Asta Paloviita, Kalle-Antti Suominen, Stig Stenholm
We consider a laser induced molecular excitation process as a decay of a single energy state into a continuum. The analytic results based on Weisskopf-Wigner approach and perturbation calculations are compared with numerical wave packet results. We find that the decay model describes the excitation process well within the expected parameter region.
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We generalize the Weisskopf-Wigner theory for the line shape and transition rates of decaying states to the case of the energy-driven stochastic Schrödinger equation that has been used as a phenomenology for state vector reduction. Within the standard approximations used in the Weisskopf-Wigner analysis, and assuming that the perturbing potential inducing the decay has vanishing matrix elements within the degenerate manifold containing the decaying state, the stochastic Schrödinger equation linearizes. Solving the linearized equations, we find no change from the standard analysis in the line s…
In this paper, we use the Weisskopf-Wigner theory to study the entanglement in the state of the free-space radiation field produced from vacuum due to atomic decay. We show how bipartite entanglement is shared between different partitions of the radiation modes. We investigate the role played by the size of the partitions and their detuning with the decaying atom. The dynamics of the atom-field entanglement during the atomic decay is also briefly discussed. From this dynamics, we assert that such entanglement is the physical quantity that fix the statistical atomic decay time.
Non-Markovian dynamics of giant emitters beyond the Weisskopf-Wigner approximation
针对巨型量子发射体在标准 Weisskopf-Wigner 近似外的非马尔可夫行为，研究耦合腔阵列波导的可精确求解最小模型，揭示连续谱内外束缚态及相干叠加工程，并给出超导电路实现方案。
When a discrete state is coupled to a continuum, the dynamics can be described either by the Weisskopf-Wigner exponential decay or by the Rabi oscillation, depending on the relative magnitudes of the continuum width and of the Rabi frequency. A continuous transition between these two regimes exists, as demonstrated in 1977 by C. Cohen-Tannoudji and P. Avan. Here, we describe a fully analogous transition in classical mechanics, by studying the dynamics of two coupled mechanical oscillators in the presence of damping. By varying the relative magnitudes of the damping and coupling terms, we obser…
High entanglement regimes in the Weisskopf-Wigner theory for spontaneous decay
本文回顾 Weisskopf-Wigner 自发辐射理论，通过纯度计算发现基于初始原子动量不确定性的两个高纠缠区域：反冲纠缠与多普勒纠缠，并给出各自阈值。
The Adiabatic Wigner-Weisskopf Model
该研究提出Wigner-Weisskopf模型的时间相关推广版本，针对缓变d能级原子与光子场相互作用的单激发体系，在绝热和小耦合近似下分析不同区域的动力学，同时刻画了原子辐射衰减与场中光子激发的累积过程。
We establish the relation between the Wigner-Weisskopf theory for the description of an unstable system and the theory of coupling to an environment. According to the Wigner-Weisskopf general approach, even within the pole approximation (neglecting the background contribution) the evolution of a total system subspace is not an exact semigroup for the multi-channel decay, unless the projectors into eigesntates of the reduced evolution generator $W(z)$ are orthogonal. In this case these projectors must be evaluated at different pole locations $z_α\neq z_β$. Since the orthogonality relation does …
We extend the quantum theory of dissipation in the context of system-reservoir model, where the reservoir in question is kept in a nonequilibrium condition. Based on a systematic separation of time scales involved in the dynamics, appropriate generalizations of the fluctuation-dissipation and Einstein's relations have been pointed out. We show that the Wigner-Weisskopf decay of the system mode results in a rate constant which depending on the relaxation of nonequilibrium bath is dynamically modified. We also calculate the time-dependent spectra of a cavity mode with a suitable gain when the ca…
The Wigner-Weisskopf-type model describing the energy transfer between two centers mediated by a continuum of energy levels is studied. This work is motivated by the recent interest in transport phenomena at nanoscale in biology and quantum engineering. The analytical estimation for the energy transfer efficiency is derived in the weak coupling regime and the conditions for the almost perfect transfer are discussed. The embedding of the standard tight-binding model into Wigner-Weisskopf one which includes the environmental noise is presented.
