The traversal of an elliptically polarized optical field through a thermal vapour cell can give rise to a rotation of its polarization axis. This process, known as polarization self-rotation (PSR), has been suggested as a mechanism for producing squeezed light at atomic transition wavelengths. In this paper, we show results of the characterization of PSR in isotopically enhanced Rubidium-87 cells, performed in two independent laboratories. We observed that, contrary to earlier work, the presence of atomic noise in the thermal vapour overwhelms the observation of squeezing. We present a theory that contains atomic noise terms and show that a null result in squeezing is consistent with this theory.
We demonstrate experimentally the delay of squeezed light and entanglement using Electromagnetically Induced Transparency (EIT) in a rubidium vapour cell. We perform quadrature amplitude measurements of the probe field and find no appreciable excess noise from the EIT process. From an input squeezing of 3.1 dB at low sideband frequencies, we observed the survival of 2 dB of squeezing at the EIT output. By splitting the squeezed light on a beam-splitter, we generated biased entanglement between two beams. We transmit one of the entangled beams through the EIT cell and correlate the quantum stat…
We report on the use of parametric excitation to coherently manipulate the collective spin state of an atomic vapour at room temperature. Signatures of the parametric excitation are detected in the ground-state spin evolution. These include the excitation spectrum of the atomic coherences, which contains resonances at frequencies characteristic of the parametric process. The amplitudes of the signal quadratures show amplification and attenuation, and their noise distribution is characterized by a strong asymmetry, similarly to those observed in mechanical oscillators. The parametric excitation…
We analyse a novel squeezing and entangling mechanism which is due to correlated Stokes and anti-Stokes photon forward scattering in a multi-level atom vapour. Following the proposal we present an experimental demonstration of 3.5 dB pulsed frequency nondegenerate squeezed (quadrature entangled) state of light using room temperature caesium vapour. The source is very robust and requires only a few milliwatts of laser power. The squeezed state is generated in the same spatial mode as the local oscillator and in a single temporal mode. The two entangled modes are separated by twice the Zeeman fr…
When linearly polarized light propagates through a medium in which elliptically polarized light would undergo self-rotation, squeezed vacuum can appear in the orthogonal polarization. A simple relationship between self-rotation and the degree of vacuum squeezing is developed. Taking into account absorption, we find the optimum conditions for squeezing in any medium that can produce self-rotation. We then find analytic expressions for the amount of vacuum squeezing produced by an atomic vapor when light is near-resonant with a transition between various low-angular-momentum states. Finally, we …
We show that it is possible to generate continuous-wave fields and pulses of polarization squeezed light by sending classical, linearly polarized laser light twice through an atomic sample which causes an optical Faraday rotation of the field polarization. We characterize the performance of the process, and we show that an appreciable degree of squeezing can be obtained under realistic physical assumptions.
We report the generation of optical squeezed vacuum states by means of polarization self-rotation in rubidium vapor following a proposal by Matsko et al. [Phys. Rev. A 66, 043815 (2002)]. The experimental setup, involving in essence just a diode laser and a heated rubidium gas cell, is simple and easily scalable. A squeezing of 0.85+-0.05 dB was achieved.
