We investigated the preservation of information encoded into the relative phase and amplitudes of optical pulses during storage and retrieval in an optical memory based on stimulated photon echo. By interfering photon echoes produced in a Ti-indiffused single-mode Er-doped LiNbO$_{3}$ waveguiding structure at telecom wavelength, we found that decoherence in the atomic medium translates only as losses (and not as degradation) of information, as long as the data pulse series is short compared to the atomic decoherence time. The experimentally measured value of the visibility for interfering echoes is close to 100 %. In addition to the expected three-pulse photon-echo interferences we also observed interference due to a four-pulse photon echo. Our findings are of particular interest for future long-distance quantum communication protocols, which rely on the reversible transfer of quantum states between light and atoms with high fidelity.
Using on-demand coherence conversion via optical locking in conventional stimulated (three-pulse) photon echoes, ultralong, ultraefficient photon storage has been observed in a rare-earth Pr3+ doped Y2SiO5, where storage time is several orders of magnitude longer and retrieval efficiency is enhanced by fifty times. Compared with the same method applied to two-pulse photon echoes for a rephasing halt, use of spectral grating in the stimulated photon echoes offers a phase-independent coherence conversion between optical and spin states. Eventually an ultralong spin population decay-dependent pho…
We show experimentally and describe theoretically how a conventional magnetic resonance Hahn echo sequence can lead to a self-stimulated pulse echo train when an inhomogeneously broadened spin ensemble is coupled to a resonator. Effective strong coupling between the subsystems assures that the first Hahn echo can act as a refocussing pulse on the spins, leading to self-stimulated secondary echoes. Within the framework of mean field theory, we show that this process can continue multiple times leading to a train of echoes. We introduce an analytical model that explains the shape of the first ec…
To overcome fundamental limitations of the πoptical pulse-induced population inversion and optical decay-caused short storage time in conventional photon echoes, a coherent control of collective atoms is studied for inversion-free, optical decay-halted photon echoes, where the constraint of photon storage time is now replaced by a spin population decay process. Using phase-controlled double rephasing, an inversion-free photon echo scheme is obtained, where no spontaneous or stimulated emission-driven quantum noise exists. Thus, the present method can be applied for ultralong quantum memories i…
We experimentally demonstrate and systematically study the stimulated revival (echo) of motional wave packet oscillations. For this purpose, we prepare wave packets in an optical lattice by non-adiabatically shifting the potential and stimulate their reoccurence by a second shift after a variable time delay. This technique, analogous to spin echoes, enables one even in the presence of strong dephasing to determine the coherence time of the wave packets. We find that for strongly bound atoms it is comparable to the cooling time and much longer than the inverse of the photon scattering rate.
Fidelity serves as a benchmark for the relieability in quantum information processes, and has recently atracted much interest as a measure of the susceptibility of dynamics to perturbations. A rich variety of regimes for fidelity decay have emerged. The purpose of the present review is to describe these regimes, to give the theory that supports them, and to show some important applications and experiments. While we mention several approaches we use time correlation functions as a backbone for the discussion. Vanicek's uniform approach to semiclassics and random matrix theory provides an import…
It is proved that a qubit encoded in excited states of a V-type quantum system cannot be perfectly transferred to the state of the cavity field mode using a single rectangular laser pulse. This obstacle can be overcome by using a two-stage protocol, in which the fidelity of a state-mapping operation can be increased to nearly one.
