existence of the Mar…
Noisy quantum walks are studied from the perspective of comparing their quantumness as defined by two popular measures, measurement-induced disturbance (MID) and quantum discord (QD). While the former has an operational definition, unlike the latter, it also tends to overestimate non-classicality because of a lack of optimization over local measurements. Applied to quantum walks, we find that MID, while acting as a loose upper bound on QD, still tends to reflect correctly the trends in the behavior of the latter. However, there are regimes where its behavior is not indicative of non-classicali…
The experimental observation of a clear quantum signature of gravity is believed to be out of the grasp of current technology. However, several recent promising proposals to test the possible existence of non-classical features of gravity seem to be accessible by the state-of-art table-top experiments. Among them, some aim at measuring the gravitationally induced entanglement between two masses which would be a distinct non-classical signature of gravity. We explicitly study, in two of these proposals, the effects of decoherence on the system's dynamics by monitoring the corresponding degree o…
We study various measures of classicality of the states of open quantum systems subject to decoherence. Classical states are expected to be stable in spite of decoherence, and are thought to leave conspicuous imprints on the environment. Here these expected features of environment-induced superselection (einselection) are quantified using four different criteria: predictability sieve (which selects states that produce least entropy), purification time (which looks for states that are the easiest to find out from the imprint they leave on the environment), efficiency threshold (which finds stat…
The lack of superposition of different position states or the emergence of classicality in macroscopic systems have been a puzzle for decades. Classicality exists in every measuring apparatus, and is the key for understanding what can be measured in quantum theory. Different theories have been proposed, including decoherence, einselection and the spontaneous wave-function collapse, with no consensus reached up to now. In this paper, we propose a stochastic dynamics for the wave-function in an open system (e.g. the measuring apparatus) that interacts with its environment. The trajectory of wave…
The ongoing exploration of the ambiguous boundary between the quantum and the classical worlds has spurred substantial developments in quantum science and technology. Recently, the nonclassicality of dynamical processes has been proposed from a quantum-information-theoretic perspective, in terms of witnessing nonclassical correlations with Hamiltonian ensemble simulations. To acquire insights into the quantum-dynamical mechanism of the process nonclassicality, here we propose to investigate the nonclassicality of the electron spin free-induction-decay process associated with an NV$^-$ center. …
We provide a detailed discussion about the unitary and reduced evolution induced by family of Hamiltonian models describing a multilevel system, with a ground state and a possibly multilevel excited sector, coupled to a multimode boson field via a rotating-wave interaction. We prove explicitly that the system, in the limit in which the coupling is flat with respect to the boson frequencies, is Markovian under sharp measurements in arbitrary bases; we also find necessary and sufficient conditions under which the process is classical, i.e. its family of multitime joint probability distributions …
In this paper we will present the \QTR{it}{self-induced approach} to decoherence, which does not require the interaction between the system and the environment: decoherence in closed quantum systems is possible. This fact has relevant consequences in cosmology, where the aim is to explain the emergence of classicality in the universe conceived as a closed (non-interacting) quantum system. In particular, we will show that the self-induced approach may be used for describing the evolution of a closed quantum universe, whose classical behavior arises as a result of decoherence.
Advancing the debate on quantum effects in light-initiated reactions in biology requires clear identification of non-classical features that these processes can exhibit and utilise. Here we show that in prototype dimers present in a variety of photosynthetic antennae, efficient vibration-assisted energy transfer in the subpicosecond timescale and at room temperature can manifest and benefit from non-classical fluctuations of collective pigment motions. Non-classicality of initially thermalised vibrations is induced via coherent exciton-vibration interactions and is unambiguously indicated by n…
A recent debate has ensued over the claim by Pikovski et al. [Nat. Phys. 11, 668 (2015)] that systems with internal degrees of freedom undergo a universal, gravity-induced, type of decoherence that explains their quantum-to-classical transition. This decoherence is supposed to arise from the different gravitational redshifts experienced by such systems when placed in a superposition of two wave packets at different heights in a gravitational field. Here we investigate some aspects of the discussion with the aid of simple examples. In particular, we first resolve an apparent conflict between th…
Environmentally-induced superselection or "einselection" has been proposed as an observer-independent mechanism by which apparently classical systems "emerge" from physical interactions between degrees of freedom described completely quantum-mechanically. It is shown that einselection can only generate classical systems if the "environment" is assumed \textit{a priori} to be classical; einselection therefore does not provide an observer-independent mechanism by which classicality can emerge from quantum dynamics. Einselection is then reformulated in terms of positive operator-valued measures (…
The employment of path entangled multiphoton states enables measurement of phase with enhanced precision. It is common practice to demonstrate the unique properties of such quantum states by measuring super-resolving oscillations in the coincidence rate of a Mach-Zehnder interferometer. Similar oscillations, however, have also been demonstrated in various configurations using classical light only; making it unclear what, if any, are the classical limits of this phenomenon. Here we derive a classical bound for the visibility of super-resolving oscillations in a Mach-Zehnder. This provides an ea…
