The formation of domains comprising alternating 'hole rich' and 'hole poor' ladders recently observed by Scanning Tunneling Microscopy by Kohsaka et al., on lightly hole doped cuprates, is interpreted in terms of an attractive mechanism which favors the presence of doped holes on Cu sites located each on one side of an oxygen atom. This mechanism leads to a geometrical pattern of alternating hole-rich and hole-poor ladders with a periodicity equal to 4 times the lattice spacing in the CuO plane, as observed experimentally. To cite this article: G. Deutscher, P.-G. de Gennes, C. R. Physique 8 (2007).
We amend ab initio strongly-correlated band structures by taking into account the band-tailing phenomenon in doped charge-transfer Mott-Hubbard insulators. We show that the photoemission from band tails accounts for sharp "quasi-particle" peaks, rapid loss of their intensities in some directions of the Brillouin zone ("Fermi-arcs") and high-energy "waterfall" anomalies as a consequence of matrix-element effects of disorder-localised states in the charge-transfer gap of doped cuprates.
We investigate magnetic properties of lightly doped antiferromagnetic Mott insulators in the presence of non-magnetic impurities. Within the framework of the t-J model we calculate the doping dependence of the antiferromagnetic order parameter using the self-consistent diagrammatic techniques. We show that in the presence of non-magnetic impurities the antiferromagnetic order is more robust against hole doping in comparison with the impurity-free host, implying that magnetic order can re-appear upon Zn doping into lightly hole-doped cuprates. We argue that this is primarily due to the loss of …
A central question in the high temperature cuprate superconductors is the fate of the parent Mott insulator upon charge doping. Here we use scanning tunneling microscopy to investigate the local electronic structure of lightly doped cuprate in the antiferromagnetic insulating regime. We show that the doped charge induces a spectral weight transfer from the high energy Hubbard bands to the low energy in-gap states. With increasing doping, a V-shaped density of state suppression occurs at the Fermi level, which is accompanied by the emergence of checkerboard charge order. The new STM perspective…
Behavior of ρ_{ab}(T) and R_{H}(T) is presented for LSCO and YBCO single crystals in the lightly hole-doped antiferromagnetic region, with an emphasis on the R_{H}(T) data. In both systems, R_{H} is virtually constant at moderate temperatures and tends to increase at low temperatures. Since essentially the same behavior of ρ_{ab}(T) and R_{H}(T) is observed in both LSCO and YBCO, we discuss that the in-plane charge transport properties are universal among the cuprates in the lightly-doped regime and that the R_{H}(T) data we obtained represent the genuine behavior of the Hall effect in this re…
One of the major puzzles regarding unconventional superconductivity is how some of the most interesting superconductors are related to an insulating phase that lies in close proximity. Here we report scanning tunneling microscopy studies of the local electronic structure of Cu doped NaFeAs across the superconductor to insulator transition. We find that in the highly insulating regime the electronic spectrum develops an energy gap with diminishing density of state at the Fermi level. The overall lineshape and strong spatial variations of the spectra are strikingly similar to that of lightly dop…
Lightly-doped La$_{2-x}$Sr$_x$CuO$_4$ in the so-called "insulating" spin-glass/diagonal-stripe phase has been studied by angle-resolved photoemission spectroscopy. A quasi-particle (QP) peak crossing the Fermi level has been observed in the node direction of the d-wave superconducting gap, forming an "arc" of Fermi surface consistent with the recently observed metallic transport behavior at high temperatures of lightly-doped materials. The spectral weight of the nodal QP smoothly increases with hole doping, corresponding to the $n \sim x$ behavior of the carrier number in the underdoped and li…
Resistivity and magnetization measurements are used for studying the transverse sliding of AF domain boundaries in lightly doped La_{2-x}Sr_{x}CuO_{4}. We discuss that it is the freezing of the transverse boundary motion that is responsible for the appearance of ``spin-glass'' features at low temperatures.
