Large spin cold atom systems can exhibit novel magnetic properties which do not appear in usual spin-1/2 systems. We investigate the SU(4) resonating plaquette state in the three dimensional cubic optical lattice with spin-3/2 cold fermions. A novel gauge field formalism is constructed to describe the Rokhsar-Kivelson type of Hamiltonian and a duality transformation is used to study the phase diagram. Due to the proliferation of topological defects, the system is generally gapped for the whole phase diagram of the quantum model, which agrees with the recent numerical studies. A critical line is found for the classical plaquette system, which also corresponds to a quantum many-body wavefunction in a "plaquette liquid phase".
We consider the simplest generalizations of the valence bond physics of SU(2) singlets to SU(N) singlets that comprise objects with N sites -- these are SU(N) singlet plaquettes with N=3 and N=4 in three spatial dimensions. Specifically, we search for a quantum mechanical liquid of such objects -- a resonating singlet valence plaquette phase that generalizes the celebrated resonating valence bond phase for SU(2) spins. We extend the Rokhsar-Kivelson construction of the quantum dimer model to the simplest SU(4) model for valence plaquette dynamics on a cubic lattice. The phase diagram of the re…
The simplest quantum generalization of the six-vertex model describes fluctuations of the order parameter of the d-density wave (DDW), believed to compete with superconductivity in the high-Tc superconductors. The ground state of this model undergoes a first order transition from the DDW phase to a resonating plaquette phase as the quantum fluctuations are increased, which is explored with the help of quantum Monte Carlo simulations and analytic considerations involving the n-vector (n=2) model with cubic anisotropy. In addition to finding a new quantum state, we show that the DDW is robust ag…
We study the quantum phases of fermions with an explicit SU(N)-symmetric, Heisenberg-like nearest-neighbor flavor exchange interaction on the honeycomb lattice at half-filling. Employing projective (zero temperature) quantum Monte Carlo simulations for even values of N, we explore the evolution from a weak-coupling semimetal into the strong-coupling, insulating regime. Furthermore, we compare our numerical results to a saddle-point approximation in the large-N limit. From the large-N regime down to the SU(6) case, the insulating state is found to be a columnar valence bond crystal, with a dire…
We propose a theory of the spin dynamics of frustrated quantum antiferromagnets, which is based on an effective action for a plaquette embedded in a self-consistent bath. This approach, supplemented by a low-energy projection, is applied to the kagome antiferromagnet. We find that a spin-liquid regime extends to very low energy, in which local correlation functions have a slow decay in time, well described by a power law behaviour and $ω/T$ scaling of the response function: $χ''(ω)\propto ω^{-α}F(ω/T)$.
We examine the topological order in the resonating singlet valence plaquette (RSVP) phase of the hard-core quantum plaquette model (QPM) on the face centered cubic (FCC) lattice. To do this, we construct a Rohksar-Kivelson type Hamiltonian of local plaquette resonances. This model is shown to exhibit a $\mathbb{Z}_3$ topological order, which we show by identifying a $\mathbb{Z}_3$ topological constant (which leads to a $3^3$-fold topological ground state degeneracy on the $3$-torus) and topological point-like charge and loop-like magnetic excitations which obey $\mathbb{Z}_3$ statistics. We al…
The plaquette phase of the square lattice quantum dimer model is studied using a continuous-time reptation quantum Monte Carlo method for lattices of sizes up to 48x48 sites. We determine the location of the phase transition between the columnar and plaquette phases to occur at V_c/J=0.60 +- 0.05 which is significantly larger than inferred from previous exact diagonalization studies on smaller lattices. Offdiagonal correlation functions are obtained. They exhibit long-range order in the plaquette phase but not at the Rokhsar-Kivelson point. We also observe significant finite-size corrections t…
We present a strong-coupling approach to the theory of high-temperature superconductivity based on the observation of a quantum critical point in the plaquette within the t,t' Hubbard model. The crossing of ground state energies in the N=2,3,4 sectors occurs for parameters close to the optimal doping. The theory predicts the maximum of the d(x2-y2)-wave order parameter at the border between localized and itinerant electron behavior and gives a natural explanation for the pseudo-gap formation via soft-fermion mode related to local singlet states of the plaquette in the environment. Our approach…