In a quantum measurement process, classical information about the measured system spreads throughout the environment. Meanwhile, quantum information about the system becomes inaccessible to local observers. Here we prove a result about quantum channels indicating that an aspect of this phenomenon is completely general. We show that for any evolution of the system and environment, for everywhere in the environment excluding an $O(1)$-sized region we call the "quantum Markov blanket," any locally accessible information about the system must be approximately classical, i.e. obtainable from some f…
According to the so-called Quantum Darwinist approach, the emergence of "classical islands" from a quantum background is assumed to obey a (selection) principle of maximal information. We illustrate this idea by considering the coupling of two oscillators (modes). As our approach suggests that the classical limit could have emerged throughout a long and progressive Evolution mechanism, it is likely that primitive living organisms behave in a "more quantum", "less classical" way than more evolved ones. This brings us to seriously consider the possibility to measure departures from classicality …
Quantum entanglement between two or more bipartite entities is a core concept in quantum information areas limited to microscopic regimes directly governed by Heisenberg uncertainty principle via quantum superposition, resulting in nondeterministic and probabilistic quantum features. Such quantum features cannot be generated by classical means. Here, a pure classical method of on-demand entangled light-pair generation is presented in a macroscopic regime via basis randomness. This conflicting idea of conventional quantum mechanics invokes a fundamental question about both classicality and quan…
We analyze the time dependence of entanglement and total correlations between a system and fractions of its environment in the course of decoherence. For the quantum Brownian motion model we show that the entanglement and total correlations have rather different dependence on the size of the environmental fraction. Redundancy manifests differently in both types of correlations and can be related with induced--classicality. To study this we introduce a new measure of redundancy and compare it with the existing one.
One interpretation of how the classical world emerges from an underlying quantum reality involves the build-up of certain robust entanglements between particles due to scattering events [Science Vol.301 p.1081]. This is an appealing view because it unifies two apparently disparate theories. It says that the uniquely quantum effect of entanglement is associated with classical behaviour. This is distinct from other interpretations that says classicality arises when quantum correlations are lost or neglected in measurements. To date the weakness of this interpretation has been the lack of a clear…
Recent work has demonstrated that quantum Fisher information (QFI), a witness of multipartite entanglement, and magnetic Van Hove correlations $G(r,t)$, a probe of local real-space real-time spin dynamics, can be successfully extracted from inelastic neutron scattering on spin systems through accurate measurements of the dynamical spin structure factor $S(k,ω)$. Here we apply theoretically these ideas to the half-filled Hubbard chain with nearest-neighbor hopping, away from the strong-coupling limit. This model has nontrivial redistribution of spectral weight in $S(k,ω)$ going from the non-int…
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phon…
Despite the impressive advances in biological imaging, no imaging modality today generates, in a comprehensive manner, high-resolution images of crowded molecules working deep inside the living cell in real time. In this paper, instead of tackling this engineering problem in the hope of solving it, we ask a converse question: What if such imaging is \emph{fundamentally} impossible? We argue that certain decoherence processes could be suppressed because the internal workings of the cell are not being closely "observed" in the quantum mechanical sense, as implied by the assumed impossibility of …
We study the process of observation (measurement), within the framework of a `perspectival' (`relational', `relative state') version of the modal interpretation of quantum mechanics. We show that if we assume certain features of discreteness and determinism in the operation of the measuring device (which could be a part of the observer's nerve system), this gives rise to classical characteristics of the observed properties, in the first place to spatial localization. We investigate to what extent semi-classical behavior of the object system itself (as opposed to the observational system) is ne…
In this paper we propose a chiral resolution technique based on laser-induced continuum structure (LICS). We show that the two enantiomers can have a different ionization profile based on implemented LICS excitation. We treat a cyclic excitation between two bound states and a continuum state and show how asymmetric ionization can be achieved based on different trapping of the enantiomers due to the additional coupling between the bound states. Alternatively, when multiple states are involved in the interaction we investigate a multilevel LICS strategy of asymmetric ionization based on dark-bri…
Decoherence is caused by the interaction with the environment. Environment monitors certain observables of the system, destroying interference between the pointer states corresponding to their eigenvalues. This leads to environment-induced superselection or einselection, a quantum process associated with selective loss of information. Einselected pointer states are stable. They can retain correlations with the rest of the Universe in spite of the environment. Einselection enforces classicality by imposing an effective ban on the vast majority of the Hilbert space, eliminating especially the fl…
We report on the all-optical detection of Rydberg states in a effusive atomic beam of strontium atoms using electromagnetically induced transparency (EIT). Using narrow-linewidth CW lasers we obtain an EIT linewidth of 5 MHz. To illustrate the high spectroscopic resolution offered by this method, we have measured isotope shifts of the 5s18d ^1D_2 and 5s19s ^1S_0 Rydberg states. This technique could be applied to high-resolution, non-destructive measurements of ultra-cold Rydberg gases and plasmas.