At the dawn of Quantum Physics, Wigner and Weisskopf obtained a full analytical description (a \textit{photon portrait}) of the emission of a single photon by a two-level system, using the basis of frequency modes (Weisskopf and Wigner, "Zeitschrift für Physik", 63, 1930). A direct experimental reconstruction of this portrait demands an accurate measurement of a time resolved fluorescence spectrum, with high sensitivity to the off-resonant frequencies and ultrafast dynamics describing the photon creation. In this work we demonstrate such an experimental technique in a superconducting waveguide…
The transient Casimir-Polder force on a two-level atom introduced into a three-dimensional, inhomogeneous, generally non-reciprocal environment is evaluated using non-Markovian Weisskopf-Wigner theory in the strong and weak coupling regimes. Ground-state and excited atoms are considered as two separate initial-value problems, and both the short-time and long-time atomic population and force are evaluated. The results are compared with various Markov approximation of the Weisskopf-Wigner theory, and with previous Markov results from the Heisenberg picture.
We calculate atom-photon resonances in the Wigner-Weisskopf model, admitting two photons and choosing a particular coupling function. We also present a rough description of the set of resonances in a model for a three-level atom coupled to the photon field. We give a general picture of matter-field resonances these results fit into.
We calculate the Wigner quasi-probability distribution for position and momentum, P_W^(n)(x,p), for the energy eigenstates of the standard infinite well potential, using both x- and p-space stationary-state solutions, as well as visualizing the results. We then evaluate the time-dependent Wigner distribution, P_W(x,p;t), for Gaussian wave packet solutions of this system, illustrating both the short-term semi-classical time dependence, as well as longer-term revival and fractional revival behavior and the structure during the collapsed state. This tool provides an excellent way of demonstrating…
Using an exactly solvable model of the Wigner-Weisskopf atom it is shown that an unstable quantum state cannot be recovered completely by the procedure involving detection of the decay products followed by creation of the time reversed decay products state, as proposed in \cite{Son}. The universal lower bound on the recovery error is approximately equal to $5% $ of the \emph{error per cycle} - the dimensionless parameter characterizing decay process in the Markovian approximation. This result has consequences for the efficiency of quantum error correction procedures which are based on syndrome…
We investigate non-classical effects such as fractional revivals, squeezing and higher-order squeezing of photon-added coherent states propagating through a Kerr-like medium.The Wigner functions corresponding to these states at the instants of fractional revivals are obtained, and the extent of non-classicality quantified.
Within a plane-wave approximation in scattering, an incoming wave packet's Wigner function stays everywhere positive, which obscures such purely quantum phenomena as non-locality and entanglement. With the advent of the electron microscopes with subnanometer-sized beams one can enter a genuinely quantum regime where the latter effects become only moderately attenuated. Here we show how to probe negative values of the Wigner function in scattering of a coherent superposition of two Gaussian packets with a non-vanishing impact-parameter between them (a Schrödinger's cat state) by atomic targets.…
Asymptotic time evolution of a wave packet describing a non-relativistic particle incident on a potential barrier is considered, using the Wigner phase-space distribution. The distortion of the trasmitted wave packet is determined by two time-like parameters, given by the energy derivative of the complex transmission amplitude. The result is consistent with various definitions of the tunneling time (e.g. the Büttiker-Landauer time, the complex time and Wigner's phase time). The speed-up effect and the negative dispersion are discussed, and new experimental implications are considered.
We investigate the dynamics of a rotating Morse wave packet, appropriate for a ro-vibrating diatomic molecule. The coupling between vibrational and rotational degrees of freedom is explicated in real position space as well as in phase space Wigner distribution of a SU(2) coherent state at various dynamically evolved times. We choose the well studied $I_{2}$ molecule with the parameter values in good agrement with experiments. A quantitative measure of the angles of rotations for different angular momenta is also given.
