In this work we have shown bulk superconductivity and studied the anisotropy in both the normal and superconducting states in quasi-1D conductor Nb2Se3. Electron - electron Umklapp scattering dominates electronic transport along the direction of Nb metal chains as well as perpendicular to it. The superconducting state is rather anisotropic with possible multi - band features.
We report a systematic study of anisotropy resistivity, magnetoresistance and Hall effect of Li0.32(NH3)yFe2Te1.2Se0.8 single crystals. When compared to the parent compound FeTe0.6Se0.4, the Li-NH3 intercalation not only increases the superconducting transition temperature, but also enhances the electronic anisotropy in both normal and superconducting states. Moreover, in contrast to the parent compound, the Hall coefficient RH becomes negative at low temperature, indicating electron-type carriers are dominant due to Li doping. On the other hand, the sign reverse of RH at high temperature and …
We investigate the superconducting properties and possible nematic superconductivity of self-doped BiCh2-based (Ch: S, Se) superconductor CeOBiS1.7Se0.3 through the measurements of in-plane anisotropy of magnetoresistance. Single crystals of CeOBiS1.7Se0.3 were grown using a flux method. Single-crystal structural analysis revealed that the crystal structure at room temperature is tetragonal (P4/nmm). Bulk superconductivity with a transition temperature of 3.3 K was observed through electrical resistivity and magnetization measurements. Investigation of anisotropy of upper critical field sugges…
Exotic superconductivity is formed by unconventional electron pairing and exhibits various unique properties that cannot be explained by the basic theory. The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state is known as an exotic superconducting state in that the electron pairs have a finite center-of-mass momentum leading to a spatially modulated pattern of superconductivity. The spatial modulation endows the FFLO state with emergent anisotropy. However, the anisotropy has never been experimentally verified despite numerous efforts over the years. Here, we report detection of anisotropic acousti…
FeSe is a unique superconductor that can be manipulated to enhance its superconductivity using different routes while its monolayer form grown on different substrates reaches a record high temperature for a two-dimensional system. In order to understand the role played by the substrate and the reduced dimensionality on superconductivity, we examine the superconducting properties of exfoliated FeSe thin flakes by reducing the thickness from bulk down towards 9 nm. Magnetotransport measurements performed in magnetic fields up to 16T and temperatures down to 2K help to build up complete supercond…
The interaction between superconductivity and ferromagnetism in thin film superconductor/ferromagnet heterostructures is usually reflected by a change in superconductivity of the S layer set by the magnetic state of the F layers. Here we report the converse effect: transformation of the magnetocrystalline anisotropy of a single Fe(001) layer, and thus its preferred magnetization orientation, driven by the superconductivity of an underlying V layer through a spin-orbit coupled MgO interface. We attribute this to an additional contribution to the free energy of the ferromagnet arising from the c…
We have investigated Se substitution effect to superconductivity of an optimally-doped BiS2-based superconductor Eu0.5La0.5FBiS2. Eu0.5La0.5FBiS2-xSex samples with x = 0-1 were synthesized. With increasing x, in-plane chemical pressure is enhanced. For x = 0.6, 0.8, and 1, superconducting transitions with a large shielding volume fraction are observed in magnetic susceptibility measurements, and the highest Tc is 3.8 K for x = 0.8. From low-temperature electrical resistivity measurements, a zero-resistivity state is observed for all the samples, and the highest Tc is observed for x = 0.8. With…
Sn0.8Ag0.2Te is a new superconductor with Tc ~ 2.4 K. The superconducting properties of Sn0.8Ag0.2Te have been investigated by specific heat measurements under magnetic fields. Bulk nature of superconductivity was confirmed from the amplitude of the specific heat jump at the superconducting transition, and the amplitude is consistent with fully-gapped superconductivity. Upper critical field was estimated from specific heat and electrical resistivity measurements under magnetic fields. The Hall coefficient was positive, suggesting that the Ag acts as a p-type dopant in Sn0.8Ag0.2Te.
