We show experimentally that parametric interaction can induce a cooperative oscillation of non simultaneously resonant transverse modes in an optical parametric oscillator. More generally, this effect is expected to occur in any spatially extended system subjected to boundary conditions where nonlinear wave mixing of two nonresonant spatial modes can generate a resonant oscillation.
Dynamical radiation pressure effects in cavity optomechanical systems give rise to self-sustained oscillations or `phonon lasing' behavior, producing stable oscillators up to GHz frequencies in nanoscale devices. Like in photonic lasers, phonon lasing normally occurs in a single mechanical mode. We show here that phase-locked, multimode phonon lasing can be established in a multimode optomechanical system through Floquet dynamics induced by a temporally modulated laser drive. We demonstrate this concept in a suitably engineered silicon photonic nanocavity coupled to multiple GHz-frequency mech…
We present a spatiotemporally mode-locked Mamyshev oscillator. A wide variety of multimode mode-locked states, with varying degrees of spatiotemporal coupling, are observed. We find that some control of the modal content of the output beam is possible through the cavity design. Comparison of simulations to experiments indicates that spatiotemporal mode-locking is enabled by nonlinear intermodal interactions and spatial filtering, along with the Mamyshev mechanism. This work represents a first exploration of spatiotemporal mode-locking in an oscillator with the Mamyshev saturable absorber.
We demonstrate the first multimode fiber interference-based filtering in an all-fiber spatiotemporally mode-locked laser. The oscillator generates dissipative soliton pulses at 1036 nm with 12 mW average power, 6.24 ps duration and 24.3 MHz repetition rate. The reported pulse energy (0.5 nJ) represents ~4 times improvement over the previously reported single-mode all-normal dispersion mode-locked lasers with multimode interference-based filtering. Numerical simulations are performed to reveal cavity and spatiotemporal mode-locking dynamics. The proposed oscillator presents an alternative appro…
The performance of fiber mode-locked lasers is limited due to the high nonlinearity induced by the spatial confinement of the single-mode fiber core. To massively increase the pulse energy of the femtosecond pulses, amplification is obtained outside the oscillator. Recently, spatiotemporal mode-locking has been proposed as a new path to fiber lasers. However, the beam quality was either highly multimode and/or with low pulse energy. Here we present an approach to reach high energy per pulse directly in the mode-locked multimode fiber oscillator with a near single-mode output beam. Our approach…
Photo-induced forces can be used to manipulate and cool the mechanical motion of oscillators. When the oscillator is used as a force sensor, such as in atomic force microscopy, active feedback is an enticing route to enhancing measurement performance. Here, we show broadband multimode cooling of $-23$ dB down to a temperature of $8 \pm 1$~K in the stationary regime. Through the use of periodic quiescence feedback cooling, we show improved signal-to-noise ratios for the measurement of transient signals. We compare the performance of real feedback to numerical post-processing of data and show th…
The quantum features of ultrashort-pulse optical parametric oscillators (OPOs) are investigated theoretically in the nonlinear regime near and above threshold. Viewing the pulsed OPO as a multimode open quantum system, we rigorously derive a general input-output model that features nonlinear coupling among many cavity (i.e., system) signal modes and a broadband single-pass (i.e., reservoir) pump field. Under appropriate assumptions, our model produces a Lindblad master equation with multimode nonlinear Lindblad operators describing two-photon dissipation and a multimode four-wave-mixing Hamilt…
We develop a universal approach enabling the study of any multimode quantum optical system evolving under a quadratic Hamiltonian. Our strategy generalizes the standard symplectic analysis and permits the treatment of multimode systems even in situations where traditional theoretical methods cannot be applied. This enables the description and investigation of a broad variety of key-resources for experimental quantum optics, ranging from optical parametric oscillators, to silicon-based micro-ring resonator, as well as opto-mechanical systems.
