Magnetic properties of high purity stoichiometric La$_2$CuO$_4$ nanoparticles are systematically investigated as a function of particle size. Ferromagnetic single-domain spin clusters are shown to spontaneously form at the surface of fine grains as well as paramagnetic defects. Hysteresis loops and thermomagnetic irreversibility are observed in a wide temperature range $5 - 350$ K with the remnant moment and coercivity gradually decreasing with increasing temperature. Possible origins of the spontaneous surface ferromagnetic clusters and the relation of our data to the appearance of unusual magnetic phenomena and phase separation of doped cuprates are discussed.
A study of the ferromagnetic transition of $SrRuO_3$ in nanometer thick bilayers with $YBa_2Cu_3O_y$, $La_{1.88}Sr_{0.12}CuO_{4-y}$, Au and Cr: Signature of injected carriers in the pseudogap regime
Selective interlayer ferromagnetic coupling between the Cu spins in YBa$_2$ Cu$_3$ O$_{7-x}$ grown on top of La$_{0.7}$ Ca$_{0.3}$ MnO$_3$
铁磁/d波超导异质结构的研究主要集中在界面处或界面附近的影响,而忽略了体性质对异质结构的响应。本文利用共振软X射线散射谱研究了在铁磁La $_{0.7}$ Ca $_{0.3}$ MnO $_3$(LCMO)锰氧化物层上生长的YBa $_2$ Cu $_3$ O $_{7-x}$(YBCO)超导体中,面内Cu自旋之间的c轴铁磁耦合.这种耦合存在于YBCO的正常态和超导态,对界面终止敏感,仅在MnO_2界面终止的双层膜中观察到,而在La $_{0.7}$ Ca $_{0.3}$界面终止的双层膜中观察不到。这种不同的行为,我们认为,是由于不同的能量的CuO链和CuO $_2$平面在La $_{0.7}$钙$_{0.3}$和MnO $_2$终止界面,从而影响不同的自旋极化电子从锰氧化物到铜酸盐的转移。我们的研究结果表明,超导/铁磁双层膜与适当的界面工程可以很好的候选人搜索理论的Fulde-Ferrel-Larkin-Ovchinnikov(FFLO)状态在铜酸盐和研究竞争的量子级在高度相关的电子系统。
Transport and spectroscopic properties of superconductor - ferromagnet - superconductor junctions of $La_{1.9}Sr_{0.1}CuO_4$ - $La_{0.67}Ca_{0.33}MnO_3$ - $La_{1.9}Sr_{0.1}CuO_4$
Synthesis, Structure and Properties of Tetragonal Sr2M3As2O2 (M3 = Mn3, Mn2Cu and MnZn2) Compounds Containing Alternating CuO2-Type and FeAs-Type Layers
High-Temperature Charge-Stripe Correlations in La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$
我们用共振非弹性X射线散射研究了La $_{1.675}$ Eu $_{0.2}$ Sr $_{0.125}$ CuO $_4$中的电荷条纹相关。通过区分弹性和非弹性散射,它表明,电荷条纹相关性之前的结构低温tetraxide相和运输定义的pseudogap发病。从电荷条纹的散射峰振幅衰减约为$T^{-2}$对我们的检测限。然而,面内积分强度大致保持与温度无关。因此,虽然在高温下的不可逆性显示出显着的大幅度增加,我们的结果是通过一个单一的散射成分解释。事实上,与其他条纹有序化合物(La $_{1.875}$ Ba $_{0.125}$ CuO $_4$、La $_{1.475}$ Nd $_{0.4}$ Sr $_{0.125}$ CuO $_4$和La $_{1.875}$ Sr $_{0.125}$ CuO $_4$)的直接比较表明,所有这些化合物的积分散射强度大致恒定。因此,我们的研究结果提供了一个统一的图片的La为基础的铜酸盐的电荷条纹有序。当La $_{1.675}$ Eu $_{0.2}$ Sr $_{0.125}$ CuO $_4$中的电荷关联超出低温四元相和赝隙相时,它们的出现预示着该化合物中的自发对称性破缺。
Cu-spin Correlation in the Electron-overdoped High-Tc Cuprate Thin Films of La_2-x_Ce_x_CuO_4_ Probed by Low-energy Muons
Sophia University(上智大学);PSI Center for Neutron and Muon Sciences(瑞士保罗谢尔研究所中子与μ子科学中心);Institute of Materials Structure Science, High Energy Accelerator Research Organization (KEK-IMSS)(高能加速器研究机构材料结构科学研究所)
X-ray absorption spectroscopy study of the electronic and magnetic proximity effects in YBa$_2$Cu$_3$O$_{7}$/La$_{2/3}$Ca$_{1/3}$MnO$_3$ and La$_{2-x}$Sr$_x$CuO$_4$/La$_{2/3}$Ca$_{1/3}$MnO$_3$ multilayers