The antiferromagnetic Ising model on a checkerboard lattice has an ice-like ground state manifold with extensive degeneracy. and, to leading order in J_xy, deconfined spinon excitations. We explore the role of cyclic exchange arising at order J^2_xy/J_z on the ice states and their associated spinon excitations. By mapping the original problem onto an equivalent quantum six--vertex model, we identify three different phases as a function of the chemical potential for flippable plaquettes - a phase with long range Neel order and confined spinon excitations, a non-magnetic state of resonating squa…
We study the quantum phase transition between the $Z_2$ spin liquid and valence bond solid (VBS) orders on a triangular lattice. With a fully isotropic triangular lattice, the transition from a columnar or resonating-plaquette VBS order can be either first order or there could be two transitions with an intermediate phase. If the transition splits into two, then the $Z_2$ spin liquid will first experience a first order $q=3$ Potts transition to a new nematic $Z_2$ spin liquid that breaks the $2π/3$ lattice rotation symmetry (but retain translation symmetry unlike the VBS states). The second tr…
We relate properties of nearest-neighbour resonating valence bond (nnRVB) wavefunctions for $SU(g)$ spin systems on two dimensional bipartite lattices to those of fully-packed classical dimer models with potential energy $V$ on the same lattice. We define a cluster expansion of $V$ in terms of $n$-body potentials $V_n$, which are recursively determined from the nnRVB wavefunction on {\em finite subgraphs} of the original lattice. The magnitude of the $n$-body interaction $V_n$ ($n>1$) is of order ${\mathcal O}(g^{-(n-1)})$ for small $g^{-1}$, while $V_1$ reduces to a constant due to the fully-…
We study a model of strongly correlated S=1/2 fermions on the planar pyrochlore, or checkerboard, lattice, at fractional (1/8) filling. Starting with the extended Hubbard model in the limit of strong Coulomb repulsion, low-energy configurations can be mapped onto hard-core dimer configurations whose dimers carry a spin degree of freedom. An effective Hamiltonian similar to the kinetic term of a quantum dimer model on the square lattice which rotates two parallel dimers (in a spin-singlet configuration) by 90 degrees naturally emerges. We also introduce an additional term in the Hamiltonian, a …
The power of machine learning algorithms to automatically classify different phases of matter and detect quantum phase transitions without necessity to characterize phases by various quantities like local order parameters or topological invariants as in conventional approaches defined machine learning phases of matter as a new research frontier and basic research tool in condensed matter and statistical physics. We study quantum criticality in the spin-1/2 square-lattice J1-J2 model with additional plaquette structure by combination of reinforcement and supervised machine learning techniques. …
Implementation of the hardcore-dimer Hilbert space in cold Rydberg-atom simulators opens a new route of investigating real-time dynamics of dimer liquids under Hamiltonian quench. Here, we consider an initial Resonating Valence Bond (RVB) state on the square lattice realizing a critical Coulomb phase with algebraic and dipolar correlations. Using its representation as a special point of a broad manifold of SU($2$)-symmetric, translationnally invariant, Projected Entangled Pair States (PEPS), we compute its non-equilibrium dynamics upon turning on inter-site Heisenberg interactions. We show tha…
Classification of possible quantum spin liquid (QSL) states of interacting spin-1/2's in two dimensions has been a fascinating topic of condensed matter for decades, resulting in enormous progress in our understanding of low-dimensional quantum matter. By contrast, relatively little work exists on the identification, let alone classification, of QSL phases for spin-1 systems in dimensions higher than one. Employing the powerful ideas of tensor network theory and its classification, we develop general methods for writing QSL wave functions of spin-1 respecting all the lattice symmetries, spin r…