Motivated by recent experiments, we consider a Schrödinger cat superposition of two widely separated coherent states in thermal equilibrium. The time development of our system is obtained using Wigner distribution functions. In contrast to our discussion for a two-Gaussian wave packet [Phys. Lett. A 286 (2001) 87], we find that, in the absence of dissipation, the interference term does not decay rapidly in time, but in common with the other two terms, it oscillates in time and persists for all times
We demonstrate the possibility of realizing sub-Planck-scale structures in the mesoscopic superposition of molecular wave packets involving vibrational levels. The time evolution of the wave packet, taken here as the SU(2) coherent state of the Morse potential describing hydrogen iodide molecules, produces macroscopicquantum- superposition-like states, responsible for the above phenomenon. We investigate the phase-space dynamics of the coherent state through the Wigner function approach and identify the interference phenomena behind the sub-Planck-scale structures. The optimal parameter ranges…
We study the dynamics of superposed wave packets in a specific nonlinear Hamiltonian which models the wave packet propagation in Kerr-like media and the dynamics of Bose-Einstein condensates. We show the dependence of initial wave packet superposition on fractional revival times using analysis based on the expectation values, Rényi entropy and Wigner function. We also show how the selective identification of fractional revivals using moments of appropriate observables depends on the number of wave packets present in the initial state.
The quantum clock of Salecker-Wigner-Peres is used, by performing a post-selection of the final state, to obtain average transmission and reflection times associated to the scattering of localized wave packets by static potentials in one dimension. The behavior of these average times is studied for a gaussian wave packet, centered around a tunneling wave number, incident on a rectangular barrier and, in particular, on a double delta barrier potential. The regime of opaque barriers is investigated and the results show that the average transmission time does not saturate, showing no evidence of …
No, we cannot! The concept of Wigner time delay was introduced in scattering theory to quantify the delay or advance of an incoming particle in its interaction with the scattering potential. It was assumed that this concept can be transferred to ionization considering it as a half scattering process. In the present work we show, by analyzing the corresponding wave packets, that this assumption is incorrect since the wave function of the liberated particle has to satisfy the incoming-wave boundary condition. We show that the electron released in photoionization carries no imprint of the scatter…
The analysis of wave-packet dynamics may be greatly simplified when viewed in phase-space. While harmonic oscillators are often used as a convenient platform to study wave-packets, arbitrary state preparation in these systems is more challenging. Here, we demonstrate a direct measurement of the Wigner distribution of complex photon states in an anharmonic oscillator - a superconducting phase circuit, biased in the small anharmonicity regime. We test our method on both non-classical states composed of two energy eigenstates and on the dynamics of a phase-locked wavepacket. This method requires …
Models of the spontaneous emission of photons coupled to the electronic states of quantum dots are important for understanding quantum interactions in dielectric media as applied to proposed solid-state quantum computers, single photon emitters, and single photon detectors. The characteristic lifetime of photon emission is traditionally modeled in the Weisskopf-Wigner approximation. Here we model the fully quantized spontaneous emission, including near field effects, of a photon from the excited state of a quantum dot beyond theWeisskopf-Wigner approximation. We propose the use of discretized …
Quantum versus classical quenches and the broadening of wave packets
本文分析一维势场猝灭后量子概率密度的时间演化，并与经典统计力学比较，给出谐振子情形的解析结果及自由波包展宽，借助 Wigner 函数说明 Gaussian 波包例子的特殊性。
The left-to-right motion of a free quantum Gaussian wave packet can be accompanied by the right-to-left flow of the probability density, the effect recently studied by Villanueva [Am. J. Phys. 88, 325 (2020)]. Using the Wigner representation of the wave packet, we analyze the effect in phase space, and demonstrate that its physical origin is rooted in classical mechanics.