We investigated the doping dependence of magnetic excitations in the lightly doped cuprate La2-xSrxCuO4 via combined studies of resonant inelastic x-ray scattering (RIXS) at the Cu L3-edge and theoretical calculations. With increasing doping, the magnon dispersion is found to be essentially unchanged, but the spectral width broadens and the spectral weight varies differently at different momenta. Near the Brillouin zone center, we directly observe bimagnon excitations which possess the same energy scale and doping dependence as previously observed by Raman spectroscopy. They disperse weakly in…
The low-energy excitations of the lightly doped cuprates were studied by angle-resolved photoemission spectroscopy. A finite gap was measured over the entire Brillouin zone, including along the d_{x^2 - y^2} nodal line. This effect was observed to be generic to the normal states of numerous cuprates, including hole-doped La_{2-x}Sr_{x}CuO_{4} and Ca_{2-x}Na_{x}CuO_{2}Cl_{2} and electron-doped Nd_{2-x}Ce_{x}CuO_{4}. In all compounds, the gap appears to close with increasing carrier doping. We consider various scenarios to explain our results, including the possible effects of chemical disorder,…
We investigate the electronic properties of Ba[Fe(1-x)Co(x)]2As2 (x =0.02, 0.04) in the lightly electron-doped regime by 59Co and 75As NMR. We demonstrate that Co doping significantly suppresses the magnetic ordering temperature to the SDW state, T_{SDW}. Furthermore, ordered moments below T_{SDW} exhibit large distribution. Strong spin fluctuations remain even below T_{SDW}, persisting all the way down to 4.2 K. We find no signature of additional freezing of spin degrees of freedom unlike the case of the lightly hole-doped stripe phase of the cuprates.
We calculate the charge compressibility and uniform spin susceptibility for the two-dimensional (2D) Hubbard model slightly away from half-filling within a two-loop renormalization group scheme. We find numerically that both those quantities flow to zero as we increase the initial interaction strength from weak to intermediate couplings. This result implies gap openings in both charge and spin excitation spectra for the latter interaction regime. When this occurs, the ground state of the lightly doped 2D Hubbard model may be interpreted as an insulating spin liquid as opposed to a Mott insulat…
The AC and DC conductivity anisotropies in the low temperature orthorhombic phase of lightly doped La(2-x)Sr(x)CuO(4) are ascribed to the rotational symmetry broken, localized impurity states resulting from the trapping of doped holes by Sr ions. The two lowest-energy p-wave-like states are split by orthorhombicity and partially filled with holes. This leaves a unique imprint in AC conductivity, which shows two distinct infrared continuum absorption energies. Furthermore, the existence of two independent channels for hopping conductivity, associated to the two orthorhombic directions, explains…
We show that lightly doped holes will be self-trapped in an antiferromagnetic spin background at low-temperatures, resulting in a spontaneous translational symmetry breaking. The underlying Mott physics is responsible for such novel self-localization of charge carriers. Interesting transport and dielectric properties are found as the consequences, including large doping-dependent thermopower and dielectric constant, low-temperature variable-range-hopping resistivity, as well as high-temperature strange-metal-like resistivity, which are consistent with experimental measurements in the high-T$_c…
We present a study of the magnetic susceptibility in carefully detwinned La_{2-x}Sr_{x}CuO_4 single crystals in the lightly-doped region (x=0-0.03), which demonstrates a remarkable in-plane anisotropy of the spin system. This anisotropy is found to persist after the long-range antiferromagnetic (AF) order is destroyed by hole doping, suggesting that doped holes break the AF order into domains in which the spin alignment is kept essentially intact. It turns out that the freezing of the spins taking place at low temperatures is also notably anisotropic, implying that the "spin-glass" feature is …
Hole induced changes in the antiferromagnetic structure of a lightly Ca doped Gd:Y_{1-x}Ca_xBa_2Cu_3O_6 copper oxide single crystal with x~0.008 is investigated by Gd3+ electron spin resonance. Holes do not localize to Ca2+ ions above 2.5 K since the charge distribution and spin susceptibility next to the Ca2+ are independent of temperature. Both hole doped and pristine crystals are magnetically twinned with an external magnetic field dependent antiferromagnetic domain structure. Unlike the undoped crystal, where the easy magnetic axis is along [100] at all temperatures, the easy direction in …
