在α-团簇模型的框架内结合系统双折叠势研究了中等质量核的性质。以前，该α-簇模型已被广泛应用于轻核，特别是8Be = α \otimes α、20 Ne = 16 O \otimes α和44 Ti = 40 Ca \otimes α，以及重核，特别是212 Po = 208 Pb \otimes α。本文研究了幻数N = 50，质量范围在\approx 80 - 100：（A+4，N=52）=（A，N=50）\otimes α附近的各种核.结果表明，该模型能很好地描述激发能、衰变性质和跃迁强度。α-核势的基本参数的平滑和小的变化可以用于外推，以预测所研究的核中的实验未知性质。
英文摘要：
Properties of intermediate mass nuclei have been investigated within the framework of the alpha-cluster model in combination with systematic double-folding potentials. Previously, this alpha-cluster model has been widely applied to light nuclei, in particular to 8Be = alpha \otimes alpha, 20Ne = 16O \otimes alpha, and 44Ti = 40Ca \otimes alpha, and to heavy nuclei, in particular to 212Po = 208Pb \otimes alpha. In the present work a wide range of nuclei is investigated with the magic neutron number N = 50 in the mass range around A \approx 80 - 100: (A+4,N=52) = (A,N=50) \otimes alpha. It is found that excitation energies, decay properties, and transition strengths can be described successfully within this model. The smooth and small variation of the underlying parameters of the alpha-nucleus potential may be used for extrapolations to predict experimentally unknown properties in the nuclei under study.
We have constructed new proximity function particularly for interaction between two superheavy nuclei based on the experimental alpha decay half-lives. The new proximity function is used to produce the alpha decay half-lives of superheavy nuclei whose experimental values are known. The new proximity function produces the alpha decay half-lives close to the experiments. Hence we can conclude that the new proximity function can be used to study the interaction between two superheavy nuclei.
Spontaneous fission and alpha decay are the main decay modes for superheavy nuclei. The superheavy nuclei which have small alpha decay half-life compared to spontaneous fission half-life will survive fission and can be detected in the laboratory through alpha decay. We have studied the alpha decay half-life and spontaneous half-life of some superheavy elements in the atomic range Z = 100-130. Spontaneous fission half-lives of superheavy nuclei have been calculated using the phenomenological formula and the alpha decay half-lives using Viola-Seaborg-Sobiczewski formula (Sobiczewski et al. 1989)…
The competition between alpha- and beta+/EC-decay modes is studied systematically in nuclei along the alpha-decay chains following the synthesis of superheavy nuclei with Z = 119 and Z = 120. A microscopic approach based on deformed self-consistent Hartree-Fock mean-field calculations with Skyrme forces and pairing correlations is used to describe the beta+ and electron capture weak decays, whereas the alpha-decay is estimated from existing phenomenological expressions. It is shown that alpha-decay is in most cases the dominant decay mode, but interesting instances are identified where the hal…
Recently synthesis of superheavy nuclei has been achieved in hot fusion reactions. A systematic theoretical calculation of alpha decay half-lives in this region of the periodic system, may be useful in the identification of new nuclei in these type of reactions. Alpha decay half-lives are obtained in the framework of the barrier penetration theory, built with the use of proximity and Coulomb forces. It is estimated from a classical viewpoint, a possible angular momentum maximum value for odd and odd-odd nuclei alpha particles. The masses of the nuclei are obtained from a macro-microscopic mode…
The nuclear equation of state is explored with the constrained HFB approach for self conjugate nuclei. It is found that beyond a certain low, more or less universal density, those nuclei spontaneously cluster into A/4 alpha particles with A the nucleon number. The energy at the threshold density increases linearly with the number of alpha particles as does the experimental threshold energy. Taking off the spurious c.o.m. energy of each alpha particle almost gives agreement between theory and experiment. The implications of these results with respect to alpha clustering and the nuclear EOS at l…
We propose a novel mechanism to explain nuclear decay by emission of an alpha particle. We show that the famous Geiger-Nuttall law can be explained by post-forming an alpha particle outside the range of the nuclear interaction with the daughter nucleus. This contrasts with the commonly accepted mechanism of first alpha particle pre-formation followed by emission through barrier penetration. We predict that the post-formation mechanism is more likely to occur for alpha-particles with higher energy.
