Using a conventional Hall-bar geometry with a micro-metal strip on top of the surface, we demonstrate an electrical coherent control of nuclear spins in an AlGaAs/GaAs semiconductor heterostructure. A breakdown of integer quantum Hall (QH) effect is utilized to dynamically polarize nuclear spins. By applying a pulse rf magnetic field with the metal strip, the quantum state of the nuclear spins shows Rabi oscillations, which is detected by measuring longitudinal voltage of the QH conductor.
Several data sets of electrical breakdown in air of single-wall carbon nanotubes (SWNTs) on insulating substrates are collected and analyzed. A universal scaling of the Joule breakdown power with nanotube length is found, which appears independent of the insulating substrates used or their thickness. This suggests the thermal resistances at the interface between SWNT and insulator, and between SWNT and electrodes, govern heat sinking from the nanotube. Analytical models for the breakdown power scaling are presented, providing an intuitive, physical understanding of the breakdown process. The e…
We have measured the electrical properties of a V2O3 thin film micro bridge at the insulator metal transition (IMT). Discontinuous jumps to lower voltages in the current voltage characteristic (IV) followed by an approximately constant voltage progression for high currents indicate an electrical breakdown of the device. In addition, the IV curve shows hysteresis and a training effect, i.e. the subsequent IV loops are different from the first IV loop after thermal cycling. Low temperature scanning electron microscopy (LTSEM) reveals that the electrical breakdown over the whole device is caused …
We have analyzed the breakdown of the quantum Hall effect in 1 micrometer wide Hall devices fabricated from an exfoliated monolayer graphene transferred on SiOx. We have observed that the deviation of the Hall resistance from its quantized value is weakly dependent on the longitudinal resistivity up to current density of 5 A/m, where the Hall resistance remains quantized even when the longitudinal resistance increases monotonously with the current. Then a collapse in the quantized resistance occurs while longitudinal resistance keeps its gradual increase. The exponential increase of the conduc…
We study high-field electrical breakdown and heat dissipation from carbon nanotube (CNT) devices on SiO2 substrates. The thermal "footprint" of a CNT caused by van der Waals interactions with the substrate is revealed through molecular dynamics (MD) simulations. Experiments and modeling find the CNT-substrate thermal coupling scales proportionally to CNT diameter and inversely with SiO2 surface roughness (~d/Δ). Comparison of diffuse mismatch modeling (DMM) and data reveals the upper limit of thermal coupling ~0.4 W/K/m per unit length at room temperature, and ~0.7 W/K/m at 600 C for the large…
Narrow gaps are formed in suspended single to few layer graphene devices using a pulsed electrical breakdown technique. The conductance of the resulting devices can be programmed by the application of voltage pulses, with a voltage of 2.5V~4.5V corresponding to an ON pulse and voltages ~8V corresponding to OFF pulses. Electron microscope imaging of the devices shows that the graphene sheets typically remain suspended and that the device conductance tends to zero when the observed gap is large. The switching rate is strongly temperature dependent, which rules out a purely electromechanical swit…
We observed a huge volume expansion of aligned single walled carbon nanotube (SWNT) arrays accompanied by structural transformation during electrical breakdown in vacuum. The SWNT arrays were assembled between prefabricated Pd source and drain electrodes of 2 μm separation on Si/SiO_2 substrate via dielectrophoresis. At high electrical field, the SWNT arrays erupt into large mushroom-like structure. Systematic studies with controlled electrical bias show that above a certain field SWNTs swell and transform to nanoparticles and flower-like structures with small volume increase. Further increase…
Our study presents experimental measurements of the contact and longitudinal voltage drops in Hall bars, as a function of the current amplitude. We are interested in the heating phenomenon which takes place before the breakdown of the quantum Hall effect, i.e. the pre-breakdown regime. Two types of samples has been investigated, at low temperature (4.2 and 1.5K) and high magnetic field (up to 13 T). The Hall bars have several different widths, and our observations clearly demonstrate that the size of the sample influences the heating phenomenon. By measuring the critical currents of both conta…
We have developed a method for electrical polarization of nuclear spins in quantum Hall systems. In a breakdown regime of odd-integer quantum Hall effect (QHE), excitation of electrons to the upper Landau subband with opposite spin polarity dynamically polarizes nuclear spins through the hyperfine interaction. The polarized nuclear spins in turn accelerate the QHE breakdown, leading to hysteretic voltage-current characteristics of the quantum Hall conductor.
