We show that quantum-interference-related phenomena, such as electromagnetically induced transparency, gain without inversion and enhanced refractive index may occur on electric-dipole forbidden transitions. Gain/dispersion characteristics of such transitions strongly depend upon the relative phase between the driving and probe fields. Unlike allowed transitions, gain/absorption behavior of forbidden transitions exhibit antisymmetric feature on the Rabi sidebands. Absorption/gain spectra possess extremely narrow sub-natural resonances.
We propose a technique to prepare coherent superpositions of two nondegenerate quantum states in a three-state ladder system, driven by two simultaneous fields near resonance with an intermediate state. The technique, of potential application to enhancement of nonlinear processes, uses adiabatic passage assisted by dynamic Stark shifts induced by a third laser field. The method offers significant advantages over alternative techniques: (ı) it does not require laser pulses of specific shape and duration and (\ii) it requires less intense fields than schemes based on two-photon excitation with n…
Quantum memories for quantum communication need to be able to store photons for an extended time and then to release them on demand. This can be achieved in atomic frequency comb ensemble based quantum memories by control pulses that transfer the excitation to and from long-lived spin states. However, such pulses can give rise to coherent and incoherent noise due to their interaction with the memory ensemble. In this article, we experimentally demonstrate the ability to switch off the coherent noise from such control pulses during the echo emission in a spin-wave quantum memory, using the line…
An exact analytic solution for two two-level atoms coupled with a multi-photon single-mode electromagnetic cavity field in the presence of the Stark shift is derived. We assume that the field is initially prepared in a coherent state and the two atoms are initially prepared in an excited state. Considering the atomic level shifts generated by the Stark shift effect, the dynamical behavior of both quantum coherence (QC) measured using a quantum Jensen-Shannon divergence and of quantum correlations captured by quantum discord (QD) are investigated. It is shown that the intensity-dependent Stark-…
This papers presents a formalism describing the dynamics of a quantum particle in a one-dimensional tilted time-dependent lattice. The description uses the Wannier-Stark states, which are localized in each site of the lattice and provides a simple framework leading to fully-analytical developments. Particular attention is devoted to the case of a time-dependent potential, which results in a rich variety of quantum coherent dynamics is found.
The resonance frequency of an InAs quantum dot strongly coupled to a GaAs photonic crystal cavity was electrically controlled via quantum confined Stark effect. Stark shifts up to 0.3meV were achieved using a lateral Schottky electrode that created a local depletion region at the location of the quantum dot. We report switching of a probe laser coherently coupled to the cavity up to speeds as high as 150MHz, limited by the RC constant of the transmission line. The coupling rate and the magnitude of the Stark shift with electric field were investigated while coherently probing the system.
A quantum memory protocol of controlled ac Stark echoes (CASE) based on a double rephasing photon echo scheme via controlled Rabi flopping is proposed. A double rephasing scheme of photon echoes inherently satisfies the no-population inversion requirement for quantum memories, but the resultant absorptive echo has been a fundamental problem. In the present studies, firstly, the first echo in the double rephasing scheme is dynamically controlled not to affect the second echo by using unbalanced ac Stark shifts. Secondly, a control Rabi pulse coherently manipulates the second echo to be emissive…
The old quantum theory and Schrödinger's wave mechanics (and other forms of quantum mechanics) give the same results for the line splittings in the first-order Stark effect in hydrogen, the leading terms in the splitting of the spectral lines emitted by a hydrogen atom in an external electric field. We examine the account of the effect in the old quantum theory, which was hailed as a major success of that theory, from the point of view of wave mechanics. First, we show how the new quantum mechanics solves a fundamental problem one runs into in the old quantum theory with the Stark effect. It t…