The experimentally available data on the alpha decay half lives and Q? values for 96 superheavy nuclei are used to fix the parameters for a modified version of the Brown empirical formula through two fitting procedures which enables its comparison with similar fits using Viola-Seaborg and Royer formulas. The new expressions provide very good agreement with experimental data having fewer or the same number of parameters. All formulas with the obtained parameters are then extrapolated to generate half lives predictions for 125 unknown superheavy alpha emitters. The nuclei where the employed empi…
We discuss the treatment of isovector pairing by an alpha-like quartet condensate which conserves exactly the particle number, the spin and the isospin. The results show that the quartet condensate describes accurately the isovector pairing correlations in the ground state of systems with an equal number of protons and neutrons
It is shown, that the Gamow-like model with only one adjustable parameter - radius constant is able to reproduce well the alpha-decay half-lives for all even-even nuclei with the proton number larger than 50. The systematics for odd-A and odd-odd isotopes can be also well described when ones introduces an additional hindrance factor. Similar model based on the W. J. Swiatecki idea from 1955 is developed to reproduce the spontaneous fission half-lives of transactinide nuclei. The achieved accuracy of reproduction of the data is better than that obtained in more advanced theories.
The classical trajectory model with stochastic breakup for nuclear collision dynamics of weakly-bound nuclei is further developed. It allows a quantitative study of the importance of incomplete fusion dynamics in the angular distribution of direct alpha-production. Model calculations indicate that the incomplete fusion contribution diminishes with decreasing energy towards the Coulomb barrier, notably separating in angles from the contribution of no-capture breakup events. This should facilitate the experimental disentanglement of these competing reaction processes.
Alpha-decay energies for several chains of super-heavy nuclei are calculated within the self-consistent mean-field approach by using the Fayans functional FaNDF$^0$. They are compared to the experimental data and predictions of two Skyrme functionals, SLy4 and SkM*, and of the macro-micro method as well. The corresponding lifetimes are calculated with the use of the semi-phenomenological formulas by Parkhomenko and Sobiczewski and by Royer and Zhang.
The Woods-Saxon-Gaussian (WSG) potential is proposed as a new phenomenological potential to describe systematically the level scheme, electromagnetic transitions, and alpha-decay half-lives of the alpha-cluster structures in various alpha+closed shell nuclei. It modifies the original Woods-Saxon (WS) potential with a shifted Gaussian factor centered at the nuclear surface. We determine the free parameters in the WSG potential by reproducing the correct level scheme of $^{212}\text{Po}={}^{208}\text{Pb}+α$. It is found that the resulting WSG potential matches with the M3Y double-folding potenti…
We study the possibility to use the cluster-daughter overlap as a new probe of alpha-cluster formation in medium-mass and heavy even-even nuclei. We introduce a dimensionless parameter $\mathfrak{O}$, which is the ratio between the root-mean-square (rms) intercluster separation and the sum of rms point radii of the daughter nucleus and the alpha particle, to measure the degree of the cluster-daughter overlap quantitatively. By using this parameter, a large (small) cluster-daughter overlap between the alpha cluster and daughter nucleus corresponds to a small (large) $\mathfrak{O}$ value. The al…
The updated data for the ground-state-to-ground-state alpha-transition half-lives in 401 nuclei and the alpha capture cross sections of 40Ca, 44Ca, 59Co, 208Pb and 209Bi are well described in the framework of the unified model for alpha-decay and alpha-capture. The updated values of the alpha decay half-lives, the binding energies of nuclei, the spins of parent and daughter nuclei, and the surface deformation parameters are used for the reevaluation of the model parameters. The data for the ground-state-to-ground-state alpha-decay half-lives are also well described by the empirical relationshi…
Description of a nuclear system in its ground state and at low excitations based on the equation of state (EoS) around normal density is presented. In the expansion of the EoS around the saturation point additional spin polarization terms are taken into account. These terms, together with the standard symmetry term, are responsible for appearance of the $α$-like clusters in the ground state configurations of the N=Z even-even nuclei. At the nuclear surface these clusters can be identified as alpha particles. A correction for the surface effects is introduced for atomic nuclei. Taking into acco…
The nucleonic localization function has been used for a decade to study the formation of alpha-particles in nuclei, by providing a measure of having nucleons of a given spin in a single place. However, differences in interpretation remain, compared to the nucleonic density of the nucleus. In order to better understand the respective role of the nucleonic localization function and the densities in the alpha-particle formation in cluster states or in alpha-decay mechanism, both an analytic approximation and microscopic calculations, using energy density functionals, are undertaken. The nucleonic…
We considered the systematics of $α$-decay (AD) half-life (HL) of super-heavy nuclei versus the decay energy and the total $α$-kinetic energy. We calculated the HL using the experimental Q_{$α$} values. The computed half-lives are compared with the experimental data and also with the existing empirical estimates and are found in good agreement. Also, we obtained $α$-preformation factors from the ratio between theoretical and experimental results for some super heavy nuclei SHN and evaluated the standard deviation. The results indicate the acceptability of the approach.
In this work, the $β$-stable region for Z $\geq$ 90 is proposed. The calculated $β$-stable nuclei in the $β$-stable region are in good agreement with the ones obtained by Möller \emph{et al}.. The half-lives of the nuclei close to the $β$-stable region are calculated and the competition between $α$-decay and $β$-decay is systematically investigated. The calculated half-lives and the suggested decay modes are well in line with the experimental results. The predictions for half-lives and decay modes of the nuclei with Z = 107$-$110 are presented.
