One-way quantum computing is an important and novel approach to quantum computation. By exploiting the existing particle-particle interactions, we report the first experimental realization of the complete process of deterministic one-way quantum Deutsch-Josza algorithm in NMR, including graph state preparation, single-qubit measurements and feed-forward corrections. The findings in our experiment may shed light on the future scalable one-way quantum computation.
We experimentally test quantum contextuality of a single qutrit using NMR. The contextuality inequalities based on nine observables developed by Kurzynski et. al. are first reformulated in terms of traceless observables which can be measured in an NMR experiment. These inequalities reveal the contextuality of almost all single-qutrit states. We demonstrate the violation of the inequality on four different initial states of a spin-1 deuterium nucleus oriented in a liquid crystal matrix, and follow the violation as the states evolve in time. We also describe and experimentally perform a single-s…
The existence of contextuality in quantum mechanics is a fundamental departure from the classical description of the world. Currently, the quest to identify scenarios which cannot be more contextual than quantum theory is at the forefront of research in quantum contextuality. In this work, we experimentally test two inequalities, which are capable of revealing fully contextual quantum correlations, on a Hilbert space of dimension 8 and 4 respectively, on an NMR quantum information processor. The projectors associated with the contextuality inequalities are first reformulated in terms of Pauli …
The Greenberger-Horne-Zeilinger (GHZ) effect provides an example of quantum correlations that cannot be explained by classical local hidden variables. This paper reports on the experimental realization of GHZ correlations using nuclear magnetic resonance (NMR). The NMR experiment differs from the originally proposed GHZ experiment in several ways: it is performed on mixed states rather than pure states; and instead of being widely separated, the spins on which it is performed are all located in the same molecule. As a result, the NMR version of the GHZ experiment cannot entirely rule out class…
The method of quantum cloning is divided into two main categories: approximate and probabilistic quantum cloning. The former method is used to approximate an unknown quantum state deterministically, and the latter can be used to faithfully copy the state probabilistically. So far, many approximate cloning machines have been experimentally demonstrated, but probabilistic cloning remains an experimental challenge, as it requires more complicated networks and a higher level of precision control. In this work, we designed an efficient quantum network with a limited amount of resources, and perform…
We present the first NMR implementation of a scheme for selective and efficient quantum process tomography without ancilla. We generalize this scheme such that it can be implemented efficiently using only a set of measurements involving product operators. The method allows us to estimate any element of the quantum process matrix to a desired precision, provided a set of quantum states can be prepared efficiently. Our modified technique requires fewer experimental resources as compared to the standard implementation of selective and efficient quantum process tomography, as it exploits the speci…
This paper surveys our recent research on quantum information processing by nuclear magnetic resonance (NMR) spectroscopy. We begin with a geometric introduction to the NMR of an ensemble of indistinguishable spins, and then show how this geometric interpretation is contained within an algebra of multispin product operators. This algebra is used throughout the rest of the paper to demonstrate that it provides a facile framework within which to study quantum information processing more generally. The implementation of quantum algorithms by NMR depends upon the availability of special kinds of m…
We describe Nuclear Magnetic Resonance (NMR) demonstrations of the quantum Zeno effect, and discuss briefly how these are related to similar phenomena in more conventional NMR experiments.