A numerical study is made of current distribution in small Hall bars with disorder. It is observed, in particular, that in the Hall-plateau regime the Hall current tends to concentrate near the sample edges while it diminishes on average in the sample interior as a consequence of localization. Also reported is another numerical experiment on a related, but rather independent topic, the breakdown of the quantum Hall effect. It is pointed out that the competition of the Hall field with disorder in the sample interior, an intra-subband process, can account for both the magnitude and magnetic-fiel…
We study dynamic nuclear polarization (DNP) induced by breakdown of the fractional quantum Hall (FQH) effect. We find that voltage-current characteristics depend on current sweep rates at the quantum Hall states of Landau level filling factors $ν$ = 1, 2/3, and 1/3. The sweep rate dependence is attributed to DNP occurring in the breakdown regime of FQH states. Results of a pump and probe experiment show that the polarities of the DNP induced in the breakdown regimes of the FQH states is opposite to that of the DNP induced in the breakdown regimes of odd-integer quantum Hall states.
In samples used to maintain the US resistance standard the breakdown of the dissipationless integer quantum Hall effect occurs as a series of dissipative voltage steps. A mechanism for this type of breakdown is proposed, based on the generation of magneto-excitons when the quantum Hall fluid flows past an ionised impurity above a critical velocity. The calculated generation rate gives a voltage step height in good agreement with measurements on both electron and hole gases. We also compare this model to a hydrodynamic description of breakdown.
In samples used to maintain the US resistance standard the breakdown of the dissipationless integer quantum Hall effect occurs as a series of dissipative voltage steps. A mechanism for this type of breakdown is proposed, based on the generation of magneto-excitons when the quantum Hall fluid flows past an ionised impurity above a critical velocity. The calculated generation rate gives a voltage step height in good agreement with measurements. We also compare this model to a hydrodynamic description of breakdown.
A numerical analysis is made of the breakdown of the quantum Hall effect caused by the Hall electric field in competition with disorder. It turns out that in the regime of dense impurities, in particular, the number of localized states decreases exponentially with the Hall field, with its dependence on the magnetic and electric field summarized in a simple scaling law. The physical picture underlying the scaling law is clarified. This intra-subband process, the competition of the Hall field with disorder, leads to critical breakdown fields of magnitude of a few hundred V/cm, consistent with ob…
By studying the quantum Hall effect of stationary states with high values of injected current using a von Neumann lattice representation, we found that broadening of extended state bands due to a Hall electric field occurs and causes the breakdown of the quantum Hall effect. The Hall conductance agrees with a topological invariant that is quantized exactly below a critical field and is not quantized above a critical field. The critical field is proportional to $B^{3/2}$ and is enhanced substantially if the extended states occupy a small fraction of the system.
We studied spatial distribution of dynamic nuclear polarization (DNP) in a Hall-bar device in a breakdown regime of the quantum Hall effect (QHE). We detected nuclear magnetic resonance (NMR) signals from the polarized nuclear spins by measuring the Hall voltage $V_{xy}$ using three pairs of voltage probes attached to the conducting channel of the Hall bar. We find that the amplitude of the NMR signal depends on the position of the Hall voltage probes and that the largest NMR signal is obtained from the pair of probes farthest from the electron-injecting electrode. Combined with results on pum…
High bias electrical transport characteristics of freely suspended metallic single-walled carbon nanotubes (SWNTs) are investigated at 250-400K in vacuum and various gases. Self-heating is exploited to examine the temperature dependence of phonon transport and optical phonon decay in SWNTs. The acoustic phonon thermal conductivity of a SWNT follows ~1/T at high temperatures. Non-equilibrium optical phonon effects in suspended nanotubes decrease as the ambient temperature increases. Gas molecules assist the relaxation of hot optical phonons along the tube length and enable enhanced current flow…
Nuclear spins are polarized electrically in a breakdown regime of an odd-integer quantum Hall effect (QHE). Electron excitation to the upper Landau subband with the opposite spin polarity flips nuclear spins through the hyperfine interaction. The polarized nuclear spins reduce the spin-splitting energy and accelerate the QHE breakdown. The Knight shift of the nuclear spins is also measured by tuning electron density during the irradiation of radio-frequency magnetic fields.