Stark-chirped rapid adiabatic passage (SCRAP) is an important technique used for coherent quantum controls. In this paper we investigate how the practically-existing dissipation of the system influences on the efficiency of the passage, and thus the fidelities of the SCRAP-based quantum gates. With flux-biased Josephson qubits as a specifical example, our results show clearly that the efficiency of the logic gates implemented by SCRAP are robust against the weak dissipation. The influence due to the non-adiabtic transitions between the adiabatic passages is comparatively significantly small. T…
Realization of Backward Retrieval in a Stark-modulated Spin-wave Quantum Memory
Southern University of Science and Technology（南方科技大学）；International Quantum Academy, and Shenzhen Branch, Hefei National Laboratory（国际量子学院合肥国家实验室深圳分院）；CAS Key Laboratory of Quantum Information, University of Science and Technology of China（中国科学院量子信息重点实验室中国科学技术大学）；Anhui Province Key Laboratory of Quantum Network, University of Science and Technology of China（安徽省量子网络重点实验室中国科学技术大学）；CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China（中国科学院量子信息与量子物理前沿卓越创新中心中国科学技术大学）；Hefei National Laboratory, University of Science and Technology of China（合肥国家实验室中国科学技术大学）
Entangled state, as an essential tool in quantum information processing, may be generated through the interaction between light and matter in cavity quantum electrodynamics. In this paper, we study the interaction between two two-level atoms and a two-mode field in an optical cavity enclosed by a medium with Kerr nonlinearity in the presence of detuning parameter and Stark effect. It is assumed that atom-field coupling and third-order susceptibility of the Kerr medium depend on the intensity of light. In order to investigate the dynamics of the introduced system, we obtain the exact analytical…
Quantum memories for light are essential components in quantum technologies like long-distance quantum communication and distributed quantum computing. Recent studies have shown that long optical and spin coherence lifetimes can be observed in rare earth doped nanoparticles, opening exciting possibilities over bulk materials e.g. for enhancing coupling to light and other quantum systems, and material design. Here, we report on coherent light storage in Eu$^{3+}$:Y$_2$O$_3$ nanoparticles using the Stark Echo Modulation Memory (SEMM) quantum protocol. We first measure a nearly constant Stark coe…
A three level ladder system is analyzed and the coherence of initially electric-dipole forbidden transition is calculated. Due to the presence of two laser fields the initially dipole forbidden transition becomes dynamically permitted due to ac Stark effect. It is shown that such transitions exhibit quantum-interference-related phenomena, such as electromagnetically induced transparency, gain without inversion and enhanced refractive index. Gain and dispersion characteristics of such transitions strongly depend upon the relative phase between the driving and the probe fields. Unlike allowed tr…
We report on the realization of dynamical control of transport for ultra-cold Sr88 atoms loaded in an accelerated and amplitude-modulated 1D optical lattice. We tailor the energy dispersion of traveling wave packets and reversibly switch between Wannier-Stark localization and driven transport based on coherent tunneling. Within a Loschmidt-echo scheme where the atomic group velocities are reversed at once, we demonstrate a novel mirror for matter waves working independently of the momentum state and discuss possible applications to force measurements at micrometric scales.
A strong, far-detuned laser can shift the energy levels of an optically active quantum system via the AC Stark effect. We demonstrate that the polarization of the laser results in a spin-selective modification to the energy structure of a charged quantum dot, shifting one spin manifold but not the other. An additional shift occurs due to the Overhauser field of the nuclear spins, which are pumped into a partially polarized state. This mechanism offers a potentially rapid, reversible, and coherent control of the energy structure and polarization selection rules of a charged quantum dot.