Photon echo is a fundamental tool for the manipulation of electromagnetic fields. Unavoidable spontaneous emission noise is generated in this process due to the strong rephasing pulse, which limits the achievable signal-to-noise ratio and represents a fundamental obstacle towards their applications in the quantum regime. Here we propose a noiseless photon-echo protocol based on a four-level atomic system. We implement this protocol in a Eu3+:Y2SiO5bcrystal to serve as an optical quantum memory. A storage fidelity of 0.952 is obtained for time-bin qubits encoded with single-photon-level coheren…
We developed single-shot shaped pulses for ultra high fidelity (UH-fidelity) population transfer on a 3-level quantum system in lambda configuration. To ensure high fidelity, we use the Lewis-Riesenfeld (L-R) method to derive a family of solutions leading to an exact transfer, where the solutions follow a single dynamical mode of the L-R invariant. Among this family, we identify a tracking solution with a single parameter to control simultaneously the fidelity of the transfer, the population of the excited state, and robustness. We define a measure of the robustness of an UH-fidelity transfer …
We introduce a high-fidelity technique for coherent control of three-state quantum systems, which combines two popular control tools --- stimulated Raman adiabatic passage (STIRAP) and composite pulses. By using composite sequences of pairs of partly delayed pulses with appropriate phases the nonadiabatic transitions, which prevent STIRAP from reaching unit fidelity, can be canceled to an arbitrary order by destructive interference, and therefore the technique can be made arbitrarily accurate. The composite phases are given by simple analytic formulas, and they are universal for they do not de…
We present an improvement to the cross resonance gate realized with the addition of resonant, target rotary pulses. These pulses, applied directly to the target qubit, are simultaneous to and in phase with the echoed cross resonance pulses. Using specialized Hamiltonian error amplifying tomography, we confirm a reduction of error terms with target rotary -- directly translating to improved two-qubit gate fidelity. Beyond improvement in the control-target subspace, the target rotary reduces entanglement between target and target spectators caused by residual quantum interactions. We further cha…
Accurate control of a quantum system is a fundamental requirement in many areas of modern science ranging from quantum information processing to high-precision measurements. A significantly important goal in quantum control is to prepare a desired state as fast as possible with sufficiently high fidelity allowed by available resources and experimental constraints. Stimulated Raman adiabatic passage (STIRAP) is a robust way to realize high-fidelity state transfer but it requires a sufficiently long operation time to satisfy the adiabatic criteria. We here theoretically propose and then experime…
This paper reexamines the results of Cummings in which the quantum mechanical two-level-system (TLS) interacts with the electromagnetic field with various initial distributions and extends that work for both resonant and non-resonant to times large enough to display multiple photon echoes. The results presented here include the initial pure coherent state, the field whose initial density matrix is the Gaussian superposition of coherent states (blackbody radiation) and density matrices of the field represented by various combinations of mixed coherent and thermal states with and without squeezi…
In this paper we review our recent work on the theoretical approach to quantum Loschmidt echoes, i.e. various properties of the so called echo dynamics -- the composition of forward and backward time evolutions generated by two slightly different Hamiltonians, such as the state autocorrelation function (fidelity) and the purity of a reduced density matrix traced over a subsystem (purity fidelity). Our main theoretical result is a linear response formalism, expressing the fidelity and purity fidelity in terms of integrated time autocorrelation function of the generator of the perturbation. Surp…
We define a quantity, the so-called purity fidelity, which measures the rate of dynamical irreversibility due to decoherence, observed e.g in echo experiments, in the presence of an arbitrary small perturbation of the total (system + environment) Hamiltonian. We derive a linear response formula for the purity fidelity in terms of integrated time correlation functions of the perturbation. Our relation predicts, similarly to the case of fidelity decay, faster decay of purity fidelity the slower decay of time correlations is. In particular, we find exponential decay in quantum mixing regime and f…
Stimulated Raman adiabatic passage (STIRAP), driven with pulses of optimum shape and delay has the potential of reaching fidelities high enough to make it suitable for fault-tolerant quantum information processing. The optimum pulse shapes are obtained upon reduction of STIRAP to effective two-state systems. We use the Dykhne-Davis-Pechukas (DDP) method to minimize nonadiabatic transitions and to maximize the fidelity of STIRAP. This results in a particular relation between the pulse shapes of the two fields driving the Raman process. The DDP-optimized version of STIRAP maintains its robustnes…
We show how to reach high fidelity NOON states with a high count rate inside optical interferometers. Recently it has been shown that by mixing squeezed and coherent light at a beamsplitter it is possible to generate NOON states of arbitrary N with a fidelity as high as 94%. (Afek I. et al. Science 328, 879 (2010)). The scheme is based on higher order interference between "quantum" down-converted light and "classical" coherent light. However, this requires optimizing the amplitude ratio of classical to quantum light thereby limiting the overall count rate for the interferometric super-resoluti…
We propose a simple technique for the generation of arbitrary-sized Dicke states in a chain of trapped ions. The method uses global addressing of the entire chain by two pairs of delayed but partially overlapping laser pulses to engineer a collective adiabatic passage along a multi-ion dark state. Our technique, which is a many-particle generalization of stimulated Raman adiabatic passage (STIRAP), is decoherence-free with respect to spontaneous emission and robust against moderate fluctuations in the experimental parameters. Furthermore, because the process is very rapid, the effects of heati…