We study theoretically the dynamics of multiple mechanical oscillators coupled to a single cavity field mode via linear or quadratic optomechanical interactions. We focus specifically on the strong coupling regime where the cavity decays much faster than the mechanical modes, and the optomechanical coupling is comparable to or larger than the mechanical frequency, so that both the optical and mechanical systems operate in the deep quantum regime. Using the examples of one and two mechanical oscillators we show that the system can classically exhibit bistability and bifurcations, and we explore…
We study a multimode optomechanical system where two mechanical oscillators are coupled to an electromagnetic cavity. Previously it has been shown that if the mechanical resonances have nearly equal frequencies, one can make the oscillators to interact via the cavity by strong pumping with a coherent pump tone. One can view the interaction also as emergence of an electromagnetically dark mode which gets asymptotically decoupled from the cavity and has a linewidth much smaller than that of the bare cavity. The narrow linewidth and long lifetime of the dark mode could be advantageous for example…
Cavity optomechanics offers powerful methods for controlling optical fields and mechanical motion. A number of proposals have predicted that this control can be extended considerably in devices where multiple cavity modes couple to each other via the motion of a single mechanical oscillator. Here we study the dynamical properties of such a multimode optomechanical device, in which the coupling between cavity modes results from mechanically-induced avoided crossings in the cavity's spectrum. Near the avoided crossings we find that the optical spring shows distinct features that arise from the i…
We demonstrate optomechanical interference in a multimode system, in which an optical mode couples to two mechanical modes. A phase-dependent excitation-coupling approach is developed, which enables the observation of constructive and destructive optomechanical interferences. The destructive interference prevents the coupling of the mechanical system to the optical mode, suppressing optically-induced mechanical damping. These studies establish optomechanical interference as an essential tool for controlling the interactions between light and mechanical oscillators.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables, for example in cluster state computation. They can be generated either by mixing different squeezed light sources using linear optical operations, or directly in a multimode optical device. In parallel, frequency combs are perfect tools for high precision metrological applications and for quantum time transfer. Synchronously Pumped Optical Parametric Oscillators (SPOPOs) have been theoretically shown to produce multimode non-classical frequency combs. In this paper, we present the…
In this letter, we demonstrate the first all-fiber all-normal dispersion ytterbium-doped oscillator with nonlinear multimodal interference based saturable absorber capable to generate ultrashort dissipative soliton pulses. Additional to functioning as a saturable absorber, the use of multimode fiber segments between single mode fibers also ensures the bandpass filtering via multimode interference reimaging necessary to obtain dissipative soliton mode-locking. The oscillator generates dissipative soliton pulses at 1030 nm with 5.8 mW average power, 5 ps duration and 44.25 MHz repetition rate. P…
Reconfigurable Resonant Multimode Nonlinear Coupling for UV-to-infrared Frequency Generation
École Polytechnique Fédérale de Lausanne（洛桑联邦理工学院）；Università di Pavia（帕维亚大学）；International Quantum Academy and Shenzhen Futian SUSTech Institute for Quantum Technology and Engineering（国际量子学院及深圳福田南方科技大学量子技术与工程研究院）；Hefei National Laboratory, University of Science and Technology of China（合肥国家实验室，中国科学技术大学）
Mode locking in lasers is a collective effect, where due to a weak coupling a large number of frequency modes lock their phases to oscillate in unison, forming an ultrashort pulse in time. We demonstrate an analogous collective effect in coupled parametric oscillators, which we term "pairwise mode-locking", where many pairs of modes with twin frequencies (symmetric around the center carrier) oscillate simultaneously with a locked phase-sum, while the phases of individual modes remain undefined. Thus, despite being broadband and multimode, the emission is not pulsed and lacks first-order cohere…
Exciton-Tunable Phase Control and Superstrong Coupling Through Multimode Polariton Engineering in Planar Waveguides
CNR Nanotec, Institute of Nanotechnology（国家研究委员会纳米技术研究所）；School of Physics and Astronomy, University of Southampton（南安普顿大学物理与天文学学院）；Istituto di Fotonica e Nanotecnologie—Consiglio Nazionale delle Ricerche (CNR)（国家研究委员会光子学与纳米技术研究所）
In this Letter, we demonstrate, to the best of our knowledge, the first spatiotemporally mode-locked fiber laser with self-similar pulse evolution. The multimode fiber oscillator generates parabolic amplifier similaritons at 1030 nm with 90 mW average power, 2.3 ps duration, and 37.9 MHz repetition rate. Remarkably, we observe experimentally a near-Gaussian beam quality (M^2<1.4) at the output of the highly multimode fiber. The output pulses are compressed to 192 fs via an external grating compressor. Numerical simulations are performed to investigate the cavity dynamics which confirm experime…