We report an ensemble nuclear magnetic resonance (NMR) implementation of a quantum lattice gas algorithm for the diffusion equation. The algorithm employs an array of quantum information processors sharing classical information, a novel architecture referred to as a type-II quantum computer. This concrete implementation provides a test example from which to probe the strengths and limitations of this new computation paradigm. The NMR experiment consists of encoding a mass density onto an array of 16 two-qubit quantum information processors and then following the computation through 7 time step…
We present a generalized quantum scattering circuit which can be used to perform non-invasive quantum measurements, and implement it on NMR qubits. Such a measurement is a key requirement for testing temporal non-contextual inequalities. We use this circuit to experimentally demonstrate the violation of the Peres-Mermin inequality (which is the temporal analog of a Klyachko-Can- Binicioglu-Shumovsky (KCBS) inequality), on a three-qubit NMR quantum information processor. Further, we experimentally demonstrate the violation of a transformed Bell-type inequality (the spatial equivalent of the tem…
Quantum simulation can beat current classical computers with minimally a few tens of qubits and will likely become the first practical use of a quantum computer. One promising application of quantum simulation is to attack challenging quantum chemistry problems. Here we report an experimental demonstration that a small nuclear-magnetic-resonance (NMR) quantum computer is already able to simulate the dynamics of a prototype chemical reaction. The experimental results agree well with classical simulations. We conclude that the quantum simulation of chemical reaction dynamics not computable on cu…
Quantum computing exploits fundamentally new models of computation based on quantum mechanical properties instead of classical physics, and it is believed that quantum computers are able to dramatically improve computational power for particular tasks. At present, nuclear magnetic resonance (NMR) has been one of the most successful platforms amongst all current implementations. It has demonstrated universal controls on the largest number of qubits, and many advanced techniques developed in NMR have been adopted to other quantum systems successfully. In this review, we show how NMR quantum proc…
We experimentally demonstrate in NMR a quantum interferometric multi-meter for extracting certain properties of unknown quantum states without resource to quantum tomography. It can perform direct state determinations, eigenvalue/eigenvector estimations, purity tests of a quantum system, as well as the overlap of any two unknown quantum states. Using the same device, we also demonstrate one-qubit quantum fingerprinting.
Knill, Laflamme, and Milburn recently showed that non-deterministic quantum logic operations could be performed using linear optical elements, additional photons (ancilla), and post-selection based on the output of single-photon detectors [Nature 409, 46 (2001)]. Here we report the experimental demonstration of two logic devices of this kind, a destructive controlled-NOT (CNOT) gate and a quantum parity check. These two devices can be combined with a pair of entangled photons to implement a conventional (non-destructive) CNOT that succeeds with a probability of 1/4.
We experimentally demonstrate a new dynamic fashion of quantum Zeno effect in nuclear magnetic resonance systems. The frequent measurements are implemented through quantum entanglement between the target qubit(s) and the measuring qubit, which dynamically results from the unitary evolution of duration $τ_{m}$ due to dispersive-coupling. Experimental results testify the presence of "the critical measurement time effect", that is, the quantum Zeno effect does not occur when $τ_{m}$ takes the some critical values, even if the measurements are frequent enough. Moreover, we provide a first experime…
Linear optics is a promising candidate to enable the construction of quantum computers. A number of quantum protocols gates based on linear optics have been demonstrated. However, it is well-known that these gates are non-deterministic and that higher order nonlinearity is necessary for deterministic operations. We found the quantum leader election protocol (QLE) can be operated deterministically only with linear optics, and we have demonstrated the nearly deterministic operation which overcomes classical limit.
Anyons have exotic statistical properties, fractional statistics, differing from Bosons and Fermions. They can be created as excitations of some Hamiltonian models. Here we present an experimental demonstration of anyonic fractional statistics by simulating a version of the Kitaev spin lattice model proposed by Han et al[Phys. Rev.Lett. 98, 150404 (2007)] using an NMR quantum information processor. We use a 7-qubit system to prepare a 6-qubit pseudopure state to implement the ground state preparation and realize anyonic manipulations, including creation, braiding and anyon fusion. A $π/2\times…
The quantum Fourier transform (QFT) has been implemented on a three bit nuclear magnetic resonance (NMR) quantum computer, providing a first step towards the realization of Shor's factoring and other quantum algorithms. Implementation of the QFT is presented with fidelity measures, and state tomography. Experimentally realizing the QFT is a clear demonstration of NMR's ability to control quantum systems.