By using a hydrothermal method, we have successfully grown crystals of the newly discovered superconductor FeS, which has an isostructure of the iron based superconductor FeSe. The superconductivity appears at about 4.5K, as revealed by both resistive and magnetization measurements. It is found that the upper critical field is relatively low, with however an rather large anisotropy $Γ=[(dH_{c2}^{ab}/dT)/(dH_{c2}^{c}/dT)]_{T_c}\approx5.8$. A huge magnetoresistivity (290$\%$ at 9T and 10K, ${H}$ $\parallel$ c-axis) together with a non-linear behavior of Hall resistivity vs. external field are ob…
We investigated the effects of $c/a$ anisotropy and local crystal structure on superconductivity (SC) in As/P solid solution systems, $A\mathrm{Fe_{2}}(\mathrm{As}_{1-x}\mathrm{P}_{x}\mathrm{)_{2}}$ ($A$122P) with various $A$ ions. With decreasing $A$ site atomic size from $A$=Ba to Eu, the structural anisotropy decreases, and the rate of decreasing with $x$ also increases. The rapid narrowing of the region of antiferromagnetic composition ($x$) can be considered to be a result of this anisotropy change due mainly to the change in the Fermi surface (FS) nesting condition. By contrast, although…
Anisotropy in the electrical resistivity and susceptibility of superconducting BaFe$_{2}$As$_{2}$ single crystals
用自熔法生长了$BaFe_2As_2$单晶。晶体呈板状，c轴垂直于平面。尺寸可以大到3 x 5 x 0.2 $mm^3$。电阻率各向异性（$ρ_c/ρ_{ab}$）大到约150，并且与温度无关。在ab平面和沿c轴方向的输运具有相同的散射机制。与多晶样品的磁行为相反，没有观察到Curie-Weiss行为，在自旋密度波（SDW）转变以上出现了与温度线性相关的磁化率。磁化率行为与反铁磁SDW铬非常相似。除了巡游电子对磁化率的贡献外，单晶的磁行为也明确地证明了局域磁矩的存在。观察到电阻率极小值强烈依赖于磁场。在低温下，与低掺杂铜酸盐类似，出现log（1/T）发散。在这里，我们首先介绍了高质量单晶的内禀输运和磁性，以及它们的各向异性。
The recent study of $^{77}$Se nuclear magnetic resonance (NMR) in a $β$-FeSe single crystal proposed that ferro-orbital order breaks the $90^\circ$ $C_4$ rotational symmetry, driving nematic ordering. Here, we report an NMR study of the impact of small strains generated by gluing on nematic state and spin fluctuations. We observe that the local strains strongly affect the nematic transition, considerably enhancing its onset temperature. On the contrary, no effect on low-energy spin fluctuations was found. Furthermore we investigate the interplay of the nematic phase and superconductivity. Our …
The capability to switch electrically between superconducting and insulating states of matter represents a novel paradigm in the state-of-the-art engineering of correlated electronic systems. An exciting possibility is to turn on superconductivity in a topologically non-trivial insulator, which provides a route to search for non-Abelian topological states. However, existing demonstrations of superconductor-insulator switches have involved only topologically trivial systems, and even those are rare due to the stringent requirement to tune the carrier density over a wide range. Here we report re…
Twisted graphene multilayers have demonstrated to yield a versatile playground to engineer controllable electronic states. Here, by combining first-principles calculations and low-energy models, we demonstrate that twisted graphene trilayers provide a tunable system where van Hove singularities can be controlled electrically. In particular, it is shown that besides the band flattening, bulk valley currents appear, which can be quenched by local chemical dopants. We finally show that in the presence of electronic interactions, a non-uniform superfluid density emerges, whose non-uniformity gives…
We investigate the physical mechanisms for achieving an electrical control of conventional spin-singlet superconductivity in thin films by focusing on the role of surface orbital polarization. Assuming a multi-orbital description of the metallic state, due to screening effects the electric field acts by modifying the strength of the surface potential and, in turn, yields non-trivial orbital-Rashba couplings. The resulting orbital polarization at the surface and in its close proximity is shown to have a dramatic impact on superconductivity. We demonstrate that, by varying the strength of the el…
Weakly anisotropic superconductivity of Pr4Ni3O10 single crystals
ShanghaiTech University（上海科技大学）；Center for High Pressure Science and Technology Advanced Research（高压科学与技术先进研究中心）；Institute for Shanghai Advanced Research in Physical Sciences (SHARPS)（上海物理科学研究院）；Songshan Lake Materials Laboratory（松山湖材料实验室）；Qufu Normal University（曲阜师范大学）；University of Oxford（牛津大学）；Southeast University（东南大学）；Tsinghua University（清华大学）
Comment on ``Anisotropic s-wave superconductivity: comparison with experiments on MgB_2 [A. I. Posazhennikova, T. Dahm and K. Maki, cond-mat/0204272; submitted to Europhys. Lett.]