A broad extension of periodic system into the sector of antimatter could be possible sometimes in a remote future. We expect that anti-alpha spontaneous emission from an antimatter nucleus will have the same Q-value and half-life as alpha emission from the corresponding mirror nucleus. This is the consequence of the invariance of binding energy as well as of the surface and Coulomb energy when passing from matter to antimatter nuclei with the the same mass number and the same atomic number. The Q-values and half-lives of all measured up to now 27 cluster radioactivities are given together with…
We propose a simple quartet condensation model (QCM) which describes with very high accuracy the isovector pairing correlations in self-conjugate nuclei. The quartets have an alpha-like structure and are formed by collective isovector pairs. The accuracy of the QCM is tested for N=Z nuclei for which exact shell model diagonalizations can be performed. The calculations are done with two isovector pairing forces, one extracted from standard shell model interactions and the other of seniority type, acting, respectively, upon spherical and axially-deformed single-particle states. It is shown that …
In the framework of a recently developed alpha-cluster model a nucleus is represented as a core (alpha-cluster liquid drop with dissolved excess neutron pairs in it) and a nuclear molecule on its surface. From analysis of experimental nuclear binding energies one can find the number of alpha-clusters in the molecule and calculate the nuclear charge radii. It was shown that for isotopes of one Z with growing A the number of alpha-clusters in the molecule decreases to three, which corresponds to the nucleus 12C for even Z and 15N for odd Z, and the specific density of the core binding energy ρgr…
We study the competition between alpha-type and conventional pair condensation in the ground state of nuclei with neutrons and protons interacting via a charge-independent pairing interaction. The ground state is described by a product of two condensates, one of alpha-like quartets and the other one of pairs in excess relative to the isotope with N=Z. It is shown that this ansatz for the ground state gives very accurate pairing correlation energies for nuclei with the valence nucleons above the closed cores 16O, 40Ca and 100Sn. These results indicate that alpha-type correlations are important …
A systematic study on the probability for the emission of 4^He and 14^C cluster from hyper ${207-234}^$Ac and non-strange normal ${207-234}^$Ac nuclei are performed for the first time using our fission model, the Coulomb and proximity potential model (CPPM). The predicted half lives show that hyper ${207-234}^$Ac nuclei are unstable against 4^He emission and 14^C emission from hyper ${217-228}^$Ac are favorable for measurement. Our study also show that hyper ${207-234}^$Ac are stable against hyper 4^He and 14^C emission. The role of neutron shell closure (N=126) in hyper 214^Fr daughter and ro…
Bose-Einstein condensation of alpha clusters in light and medium-heavy nuclei is studied in the frame of the field theoretical superfluid cluster model. The order parameter of the phase transition from the Wigner phase to the Nambu-Goldstone phase is a superfluid amplitude, square of the moduli of which is the superfluid density distribution. The zero mode operators due to the spontaneous symmetry breaking of the global phase in the finite number of alpha clusters are rigorously treated. The theory is systematically applied to N alpha nuclei from12C-52Fe at various condensation rates. In 12C i…
The advent of radioactive ion beam facilities and new detector technologies have opened up new possibilities to investigate the radioactive decays of highly unstable nuclei, in particular the proton emission, $α$ decay and heavy cluster decays from neutron-deficient (or proton-rich) nuclei around the proton drip line. It turns out that these decay measurements can serve as a unique probe for studying the structure of the nuclei involved. On the theoretical side, the development in nuclear many-body theories and supercomputing facilities have also made it possible to simulate the nuclear cluste…
In this contribution, I discuss an algebraic treatment of alpha-cluster nuclei based on the introduction of a spectrum generating algebra for the relative motion of the alpha-clusters. Particular attention is paid to the discrete symmetry of the geometric arrangement of the alpha-particles, and the consequences for the structure of the rotational bands in the 12C and 16O nuclei.
