We study heat transport in normal/superconducting graphene junctions. We find that while the thermal conductance displays the usual exponential dependence on temperature, reflecting the s-wave symmetry of the superconductor, it exhibits an unusual oscillatory dependence on the potential height or the length of the barrier region. This oscillatory dependence stems from the emergent low-energy relativistic nature of fermions in graphene, essentially different from the result in conventional normal metal/superconductor junctions.
We show that in contrast to conventional normal metal-insulator-superconductor (NIS) junctions, the tunneling conductance of a NIS junction in graphene is an oscillatory function of the effective barrier strength of the insulating region, in the limit of a thin barrier. The amplitude of these oscillations are maximum for aligned Fermi surfaces of the normal and superconducting regions and vanishes for large Fermi surface mismatch. The zero-bias tunneling conductance, in sharp contrast to its counterpart in conventional NIS junctions, becomes maximum for a finite barrier strength. We also sugge…
We study the supercurrent in a superconductor/ferromagnet/superconductor graphene junction. In contrast to its metallic counterpart, the oscillating critical current in our setup decays only weakly upon increasing exchange field and junction width. We find an unusually large residual value of the supercurrent at the oscillatory cusps due to a strong deviation from a sinusoidal current-phase relationship. Our findings suggest a very efficient device for dissipationless supercurrent switching.
We investigate the conductance spectra of a normal/superconductor graphene junction using the extended Blonder-Tinkham-Klapwijk formalism, considering pairing potentials that are both conventional (isotropic s-wave) and unconventional (anisotropic d-wave). In particular, we study the full crossover from normal to specular Andreev reflection without restricting ourselves to special limits and approximations, thus expanding results obtained in previous work. In addition, we investigate in detail how the conductance spectra are affected if it is possible to induce an unconventional pairing symmet…
We theoretically calculate the charge-supercurrent through a ballistic graphene junction where superconductivity is induced via the proximity-effect. Both monolayer and bilayer graphene are considered, including the possibility of strain in the systems. We demonstrate that the supercurrent at the charge neutrality point can be tuned efficiently by means of mechanical strain. Remarkably, the supercurrent is enhanced or suppressed relative to the non-strained case depending on the direction of this strain. We also calculate the Fano factor in the normal-state of the system and show how its behav…
Within the tunneling Hamiltonian formulation for the eight-component spinors,the Josephson critical super-current has been calculated in a planar superconductor-normal graphene-superconductor junction. Coupling between superconductor regions and graphene is taken into account by a tunneling Hamiltonian which contains two types of tunneling, intra-valley and inter-valley tunneling. Within the present tunneling approach, we find that the contributions of two kinds of tunneling to the critical super-current, are completely separable. Therefore, it is possible to consider the effect of the inter-v…
Transparent contact interfaces in superconductor-graphene hybrid systems are critical for realizing superconducting quantum applications. Here, we examine the effect of the edge-contact fabrication process on the transparency of the superconducting aluminum-graphene junction. We show significant improvement in the transparency of our superconductor-graphene junctions by promoting the chemical component of the edge contact etch process. Our results compare favorably with state-of-the-art graphene Josephson junctions. The findings of our study contribute to advancing the fabrication knowledge of…
We perform extensive analysis of graphene Josephson junctions embedded in microwave circuits. By comparing a diffusive junction at 15 mK with a ballistic one at 15 mK and 1 K, we are able to reconstruct the current-phase relation.
Josephson junctions with graphene as the weak link between superconductors have been intensely studied in recent years, with respect to both fundamental physics and potential applications. However, most of the previous work was based on mechanically exfoliated graphene, which is not compatible with mass production. Here we present our research using graphene grown by chemical vapour deposition (CVD) as the weak link of Josephson junctions. We demonstrate that CVD-graphene-based Josephson junctions with Nb electrodes can work effectively without any thermal hysteresis from 1.5 K down to a base …
Superconductor-graphene-superconductor (SGS) junction provides a unique platform to study relativistic electrodynamics of Dirac fermions combined with proximity-induced superconductivity. We report observation of the Josephson effect in proximity-coupled superconducting junctions of graphene in contact with Pb1-xInx (x=0.07) electrodes for temperatures as high as T = 4.8K, with a large IcRn (~ 255 microV). This demonstrates that Pb1-xInx SGS junction would facilitate the development of the superconducting quantum information devices and superconductor-enhanced phase-coherent transport of graph…
Graphene on silicon carbide (SiC) has proved to be highly successful in Hall conductance quantization for its homogeneity at the centimetre scale. Robust Josephson coupling has been measured in co-planar diffusive Al/monololayer graphene/Al junctions. Graphene on SiC substrates is a concrete candidate to provide scalability of hybrid Josephson graphene/superconductor devices, giving also promise of ballistic propagation.