By employing at recent proposal (R. Filip, P. Marek and U.L. Andersen, Phys. Rev. A {\bf 71}, 042308 (2005) \cite{Filip05.pra}), we experimentally demonstrate a universal, deterministic and high-fidelity squeezing transformation of an optical field. It relies only on linear optics, homodyne detection, feedforward and an ancillary squeezed vacuum state, thus direct interaction between a strong pump and the quantum state is circumvented. We demonstrate three different squeezing levels for a coherent state input. This scheme is highly suitable for the fault-tolerant squeezing transformation in a …
We experimentally emulate interaction induced blockade and local spin freezing in two and three qubit Nuclear Magnetic Resonance (NMR) architecture. These phenomena are identical to the Rydberg blockade and Rydberg biased freezing. In Rydberg blockade, the simultaneous excitation of two or more atoms is blocked due to the level shift induced by the strong Van der Waal's interaction. In such a strong interaction regime, one can also observe Rydberg biased freezing, wherein the dynamics is confined to a subspace, with the help of multiple drives with unequal amplitudes. Here we drive NMR qubits …
We report the first experimental demonstration of quantum delayed-choice experiment via nuclear magnetic resonance techniques. An ensemble of molecules each with two spin-1/2 nuclei are used as target and the ancilla qubits to perform the quantum circuit corresponding the delayed-choice setup. As expected in theory, our experiments clearly demonstrate the continuous morphing of the target qubit between particle-like and wave-like behaviors. The experimental visibility of the interference patterns shows good agreement with the theory.
Algorithmic Cooling is a method that uses novel data compression techniques and simplecquantum computing devices to improve NMR spectroscopy, and to offer scalable NMR quantum computers. The algorithm recursively employs two steps. A reversible entropy compression of the computation quantum-bits (qubits) of the system and an irreversible heat transfer from the system to the environment through a set of reset qubits that reach thermal relaxation rapidly. Is it possible to experimentally demonstrate algorithmic cooling using existing technology? To allow experimental algorithmic cooling, the the…
We describe a nuclear magnetic resonance (NMR) experiment which implements an efficient one-to-two qubit phase-covariant cloning machine(QPCCM). In the experiment we have achieved remarkably high fidelities of cloning, 0.848 and 0.844 respectively for the original and the blank qubit. This experimental value is close to the optimal theoretical value of 0.854. We have also demonstrated how to use our phase-covariant cloning machine for quantum simulations of bit by bit eavesdropping in the four-state quantum key distribution protocol.
We present experimental results on the measurement of fidelity decay under contrasting system dynamics using a nuclear magnetic resonance quantum information processor. The measurements were performed by implementing a scalable circuit in the model of deterministic quantum computation with only one quantum bit. The results show measurable differences between regular and complex behaviour and for complex dynamics are faithful to the expected theoretical decay rate. Moreover, we illustrate how the experimental method can be seen as an efficient way for either extracting coarse-grained informatio…
Dynamic nuclear polarization (DNP) is used in nuclear magnetic resonance (NMR) to transfer polarization from electron spins to nuclear spins. The resulting nuclear polarization enhancement can, in theory, be two or three orders of magnitude depending on the sample. In solid state systems, however, there are competing mechanisms of DNP, which, when occurring simultaneously, reduce the net polarization enhancement of the nuclear spin. We present a simple quantum description of DNP and apply optimal control theory (OCT) with an open quantum system framework to design pulses that select one DNP pr…