An intense study of the alpha decay properties of the isotopes of superheavy element Z=113 have been performed within the Coulomb and proximity potential model for deformed nuclei (CPPMDN) within the wide range 255 l.e. A l.e. 314. The predicted alpha decay half lives of $^{278}$113 and $^{282}$113 and the alpha half lives of their decay products are in good agreement with the experimental data. 6{α) chains and 4α chains predicted respectively for $^{278}$113 and $^{282}$113 are in agreement with the experimental observation. Our study shows that the isotopes in the mass range 278 l.e. A l.e. …
The breaking of rotational symmetry on the lattice for bound eigenstates of the two lightest alpha conjugate nuclei is explored. Moreover, a macroscopic alpha-cluster model is used for investigating the general problems associated with the representation of a physical many-body problem on a cubic lattice. In view of the descent from the 3D rotation group to the cubic group symmetry, the role of the squared total angular momentum operator in the classification of the lattice eigenstates in terms of SO(3) irreps is discussed. In particular, the behaviour of the average values of the latter opera…
In this work study on alpha decay chains emerging from isotopes of Z = 122 superheavy nuclei is carried out with emphasize on nuclear deformations and Langer modification. The interest in this particular superheavy nuclei is due to the recent experimental efforts to synthesize the isotope ^{299}120 in a fusion reaction at the velocity filter SHIP (GSI Darmstadt), which makes synthesis of Z = 122 nuclei to occur in the near future, and in turn will give the experimentalist the chance observe the decays associated with the isotopes of this nuclei. We perform our calculations by choosing the Wood…
The formation of alpha-clusters in nuclei close to the decay thresholds is discussed. These states can be considered to be boson-condensates, which are formed in a second order phase transition in a mixture of nucleons and alpha-particles. The de Broglie wavelength of the alpha-particles is larger than the nuclear diameter, therefore the coherent properties of the alpha-particles give particular effects for the study of such states. The states are above the thresholds thus the enhanced emission of multiple-alphas into the same direction is observed. The probability for the emission of multiple…
Masses of superheavy (SH) nuclei with $Z=98-128$, including odd and odd-odd nuclei, are systematically calculated within the microscopic-macroscopic model based on the deformed Woods-Saxon potential. Ground states are found by minimizing energy over deformations and configurations. Pairing in odd particle-number systems is treated either by blocking or by adding the BCS energy of the odd quasiparticle. Three new parameters are introduced which may be interpreted as the constant mean pairing energies for even-odd, odd-even and odd-odd nuclei. They are adjusted by a fit to masses of heavy nuclei…
The alpha-decay half-lives of recently synthesized superheavy nuclei (SHN) are investigated based on a unified fission model (UFM) where a new method to calculate the assault frequency of alpha-emission is used. The excellent agreement with the experimental data indicates the UFM is a useful tool to investigate these alpha-decays. It is found that the half-lives become more and more insensitive to the Q_alpha values as the atomic number increases on the whole, which is favorable for us to predict the half-lives of SHN. In addition, a formula is suggested to compute the Q_alpha values for the n…
The universal curve is one of the simple ways to get preliminary information about the Alpha-decay half-life times of heavy nuclei. We try to find parameterization for the universal curve of Alpha decay based on semi-microscopic calculations, starting from the realistic M3Y-Reid nucleon-nucleon interaction. Within the deformed density-dependent cluster model, the penetration probability and the assault frequency are calculated using the WKB penetration probability. The deformations of daughter nuclei and the ground-state spin and parity of the involved nuclei are considered. We found that it i…
We report variational Monte Carlo calculations of single-nucleon momentum distributions for A <= 12 nuclei and nucleon-pair and nucleon-cluster momentum distributions for A <= 8. The wave functions have been generated for a Hamiltonian containing the Argonne v18 two-nucleon and Urbana X three-nucleon potentials. The single-nucleon and nucleon-pair momentum distributions exhibit universal features attributable to the one-pion-exchange tensor interaction. The single-nucleon distributions are broken down into proton and neutron components and spin-up and spin-down components where appropriate. Th…
A systematic study on $α$-decay half-lives for the nuclei in the range $93\leq Z \leq 118$ is done by employing various versions of proximity potentials. To obtain the more reliable results, the deformation terms are included up to hexadecapole ($β_{4}$) in the spherical-deformed nuclear and Coulomb interaction potentials. The favored $α$-decays process in this region are categorized as the even-even, odd A, and odd-odd nuclei, first, and second they are grouped into two parts as a ground state to ground state and ground state to isomeric states transition. Due to their root-mean-square deviat…
The nuclear $α$ decay of heavy nuclei is investigated based on the nuclear energy density functional, which leads to the $α$ potential inside the parent nucleus in terms of the proton and neutron density profiles of the daughter nucleus. We use the Skyrme force model, Gogny force model, and relativistic mean field model to get the nucleon density profiles inside heavy nuclei. Once the nucleon density profiles are determined, the parameters of the nuclear $α$ potential are fitted to the observed $α$ decay half-lives of heavy nuclei. This approach is then applied to predict unknown $α$ decay hal…
The antisymmetrized quasi-cluster model (AQCM) is a method to describe a transition from the alpha-cluster wave function to the jj-coupling shell model wave function. In this model, the cluster-shell transition is characterized by only two parameters; R representing the distance between alpha clusters and Lambda describing the breaking of alpha clusters, and the contribution of the spin-orbit interaction, very important in the jj-coupling shell model, can be taken into account starting with the alpha cluster model wave function. In this article we show the generality of AQCM by extending the a…