We extend the methods recently introduced in Phys. Rev. Lett. 106 036401 (2011) to investigate correlations between two spin-polarons in a quasi-two-dimensional CuO2 layer. The low-energy wavefunctions for two doped holes introduced in a half-filled CuO2 plane with 32 copper and 64 oxygen sites are calculated explicitly using an efficient yet accurate truncation scheme to model the antiferromagnet background. The energetics and wavefucntions show that the charges form three-spin polarons and the spin is carried by a disturbance around the three-spin polaron core. The low-energy band results fr…
Detailed behavior of the magnetoresistance (MR) is studied in lightly doped antiferromagnetic La_{1.99}Sr_{0.01}CuO_{4}, where, thanks to the weak ferromagnetic moment due to spin canting, the antiferromagnetic (AF) domain structure can be manipulated by the magnetic field. The MR behavior demonstrates that CuO_2 planes indeed contain anti-phase AF domain boundaries in which charges are confined, forming anti-phase stripes. The data suggest that a high magnetic field turns the anti-phase stripes into in-phase stripes, and the latter appear to give better conduction than the former, which chall…
We consider the extended 2D $t-t'-t''-J$ model at zero temperature. Parameters of the model corresponds to doping by holes. Using the low doping effective action we demonstrate that the system can 1) preserve the long range collinear antiferromagnetic order, 2) lead to a spin spiral state (static or dynamic), 3) lead to the phase separation instability. We show that at parameters of the effective action corresponding to the single layer cuprate La$_{2-x}$Sr$_x$CuO$_4$ the spin spiral ground state is realized. We derive properties of magnetic excitations and calculate quantum fluctuations. Quan…
In a recent study Viskadourakis et al. discovered that extremely underdoped La_2CuO_(4+x) is a relaxor ferroelectric and a magnetoelectric material at low temperatures. It is further observed that the magnetoelectric response is anisotropic for different directions of electric polarization and applied magnetic field. By constructing an appropriate Landau theory, we show that a bi-quadratic magnetoelectric coupling can explain the experimentally observed polarization dependence on magnetic field. This coupling leads to several novel low-temperature effects including a feedback enhancement of th…
Much progress has been made recently in the study of the effects of electron-phonon (el-ph) coupling in doped insulators using angle resolved photoemission (ARPES), yielding evidence for the dominant role of el-ph interactions in underdoped cuprates. As these studies have been limited to doped Mott insulators, the important question arises how this compares with doped band insulators where similar el-ph couplings should be at work. The archetypical case is the perovskite SrTiO$_3$ (STO), well known for its giant dielectric constant of 10000 at low temperature, exceeding that of La$_2$CuO$_4$ b…
Recent ESR data shows rotation of the antiferromagnetic (AF) easy axis in lightly doped layered cuprates upon lowering the temperature. We account for the ESR data and show that it has significant implications on spin and charge ordering according to the following scenario: In the high temperature phase AF domain walls coincide with (110) twin boundaries of an orthorhombic phase. A magnetic field leads to annihilation of neighboring domain walls resulting in antiphase boundaries. The latter are spin carriers, form ferromagnetic lines and may become charged in the doped system. However, hole or…
We investigate the occurrence of a two-step spin-flop transition and spin reorientation when a longitudinal magnetic field is applied to lightly hole-doped La(2)CuO(4). We find that for large and strongly frustrating impurities, such as Sr in La(2-x)Sr(x)CuO(4), the huge enhancement of the longitudinal susceptibility suppresses the intermediate flop and the reorientation of spins is smooth and continuous. Contrary, for small and weakly frustrating impurities, such as O in La(2)CuO(4+y), a discontinuous spin reorientation (two-step spin-flop transition) takes place. Furthermore, we show that fo…