While a bit is the fundamental unit of binary classical information, a qubit is the fundamental unit of quantum information. In quantum information processing (QIP), it is customary to call the qubits under study as system qubits, and the additional qubits as ancillary qubits. In this thesis, I describe various schemes to exploit the ancillary qubits to efficiently perform many QIP tasks and their experimental demonstrations in nuclear magnetic resonance (NMR) systems. Particularly, we have showed that, in the presence of sufficient ancillary qubits, it is possible to completely characterize a…
Recently developed quantum algorithms suggest that in principle, quantum computers can solve problems such as simulation of physical systems more efficiently than classical computers. Much remains to be done to implement these conceptual ideas into actual quantum computers. As a small-scale demonstration of their capability, we simulate a simple many-fermion problem, the Fano-Anderson model, using liquid state Nuclear Magnetic Resonance (NMR). We carefully designed our experiment so that the resource requirement would scale up polynomially with the size of the quantum system to be simulated. T…
Quantum no-Hiding theorem, first proposed by Braunstein and Pati [Phys. Rev. Lett. 98, 080502 (2007)], was verified experimentally by Samal et al. [Phys. Rev. Lett. 186, 080401 (2011)] using NMR quantum processor. Till then, this fundamental test has not been explored in any of the experimental architecture. Here, we demonstrate the above no-hiding theorem using the IBM 5Q quantum processor. Categorical algebra developed by Coecke and Duncan [New J. Phys. 13, 043016 (2011)] has been used for better visualization of the no-hiding theorem by analyzing the quantum circuit using the ZX calculus. T…
Quantum algorithms are known for presenting more efficient solutions to certain computational tasks than any corresponding classical algorithm. It has been thought that the origin of the power of quantum computation has its roots in non-classical correlations such as entanglement or quantum discord. However, it has been recently shown that even a single pure qudit is sufficient to design an oracle-based algorithm which solves a black-box problem faster than any classical approach to the same problem. In particular, the algorithm that we consider determines whether eight permutation functions d…
We experimentally demonstrate quantum machine learning using NMR based on a framework of quantum reservoir computing. Reservoir computing is for exploiting natural nonlinear dynamics with large degrees of freedom, which is called a reservoir, for a machine learning purpose. Here we propose a concrete physical implementation of a quantum reservoir using controllable dynamics of a nuclear spin ensemble in a molecular solid. In this implementation, we demonstrate learning of nonlinear functions with binary or continuous variable inputs with low mean squared errors. Our implementation and demonstr…
A protocol for non-destructive descrimination of arbitrary set of orthogonal quantum states was proposed by V. S. Manu et al., using an algorithm based on quantum phase estimation. IBM Corporation has released a superconductivity based 5-qubit (5-qubit transmon bowtie chip 3 and IBM 5-qubit real processor) quantum computer named Quantum Experience and placed it on cloud. In this paper we take advantage of the online availability of those real quantum processors(ibmqx2 amd ibmqx4) and carry out the above protocol that has experimentally demonstrated earlier using NMR quantum processor. Here, we…
The non-local nature of the correlations possessed by quantum systems may be revealed by experimental demonstrations of the violation of Bell-type inequalities. Recent work has placed bounds on the correlations that quantum systems can possess in an actual experiment. These bounds were limited to a composite quantum system comprising of a few lower-dimensional subsystems. In a more general approach, it has been shown that fewer body correlations can reveal the non-local nature of the correlations arising from a quantum mechanical description of nature. Such tests on the correlations can be tra…
We present experimental NMR demonstration of a scheme of reversible projective measurement, which allows extracting information on outcomes and probabilities of a projective measurement in a non-destructive way, with a minimal net effect on the quantum state of an ensemble. The scheme uses reversible dynamics and weak measurement of the intermediate state. The experimental system is an ensemble of 133Cs (S = 7/2) nuclei in a liquid-crystalline matrix.