The 12442 compounds are a recently discovered family of iron-based superconductors, that share several features with the cuprates due to their strongly anisotropic structure, but are so far poorly understood. Here, we report on the gap structure and anisotropy of RbCa2(Fe1-xNix)4As4F2 single crystals, investigated by a combination of directional point-contact Andreev-reflection spectroscopy and coplanar waveguide resonator measurements. Two gaps were identified, with clear signatures of d-wave-like nodal structures which persist upon Ni doping, well described by a two-band d-d state with symme…
The missing hole packets near the Brillouin zone center render unique electronic structures to the heavily electron doped FeSe-based superconductors with Tc above 40 K. It challenges the existing scenario accounting for the nature of superconductivity in the iron-based family. Yet, one hurdle that has to be overcome is the materials complexity in the rather limited number of compounds. Here we report the growth of heavily electron doped Li-NH3 intercalated FeSe single crystals that are free of such complexities and allow access to the intrinsic superconducting properties. Our results show extr…
Controlling the perpendicular magnetic anisotropy (PMA) in thin films has received considerable attention in recent years due to its technological importance. PMA based devices usually involve heavy-metal (oxide)/ferromagnetic-metal bilayers, where, thanks to interfacial spin-orbit coupling (SOC), the in-plane (IP) stability of the magnetization is broken. Here we show that in V/MgO/Fe(001) epitaxial junctions with competing in-plane and out-of-plane (OOP) magnetic anisotropies, the SOC mediated interaction between a ferromagnet (FM) and a superconductor (SC) enhances the effective PMA below t…
The recent observation of superconductivity in thin film infinite-layer nickelates$^{1-3}$ offers a different angle to investigate superconductivity in layered oxides$^{4}$. A wide range of candidate models have been proposed$^{5-10}$, emphasizing single- or multi-orbital electronic structure, Kondo or Hund's coupling, and analogies to cuprates. Clearly, further experimental characterization of the superconducting state is needed to develop a full understanding of the nickelates. Here we use magnetotransport measurements to probe the superconducting anisotropy in Nd$_{0.775}$Sr$_{0.225}$NiO$_{…
Recent studies on superconductivity in NbSe$_2$ have demonstrated a large anisotropy in the superconducting critical field when the material is reduced to a single monolayer. Motivated by this recent discovery, we use density functional theory (DFT) calculations to quantitatively address the superconducting properties of bulk and monolayer NbSe$_2$. We demonstrate that NbSe$_2$ is close to a ferromagnetic instability, and analyze our results in the context of experimental measurements of the spin susceptibility in NbSe$_2$. We show how this magnetic instability, which is pronounced in a single…
In-plane anisotropy of electrical resistivity in the strain-detwinned SrFe2As2
本征的，在平面内的电阻率的各向异性进行了研究的SrFe $_2$作为$_2$的机械解孪单晶的温度以上和以下的耦合结构/磁性转变，$T_{\textrm{TO}}$。电阻率对于沿正交$a_o$方向（反铁磁交替磁矩的方向）的电流流动较小，并且对于沿$b_o$方向（铁磁链的方向）的传输较大，这类似于CaFe $_2$ As $_2$和BaFe $_2$ As $_2$化合物。高能X射线衍射结果证实了SrFe $_2$ As $_2$的一级结构转变，其转变温度和性质不受中等应变的影响。对于小的应变水平，这是刚刚足以detwin的样品，我们发现一个可以忽略不计的影响电阻率以上$T_{\textrm{TO}}$。随着应变的增加，电阻率各向异性开始发展到高于$T_{\textrm{TO}}$，清楚地表明各向异性与对应变的强烈响应的关系。我们的研究表明，电子向列性不能观察到的FeAs基化合物中的结构转变是强烈的一级。
Superconductivity in many strongly correlated materials appears in proximity to a density-wave or nematic order and is believed to be mediated by quantum-critical (QC) fluctuations of the corresponding order parameter. We argue that fingerprints of QC pairing can be extracted from the angular dependence of the gap $Δ(θ)$. We consider pairing by QC nematic fluctuations and show that there exist multiple pairing instabilities within the same symmetry ($s-$wave in our case), with closely spaced transition temperatures $T_{c,n}$. The corresponding $Δ_n (θ)$ change sign $8n$ times along the FS. Onl…
We study the intrinsic anisotropy of the superconducting state in KFe$_2$As$_2$, using small-angle neutron scattering to image the vortex lattice as the applied magnetic field is rotated towards the FeAs crystalline planes. The anisotropy is found to be strongly field dependent, indicating multiband superconductivity. Furthermore, the high field anisotropy significantly exceeds that of the upper critical field, providing further support for Pauli limiting in KFe$_2$As$_2$ for field applied in the basal plane. The effect of Pauli paramagnetism on the unpaired quasiparticles in the vortex cores …
Superconductivity in the presence of disorder in skutterudite-related La$_3$Co$_4$Sn$_{13}$ and La$_3$Ru$_4$Sn$_{13}$ compounds; electrical transport and magnetic studies
La $_3$ Co $_4$ Sn $_{13}$和La $_3$ Ru $_4$ Sn $_{13}$被归类为BCS超导体。在临界场$H_{c2}$对$T$的曲线图中，La $_3$ Ru $_4$ Sn $_{13}$在较高的临界温度$T_c^{\star}$下显示第二超导相，这是非均匀超导体的特征，而La $_3$ Co $_4$ Sn $_{13}$在低于$T_c$下显示体超导性。我们观察到的临界温度与外部压力和磁场的降低与$\frac{dT_c^{\star}}{dP} > \frac{dT_c}{dP}$的两种化合物。根据McMillan理论解释了$T_c$的压力依赖性，并将其理解为晶格硬化的结果。对La-$_3$-Co-$_x$-Ru-$_{4-x}$-Sn-$_{13}$超导态的研究表明，对于$x<4$，$T_c^{\star}$大于$T_c$.这种独特的和意想不到的观察结果进行了讨论，作为一个结果的局部无序和/或化学压力的影响时，Ru原子被部分取代较小的Co原子。
