We report on far infrared measurements of interplane conductivity for underdoped single-crystal YBa2Cu3Oy in magnetic field and situate these new data within earlier work on two other high-Tc cuprate superconductors, La(2-x)SrxCuO4 and Bi2Sr2CaCu2O(8+d). The three systems have displayed apparently disparate electrodynamic responses in the Josephson vortex state formed when magnetic field H is applied parallel to the CuO2 planes. Specifically, there is discrepancy in the number and field dependence of longitudinal modes observed. We compare and contrast these findings with several models of the electrodynamics in the vortex state and suggest that most differences can be reconciled through considerations of the Josephson vortex lattice ground state as well as the c-axis and in-plane quasiparticle dissipations.
Recently a phonon exchange d - wave pairing mechanism in cuprates was proposed. The phonons are the lateral apical oxygen atoms vibrations. They generate the attractive pairing potential peaked at X point of the Brillouin zone, V (k) = exp [-2kda], where da is distance from the CuO planes. The model explains a rather paradoxical well known negative correlation of the optimal doping critical temperature Tcmax with da and increase of Tcmax with pressure. However the large disparities in Tcmax, especially in one - layer cuprate superconductors, from 39K for La2-xSrxCuO4, to 95K for HgBa2CuO4+x, c…
The interplay between charge order and superconductivity remains one of the central themes of research in quantum materials. In the case of cuprates, the coupling between striped charge fluctuations and local electromagnetic fields is especially important, as it affects transport properties, coherence and dimensionality of superconducting correlations. Here, we study the emission of coherent terahertz radiation in single-layer cuprates of the La$_{2-x}$Ba$_x$CuO$_4$ family, for which this effect is expected to be forbidden by symmetry. We find that emission vanishes for compounds in which the …
We find systematic signatures suggesting a different superconducting nature for a triple-layered cuprate Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ with respect to a double-layer through the properties of intrinsic Josephson junctions (IJJs). Our measurements on the current-voltage characteristics reveal that the $c$-axis maximum Josephson current density is sensitive to the superfluid density in outer planes while the critical temperature and the superconducting gap remain unaffected. Switching dynamics of stacked IJJs exhibit that the fluctuation in gauge-invariant phase difference of an IJJ implies…
We report on an investigation of the redistribution of interlayer coherence in the trilayer cuprate Bi2Sr2Ca2Cu3O10. The experiment is performed under the same apical-oxygen phonon excitation discussed in the past for the bilayer cuprate YBa2Cu3O6.5. In Bi2Sr2Ca2Cu3O10, we observe a similar spectral weight loss at the transverse plasma mode resonance seen in YBa2Cu3O6.5. However, this feature is not accompanied by light-enhanced interlayer coherence that was seen in YBa2Cu3O6+x, for which the transverse plasma mode is observed at equilibrium even in the normal state. These new observations off…
The hallmark of superconductivity is the rigidity of the quantum-mechanical phase of electrons, responsible for superfluid behavior and Meissner effect. The strength of the phase stiffness is set by the Josephson coupling, which is strongly anisotropic in layered superconducting cuprates. So far, THz light pulses have been efficiently used to achieve non-linear control of the out-of-plane Josephson plasma mode, whose frequency scale lies in the THz range. However, the high-energy in-plane plasma mode has been assumed to be insensitive to THz pumping. Here, we show that THz driving of both low-…
Recent measurements of charge instabilities in overdoped compounds rekindled the proposal that cuprates become superconductors by long-range order through Josephson coupling between nanoscopic charge domains. We use the theory of phase-ordering dynamics to show that incommensurate charge density waves (CDWs) are formed in the CuO planes by a series of free-energy wells separated by steep barriers. Charge oscillations in these domains give rise to a net hole-hole attraction proportional to the height of these barriers. Concomitantly, the self-consistent calculations yield localized superconduct…
Recent advances in the development of Josephson scanning tunneling spectroscopy (JSTS) have opened a new path for the exploration of unconventional superconductors. We demonstrate that the critical current, $I_c$, measured via JSTS, images the spatial form of the superconducting order parameter in $d_{x^2-y^2}$-wave superconductors around defects and in the Fulde-Ferrell-Larkin-Ovchinnikov state. Moreover, we show that $I_c$ probes the existence of phase-incoherent superconducting correlations in the pseudo-gap region of the cuprate superconductors, thus providing unprecedented insight into it…