Franson-type nonlocal quantum correlation based on the particle nature of quantum mechanics has been intensively studied for both fundamental physics and potential applications of quantum key distribution between remotely separated parties over the last several decades. Recently, a coherence theory of deterministic quantum features has been applied for Franson-type nonlocal correlation [arXiv:2102.06463] to understand its quantumness in a purely classical manner, where the resulting features are deterministic and macroscopic. Here, nearly sub-Poisson distributed coherent photon pairs obtained …
We propose and experimentally demonstrate an efficient framework for the quantum simulation of quantum channels in NMR. Our approach relies on the suitable decomposition of non-unitary operators in a linear combination of $d$ unitary ones, which can be then experimentally implemented with the assistance of a number of ancillary qubits that grows logarithmically in $d$. As a proof-of-principle demonstration, we realize the quantum simulation of three quantum channels for a single-qubit: phase damping (PD), amplitude damping (AD), and depolarizing (DEP) channels. For these paradigmatic cases, we…
In 1985, Leggett and Garg (1985 Phys. Rev. Lett. 54 857) proposed a Bell-like inequality to test (in)compatibility between two fundamental concepts of quantum mechanics. The first concept is 'macroscopic realism', which is the quality of a physical property of a quantum system being independent of observation at the macroscopic level. The second concept is 'noninvasive measurability', which is the possibility of performing a measurement without disturbing the subsequent evolution of a system. One of the key requirement for testing the violation of the Leggett-Garg inequality, or Bell's time in…
The effects of shot noise on the quantum computation of NMR spectra
Institut für Theoretische Physik and Center for Integrated Quantum Science and Technology, Universität Tübingen（蒂宾根大学理论物理研究所与集成量子科学与技术中心）；HQS Quantum Simulations GmbH（HQS量子模拟有限公司）；The University of Nottingham（诺丁汉大学）
We show for the first time how deterministic unitary operations on time-bin qubits encoded in single photon pulses can be realized using fiber optics components that are available with current technology. We also generalize this result to operations on time-bin qudits, i.e. $d$-level systems, and show that this can be done efficiently using 2$\times$2 beamsplitters and phase modulators. Important benefits for experimental quantum communication are highlighted. This work shows how to bridge the gap between current proof-of-principle demonstrations and complete, deterministic experiments.
We report an optical one-way quantum computing experiment with stationary quantum memory involved. First we create a hybrid four-qubit cluster state with two qubits propagating as photons and the other two stationary and stored in a laser-cooled atomic-ensemble quantum memory, and characterize it with entanglement witness and quantum state tomography. Then, by making use of this cluster state and fast operations of electro-optic modulators, we realize memory-assisted feedforward operations and demonstrate deterministic single-qubit rotation as an example.
One of the main requirements in linear optics quantum computing is the ability to perform single-qubit operations that are controlled by classical information fed forward from the output of single photon detectors. These operations correspond to pre-determined combinations of phase corrections and bit-flips that are applied to the post-selected output modes of non-deterministic quantum logic devices. Corrections of this kind are required in order to obtain the correct logical output for certain detection events, and their use can increase the overall success probability of the devices. In this…
In this paper, we consider the secret-string-learning problem in the teacher-student setting: the teacher has a secret string $s\in {\{0,1\}^{n}}$, and the student wants to learn the secret $s$ by question-answer interactions with the teacher, where at each time, the student can ask the teacher with a pair $(x, q) \in {\{0,1\}^{n}}\times\{0,1,\cdots, n-1\}$ and the teacher returns a bit given by the oracle $f_{s}(x,q)$ that indicates whether the length of the longest common prefix of $s$ and $x$ is greater than $q$ or not. Our contributions are as follows. (i) We prove that any classical deter…
We demonstrate an unconditional high-fidelity teleporter capable of preserving the broadband entanglement in an optical squeezed state. In particular, we teleport a squeezed state of light and observe $-0.8 \pm 0.2$dB of squeezing in the teleported (output) state. We show that the squeezing criterion translates directly into a sufficient criterion for entanglement of the upper and lower sidebands of the optical field. Thus, this result demonstrates the first unconditional teleportation of broadband entanglement. Our teleporter achieves sufficiently high fidelity to allow the teleportation to b…
In this note we demonstrate that a quantum-like interference picture could appear as a statistical effect of interference of deterministic particles, i.e. particles that have trajectories and obey deterministic equations, if one introduces a discrete time. The nature of the resulting interference picture does not follow from the geometry of force field, but is strongly attached to the time discreetness parameter. As a demonstration of this concept we consider a scattering of charged particles on the charged screen with a single slit. The resulting interference picture has a nontrivial minimum-…
This paper demonstrates the use of entanglement resources in quantum speedup by presenting an algorithm which is the generalization of an algorithm proposed by Goswami and Panigrahi [arXiv:1706.09489 (2017)]. We generalize the algorithm and show that it provides deterministic solutions having an advantage over classical algorithm. The algorithm answers the question of whether a given function is constant or balanced and whether two functions are equal or unequal. Finally, we experimentally verify the algorithm by using IBM's five-qubit quantum computer with a high fidelity.