We use low-temperature scanning gate microscopy (SGM) to investigate the breakdown of the quantum Hall regime in an exfoliated bilayer graphene flake. SGM images captured during breakdown exhibit intricate patterns of "hotspots" where the conductance is strongly affected by the presence of the tip. Our results are well described by a model based on quantum percolation which relates the points of high responsivity to tip-induced scattering between localized Landau levels.
We demonstrate a new method for electrical manipulation of nuclear spins utilizing dynamic nuclear polarization induced by quantum Hall effect breakdown. Nuclear spins are polarized and detected through the hyperfine interaction between a nuclear spin system and a two-dimensional electron system located at an interface of GaAs/AlGaAs single heterostructure. Coherent oscillations between the nuclear-spin quantum states are observed by measuring the longitudinal voltage of the conductor.
We present an analytical scaling theory for localization in a two-dimensional hierarchical network model that is designed to represent phase-coherent electron transport in the quantum-Hall regime. Scaling expressions for both the longitudinal and Hall resistivities are derived. In agreement with recent numerical studies, we find that the Hall resistivity is quantized in the metallic phase but diverges in the insulating phase. This suggests that the characteristics of a quantized Hall insulator can occur only in the presence of a strong dephasing mechanism.
Reentrant integer quantum Hall (RIQH) states are believed to be correlated electron solid phases, though their microscopic description remains unclear. As bias current increases, longitudinal and Hall resistivities measured for these states exhibit multiple sharp breakdown transitions, a signature unique to RIQH states. We present spatially-resolved measurements of RIQH breakdown that indicate these breakdown signatures can be ascribed to a phase boundary between broken-down and unbroken regions, spreading chirally from source and drain contacts as a function of bias current and passing voltag…
In this report we experimentally probe the non-equilibrium breakdown of the quantum Hall state in monolayer graphene by injecting a high current density ($\sim$1A/m). The measured critical currents for dissipationless transport in the vicinity of integer filling factors show a dependence on filling factor. The breakdown can be understood in terms of inter Landau level (LL) scattering resulting from mixing of wavefunctions of different LLs. To further study the effect of transverse electric field, we measured the transverse resistance between the $ν=2$ to $ν=6$ plateau transition for different …
Puzzling results obtained from torque magnetometry in the quantum Hall effect (QHE) regime are presented, and a theory is proposed for their explanation. Magnetic moment saturation, which is usually attributed to the QHE breakdown, is shown to be related to the charge redistribution across the sample.
We report on the stability of the quantum Hall plateau in wide Hall bars made from a chemically gated graphene film grown on SiC. The $ν=2$ quantized plateau appears from fields $B \simeq 5$ T and persists up to $B \simeq 80$ T. At high current density, in the breakdown regime, the longitudinal resistance oscillates with a $1/B$ periodicity and an anomalous phase, which we relate to the presence of additional electron reservoirs. The high field experimental data suggest that these reservoirs induce a continuous increase of the carrier density up to the highest available magnetic field, thus en…
With unusually slow and high-resolution sweeps of magnetic field, strong, ultra-narrow (width down to $100 {\rm μT}$) resistance peaks are observed in the regime of breakdown of the quantum Hall effect. The peaks are dependent on the directions and even the history of magnetic field sweeps, indicating the involvement of a very slow physical process. Such a process and the sharp peaks are, however, not predicted by existing theories. We also find a clear connection between the resistance peaks and nuclear spin polarization.