Quantum emitters in diamond are leading optically-accessible solid-state qubits. Among these, Group IV-vacancy defect centers have attracted great interest as coherent and stable optical interfaces to long-lived spin states. Theory indicates that their inversion symmetry provides first-order insensitivity to stray electric fields, a common limitation for optical coherence in any host material. Here we experimentally quantify this electric field dependence via an external electric field applied to individual tin-vacancy (SnV) centers in diamond. These measurements reveal that the permanent elec…
When an atom strongly couples to a cavity, it can undergo coherent vacuum Rabi oscillations. Controlling these oscillatory dynamics quickly relative to the vacuum Rabi frequency enables remarkable capabilities such as Fock state generation and deterministic synthesis of quantum states of light, as demonstrated using microwave frequency devices. At optical frequencies, however, dynamical control of single-atom vacuum Rabi oscillations remains challenging. Here, we demonstrate coherent transfer of optical frequency excitation between a single quantum dot and a cavity by controlling vacuum Rabi o…
We realize a coherent transfer between a laser-accessible low-angular-momentum Rydberg state and the circular Rydberg level with maximal angular momentum. This transfer is induced by a radiofrequency field with a high-purity $σ^+$ polarization tuned at resonance on Stark transitions inside the hydrogenic Rydberg manifold. We observe over a few microseconds more than twenty coherent Rabi oscillations between the initial Rydberg state and the circular Rydberg level. We characterize in details these complex oscillations involving many Rydberg levels and find them to be in perfect agreement with a…
Stark many-body localized (SMBL) systems have been shown both numerically and experimentally to have Bloch many-body oscillations, quantum many-body scars, and fragmentation in the large field tilt limit. Likewise, they are believed to show localization similar to disordered MBL. We explain and analytically prove all these observations by rigorously showing the existence of novel algebraic structures that are exponentially stable in time, which we call dynamical l-bits. Moreover, we show that many-body Bloch oscillations persist even at infinite temperature for exponentially long-times. We num…
A setup for discriminating between arbitrary two coherent states of a single light mode with the highest success rate allowed by quantum mechanics is presented. Its application to time-multiplexed quantum key distribution is discussed.
We present an experimental proposal to achieve a strong photon blockade by employing electromagnetically induced transparency (EIT) with single alkaline-earth-metal atom trapped in an optical cavity. In the presence of optical Stark shift, both second-order correlation function and cavity transmission exhibit asymmetric structures between the red and blue sidebands of the cavity. For a weak control field, the photon quantum statistics for the coherent transparency window (i.e. atomic quasi-dark state resonance) are insensitive to the Stark shift, which should also be immune to the spontaneous …
In this paper we study a two-photon time-dependent Jaynes-Cummings model interacting with a Kerr-like medium. We assumed that the electromagnetic field is in different states such as coherent, squeezed vacuum and pair coherent, and that the atom is initially in the excited state. We studied the temporal evolution of the population of the excited level, and the second order coherence function. The results obtained show that this system has some similarities with the two-mode Stark system. We analize two photon entanglement for different initial conditions.
This communication is an enquiry into the circumstances under which entropy and subentropy methods can give an answer to the question of quantum entanglement in the composite state. Using a general quantum dynamical system we obtain the analytical solution when the atom initially starts from its excited state and the field in different initial states. Different features of the entanglement are investigated when the field is initially assumed to be in a coherent state, an even coherent state (Schrodinger cate state) and a statistical mixture of coherent states. Our results show that the setting…
The explanation of the first-order Stark effect in hydrogen by Epstein and Schwarzschild in 1916 was seen as a great success for the old quantum theory. Yet, it also revealed some serious limitations of the theory. To recover the experimentally found line splittings, one had to make some arbitrary assumptions in addition to the basic quantum conditions to rule out certain orbits. The calculation of intensities of lines on the basis of Bohr's correspondence principle likewise required arbitrary additional assumptions. Finally, the actual orbits predicted by the old quantum theory depend on the …
Solid-state spin defects are a promising platform for quantum science and technology, having realized demonstrations of a variety of key components for quantum information processing, particularly in the area of quantum networks. An outstanding challenge for building larger-scale quantum systems with solid-state defects is realizing high-fidelity control over multiple defects with nanoscale separations, which is required to realize strong spin-spin interactions for multi-qubit logic and the creation of entangled states. In this work, we experimentally demonstrate an optical frequency-domain mu…
Recent studies using the quantum information theoretic approach to thermodynamics show that the presence of coherence in quantum systems generates corrections to classical fluctuation theorems. To explicate the physical origins and implications of such corrections, we here convert an abstract framework of an autonomous quantum Crooks relation into quantum Crooks equalities for well-known coherent, squeezed and cat states. We further provide a proposal for a concrete experimental scenario to test these equalities. Our scheme consists of the autonomous evolution of a trapped ion and uses a posit…