We report $^{75}$As NMR measurements in BaFe$_2$As$_2$ doped with Ni. Like Co, Ni doping suppresses the antiferromagnetic and structural phase transitions and gives rise to superconductivity for sufficiently large Ni doping. The spin lattice relaxation rate diverges at $T_N$, with a critical exponent consistent with 3D ordering of local moments. In the ordered state the spectra quickly broaden inhomogeneously with doping. We extract the average size of the ordered moment as a function of doping, and show that a model in which the order remains commensurate but with local amplitude variations i…
Electronic structure has been studied in lightly electron doped correlated spin-orbit insulator Sr$_2$IrO$_4$ by angle-resolved photoelectron spectroscopy. We have observed coexistence of the lower Hubbard band and the in-gap band, the momentum dependence of the latter traces that of the band calculations without on-site Coulomb repulsion. The in-gap state remained anisotropically gapped in all observed momentum area, forming a remnant Fermi surface state, evolving towards the Fermi energy by carrier doping. These experimental results show a striking similarity with those observed in deeply un…
The hole concentration dependence of the magnetic correlations is studied in very lightly-doped La$_{2-x}$Sr$_x$CuO$_4$ ($x<$0.02), which shows coexistence of a three-dimensional antiferromagnetic (AF) long-range ordered phase and a spin-glass phase at low temperatures. It is found that the spin-glass phase in the coexistence region also shows a diagonal spin modulation as in the pure spin-glass phase in La$_{2-x}$Sr$_x$CuO$_4$ (0.02$\le x\le$0.055). Below $x\sim$0.02 the diagonal stripe structure is the same as that in $x\sim$0.02 with a volume fraction almost proportional to hole concentrati…
We study two-leg spin ladder systems analytically by using a t-J model which includes the interchain spin exchange and the interchain hopping term. The spin part is mapped to a quantum sine-Gordon model via a bosonization method that fully accounts for the phase fluctuation. The spin gap in the Luther-Emery phase evolves to gapless Luttinger liquid phases in even-ladders at certain doping concentration. This transition occurs as doping rate increases and/or the ratio of the interchain spin exchange and hopping to the intrachain couplings decreases. We also estimate the transition temperature a…
Understanding the rich and competing electronic orders in cuprate superconductors may provide important insight into the mechanism of high-temperature superconductivity. Here, by measuring Bi2Sr2CaCu2O8+x in the extremely underdoped regime, we obtain evidence for a distinct type of ordering, which manifests itself as resistance oscillations at low magnetic fields (<10 T) and at temperatures around the superconducting transition. By tuning the doping level p continuously, we reveal that these low-field oscillations occur only when p<0.1. The oscillation amplitude increases with decreasing p but…
Both ab-plane and c-axis thermal conductivities ($κ_{ab}$ and $κ_c$) of lightly doped La$_{2-x}$Sr$_x$CuO$_4$ and La$_2$Cu$_{1-y}$Zn$_y$O$_4$ single crystals ($x$ or $y$ = 0 -- 0.04) are measured from 2 to 300 K. It is found that the low-temperature phonon peak (at 20 -- 25 K) is significantly suppressed upon Sr or Zn doping even at very low doping, though its precise doping dependences show interesting differences between the Sr and Zn dopants, or between the $ab$ plane and the c axis. Most notably, the phonon peak in $κ_c$ decreases much more quickly with Sr doping than with Zn doping, while…
Whether the doped t-J model on the Kagome lattice supports exotic superconductivity has not been decisively answered. In this paper, we propose a new class of variational states for this model and perform large-scale variational Monte Carlo simulation on it. The proposed variational states are parameterized by the SU(2)-gauge-rotation angles, as the SU(2)-gauge structure hidden in the Gutzwiller-projected mean-field ansatz for the undoped model is broken upon doping. These variational doped states smoothly connect to the previously studied U(1) $π$-flux or $0$-flux states, and energy minimizat…
