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arXiv 0806.0147cond-mat.str-el
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耦合自旋四面体系统集体模和局域模的反常频率和强度标度

Anomalous frequency and intensity scaling of collective and local modes in a coupled spin tetrahedron system

Kwang-Yong Choi, Hiroyuki Nojiri, Naresh S. Dalal, Helmuth Berger, Wolfram Brenig, Peter Lemmens

摘要:

本文报道了用单晶Raman散射研究耦合自旋四面体体系Cu $_{2}$ Te $_{2}$ O $_{5}$ Cl $_{2}$的磁激发谱。从热力学数据证明T $_{N}^{Cl}$ =18.2 K时向有序状态的转变导致叠加了宽的最大值的不同的低能磁激发的演变。这些模式被归因于具有不同程度的本地化和两个磁振子连续的磁振子。两个模式开发一个实质性的能量转移,降低温度类似的序参量的其他Neel有序系统。其他两种模式只显示出可以忽略不计的温度依赖性和溶解在一个连续的激发在有限的能量的有序温度以上。这些观测结果表明,四面体内部和内部的磁性自由度之间存在微妙的相互作用,并且在描述自旋动力学时单线态波动具有重要意义。

英文摘要:

We report on the magnetic excitation spectrum of the coupled spin tetrahedral system Cu$_{2}$Te$_{2}$O$_{5}$Cl$_{2}$ using Raman scattering on single crystals. The transition to an ordered state at T$_{N}^{Cl}$=18.2 K evidenced from thermodynamic data leads to the evolution of distinct low-energy magnetic excitations superimposed by a broad maximum. These modes are ascribed to magnons with different degree of localization and a two-magnon continuum. Two of the modes develop a substantial energy shift with decreasing temperature similar to the order parameter of other Neel ordered systems. The other two modes show only a negligible temperature dependence and dissolve above the ordering temperature in a continuum of excitations at finite energies. These observations point to a delicate interplay of magnetic inter- and intra-tetrahedra degrees of freedom and an importance of singlet fluctuations in describing a spin dynamics.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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