We study the crucial role played by the solid-state environment in determining the photon emission characteristics of a driven quantum dot. For resonant driving, we predict a phonon-enhancement of the coherently emitted radiation field with increasing driving strength, in stark contrast to the conventional expectation of a rapidly decreasing fraction of coherent emission with stronger driving. This surprising behaviour results from thermalisation of the dot with respect to the phonon bath, and leads to a nonstandard regime of resonance fluorescence in which significant coherent scattering and …
Utilization of the spatial degree of freedom vastly enhances informational capacity of light at the cost of stringent requirements on the processing devices. Multi-mode quantum memories constitute a viable candidate for quantum and classical information processing; however, full utilization of the assets of high-dimensionality requires a flexible processing technique. We employ a spatially varying ac-Stark effect to perform arbitrary 1D phase modulation of a coherent spin-wave state stored in a wavevector-multiplexed quantum memory. A far-field and an interferometric near-field characterizatio…
In order to beat any type of photon-number-splitting attack, we propose a protocol for quantum key distributoin (QKD) using 4 different intensities of pulses. They are vacuum and coherent states with mean photon number $μ,μ'$ and $μ_s$. $μ_s$ is around 0.55 and this class of pulses are used as the main signal states. The other two classes of coherent states ($μ,μ'$) are also used signal states but their counting rates should be studied jointly with the vacuum. We have shown that, given the typical set-up in practice, the key rate from the main signal pulses is quite close to the theoretically …
We theoretically study the conditions under which two laser fields can undergo Coherent Perfect Absorption (CPA) when shined on a single-mode bi-directional optical cavity coupled with two two- level quantum emitters (natural atoms, artificial atoms, quantum dots, qubits, etc.). In addition to being indirectly coupled through the cavity-mediated field, in our Tavis-Cummings model the two quantum emitters (QEs) are allowed to interact directly via the dipole-dipole interaction (DDI). Under the mean-field approximation and low-excitation assumption, in this work, we particularly focus on the imp…
A coherent control scheme for the population distribution in the vibrational states of nonpolar molecules is proposed. Our theoretical analysis and results of numerical simulations for the interaction of the hydrogen molecular ion in its electronic ground state with an infrared laser pulse reveal a selective two-photon transition between the vibrational states via a coupling with the first excited dissociative state. We demonstrate that for a given temporal intensity profile the population transfer between vibrational states, or a superposition of vibrational states, can be made complete for a…
We experimentally observe Floquet Raman transitions in the weakly driven solid state spin system of nitrogen-vacancy center in diamond. The periodically driven spin system simulates a two-band Wannier-Stark ladder model, and allows us to observe coherent spin state transfer arising from Raman transition mediated by Floquet synthetic levels. It also leads to the prediction of analog photon-assisted Floquet Raman transition and dynamical localisation in a driven two-level quantum system. The demonstrated rich Floquet dynamics offers new capabilities to achieve effective Floquet coherent control …
We propose an approach to coherently transfer populations between selected quantum states in one- and two-qubit systems by using controllable Stark-chirped rapid adiabatic passages (SCRAPs). These {\it evolution-time insensitive} transfers, assisted by easily implementable single-qubit phase-shift operations, could serve as elementary logic gates for quantum computing. Specifically, this proposal could be conveniently demonstrated with existing Josephson phase qubits. Our proposal can find an immediate application in the readout of these qubits. Indeed, the broken parity symmetries of the boun…
We present an open-system master equation study of the coherent and incoherent resonance fluorescence spectrum from a two-level quantum system under coherent pulsed excitation. Several pronounced features which differ from the fluorescence under a constant drive are highlighted, including a multi-peak structure and a pronounced off-resonant spectral asymmetry, in stark contrast to the conventional symmetrical Mollow triplet. We also study semiconductor quantum dot systems using a polaron master equation, and show how the key features of dynamic resonance fluorescence change with electron--acou…
A quantum cipher supported by a secret key so called keyed communication in quantum noise (KCQ) is very attractive in implementing high speed key generation and secure data transmission. However, Yuen-2000 as a basic model of KCQ has a difficulty to ensure the quantitative security evaluation because all physical parameter for the cipher system is finite. Recently, an outline of a generalized scheme so called coherent pulse position modulation(CPPM) to show the rigorous security analysis is given, where the parameters are allowed to be asymptotical. This may open a new way for the quantum key …
We present coherent reflection spectroscopy on a charge and DC Stark tunable quantum dot embedded in a high-quality and externally mode-matched microcavity. The addition of an exciton to a single-electron charged quantum dot forms a trion that interacts with the microcavity just below strong coupling regime of cavity quantum electrodynamics. Such an integrated, monolithic system is a crucial step towards the implementation of scalable hybrid quantum information schemes that are based on an efficient interaction between a single photon and a confined electron spin.