Quantum computation and communication protocols require quantum resources which are in the continuous variable regime squeezed and/or quadrature entangled optical modes. To perform more and more complex and robust protocols, one needs sources that can produce in a controlled way highly multimode quantum states of light. One possibility is to mix different single mode quantum resources. Another is to directly use a multimode device, either in the spatial or in the frequency domain. We present here the first experimental demonstration of a device capable of producing simultanuously several squee…
The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this study, we design a voltage-tunable open microcavity and we show the formation of multiple vibrational polaritons in methyl salicylate. A Rabi splitting and polariton anticrossing behaviour is observed when the cavity mode hybridizes with the C=O stretching vibration of methyl salicylate. As this vibration contributes to the reaction coordinate of the photoind…
The coupling of distinct systems underlies nearly all physical phenomena and their applications. A basic instance is that of interacting harmonic oscillators, which gives rise to, for example, the phonon eigenmodes in a crystal lattice. Particularly important are the interactions in hybrid quantum systems consisting of different kinds of degrees of freedom. These assemblies can combine the benefits of each in future quantum technologies. Here, we investigate a hybrid optomechanical system having three degrees of freedom, consisting of a microwave cavity and two micromechanical beams with close…
The generation of continuous-variable multipartite entangled states is important for several protocols of quantum information processing and communication, such as one-way quantum computation or controlled dense coding. In this article we theoretically show that multimode optical parametric oscillators can produce a great variety of such states by an appropriate control of the parametric interaction, what we accomplish by tailoring either the spatio-temporal shape of the pump, or the geometry of the nonlinear medium. Specific examples involving currently available optical parametric oscillator…
Experimental investigation of the effect of dispersion on squeezing generation in a synchronously pumped optical parametric oscillator
Università degli Studi di Milano（米兰大学）；Istituto Nazionale di Fisica Nucleare, Sezione di Milano（意大利国家核物理研究所米兰分部）；Istituto di Fotonica e Nanotecnologie – CNR（光子与纳米技术研究所-国家研究委员会）
The advent of dispersion-engineered and highly nonlinear nanophotonics is expected to open up an all-optical path towards the strong-interaction regime of quantum optics by combining high transverse field confinement with ultra-short-pulse operation. Obtaining a full understanding of photon dynamics in such broadband devices, however, poses major challenges in the modeling and simulation of multimode non-Gaussian quantum physics, highlighting the need for sophisticated reduced models that facilitate efficient numerical study while providing useful physical insight. In this manuscript, we revie…
Exceptional-Point-Induced Nonequilibrium Entanglement Dynamics in Bosonic Networks
Peking University（北京大学）；Hefei National Laboratory（合肥国家实验室）；ETH Zürich（苏黎世联邦理工学院）；Beihang University（北京航空航天大学）；Shanxi University（山西大学）；Peking University Yangtze Delta Institute of Optoelectronics（北京大学长三角光电科学研究院）
We experimentally demonstrate the realization of a half-polarization-maintaining (half-PM) fiber laser, in which mode-locking is provided by a reflective multimode-interference saturable absorber (SA). In the specially designed SA, linearly polarized light is coupled into a 15-cm-long graded-index multimode fiber (GIMF) through the PM fiber, and then reflected back to the PM structure through a mirror pigtailed with a single-mode fiber (SMF). The modulation depth and saturation peak power are measured to be 1.5% and 0.6 W, respectively. The proposed SA device is incorporated into a novel half-…
Hybrid quantum systems have been developed with various mechanical, optical and microwave harmonic oscillators. The coupling produces a rich library of interactions including two mode squeezing, swapping interactions, back-action evasion and thermal control. In a multimode mechanical system, coupling resonators of different scales (both in frequency and mass) leverages the advantages of each resonance. For example: a high frequency, easily manipulated resonator could be entangled with a low frequency massive object for tests of gravitational decoherence. Here we demonstrate coherent optomechan…
Two-dimensional semiconductors host excitons with very large oscillator strengths and binding energies due to significantly reduced carrier screening. Two-dimensional semiconductors integrated with optical cavities are emerging as a promising platform for studying strong light-matter interactions as a route to explore a variety of exotic many-body effects. Here, in few-layered WS2 coupled with plasmonic nanoparticle lattices, we observe the formation of a collective polaritonic mode near the exciton energy and the formation of a complete polariton band gap with energy scale comparable to the e…