We investigate the zero-bias behavior of Josephson junctions made of encapsulated graphene boron nitride heterostructures in the long ballistic junction regime. For temperatures down to 2.7K, the junctions appear non-hysteretic with respect to the switching and retrapping currents $I_C$ and $I_R$. A small non-zero resistance is observed even around zero bias current, and scales with temperature as dictated by the phase diffusion mechanism. By varying the graphene carrier concentration we are able to confirm that the observed phase diffusion mechanism follows the trend for an overdamped Josephs…
We fabricate superconductor-graphene-superconductor Josephson junctions with superconducting regions made of lead (Pb). The critical current through grapehene may be modulated by external magnetic field; the resulting Fraunhofer interference pattern shows several periods of oscillations, indicating that the junction is uniform. Deviations from the perfect Fraunhofer pattern are observed, and their cause is explained by a simulation that takes into account the sample design.
We demonstrate enhanced robustness of the supercurrent through graphene-based Josephson junctions in which strong spin-orbit interactions (SOIs) are induced. We compare the persistence of a supercurrent at high magnetic fields between Josephson junctions with graphene on hexagonal boron-nitride and graphene on WS$_2$, where strong SOIs are induced via the proximity effect. We find that in the shortest junctions both systems display signatures of induced superconductivity, characterized by a suppressed differential resistance at a low current, in magnetic fields up to 1 T. In longer junctions h…
We use a tight-binding Bogoliubov-de Gennes (BdG) formalism to self-consistently calculate the proximity effect, Josephson current, and local density of states in ballistic graphene SNS Josephson junctions. Both short and long junctions, with respect to the superconducting coherence length, are considered, as well as different doping levels of the graphene. We show that self-consistency does not notably change the current-phase relationship derived earlier for short junctions using the non-selfconsistent Dirac-BdG formalism but predict a significantly increased critical current with a stronger…
Using highly efficient simulations of the tight-binding Bogoliubov-de Gennes model we solved self-consistently for the pair correlation and the Josephson current in a Superconducting-Bilayer graphene-Superconducting Josephson junction. Different doping levels for the non-superconducting link are considered in the short and long junction regime. Self-consistent results for the pair correlation and superconducting current resemble those reported previously for single layer graphene except in the Dirac point where remarkable differences in the proximity effect are found as well as a suppression o…
The current-phase relation (CPR) of a Josephson junction reveals valuable information about the microscopic processes and symmetries that influence the supercurrent. In this Letter, we present direct measurements of the CPR for Josephson junctions with a graphene barrier, obtained by a phase-sensitive SQUID interferometry technique. We find that the CPR is skewed with respect to the commonly observed sinusoidal behavior. The amount of skewness varies linearly with critical current (Ic) regardless of whether Ic is tuned by the carrier density or temperature.
Using the Bogoliubov de-Gennes formalism, we investigate the charge and spin-dependent thermoelectric effects in superconductor graphene junctions. Results demonstrate that despite normal-superconductor junctions, there is a temperature-dependent spin thermopower both in the graphene-based ferromagnetic-superconductor (F-S) and ferromagnetic-Rashba spin-orbit region-superconductor (F-RSO-S) junctions. It is also shown that in the presence of Rashba spin-orbit interaction, the charge and spin-dependent Seebeck coefficients can reach to their maximum up to 3.5$k_B/e$ and 2.5$k_B/e$, respectively…
The Josephson Effect and Superconducting Proximity Effect were observed in Superconductor -Graphene-Superconductor (SGS) Josephson junctions with coherence lengths comparable to the distance between the superconducting leads. By comparing the measured temperature and doping dependence of the supercurrent and the proximity induced sub-gap features (multiple Andreev reflections) to theoretical predictions we find that, contrary to expectations, the ballistic transport model fails to describe the SGS junctions. In contrast, the diffusive junction model yields close quantitative agreement with the…
We have tuned in situ the proximity effect in a single graphene layer coupled to two Pt/Ta superconducting electrodes. An annealing current through the device changed the transmission coefficient of the electrode/graphene interface, increasing the probability of multiple Andreev reflections. Repeated annealing steps improved the contact sufficiently for a Josephson current to be induced in graphene.