Both the in-plane and the out-of-plane resistivities (ρ_{ab} and ρ_{c}) are measured in high-quality La_{2-x}Sr_{x}CuO_{4} (LSCO) single crystals in the lightly- to moderately-doped region, x = 0.01 to 0.10, and the resistivity anisotropy is determined. In all the samples studied, the anisotropy ratio ρ_{c}/ρ_{ab} quickly increases with decreasing temperature, although in non-superconducting samples the strong localization effect causes ρ_{c}/ρ_{ab} to decrease at low temperatures. Most notably, it is found that ρ_{c}/ρ_{ab} at moderate temperatures (100 - 300 K) is almost completely independe…
A magnetic field parallel to an electrical current does not produce a Lorentz force on the charge carriers. Therefore, orbital longitudinal magnetoresistance is unexpected. Here we report on the observation of a large and non saturating magnetoresistance in lightly doped SrTiO$_{3-x}$ independent of the relative orientation of current and magnetic field. We show that this quasi-isotropic magnetoresistance can be explained if the carrier mobility along all orientations smoothly decreases with magnetic field. This anomalous regime is restricted to low concentrations when the dipolar correlation …
The phase diagram of hole-doped copper oxides shows four different electronic phases existing at zero temperature. Familiar among these are the Mott insulator, high-transition-temperature superconductor and metallic phases. A fourth phase, ofunknown identity, occurs at light doping along the zero-temperature bound of the `pseudogap' regime. This regime is rich in peculiar electronic phenomena, prompting numerous proposals that it contains some form of hidden electronic order. Here we present low-temperature electronic structure imaging studies of a lightly hole-doped copper oxide: Ca_{2-x}Na_{…
The effects of the application of a magnetic field on the diagonal stripe spin-glass phase is studied in lightly doped La_{2-x}Sr_xCuO_4 (x=0.014 and 0.024). With increasing magnetic field, the magnetic elastic intensity at the diagonal incommensurate (DIC) positions (1,\pmε,0) decreases as opposed to the increase seen in superconducting samples. This diminution in intensity with increasing magnetic field originates from a spin reorientation transition, which is driven by the antisymmetric exchange term in the spin Hamiltonian. On the other hand, the transition temperature, the incommensurabil…
We have studied the chemical potential shift in the high-temperature superconductor Bi$_2$Sr$_2$Ca$_{1-x}${\it R}$_{x}$Cu$_2$O$_{8+y}$ ({\it R} = Pr, Er), where the hole concentration is varied from 0.025 to 0.17 per Cu, by precise measurements of core-level photoemission spectra. The result shows that the shift becomes slow in the underdoped region as in the case of La$_{2-x}$Sr$_{x}$CuO$_{4}$ (LSCO) but the effect is much weaker than in LSCO. The observed shift in the present system can be relatively well explained by numerical results on the doped two-dimensional Hubbard model, and suggests…
In a recent Letter (Phys. Rev. Lett. 106, 036401 (2011)), Lau, et al. investigated the single hole problem in an effective model containing Cu $d$ and O $2p$ orbitals by exact diagonalization on clusters composed of 32 CuO$_2$ unit cells. With full quantum fluctuations due to the antiferromagnetic (AFM) backgroud, they found that spin-polaron solutions with spin 3/2 become lowest energy solutions in certain region of Brillouin zone (BZ), which they claimed no similiar solutions were obtained in other models or approximations before. In this Comment, we would like to point out that such high-sp…
We analyze various possible superconducting pairing states and their relative stabilities in lightly doped graphene. We show that, when inter-sublattice electron-electron attractive interaction dominates and Fermi level is close to Dirac points, the system will favor intra-valley spin-triplet $p+\mathrm{i}p$ pairing state. Based on the novel pairing state, we further propose a scheme for doing topological quantum computation in graphene by engineering local strain fields and external magnetic fields.
Identification of the electronic state that appears upon doping a Mott insulator is important to understand the physics of cuprate high-temperature superconductors. Recent scanning tunneling microscopy of cuprates provides evidence that a charge-ordered state emerges before the superconducting state upon doping the parent compound. We study this phenomenon by computing the charge response function of the Hubbard model including frequency-dependent local vertex corrections that satisfy the compressibility sum-rule. We find that upon approaching the Mott phase from the overdoped side, the charge…