Gouy phase and quantum interference with cross-Wigner functions for matter-waves
本研究基于cross-Wigner变换分析物质波时空干涉，发现cross-Wigner因演化时间产生Gouy相位差，并提出从双缝实验空间强度干涉项重建cross-Wigner的技术。
The time evolution of anharmonic molecular wave packets is investigated under the influence of the environment consisting of harmonic oscillators. These oscillators represent photon or phonon modes and assumed to be in thermal equilibrium. Our model explicitly incorporates the fact that in the case of a nonequidistant spectrum the rates of the environment induced transitions are different for each transition. The nonunitary time evolution is visualized by the aid of the Wigner function related to the vibrational state of the molecule. The time scale of decoherence is much shorter than that of …
The Hu-Paz-Zhang equation is a master equation for an oscillator coupled to a linear passive bath. It is exact within the assumption that the oscillator and bath are initially uncoupled . Here an exact general solution is obtained in the form of an expression for the Wigner function at time t in terms of the initial Wigner function. The result is applied to the motion of a Gaussian wave packet and to that of a pair of such wave packets. A serious divergence arising from the assumption of an initially uncoupled state is found to be due to the zero-point oscillations of the bath and not removed …
We investigate the Wigner-Weisskopf decay of a two level atom in front of an oscillating mirror. This work builds on and extends previous theoretical and experimental studies of the effects of a static mirror on spontaneous decay and resonance fluorescence. The spontaneously emitted field is inherently non-stationary due to the time-dependent boundary conditions and in order to study its spectral distribution we employ the operational definition of the spectrum of non-stationary light due to the seminal work by Eberly and Wodkiewicz. We find a rich dependence of this spectrum as well as of the…
A general problem of $2\rightarrow N_f$ scattering is addressed with all the states being wave packets with arbitrary phases. Depending on these phases, one deals with coherent states in $(3+1)$ D, vortex particles with orbital angular momentum, the Airy beams, and their generalizations. A method is developed in which a number of events represents a functional of the Wigner functions of such states. Using width of a packet $σ_p/\langle p\rangle$ as a small parameter, the Wigner functions, the number of events, and a cross section are represented as power series in this parameter, the first non…
We investigate the interaction between a single atom and optical pulses in a coherent state with a controlled temporal envelope. In a comparison between a rising exponential and a square envelope, we show that the rising exponential envelope leads to a higher excitation probability for fixed low average photon numbers, in accordance to a time-reversed Weisskopf-Wigner model. We characterize the atomic transition dynamics for a wide range of the average photon numbers, and are able to saturate the optical transition of a single atom with ~50 photons in a pulse by a strong focusing technique. Fo…
The time evolution of a quantum wave packet in the linear gravity potential is known as Quantum Bouncing Ball. The qBounce collaboration recently observed such a system by dropping wave packets of ultracold neutrons by a height of roughly 30 microns. In this article, space and momentum spectra as well as Wigner functions of the neutron wave functions in the gravitational field of the Earth are analyzed. We investigate the quantum states in the "preparation region", into which they transition after exiting a narrow double-mirror system and where we would expect to observe free fall and bounces …
The radiation emitted by a single-electron wave packet in an intense laser field is considered. A relation between the exact quantum formulation and its classical counterpart is established via the electron's Wigner function. In particular we show that the wave packet, even when it spreads to the scale of the wavelength of the driving laser field, cannot be treated as an extended classical charge distribution but rather behaves as a point-like emitter carrying information on its initial quantum state. We outline an experimental setup dedicated to put this conclusion to the test.
The density matrix of a nonrelativistic wave-packet in an arbitrary, one-dimensional and time-dependent potential can be reconstructed by measuring hydrodynamical moments of the Wigner distribution. An n-th order Taylor polynomial in the off-diagonal variable is obtained by measuring the probability distribution at n+1 discrete time values.
Dark-state induced trapping law in single-photon emission from multiple quantum emitters
本研究揭示了多量子发射体系统中暗态诱导的普遍俘获定律，该定律仅取决于激发与总发射体数量之比，可强烈抑制单光子集体发射。
The quantum evolution of the Wigner function for Gaussian wave packets generated by a non-Hermitian Hamiltonian is investigated. In the semiclassical limit $\hbar\to 0$ this yields the non-Hermitian analog of the Ehrenfest theorem for the dynamics of observable expectation values. The lack of Hermiticity reveals the importance of the complex structure on the classical phase space: The resulting equations of motion are coupled to an equation of motion for the phase space metric---a phenomenon having no analog in Hermitian theories.
We have implemented the gedanken experiment of an individual atom scattering a wave packet of near-resonant light, and measured the associated Wigner time-delay as a function of the frequency of the light. In our apparatus the atom behaves as a two-level system and we have found delays as large as 42 nanoseconds at resonance, limited by the lifetime of the excited state. This delay is an important parameter in the problem of collective near-resonant scattering by an ensemble of interacting particles, which is encountered in many areas of physics.