X-ray absorption study of the ferromagnetic Cu moment at the $\mathbf{{YBa_2Cu_3O_7}/{La_{2/3}Ca_{1/3}MnO_3}}$ interface and the variation of its exchange interaction with the Mn moment
Highly dispersive magnons with spin-gap like features in the frustrated ferromagnetic S=1/2 chain compound Ca2Y2Cu5O10 detected by inelastic neutron scattering
我们报告的非弹性中子散射实验在Ca 2 Y2 Cu 5 O 10和映射出完整的一个磁振子分散扩展到一个创纪录的值为53毫电子伏的受抑铁磁(FM)边缘共享氧化铜链(FFESC)铜酸盐。一个均匀的自旋1/2链模型与FM最近邻(NN),反铁磁(AFM)的次近邻(NNN)inchain,和两个对角AFM链间耦合(IC)内分析线性自旋波理论(LSWT)再现以及观察到的沿链和弱的垂直分散。比率R=| J_{a2} / J_{a1}| FM NN和AFM NNN耦合的平均值为~0.23,接近单链中分离铁磁和反铁磁相关螺旋磁基态的临界点Rc=1/4,而耦合链的Rc>0.25,即使对于相对较弱的IC也有相当大的上移。虽然所测量的分散体可以通过均匀LSWT来描述,但散射强度似乎在~11.5和~28 meV处大大降低。在11.5毫电子伏的间隙状功能是由于磁振子-声子耦合,而基于DMRG模拟的动态结构因子的间隙在28毫电子伏被认为是干部分从量子效应由于AFM IC。另一个贡献是归因于内在的超结构从扭曲的不相称图案的CaY阳离子链相邻的CuO 2的。它产生了不等价的CuO 4单元和Cu-O-Cu键角Φ和所有交换积分的分布。用齐次LSWT拟合的J值被视为平均值。FFESC铜酸盐中FM NN积分J1=24 meV的记录值可以用非普适Φ(不是90 °)来解释。和Cu-O键长相关的各向异性平均FM Cu-O交换K_…
Effects of hole-doping on the magnetic ground state and excitations in the edge-sharing CuO$_2$ chains of Ca$_{2+x}$Y$_{2-x}$Cu$_5$O$_{10}$
对未掺杂和空穴掺杂的Ca $_{2+x}$ Y $_{2-x}$ Cu $_5$ O $_{10}$进行了中子散射实验。先前报道,在未掺杂的Ca $_2$ Y $_2$ Cu $_5$ O $_{10}$中,沿着链存在自旋波激发的异常加宽,这主要由反铁磁链间相互作用引起[Matsuda $et$ $al.$,Phys.Rev.B63,180403(R)(2001)]。温度和空穴浓度的依赖性的磁激发的系统研究表明,磁激发软化和扩大与温度的增加或掺杂孔的$Q$方向无关。$Q$越高,加宽越大。一个典型的特征是,空穴掺杂是更有效地扩大沿链的激发。研究还表明,虽然各向异性相互作用和链间相互作用降低,但链内相互作用并不随温度的升高或掺杂而改变。在自旋玻璃相($x$ =1.5)和近无序相($x$ =1.67)中,磁激发在能量和$Q$上加宽得多。认为自旋玻璃相起源于空穴反铁磁团簇。
On the nature of the spin frustration in the CuO2 ribbon chains of LiCuVO4: Crystal structure determination at 1.6 K, magnetic susceptibility analysis and density functional evaluation of the spin exchange constants
Thermal and Magnetoelastic Properties of the van der Waals Ferromagnet Fe$_{3-δ}$GeTe$_2$: Anisotropic Spontaneous Magnetostriction and Ferromagnetic Magnon Excitations
Molecular-field-theory fits to magnetic susceptibilities of antiferromagnetic GdCu2Si2, CuO, LiCrO2, and alpha-CaCr2O4 single crystals below their Neel temperatures
Enhanced magnetoelectric effect of exactly solved spin-electron model on a doubly decorated square lattice in vicinity of a continuous phase transition
Spontaneous nonreciprocal transport in a gate-tunable ferromagnetic Rashba 2-dimensional electron gas
Laboratoire Albert Fert, CNRS, Thales, Université Paris-Saclay(阿尔贝·费尔特实验室,法国国家科学研究中心,泰雷兹集团,巴黎萨克雷大学);Helmholtz-Zentrum Berlin(柏林赫尔姆霍兹中心);Institut für Physik, Martin-Luther-Universität, Halle-Wittenberg(马丁·路德哈勒-维滕贝格大学物理研究所);Plateforme Mesures Physiques à Basses Températures, Sorbonne Université(索邦大学低温测量平台);Saha Institute of Nuclear Physics(萨哈核物理研究所);Max Planck Institute of Microstructure Physics(马克斯·普朗克微结构物理研究所)
The route of frustrated cuprates from antiferromagnetic to ferromagnetic spin-1/2 Heisenberg chains: Li2ZrCuO4 as a missing link near the quantum critical point