The high field transport characteristics of nanostructured transistors based on layered materials are not only important from a device physics perspective but also for possible applications in next generation electronics. With the growing promise of layered materials as replacements to conventional silicon technology, we study here the high current density properties of the layered material titanium trisulfide (TiS3). We observe high breakdown current densities up to 1.7 10^6 A/cm^2 in TiS3 nanoribbon-based field-effect transistors which are among the highest found in semiconducting nanomateri…
We have determined the spin-orbit scattering length of two-dimensional layered 2H-TaSe2 metallic crystals by detailed characterization of the weak anti-localization phenomena in this strong spin-orbit interaction material. By fitting the observed magneto-conductivity, the spin-orbit scattering length for 2H-TaSe2 is determined to be 17 nm in the few-layer films. This small spin-orbit scattering length is comparable to that of Pt, which is widely used to study the spin Hall effect, and indicates the potential of TaSe2 for use in spin Hall effect devices. In addition to strong spin-orbit couplin…
Reentrant integer quantum Hall (RIQH) states are believed to be correlated electron solid phases, though their microscopic description remains unclear. As bias current increases, longitudinal and Hall resistivities measured for these states exhibit multiple sharp breakdown transitions, a signature unique to RIQH states. A comparison of RIQH breakdown characteristics at multiple voltage probes indicates that these signatures can be ascribed to a phase boundary between broken-down and unbroken regions, spreading chirally from source and drain contacts as a function of bias current and passing vo…
A branch of uniformly-propagating solitary waves of planar ferromagnets is identified. The energy dispersion and structures of the solitary waves are determined for an isotropic ferromagnet as functions of a conserved momentum. With increasing momentum, their structure undergoes a transition from a form ressembling a droplet of spin-waves to a Skyrmion/anti-Skyrmion pair. An instability to the formation of these solitary waves is shown to provide a mechanism for the electric field-induced breakdown of the spin-polarized quantum Hall effect.
The integer and fractional quantum Hall states are known to break down at high dc bias, exhibiting deviation from the ideal incompressible behavior. We measure breakdown of the ν= 2, 3, 4, 5 integer and the ν= 4/3 and 5/3 fractional states in a quantum point contact (QPC) of lithographic width ~600 nm. Dependence of the critical current on magnetic field, QPC gate voltage, and QPC width are presented. Of particular interest, the critical current of the 4/3 and 5/3 fractional states shows the opposite dependence on QPC width compared to the integer states. This previously unobserved result is n…
Breakdown of the quantum Hall effect (QHE) is commonly associated with an electric field approaching the inter Landau-level (LL) Zener field, ratio of the Landau gap and cyclotron radius. Eluded in semiconducting heterostructures, in spite of extensive investigation, the intrinsic Zener limit is reported here using high-mobility bilayer graphene and high-frequency current noise. We show that collective excitations arising from electron-electron interactions are essential. Beyond a noiseless ballistic QHE regime a large superpoissonian shot noise signals the breakdown via inter-LL scattering. T…
We report quantum Hall effect breakdown of a local filling factor v_local = 1 state formed in a bulk v_bulk = 2 system in an AlGaAs/GaAs heterostructure. When a finite source-drain bias is applied across the local system, the breakdown occurs in two steps. At low bias, quantized conductance through the v_local = 1 system breaks down due to inter-edge electron tunneling. At high bias, the incompressibility of the v_local = 1 system breaks down because the spin gap closes. The two steps are resolved by combining measurements of resistively detected nuclear magnetic resonance and shot noise, whic…
We report on results of systematic numerical studies of two-dimensional electron gas systems subject to a perpendicular magnetic field, with a high Landau level partially filled by electrons. Our results are strongly suggestive of a breakdown of translational symmetry and the presence of crystalline order in the ground state. This is in sharp contrast with the physics of the lowest and first excited Landau levels, and in good qualitative agreement with earlier Hartree-Fock studies. Experimental implications of our results are discussed.