The semiclassical long-time limit of free evolution of quantum wave packets on the torus is under consideration. Despite of simplicity of this system, there are still open questions concerning the detailed description of the evolution on time scales beyond the Ehrenfest time. One of the approaches is based on the limiting Wigner or Husimi distributions of time-evolved wave packets as the Planck constant tends to zero and time tends to infinity. We derive explicit expressions for semiclassical measures corresponding to all time scales and the corresponding stages of evolution: classical-like mo…
Second-order nonlocal shifts of scattered wave-packets: What can be measured by Goos-Hänchen and Imbert-Fedorov effects ?
研究任意色散波包在表面散射中的二阶非局域效应，提出新动量、频率位移及脉冲宽度收缩，并阐明其与介电函数测量的关系。
We present a method to extract the phase shift of a scattering process using the real-time evolution in the early and intermediate stages of the collision in order to estimate the time delay of a wave packet. This procedure is convenient when using noisy quantum computers for which the asymptotic out-state behavior is unreachable. We demonstrate that the challenging Fourier transforms involved in the state preparation and measurements can be implemented in $1+1$ dimensions with current trapped ion devices and IBM quantum computers. We compare quantum computation of the time delays obtained in …
The structure of time-dependent Gaussian solutions for the Kostin equation in dissipative quantum mechanics is analyzed. Expanding the generic external potential near the center of mass of the wave packet, one conclude that: the center of mass follows the dynamics of a classical particle under the external potential and a damping proportional to the velocity; the width of the wave packet satisfy a non-conservative Pinney equation. An appropriate perturbation theory is developed for the free particle case, solving the long standing problem of finding analytic expressions for square integrable s…
The tunneling dynamics in relativistic strong-field ionization is investigated with the aim to develop an intuitive picture for the relativistic tunneling regime. We demonstrate that the tunneling picture applies also in the relativistic regime by introducing position dependent energy levels. The quantum dynamics in the classically forbidden region features two time scales, the typical time that characterizes the probability density's decay of the ionizing electron under the barrier (Keldysh time) and the time interval which the electron spends inside the barrier (Eisenbud-Wigner-Smith tunneli…
The semiclassically scaled time-dependent multi-particle Schrödinger equation describes, inter alia, quantum dynamics of nuclei in a molecule. It poses the combined computational challenges of high oscillations and high dimensions. This paper reviews and studies numerical approaches that are robust to the small semiclassical parameter. We present and analyse variationally evolving Gaussian wave packets, Hagedorn's semiclassical wave packets, continuous superpositions of both thawed and frozen Gaussians, and Wigner function approaches to the direct computation of expectation values of observabl…
Negative transit time in non-tunneling electron transmission through graphene multilayers
该研究利用第一性原理散射理论分析电子穿过石墨烯等原子级薄膜的阿秒动力学，发现面内散射可导致负渡越时间，并揭示共振处 Wigner 延迟发散及低损耗时序操控机制。
The electron dynamics in the classically forbidden region during relativistic tunnel-ionization is investigated. The classical forbidden region in the relativistic regime is identified by defining a gauge invariant total energy operator. Introducing position dependent energy levels inside the tunneling barrier, we demonstrate that the relativistic tunnel-ionization can be well described by a one-dimensional intuitive picture. This picture predicts that, in contrast to the well-known nonrelativistic regime, the ionized electron wave packet arises with a momentum shift along the laser's propagat…
The decay of the overlap between a wave packet evolved with a Hamiltonian H and the same state evolved with H}+$Σ$ serves as a measure of the decoherence time $τ_ϕ$. Recent experimental and analytical evidence on classically chaotic systems suggest that, under certain conditions, $τ_ϕ$ depends on H but not on $Σ$. By solving numerically a Hamiltonian model we find evidence of that property provided that the system shows a Wigner-Dyson spectrum (which defines quantum chaos) and the perturbation exceeds a crytical value defined by the parametric correlations of the spectra.
Coherent motion of cold atoms in a standing-wave field is interpreted as a propagation in two optical potentials. It is shown that the wave-packet dynamics can be either regular or chaotic with transitions between these potentials after passing field nodes. Manifestations of de Broglie-wave chaos are found in the behavior of the momentum and position probabilities and the Wigner function. The probability of those transitions depends on the ratio of the squared detuning to the Doppler shift and is large in that range of the parameters where the classical motion is shown to be chaotic.
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