We report extensive muon spin rotation measurements on the lightly doped Y1-xCaxBa2Cu3O6+y compound, which allows us to disentangle the effect of disorder, controlled by random Ca2+ substitution, from that of mere doping. A 3D phase diagram of lightly doped cuprates is accurately drawn, showing that a thermally activated antiferromagnetic phase competes with superconductivity around a quantum critical point, hidden underneath a frozen insulating magnetic state. Disorder suppresses both competing order parameters and unveils the underlying frozen state. Doping and disorder destroy the activated…
We have performed an angle resolved photoemission spectroscopy (ARPES) study of lightly-doped to underdoped YBa2Cu3Oy (YBCO) untwinned single crystals and a core-level x-ray photoemission spectroscopy (XPS) study of YBCO single and polycrystals. In the zone diagonal (nodal) direction, dispersive quasi-particle (QP) features crossing the Fermi level were observed down to the hole concentration of ~ 4%, which explains the metallic transport of the lightly-doped YBCO. The chemical potential shift estimated from XPS was more rapid than in the Bi2212 cuprates. Upon hole doping, very rapid spectral …
The spatial variation of electronic states was imaged in the lightly doped Mott insulator Ca_{2-x}Na_{x}CuO_{2}Cl_{2} using scanning tunneling microscopy / spectroscopy (STM/STS). We observed nano-scale domains with a high local density of states within an insulating background. The observed domains have a characteristic length scale of 2 nm (~4-5a, a:lattice constant) with preferred orientations along the tetragonal [100] direction. We argue that such spatially inhomogeneous electronic states are inherent to slightly doped Mott insulators and play an important role for the insulator to metal …
The relaxation function theory of doped two-dimensional $S=1/2$ Heisenberg antiferromagnetic (AF) system in the paramagnetic state is presented taking into account the hole subsystem as well as both the electron and AF correlations. The expression for fourth frequency moment of relaxation shape function is derived within the $t-J$ model. The presentation obeys rotational symmetry of the spin correlation functions and is valid for all wave vectors through the Brillouin zone. The spin diffusion contribution to relaxation rates is evaluated and is shown to play a significant role in carrier free …
We have performed extensive zero field muSR experiments on pure YBa2Cu3O6+y and diluted Y-rare-earth substituted Y0.92Eu0.08Ba2Cu3O6+y and Y0.925Nd0.075Ba2Cu3O6+y at light hole-doping. A common magnetic behavior is detected for all the three families, demonstrating negligible effects of the isovalent Y-substituent disorder. Two distinct regimes are identified, separated by a crossover, whose origin is attributed to the concurrent thermal activation of spin and charge degrees of freedom: a thermally activated and a re-entrant quenched-hole antiferromagnetic regime. The peculiar temperature and …
In the low doping range of $x$ from 0.01 to 0.06 in La$_{2-x}$Sr$_{x}$CuO$_{4}$, a narrow electron paramagnetic resonance (EPR) line has been investigated. This line is distinct from the known broad line, both due to probing Mn$^{2+}$ ions. The narrow line is ascribed to metallic regions in the material, and its intensity increases exponentially upon cooling below $\sim$ 150 K. The activation energy deduced $Δ$ = 460(50) K is nearly the same as that found in the doped superconducting regime by Raman and neutron scattering. The intensity of the narrow EPR line follows the same temperature depen…
In-plane transport properties of nonsuperconducting YBa_{2}Cu_{3}O_{y} (y = 6.35) are measured using high-quality untwinned single crystals. We find that both the a- and b-axis resistivities show log(1/T) divergence down to 80 mK, and accordingly the thermal conductivity data indicate that the nodal quasiparticles are progressively localized with lowering temperature. Hence, both the charge and heat transport data do not support the existence of a "thermal metal" in nonsuperconducting YBa_{2}Cu_{3}O_{y}, as opposed to a recent report by Sutherland {\it et al.} [Phys. Rev. Lett. {\bf 94}, 14700…
The phase diagram for hole-doped cuprates is discussed. By examining some recent inelastic neutron scattering data obtained on hole-doped cuprates we conclude that the coherent gap in hole-doped cuprates has most likely the magnetic origin and scales with Tc, on average, as 2Delta/kTc = 5.4.