We show that Andreev reflection in a junction between ferromagnetic (F) and superconducting (S) graphene regions is fundamentally different from the common FS junctions. For a weakly doped F graphene with an exchange field $h$ larger than its Fermi energy $E_{\rm F}$, Andreev reflection of massless Dirac fermions is associated with a Klein tunneling through an exchange field p-n barrier between two spin-split conduction and valence subbands. We find that this Andreev-Klein process results in an enhancement of the subgap conductance of a graphene FS junction by $h$ up to the point at which the …
We present a theoretical analysis of the current-voltage characteristics of a ballistic superconductor-normal-superconductor (SNS) junction, in which a strip of graphene is coupled to two superconducting electrodes. We focus in the short-junction regime, where the length of the strip is much smaller than superconducting coherence length. We show that the differential conductance exhibits a very rich subharmonic gap structure which can be modulated by means of a gate voltage. On approaching the Dirac point the conductance normalized by the normal-state conductance is identical to that of a shor…
We study Josephson effect in graphene superconductor- barrier- superconductor junctions with short and wide barriers of thickness $d$ and width $L$, which can be created by applying a gate voltage $V_0$ across the barrier region. We show that Josephson current in such graphene junctions, in complete contrast to their conventional counterparts, is an oscillatory function of both the barrier width $d$ and the applied gate voltage $V_0$. We also demonstrate that in the thin barrier limit, where $V_0 \to \infty$ and $d \to 0$ keeping $V_0 d$ finite, such an oscillatory behavior can be understood i…
We report on Andreev reflections at clean NbSe2-bilayer graphene junctions. The high transparency of the junction, which manifests as a large conductance enhancement of up to 1.8, enables us to see clear evidence of a proximity-induced superconducting gap in bilayer graphene and two Andreev reflections through a vertical NbSe2-graphene and a lateral graphene-graphene junction respectively. Quantum transport simulations capture the complexity of the experimental data and illuminate the impact of various microscopic parameters on the transmission of the junction. Our work establishes the practic…
We present a study of a graphene-based Josephson junction with dedicated side gates carved from the same sheet of graphene as the junction itself. These side gates are highly efficient, and allow us to modulate carrier density along either edge of the junction in a wide range. In particular, in magnetic fields in the $1-2$ Tesla range, we are able to populate the next Landau level, resulting in Hall plateaus with conductance that differs from the bulk filling factor. When counter-propagating quantum Hall edge states are introduced along either edge, we observe supercurrent localized along that…
Edge-contacted superconductor-graphene-superconductor Josephson junction have been utilized to realize topological superconductivity, which have shown superconducting signatures in the quantum Hall regime. We perform the first-principles calculations to interpret electronic couplings at the superconductor-graphene edge contacts by investigating various aspects in hybridization of molybdenum d orbitals and graphene $π$ orbitals. We also reveal that interfacial oxygen defects play an important role in determining the doping type of graphene near the interface.
We report on graphene-based Josephson junctions with contacts made from lead. The high transition temperature of this superconductor allows us to observe the supercurrent branch at temperatures up to $\sim 2$ K, at which point we can detect a small, but non-zero, resistance. We attribute this resistance to the phase diffusion mechanism, which has not been yet identified in graphene. By measuring the resistance as a function of temperature and gate voltage, we can further characterize the nature of electromagnetic environment and dissipation in our samples.
We investigated the electrical transport properties of superconductor-graphene-superconductor (SGS) Josephson junctions. In low voltage bias, we observed conventional proximity-coupled Josephson effect, such as the supercurrent flow through the graphene, sub-gap structure of differential conductance due to Andreev reflection, and periodic modulation of the critical current Ic with perpendicular magnetic field H to the graphene. In high bias above the superconducting gap voltage, however, we also observed an anomalous jump of the differential conductance, the voltage position of which is sensit…
We show that interface bound states are formed at isolated graphene-superconductor junctions. These states arise due to the interplay of virtual Andreev and normal reflections taking place at these interfaces. Simple analytical expressions for their dispersion are obtained considering interfaces formed along armchair or zig-zag edges. It is shown that the states are sensitive to a supercurrent flowing on the superconducting electrode. The states provide long range superconducting correlations on the graphene layer which may be exploited for the detection of crossed Andreev processes.
We report an experimental study of Cooper pair splitting in an encapsulated graphene based multiterminal junction in the ballistic transport regime. Our device consists of two transverse junctions, namely the superconductor/graphene/superconductor and the normal metal/graphene/normal metal junctions. In this case, the electronic transport through one junction can be tuned by an applied bias along the other. We observe clear signatures of Cooper pair splitting in the local as well as nonlocal electronic transport measurements. Our experimental data can be very well described by using a modified…
Stochastic switching-current distribution in a graphene-based Josephson junction exhibits a crossover from the classical to quantum regime, revealing the macroscopic quantum tunneling (MQT) of a Josephson phase particle at low temperatures. Microwave spectroscopy measurements indicate a multi-photon absorption process occurring via discrete energy levels in washboard potential well. The crossover temperature for MQT and the quantized level spacing are controlled with the gate voltage, implying its potential application to gate-tunable superconducting quantum bits.
A graphene superlattice is formed by a one-dimensional periodic potential and is characterized by the emergence of new Dirac points in the electronic structure. The group velocity of graphene's massless Dirac fermions at the new points is drastically reduced, resulting in a measurable effect in the conductance spectroscopy. We show here that tunnel spectroscopy using a superconducting hybrid junction is more sensitive to the formation of Dirac points in the spectrum of graphene superlattices due to the additional contribution of Andreev processes. We examine the transport properties of a graph…
Short ballistic graphene Josephson junctions sustain superconducting current with a non-sinusoidal current-phase relation up to a critical current threshold. The current-phase relation, arising from proximitized superconductivity, is gate-voltage tunable and exhibits peculiar skewness observed in high quality graphene superconductors heterostructures with clean interfaces. These properties make graphene Josephson junctions promising sensitive quantum probes of microscopic fluctuations underlying transport in two-dimensions. We show that the power spectrum of the critical current fluctuations h…