Recently, a new interpretation of quantum mechanics has been developed for the wave nature of a photon, where determinacy in quantum correlations becomes an inherent property without the violation of quantum mechanics. Here, we experimentally demonstrate a direct proof of the wave natures of quantum correlation for the so-called coherence de Broglie waves (CBWs) using sub-Poisson distributed coherent photon pairs obtained from an attenuated laser. The observed experimental data coincides with the analytic solutions and the numerical calculations. Thus, the CBWs pave a road toward deterministic…
We examine three possible implementations of non-deterministic linear optical cnot gates with a view to an in-principle demonstration in the near future. To this end we consider demonstrating the gates using currently available sources such as spontaneous parametric down conversion and coherent states, and current detectors only able to distinguish between zero or many photons. The demonstration is possible in the co-incidence basis and the errors introduced by the non-optimal input states and detectors are analysed.
Any quantum information system operates with entanglement as a resource, which should be deterministically generated by a joint measurement known as complete Bell state measurement (BSM). The determinism arises from a quantum nondemolition measurement of two coupled qubits with the help of readout ancilla, which inevitably requires extra physical qubits. We here demonstrate a deterministic and complete BSM with only a nitrogen atom in a nitrogen-vacancy (NV) center in diamond as a quantum memory without reliance on any carbon isotopes by exploiting electron nitrogen (14N) double qutrits at a z…
No-cloning theorem forbids perfect cloning of an unknown quantum state. A universal quantum cloning machine (UQCM), capable of producing two copies of any input qubit with the optimal fidelity, is of fundamental interest and has applications in quantum information processing. This is enabled by delicately tailored nonclassical correlations between the input qubit and the copying qubits, which distinguish the UQCM from a classical counterpart, but whose experimental demonstrations are still lacking. We here implement the UQCM in a superconducting circuit, and investigate these correlations. The…
A hybrid interface of solid state single-photon sources and atomic quantum memories is a long sought-after goal in photonic quantum technologies. Here we demonstrate deterministic storage and retrieval of photons from a semiconductor quantum dot in an atomic ensemble quantum memory at telecommunications wavelengths. We store single photons from an InAs quantum dot in a high-bandwidth rubidium vapour based quantum memory, with a total internal memory efficiency of $(12.9 \pm 0.4) \%$. The signal-to-noise ratio of the retrieved photons is $18.2\pm 0.6$, limited only by detector dark counts. This…
Entanglement purification is to distill high-quality entangled states from low-quality entangled states. It is a key step in quantum repeaters, determines the efficiency and communication rates of quantum communication protocols, and is hence of central importance in long-distance communications and quantum networks. In this work, we report the first experimental demonstration of deterministic entanglement purification using polarization and spatial mode hyperentanglement. After purification, the fidelity of polarization entanglement arises from $0.268\pm0.002$ to $0.989\pm0.001$. Assisted wit…
Recently remarkable progress in quantum technology has been witnessed. In view of this it is important to investigate an open quantum system as a model of such quantum devices. Quantum devices often require extreme conditions such as very low temperature for the devices to operate. Dynamics can be non-Markovian in such a situation in contrast with Markovian dynamics in high temperature regime. This observation necessitates us to investigate a non-Markovian open quantum system, both theoretically and experimentally. In this paper, we report two important results: 1) Exact solution of a simple b…