The remarkable sensitivity of the c-axis resistivity and magnetoresistance in cuprates to the spin ordering is used to clarify the doping-induced transformation from an antiferromagnetic (AF) insulator to a superconducting (SC) metal in RBa_2Cu_3O_{6+x} (R = Lu, Y) single crystals. The established phase diagram demonstrates that the AF and SC regions apparently overlap: the superconductivity in RBa_2Cu_3O_{6+x}, in contrast to La_{2-x}Sr_xCuO_4, sets in before the long-range AF order is completely destroyed by hole doping. Magnetoresistance measurements of superconducting crystals with low T_c…
We develop a theory of superconducting pairing in low-density Strontium titanate due to quadratic coupling of electron density to soft transverse optical phonons. It leads to static attractive potential between electrons which decay length scales inversely with soft optical gap. For low electron densities attraction between electrons is local and transition temperature Tc was found. The Tc(n) dependence in agreement with experimental data for low doping was calculated. Next, we show that suppression of Tc by hydrostatic pressure and strong increase of Tc due to isotop substitution are explaine…
Persistent Fermi Pockets and Robust Electron Pairing in Lightly Doped CuO$_2$ Planes of Cuprate Superconductors
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；University of Chinese Academy of Sciences（中国科学院大学）；Max Planck Institute for Solid State Research（马克斯·普朗克固体研究研究所）；Technical Institute of Physics and Chemistry, Chinese Academy of Sciences（中国科学院理化技术研究所）；Songshan Lake Materials Laboratory（松山湖材料实验室）；Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）
High temperature superconductivity in cuprates is realized by doping the Mott insulator with charge carriers. A central issue is how such an insulating state can evolve into a conducting or superconducting state when charge carriers are introduced. Here, by in situ vacuum annealing and Rb deposition on the Bi2Sr2Ca0.6Dy0.4Cu2O8+delta (Bi2212) sample surface to push its doping level continuously from deeply underdoped (Tc=25 K, doping level p-0.066) to the near zero doping parent Mott insulator, angle-resolved photoemission spectroscopy measurements are carried out to observe the detailed elect…
By comparing experimental results obtained in the study of the electron transport and magnetic properties of samples of lightly strontium-substituted lanthanum cuprates and the results of a previously published numerical analysis in the reduced elastic scattering space (RPS) of the elastic scattering cross-section, we construct a phenomenological classical self-consistent strong-binding energy density profile in the superconducting $La_{2-x}Sr_xCuO_4$ cuprate. It is found that the imaginary part of the reduced phase scattering space can be zero, almost constant, or strongly self-consistent, de…
Systematic measurements of the magnetic susceptibility were performed on single crystals of lightly doped La2-xSrxCuO4 (x=0.03, 0.04 and 0.05). For all samples the temperature dependence of the in-plane magnetic susceptibility shows typical spin-glass features with spin-glass transition temperatures Tg of 6.3K, 5.5K and 5.0K for x=0.03, 0.04 and 0.05, respectively. The canonical spin-glass order parameter extracted from the in-plane susceptibility of all the samples follows a universal scaling curve. On the other hand, the out-of-plane magnetic susceptibility deviates from Curie law below a te…
Within the t-t'-J model, the charge asymmetry in superconductivity of hole- and electron-doped cuprates is studied based on the kinetic energy driven superconducting mechanism. It is shown that superconductivity appears over a narrow range of doping in electron-doped cuprates, and the superconducting transition temperature displays the same kind of the doping controlled behavior that is observed in the hole-doped case. However, the maximum achievable superconducting transition temperature in the optimal doping in electron-doped cuprates is much lower than that of the hole-doped case due to the…
The tunneling spectra of the electron-doped cuprate Pr_2-xCe_xCuO4 as a function of doping and temperature is reported. We find that the superconducting gap, delta, shows a BCS-like temperature dependence even for extremely low carrier concentrations (studied here for the first time). Moreover, delta follows the doping dependence of Tc, in strong contrast with tunneling studies of hole-doped cuprates. From our results we conclude that there is a single superconducting energy scale in the electron-doped cuprates.
It is widely believed that high-temperature superconductivity in the cuprates emerges from doped Mott insulators. The physics of the parent state seems deceivingly simple: The hopping of the electrons from site to site is prohibited because their on-site Coulomb repulsion U is larger than the kinetic energy gain t. When doping these materials by inserting a small percentage of extra carriers, the electrons become mobile but the strong correlations from the Mott state are thought to survive; inhomogeneous electronic order, a mysterious pseudogap and, eventually, superconductivity appear. How th…
We consider the lightly doped cuprates Y$_{0.97}$Ca$_{0.03}$BaCuO$_{6.05}$ and La$_{2-x}$Sr$_x$CuO$_4$ (with $x=0.02$,0.04), where the presence of a fluctuating nematic state has often been proposed as a precursor of the stripe (or, more generically, charge-density wave) phase, which sets in at higher doping. We phenomenologically assume a quantum critical character for the longitudinal and transverse nematic, and for the charge-ordering fluctuations, and investigate the effects of these fluctuations in Raman spectra. We find that the longitudinal nematic fluctuations peaked at zero transferre…