In the quantum anomalous Hall effect, quantized Hall resistance and vanishing longitudinal resistivity are predicted to result from the presence of dissipationless, chiral edge states and an insulating 2D bulk, without requiring an external magnetic field. Here, we explore the potential of this effect in magnetic topological insulator thin films for metrological applications. Using a cryogenic current comparator system, we measure quantization of the Hall resistance to within one part per million and longitudinal resistivity under 10 m$Ω$ per square at zero magnetic field. Increasing the curre…
We report the phase-space defined by the quantum Hall effect breakdown in polymer gated epitaxial graphene on SiC (SiC/G) as a function of temperature, current, carrier density, and magnetic fields up to 30T. At 2K breakdown currents ($I_c$) almost two orders of magnitude greater than in GaAs devices are observed. The phase boundary of the dissipationless state ($ρ_{xx}=0$) shows a (1-$(T/T_c)^2$) dependence and persists up to $T_c>45K$ at 29T. With magnetic field $I_c$ was found to increase $\propto B^{3/2}$ and $T_c \propto B^{1.88}$. As the Fermi energy approaches the Dirac point, the $ν=2$…
Co$_3$Sn$_2$S$_2$ is a ferromagnetic semi-metal with Weyl nodes in its band structure and a large anomalous Hall effect below its Curie temperature of 177 K. We present a detailed study of its Fermi surface and examine the relevance of the anomalous transverse Wiedemann Franz law to it. We studied Shubnikov-de Haas oscillations along two orientations in single crystals with a mobility as high as $2.7\times$10$^3$ cm$^2$V$^{-1}$s$^{-1}$ subject to a magnetic field as large as $\sim$ 60 T. The angle dependence of the frequencies is in agreement with density functional theory (DFT) calculations a…
We performed noise measurements in a two-dimensional electron gas to investigate the nonequilibrium quantum Hall effect (QHE) state. While excess noise is perfectly suppressed around the zero-biased QHE state reflecting the dissipationless electron transport of the QHE state, considerable finite excess noise is observed in the breakdown regime of the QHE. The noise temperature deduced from the excess noise is found to be of the same order as the energy gap between the highest occupied Landau level and the lowest empty one. Moreover, unexpected finite excess noise is observed at a finite source…
Electrical polarization of nuclear spins is studied in a Corbino disk under a breakdown regime of the quantum Hall effect (QHE). Since the edge channels are completely absent in the Corbino disk, we conclude that the electric current flowing in the bulk channel of a quantum Hall conductor is relevant to dynamic nuclear polarization (DNP). A pump and probe measurement demonstrates that DNP emerges near the critical voltage of the QHE breakdown. The agreement of the onset voltage of DNP with that of the QHE breakdown indicates that the underlying origin of DNP is closely related to that of the Q…
Microscopic processes giving the energy gain and loss of a two-dimensional electron system in long-range potential fluctuations are studied theoretically at the breakdown of the quantum Hall effect in the case of even-integer filling factors. The Coulomb scattering within a broadened Landau level is proposed to give the gain, while the phonon scattering to give the loss. The energy balance equation shows that the electron temperature T_e and the diagonal conductivity sigma_{xx} exhibit a bistability above the lower critical electric field E_{c1}. Calculated values of E_{c1} as well as T_e and …
The hydrodynamic equation for the spatial and temporal evolution of the electron temperature T_e in the breakdown of the quantum Hall effect at even-integer filling factors in a uniform current density j is derived from the Boltzmann-type equation, which takes into account electron-electron and electron-phonon scatterings. The derived equation has a drift term, which is proportional to j and to the first spatial derivative of T_e. Applied to the spatial evolution of T_e in a sample with an abrupt change of the width along the current direction, the equation gives a distinct dependence on the c…
Second Harmonic Hall Response in Insulators: Inter-band Quantum Geometry and Breakdown of Kleinman's Conjecture
State Key Laboratory of Quantum Functional Materials, School of Physical Science and Technology, ShanghaiTech University（上海科技大学物理科学与技术学院量子功能材料国家重点实验室）；Department of Physics, Hong Kong University of Science and Technology（香港科技大学物理系）
We used micromagnetic simulations to investigate the spatial distributions of the effective magnetic fields induced by spin chirality in crossed nanowires with three characteristic magnetic structures: a radiated-shape, an antivortex, and a uniform-like states. Our results indicate that, unlike the anomalous Hall effect, the topological Hall effect (which is related to the spin chirality) depends on both the polarity and the vorticity. Therefore, measuring the topological Hall effect can detect both the polarity and the vorticity simultaneously in crossed nanowires. This approach may be suitab…