We revisit the phase diagram of Rokhsar-Kivelson models, which are used in fields such as superconductivity, frustrated magnetism, cold bosons, and the physics of Josephson junction arrays. From an extended height effective theory, we show that one of two simple generic phase diagrams contains a mixed phase that interpolates continuously between columnar and plaquette states. For the square lattice quantum dimer model we present evidence from exact diagonalization and Green's function Monte Carlo techniques that this scenario is realised, by combining an analysis of the excitation gaps of diff…
The phase diagram of the XXZ spin-1 quantum magnet on the kagome lattice is studied for all cases where the $J_z$ coupling is antiferromagnetic. In the zero magnetic field case, the six previously introduced phases, found using various methods, are: the nondegenerate gapped photon phase which breaks no space symmetry or spin symmetry; the six-fold degenerate phase with plaquette order, which breaks both time reversal symmetry and translational symmetry; the "superfluid" (ferromagnetic) phase with an in-plane global U(1) symmetry broken, when $J_{xy} < 0$; the $\sqrt{3}\times\sqrt{3}$ order whe…
At sufficiently low temperatures, interacting electron systems tend to develop orders. Exceptions are quantum critical point (QCP) and quantum spin liquid (QSL), where fluctuations prevent the highly entangled quantum matter to an ordered state down to the lowest temperature. While the ramification of these states may have appeared in high-temperature superconductors, ultra-cold atoms, frustrated magnets and quantum Moiré materials, their unbiased presence remain elusive in microscopic two-dimensional lattice models. Here, we show by means of large-scale quantum Monte Carlo simulations of corr…
We explore the effects of artificial $U(3)$ gauge potentials on ultracold atoms. We study background gauge fields with both non-constant and constant Wilson loops around plaquettes, obtaining the energy spectra in each case. The scenario of metal-insulator transition for irrational fluxes is also examined. Finally, we discuss the effect of such a gauge potential on the superfluid-insulator transition for bosonic ultracold atoms.
We obtain the rich phase diagrams in the Hubbard model on the triangular Kagomé lattice as a function of interaction, temperature and asymmetry, by combining the cellular dynamical mean-field theory with the continuous time quantum Monte Carlo method. The phase diagrams show the asymmetry separates the critical points in Mott transition of two sublattices on the triangular Kagomé lattice and produces two novel phases called plaquette insulator with an obvious gap and a gapless Kondo metal. When the Coulomb interaction is stronger than the critical value Uc, a short range paramagnetic insulatin…
Starting from the mean-field solution of a spin-orbital model of LiNiO$_2$, we derive an effective quantum dimer model (QDM) that lives on the triangular lattice and contains kinetic terms acting on 4-site plaquettes and 6-site loops. Using numerical exact diagonalizations and Green's function Monte Carlo simulations, we show that the competition between these kinetic terms leads to a resonating valence bond (RVB) state for a finite range of parameters. We also show that this RVB phase is connected to the RVB phase identified in the Rokhsar-Kivelson model on the same lattice in the context of …
Solving strongly coupled gauge theories in two or three spatial dimensions is of fundamental importance in several areas of physics ranging from high-energy physics to condensed matter. On a lattice, gauge invariance and gauge invariant (plaquette) interactions involve (at least) four-body interactions that are challenging to realize. Here we show that Rydberg atoms in configurable arrays realized in current tweezer experiments are the natural platform to realize scalable simulators of the Rokhsar-Kivelson Hamiltonian --a 2D U(1) lattice gauge theory that describes quantum dimer and spin-ice d…
We show that a new state of matter, the d-wave Mott-insulator state (d-Mott state) (introduced recently by [H. Yao, W. F. Tsai, and S. A. Kivelson, Phys. Rev. B 76, 161104 (2007)]), which is characterized by a non-zero expectation value of a local plaquette operator embedded in an insulating state, can be engineered using ultra-cold atomic fermions in two-dimensional double-well optical lattices. We characterize and analyze the parameter regime where the $d$-Mott state is stable. We predict the testable signatures of the state in the time-of-flight measurements.