A conceptual difficulty in the foundations of quantum mechanics is the quantum measurement problem (QMP), essentially concerned with the apparent non-unitarity of the measurement process and the classicality of macroscopic systems. In an information theoretic approach proposed by us earlier (Quantum Information Processing 2, 153, 2003), which we clarify and elaborate here, QMP is understood to signal a fundamental finite resolution of quantum states, or, equivalently, a discreteness of Hilbert space. This was motivated by the notion that physical reality is a manifestation of information store…
Quantum imaging with undetected photons relies on the principle of induced coherence without induced emission and uses two sources of photon-pairs with a signal- and an idler photon. Each pair shares strong quantum correlations in both position and momentum, which allows to image an object illuminated with idler photons by just measuring signal photons that never interact with the object. In this work, we theoretically investigate the transverse resolution of this non-local imaging scheme through a general formalism that treats propagating photons beyond the commonly used paraxial approximatio…
In this article I aim to provide an intuitive and non-technical introduction to decoherence and quantum Darwinism. Together these theories explain how our classical reality emerges from an underlying quantum mechanical description. Here I focus on two aspects of this and explain, firstly, how decoherence can tell us why we never see macroscopic superpositions, such as dead-and-alive cats, in our classical surroundings; and secondly I describe and then provide a resolution to the so-called preferred basis problem. I then introduce recent results demonstrating that certain aspects of classicalit…
Weak squeezed vacuum light, especially resonant to the atomic transition, plays an important role in quantum storage and generation of various quantum sources. However, the general homodyne detection (HD) cannot determine weak squeezing due to the low signal to noise ratio and the limited resolution of the HD system. Here we provide an alternative method based on photon statistics measurement to determine the weak squeezing of the squeezed vacuum light generated from an optical parametric oscillator working far below the threshold. The approach is established the relationship between the squee…
The resilience of quantum entanglement to a classicality-inducing environment is tied to fundamental aspects of quantum many-body systems. The dynamics of entanglement has recently been studied in the context of measurement-induced entanglement transitions, where the steady-state entanglement collapses from a volume-law to an area-law at a critical measurement probability $p_{c}$. Interestingly, there is a distinction in the value of $p_{c}$ depending on how well the underlying unitary dynamics scramble quantum information. For strongly chaotic systems, $p_{c} > 0$, whereas for weakly chaotic …
To date no experiment has reached the level of sensitivity required to observe weak nuclear force induced parity violation (PV) energy differences in chiral molecules. In this paper, we present the approach, adopted at Laboratoire de Physique des Lasers (LPL), to measure frequency differences in the vibrational spectrum of enantiomers. We review different spectroscopic methods developed at LPL leading to the highest resolutions, as well as 20 years of CO2 laser stabilization work enabling such precise measurements. After a first attempt to observe PV vibrational frequency shifts using sub-Dopp…
Within the framework of the Lindblad master equation, we propose a general methodology to describe the effects of the environment on a system in dilute gas phase. The phenomenological parameters characterizing the transitions between rovibrational states of the system induced by collisions can be extracted from experimental transition kinetic constants, relying on Energy Gap fitting laws. As the availability of this kind of experimental data can be limited, the present work relied on experimental line broadening coefficients, however still using Energy Gap fitting laws. The 3 $μ$m infrared spe…
The current generation of quantum sensing technologies using color centers in diamond crystals is primarily based on the principle that the resonant microwave frequency of the luminescence between quantum levels of the nitrogen-vacancy (NV) center varies with temperature, electric and magnetic fields. This principle enables us to measure, for instance, magnetic and electric fields, as well as local temperature with nanometer resolution in conjunction with a scanning probe microscope (SPM). However, the time resolution of conventional quantum sensing technologies has been limited to microsecond…
For mesoscopic ensembles containing 100 or more atoms we measure the total atom number and the number of atoms in a specific hyperfine state with single-atom resolution. The measurement detects the atom-induced shift of the resonance frequency of an optical cavity containing the ensemble. This work extends the range of cavity-based detection with single-atom resolution by more than an order of magnitude in atom number, and provides the readout capability necessary for Heisenberg-limited interferometry with atomic ensembles.