Twisted bilayers of high-$T_c$ cuprate superconductors have been argued to form topological phases with spontaneously broken time reversal symmetry ${\cal T}$ for certain twist angles. With the goal of helping to identify unambiguous signatures of these topological phases in transport experiments, we theoretically investigate a suite of Josephson phenomena between twisted layers. We find an unusual non-monotonic temperature dependence of the critical current at intermediate twist angles which we attribute to the unconventional sign structure of the $d$-wave order parameter. The onset of the ${…
c-Axis Phase Coherence and Spin Fluctuations in Cuprates
铜酸盐的超导电性（SC）是二维的，这是一个共识。人们普遍认为，由于SC CuO_{2}（二、三、.）层次。最近的T_{c}和T12212中的电阻率测量作为施加压力的函数（Salvetat J. P.等人，欧罗巴信件：52（2000）584）表明，层间约瑟夫森耦合机制不符合数据。在这里，我们分析Andreev反射，中子散射，微波，μ子自旋弛豫，隧道和电阻率测量不同的铜氧化物，主要是，YBCO，Bi 2212和LSCO上获得的数据。分析结果表明，铜氧化物的长程相位相干性与沿c轴的反铁磁相互作用密切相关。同时，SC的面内机制似乎与沿c轴的磁相互作用没有或几乎没有关系。
Twisted interfaces between stacked van der Waals cuprate crystals enable tunable Josephson coupling between in-plane anisotropic superconducting order parameters. Employing a novel cryogenic assembly technique, we fabricate Josephson junctions with an atomically sharp twisted interface between Bi2Sr2CaCu2O8+x crystals. The Josephson critical current density sensitively depends on the twist angle, reaching the maximum value comparable to that of the intrinsic junctions at small twisting angles, and is suppressed by almost 2 orders of magnitude yet remains finite close to 45 degree twist angle. …
Imaging of order parameter induced $π$ phase shifts in cuprate superconductors by low-temperature scanning electron microscopy
利用低温扫描电子显微镜（LTSEM）研究了Nb与电子掺杂的铜酸盐Nd $_{2-x}$ Ce $_x$ CuO $_{4-y}$或空穴掺杂的铜酸盐YBa $_2$ Cu $_3$ O $_7$之间的斜坡型约瑟夫森结中的超导电流分布。在短结极限下，在零外加磁场下，双极型器件的临界电流被强烈抑制。LTSEM图像表明，这是由于约瑟夫森电流逆流在相邻的0和$π$面，这是由在铜酸盐的$d_{x^2-y^2}$序参量诱导。因此，LTSEM提供了超导序参量的符号变化的成像，这也可以应用于其他类型的约瑟夫森结。
We examine coupling interactions used to synchronize macroscopic Josephson oscillations induced in intrinsic Josephson junction (IJJ) mesa stacks made of a Bi2212 single crystal. Synchronized radiations of terahertz electromagnetic (EM) waves are detected under common voltage and current bias operations of two connected mesas with close individual radiation frequencies, while uncoupled and bimodal radiations are frequently observed in two mesas with different individual radiation frequencies. Detailed observations of the polarizations of the EM waves emitted when two mesas are biased in parall…
We demonstrate that parametric driving of suitable collective modes in cuprate superconductors results in a reflectivity $R>1$ for frequencies in the low terahertz regime. We propose to exploit this effect for the amplification of coherent terahertz radiation in a laser-like fashion. As an example, we consider the optical driving of Josephson plasma oscillations in a monolayer cuprate at a frequency that is blue-detuned from the Higgs frequency. Analogously, terahertz radiation can be amplified in a bilayer cuprate by driving a phonon resonance at a frequency slightly higher than the upper Jos…
We theoretically show that terahertz pulses with controlled amplitude and frequency can be used to switch between stable transport modes in layered superconductors, modelled as stacks of Josephson junctions. We find pulse shapes that deterministically switch the transport mode between superconducting, resistive and solitonic states. We develop a simple model that explains the switching mechanism as a destablization of the centre of mass excitation of the Josephson phase, made possible by the highly non-linear nature of the light-matter coupling.
Time-resolved synchronization analysis of stacked intrinsic Josephson junctions of a cuprate superconductor with frequency-modulated terahertz radiation spectra
Kyoto University（京都大学）；National Institute of Advanced Industrial Science and Technology (AIST)（产业技术综合研究所）
Since the discovery of high temperature superconductivity in cuprates, Josephson junction based phase-sensitive experiments are believed and used to provide the most convincing evidence for determining the pairing symmetry. Regardless of different junction materials and geometries used, quantum tunneling involved in these experiments is essentially a nanoscale process, and thus, actual experimental results are extremely sensitive to atomic details of the junction structures. The situation has led to controversial results as to the nature of the pairing symmetry of cuprates: while in-plane junc…
We show that in Pr$ _{0.5} $La$ _{0.2} $Ca$ _{0.3} $MnO$ _{3} $/YBa$ _{2} $Cu$ _{3} $O$ _{7} $ (PLCMO/YBCO) multilayers the low temperature state of YBCO is very resistive and resembles the one of a granular superconductor or a frustrated Josephson-junction network. Notably, a coherent superconducting response can be restored with a large magnetic field which also suppresses the charge-orbital order in PLCMO. This coincidence suggests that the granular superconducting state of YBCO is induced by the charge-orbital order of PLCMO. The coupling mechanism and the nature of the induced inhomogeneo…
