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arXiv 0802.2473cond-mat.str-el
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顺磁尖晶石LiV2O4自旋涨落的自洽重整化理论

Self-consistent renormalization theory of spin fluctuations in paramagnetic spinel LiV2O4

V. Yushankhai, P. Thalmeier, T. Takimoto

摘要:

用参数化的自旋涨落自洽重整化(SCR)理论对LiV $_2$ O $_4$粉末样品非弹性中子散射测量中观测到的动态自旋极化率$χ({\bf q},ω;T)$进行了唯象描述.与以前的研究在$T\to 0$兼容,一个特殊的分布在${\bf q}$ -空间的强烈增强和缓慢的自旋波动在$q \sim Q_c \simeq$ 0.6 $Å^{-1}$在LiV $_2$ O $_4$涉及到导出模式模式耦合项进入SCR理论的基本方程。该方程求解自洽的参数值从理论结果拟合实验数据。对于低温$T \lesssim 30$ K,SCR理论更可靠,静态自旋磁化率$χ(Q_c;T)$和弛豫速率$Γ_Q(T)$在$q\sim Q_c$的温度变化与理论所提出的结果很好地吻合。对于$T\gtrsim 30$ K,本SCR仅能够预测$χ(Q_c;T)$和$Γ_Q(T)$的$T$依赖性的主要趋势。讨论的重点是一个显着的演变(从$q \sim Q_c$在$T\to 0$低$q$值在较高的温度)的主要低$ω$集成中子散射强度$I(q; T)$。

英文摘要:

A phenomenological description for the dynamical spin susceptibility $χ({\bf q},ω;T)$ observed in inelastic neutron scattering measurements on powder samples of LiV$_2$O$_4$ is developed in terms of the parametrized self-consistent renormalization (SCR) theory of spin fluctuations. Compatible with previous studies at $T\to 0$, a peculiar distribution in ${\bf q}$-space of strongly enhanced and slow spin fluctuations at $q \sim Q_c \simeq$ 0.6 $Å^{-1}$ in LiV$_2$O$_4$ is involved to derive the mode-mode coupling term entering the basic equation of the SCR theory. The equation is solved self-consistently with the parameter values found from a fit of theoretical results to experimental data. For low temperatures, $T \lesssim 30$K, where the SCR theory is more reliable, the observed temperature variations of the static spin susceptibility $χ(Q_c;T)$ and the relaxation rate $Γ_Q(T)$ at $q\sim Q_c$ are well reproduced by those suggested by the theory. For $T\gtrsim 30$K, the present SCR is capable in predicting only main trends in $T$-dependences of $χ(Q_c;T)$ and $Γ_Q(T)$. The discussion is focused on a marked evolution (from $q \sim Q_c$ at $T\to 0$ towards low $q$ values at higher temperatures) of the dominant low-$ω$ integrated neutron scattering intensity $I(q; T)$.

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