The integer quantum Hall (QH) effects characterized by topologically quantized and nondissipative transport are caused by an electrically insulating incompressible phase that prevents backscattering between chiral metallic channels. We probed the incompressible area susceptible to the breakdown of topological protection using a scanning gate technique incorporating nonequilibrium transport. The obtained pattern revealed the filling-factor ($ν$)-dependent evolution of the microscopic incompressible structures located along the edge and in the bulk region. We found that these specific structures…
Instability of quantum anomalous Hall (QAH) effect has been studied as function of electric current and temperature in ferromagnetic topological insulator thin films. We find that a characteristic current for the breakdown of the QAH effect is roughly proportional to the Hall-bar width, indicating that Hall electric field is relevant to the breakdown. We also find that electron transport is dominated by variable range hopping (VRH) at low temperatures. Combining the current and temperature dependences of the conductivity in the VRH regime, the localization length of the QAH state is evaluated …
We report on measurements of direct spin Hall effect in a lightly n-doped GaAs channel. As spin detecting contacts we employed highly efficient ferromagnetic Fe/(Ga,Mn)As/GaAs Esaki diode structures. We investigate bias and temperature dependence of the measured spin Hall signal and evaluate the value of total spin Hall conductivity and its dependence on channel conductivity and temperature. From the results we determine skew scattering and side jump contribution to the total spin hall conductivity and compare it with the results of experiments on higher conductive n-GaAs channels[Phys. Rev. L…
We present a theory for the regime of coherent interlayer tunneling in a disordered quantum Hall bilayer at total filling factor one, allowing for the effect of static vortices. We find that the system consists of domains of polarized superfluid phase. Injected currents introduce phase slips between the polarized domains which are pinned by disorder. We present a model of saturated tunneling domains that predicts a critical current for the breakdown of coherent tunneling that is extensive in the system size. This theory is supported by numerical results from a disordered phase model in two dim…
We studied the unusual Quantum Hall Effect (QHE) near the charge neutrality point (CNP) in high-mobility graphene sample for magnetic fields up to 18 T. We observe breakdown of the delocalized QHE transport and strong increase in resistivities $ρ_{xx},|ρ_{xy}|$ with decreasing Landau level filling for $ν< 2$, where we identify two insulating regimes. For $1 \gtrsim |ν| \gtrsim 1/2$ we find an exponential increase of $ρ_{xx,xy} \sim e^{a(H-H_c)}$ within the range up to several resistance quanta $R_K$, while the Hall effect gradually disappears, consistent with the Hall insulator (HI) with local…
Based on a combination of $k \cdot p$ theory, band topology analysis and electronic structure calculations, we predict the (111) thin films of the SnTe class of three-dimensional (3D) topological crystalline insulators realize the quantum spin Hall phase in a wide range of thickness. The nontrivial topology originates from the inter-surface coupling of the topological surface states of TCI in the 3D limit. The inter-surface coupling changes sign and gives rise to topological phase transitions as a function of film thickness. Furthermore, this coupling can be strongly affected by an external el…
The control of the electronic properties of materials via the vacuum fields of cavity electromagnetic resonators is one of the emerging frontiers of condensed matter physics. We show here that the enhancement of vacuum field fluctuations in subwavelength split-ring resonators dramatically affects arguably one of the most paradigmatic quantum protectorates, namely the quantum Hall electron transport in high-mobility 2D electron gases. The observed breakdown of the topological protection of the integer quantum Hall effect is interpreted in terms of a long-range cavity-mediated electron hopping w…
Detection is most often the main impediment to reduce the number of spins in paramagnetic resonance experiments. Here we propose a new route to carry out electrically-detected spin resonance of an individual spin, placed at the edge of a quantum spin Hall insulator (QSHI). The edges of a QSHI host a one dimensional electron gas with perfect spin-momentum locking. Therefore, the spin relaxation induced by emission of an electron-hole pair at the edge state of the QSHI can generate current. Here we demonstrate that driving the system with an $AC$ signal, a nonequilibrium occupation can be induce…