The control and manipulation of quantum-entangled non-local states is a crucial step for the development of quantum information processing. A promising route to achieve such states on a wide scale is to couple solid-state quantum emitters through their coherent dipole-dipole interactions. Entanglement in itself is challenging, as it requires both nanometric distances between emitters and nearly degenerate electronic transitions. Implementing hyperspectral imaging to identify pairs of coupled organic molecules trapped in a low temperature matrix, we reach distinctive spectral signatures of maxi…
We present experimental results in which the unexpected zero-two transition of a circuit composed of two inductively coupled transmons is observed. This transition shows an unusual magnetic flux dependence with a clear disappearance at zero magnetic flux. In a transmon qubit the symmetry of the wave functions prevents this transition to occur due to selection rule. In our circuit the Josephson effect introduces strong couplings between the two normal modes of the artificial atom. This leads to a coherent superposition of states from the two modes enabling such transitions to occur.
We measure the AC-Stark shifts of the 5S{1/2}, F=2 to 5P{3/2}, F'=3 transitions of individual optically trapped 87Rb atoms using a non-destructive detection technique that allows us to measure the fluorescent signal of one-and-the-same atom for over 60 seconds. These measurements allow efficient and rapid characterization of single atom traps that is required for many coherent quantum information protocols. Although this method is demonstrated using a single atom trap, the concept is readily extended to resolvable atomic arrays.
Chip-based cavity quantum electrodynamics (QED) devices consisting of a self-assembled InAs quantum dot (QD) coupled to a high quality factor GaAs microdisk cavity are coherently probed through their optical channel using a fiber taper waveguide. We highlight one particularly important aspect of this all-fiber measurement setup, which is the accuracy to which the optical coupling level and optical losses are known relative to typical free-space excitation techniques. This allows for precise knowledge of the intracavity photon number and measurement of absolute transmitted and reflected signals…
We present a joint experimental and theoretical study on strong-field photo-ionization of sodium atoms using chirped femtosecond laser pulses. By tuning the chirp parameter, selectivity among the population in the highly excited states 5p, 6p, 7p and 5f, 6f is achieved. Different excitation pathways enabling control are identified by simultaneous ionization and measurement of photoelectron angular distributions employing the velocity map imaging technique. Free electron wave packets at an energy of around 1 eV are observed. These photoelectrons originate from two channels. The predominant 2+1+…
We report on the observation of magnetic dipole allowed transitions in the well-characterized $A\,^2Σ^+ - X\,^2Π$ band system of the OH radical. A Stark decelerator in combination with microwave Rabi spectroscopy is used to control the populations in selected hyperfine levels of both $Λ$-doublet components of the $X\,^2Π_{3/2},v=0,J=3/2$ ground state. Theoretical calculations presented in this paper predict that the magnetic dipole transitions in the $ν'=1 \leftarrow ν=0$ band are weaker than the electric dipole transitions by a factor of $2.58\times 10^3$ only, i.e., much less than commonly b…
The quantum capacity of a memoryless channel is often used as a single figure of merit to characterize its ability to transmit quantum information coherently. The capacity determines the maximal rate at which we can code reliably over asymptotically many uses of the channel. We argue that this asymptotic treatment is insufficient to the point of being irrelevant in the quantum setting where decoherence severely limits our ability to manipulate large quantum systems in the encoder and decoder. For all practical purposes we should instead focus on the trade-off between three parameters: the rate…