We show that optimal universal cloning of the polarization state of photons can be achieved via stimulated emission in three-level systems, both of the Lambda and the V type. We establish the equivalence of our systems with coupled harmonic oscillators, which permits us to analyze the structure of the cloning transformations realized. These transformations are shown to be equivalent to the optimal cloning transformations for qubits discovered by Buzek and Hillery, and Gisin and Massar. The down-conversion cloner discovered previously by some of the authors is obtained as a limiting case. We de…
We show theoretically that the multi-photon states obtained by cloning single-photon qubits via stimulated emission can be distinguished with the naked human eye with high efficiency and fidelity. Focusing on the "micro-macro" situation realized in a recent experiment [F. De Martini, F. Sciarrino, and C. Vitelli, Phys. Rev. Lett. 100, 253601 (2008)], where one photon from an original entangled pair is detected directly, whereas the other one is greatly amplified, we show that performing a Bell experiment with human-eye detectors for the amplified photon appears realistic, even when losses are …
In Echo experiments, imperfect time-reversal operations are performed on a subset of the total number of degrees of freedom. To capture the physics of these experiments, we introduce a partial fidelity, the Boltzmann echo, where only part of the system's degrees of freedom can be time-reversed. We present a semiclassical calculation of the Boltzmann echo. We show that, as the time-reversal operation is performed more and more accurately, the decay rate of the Boltzmann echo saturates at a value given by the decoherence rate of the controlled degrees of freedom due to their coupling to uncontro…
Dynamic stimulated emission for deterministic addition and subtraction of propagating photons
The University of Sydney（悉尼大学）；Sydney Quantum Academy（悉尼量子学院）；Institute for Photonics and Optical Sciences (IPOS)（光子与光学科学研究所）；California Institute of Technology（加州理工学院）；Moore Laboratory of Engineering（摩尔工程实验室）；Institute for Quantum Information and Matter（量子信息与物质研究所）
We present an analytic description of the effects of dephasing processes on stimulated Raman adiabatic passage in a tripod quantum system. To this end, we develop an effective two-level model. Our analysis makes use of the adiabatic approximation in the weak dephasing regime. An effective master equation for a two-level system formed by two dark states is derived, where analytic solutions are obtained by utilizing the Demkov-Kunike model. From these, it is found that the fidelity for the final coherent superposition state decreases exponentially for increasing dephasing rates. Depending on the…
Entanglement between a quantum system and its environment leads to loss of coherence in the former. In general, the temporal fate of coherences is complicated. Here, we establish the connection between decoherence of a central system and fidelity decay in the environment for a variety of situations, including both, energy conserving and dissipative couplings. We show how properties of unitary time evolution of the environment can be inferred from the non-unitary evolution of coherences in the central system. This opens up promising ways for measuring Loschmidt echoes in a variety of situations…
Although perfect copying of unknown quantum systems is forbidden by the laws of quantum mechanics, approximate cloning is possible. A natural way of realizing quantum cloning of photons is by stimulated emission. In this context the fundamental quantum limit to the quality of the clones is imposed by the unavoidable presence of spontaneous emission. In our experiment a single input photon stimulates the emission of additional photons from a source based on parametric down-conversion. This leads to the production of quantum clones with near optimal fidelity. We also demonstrate universality of …
Controlled phase (CPHASE) gates can in principle be realized with trapped neutral atoms by making use of the Rydberg blockade. Achieving the ultra-high fidelities required for quantum computation with such Rydberg gates is however compromised by experimental inaccuracies in pulse amplitudes and timings, as well as by stray fields that cause fluctuations of the Rydberg levels. We report here a comparative study of analytic and numerical pulse sequences for the Rydberg CPHASE gate that specifically examines the robustness of the gate fidelity with respect to such experimental perturbations. Anal…
Limits to Rydberg gate fidelity that arise from the entanglement of internal states of neutral atoms with the motional degrees of freedom due to the momentum kick from photon absorption and re-emission is quantified. This occurs when the atom is in a superposition of internal states but only one of these states is manipulated by visible or UV photons. The Schrödinger equation that describes this situation is presented and two cases are explored. In the first case, the entanglement arises because the spatial wave function shifts due to the separation in time between excitation and stimulated em…
Large-scale quantum information processing networks will most probably require the entanglement of distant systems that do not interact directly. This can be done by performing entangling gates between standing information carriers, used as memories or local computational resources, and flying ones, acting as quantum buses. We report the deterministic entanglement of two remote transmon qubits by Raman stimulated emission and absorption of a traveling photon wavepacket. We achieve a Bell state fidelity of 73 %, well explained by losses in the transmission line and decoherence of each qubit.
The tantalizing promise of quantum computational speedup in solving certain problems has been strongly supported by recent experimental evidence from a high-fidelity 53-qubit superconducting processor1 and Gaussian boson sampling (GBS) with up to 76 detected photons. Analogous to the increasingly sophisticated Bell tests that continued to refute local hidden variable theories, quantum computational advantage tests are expected to provide increasingly compelling experimental evidence against the Extended Church-Turing thesis. In this direction, continued competition between upgraded quantum har…
We present mirror and beamsplitter pulse designs that improve the fidelity of atom interferometry and increase its tolerance of systematic inhomogeneities. These designs are demonstrated experimentally with a cold thermal sample of $^{85}$Rb atoms. We first show a stimulated Raman inversion pulse design that achieves a ground hyperfine state transfer efficiency of 99.8(3)%, compared with a conventional $π$ pulse efficiency of 75(3)%. This inversion pulse is robust to variations in laser intensity and detuning, maintaining a transfer efficiency of 90% at detunings for which the $π$ pulse fideli…