Coulomb repulsion between electrons moving on a frustrated lattice can give rise, at simple commensurate electronic densities, to exotic insulating phases of matter. Such a phenomenon is illustrated using an extended t--J model on a planar pyrochlore lattice for which the work on the quarter-filled case [cond-mat/0702367] is complemented and extended to 1/8- and 3/8-fillings. The location of the metal-insulator transition as a function of the Coulomb repulsion is shown to depend strongly on the sign of the hopping. Quite generally, the metal-insulator transition is characterized by lattice sym…
We study electrons hopping on a kagome lattice at third filling described by an extended Hubbard Hamiltonian with on-site and nearest-neighbour repulsions in the strongly correlated limit. As a consequence of the commensurate filling and the large interactions, each triangle has precisely two electrons in the effective low energy description, and these electrons form chains of different lengths. The effective Hamiltonian includes the ring exchange around the hexagons as well as the nearest-neighbor Heisenberg interaction. Using large scale exact diagonalization, we find that the effective mode…
Ever since Heisenberg's proposal of a quantum-mechanical origin of ferromagnetism in 1928, the spin model named after him has been central to advances in magnetism, featuring in proposals of novel many-body states such as antiferromagnets, emergent gauge fields in their confined (valence bond crystal) and deconfined (resonating valence bond spin liquids) versions. Between them, these cover much of our understanding of modern magnetism specifically and topological states of matter in general. Many exciting phenomena predicted theoretically still await experimental realisation, and cold atomic s…
We study the quantum magnetism of the SU(4) Mott insulator in a square optical superlattice, in which atoms with four nuclear-spin components strongly interact with each other, in the presence of an external field that controls the imbalance between the population of two components and that of the other two. This is a natural extension of the physics of spin-dimer materials under strong magnetic field. We apply an extended linear flavor-wave theory based on four-site plaquettes and unveil the ground-state phase diagram and excitation spectra. When the population of the four components is balan…
We unveil the microscopic origin of largely debated magnetism in the Mo$_{3}$O$_{8}$ cluster systems. Upon considering an extended Hubbard model at 1/6 filling on the anisotropic kagomé lattice formed by the Mo atoms, we argue that its ground state is determined by the competition between kinetic energy and intersite Coulomb interactions, which is controlled by the trimerisation of the kagomé lattice into the Mo$_{3}$O$_{13}$ clusters. Based on first-principles calculations, we show that the strong interaction limit is realised in LiZn$_{2}$Mo$_{3}$O$_{8}$ revealing a plaquette charge order wi…
We predict the robust existence of a novel quantum orbital stripe order in the $p$-band Bose-Hubbard model of two-dimensional triangular optical lattices with cold bosonic atoms. An orbital angular momentum moment is formed on each site exhibiting a stripe order both in the superfluid and Mott-insulating phases. The stripe order spontaneously breaks time-reversal, lattice translation and rotation symmetries. In addition, it induces staggered plaquette bond currents in the superfluid phase. Possible signatures of this stripe order in the time of flight experiment are discussed.
At sufficiently low temperatures, condensed-matter systems tend to develop order. An exception are quantum spin-liquids, where fluctuations prevent a transition to an ordered state down to the lowest temperatures. While such states are possibly realized in two-dimensional organic compounds, they have remained elusive in experimentally relevant microscopic two-dimensional models. Here, we show by means of large-scale quantum Monte Carlo simulations of correlated fermions on the honeycomb lattice, a structure realized in graphene, that a quantum spin-liquid emerges between the state described by…
We examine a system of doubly degenerate $p$-orbital polarized fermions on a two-dimensional square lattice with a strong on-site interaction. We consider the system density at the half filling limit and tackle the strong attractive interaction using a perturbation theory. We treat the four-site square plaquette interaction term generated from the directional tunneling dependence of $p$-orbitals using the fourth order in perturbation theory. We map the strong coupling particle Hamiltonian into an effective spin-Hamiltonian and then use a variational mean field approach and a linear spin-wave t…
Experimental realizations of topologically ordered states of matter, such as fractional quantum Hall states, with cold atoms are now within reach. In particular, optical lattices provide a promising platform for the realization and characterization of such states, where novel detection schemes enable an unprecedented microscopic understanding. Here we show that the central charge can be directly measured in current cold atom experiments using the number entropy as a proxy for the entanglement entropy. We perform density-matrix renormalization-group simulations of Hubbard-interacting bosons on …
Quantum spin ice represents a paradigmatic example on how the physics of frustrated magnets is related to gauge theories. In the present work we address the problem of approximately realizing quantum spin ice in two dimensions with cold atoms in optical lattices. The relevant interactions are obtained by weakly admixing van der Waals interactions between laser admixed Rydberg states to the atomic ground state atoms, exploiting the strong angular dependence of interactions between Rydberg p-states together with the possibility of designing step-like potentials. This allows us to implement Abeli…