We observed squeezed vacuum light at 795 nm in 87Rb vapor via resonant polarization self-rotation, and report noise sidebands suppression of ~1 dB below shot noise level spanning from acoustic (30 kHz) to MHz frequencies. This is the first demonstration of sub-MHz quadrature vacuum squeezing in atomic systems. The spectral range of observed squeezing matches well typical bandwidths of electromagnetically induced transparency (EIT) resonances, making this simple technique for generation of optical fields with non-classical statistics at atomic transitions wavelengths attractive for EIT-based qu…
We present experimental and theoretical analysis of quantum fluctuation in a vacuum field in the presence of orthogonal linearly polarized pump field propagating through a Rb vapor cell. Previously reported theoretical and experimental studies provided somewhat contradictory conclusions regarding the possibility to observe the "squeezed vacuum" -- the reduction of vacuum fluctuations below standard quantum limit -- in this system. Here, using the D1 transitions of Rb in a cell without buffer as as an example, we demonstrate that vacuum squeezing is corrupted by incoherent processes (such as sp…
In a series of articles we studied the quantum properties of a degenerate optical parametric oscillator tuned to the first family of transverse modes at the subharmonic. We found that, for a cavity having rotational symmetry respect to the optical axis, a TEM$_{10}$ mode with an arbitrary orientation in the transverse plane is emitted above threshold. We proved then that quantum noise induces a random rotation of this bright TEM$_{10}$ mode in the transverse plane, while the mode orthogonal to it, the so-called dark mode, has perfect quadrature squeezing irrespective of the distance to thresho…
We propose a new method of spin squeezing of atomic spin, based on the interactions between atoms and off-resonant light which are known as paramagnetic Faraday rotation and fictitious magnetic field of light. Since the projection process, squeezed light, or special interactions among the atoms are not required in this method, it can be widely applied to many systems. The attainable range of the squeezing parameter is S^{-2/5}, where S is the total spin, which is limited by additional fluctuations imposed by coherent light and the spherical nature of the spin distribution.
We present a theoretical study of an ensemble of X-like 4-level atoms placed in an optical cavity driven by a linearly polarized field. We show that the self-rotation (SR) process leads to polarization switching (PS). Below the PS threshold, both the mean field mode and the orthogonal vacuum mode are squeezed. We provide a simple analysis of the phenomena responsible for the squeezing and trace the origin of vacuum squeezing not to SR, but to crossed Kerr effect induced by the mean field. Last, we show that this vacuum squeezing can be interpreted as polarization squeezing.
Planar squeezed states, i.e. quantum states which are squeezed in two orthogonal spin components, have recently attracted attention due to their applications in atomic interferometry and quantum information [Q. Y. He et al, New J. Phys. 14, 093012 (2012)]. While canonical variables such as quadratures of the radiation field can be squeezed in at most one component, simultaneous squeezing in two orthogonal spin components can be achieved due to the angular momentum commutation relations. We present a novel scheme for planar squeezing via quantum non-demolition (QND) measurements in spin-1 syste…
Semiclassical catastrophes in the dynamics of a quantum rotor (molecule) driven by a strong time-varying field are considered. We show that for strong enough fields, a sharp peak in the rotor angular distribution can be achieved via time-domain focusing phenomenon, followed by the formation of angular rainbows and glory-like angular structures. Several scenarios leading to the enhanced angular squeezing are proposed that use specially designed and optimized sequences of pulses. The predicted effects can be observed in many processes, ranging from molecular alignment (orientation) by laser fiel…
We demonstrate compact and accessible squeezed-light magnetometry using four-wave mixing in a single hot rubidium vapor cell. The strong intrinsic coherence of the four wave mixing process results in nonlinear magneto-optical rotation (NMOR) on each mode of a two mode relative-intensity squeezed state. This framework enables 4.7 dB of quantum noise reduction while the opposing polarization rotation signals of the probe and conjugate fields add to increase the total signal to noise ratio.
We report the demonstration of a magnetometer with noise-floor reduction below the shot-noise level. This magnetometer, based on a nonlinear magneto-optical rotation effect, is enhanced by the injection of a squeezed vacuum state into its input. The noise spectrum shows squeezed noise reduction of about 2 dB spanning from close to 100 Hz to several megahertz. We also report on the observation of two different regimes of operation of such a magnetometer: one in which the detection noise is limited by the quantum noise of the light probe only, and one in which we see additional noise originating…
We consider an ensemble of trapped atoms interacting with a continuous wave laser field. For sufficiently polarized atoms and for a polarized light field, we may approximate the non-classical components of the collective spin angular momentum operator for the atoms and the Stokes vectors of the field by effective position and momentum variables for which we assume a gaussian state. Within this approximation, we present a theory for the squeezing of the atomic spin by polarization rotation measurements on the probe light. We derive analytical expressions for the squeezing with and without inclu…
We propose a method to achieve quantum supremacy using ensembles of qubits, using only spin squeezing, basis rotations, and Fock state measurements. Each ensemble is assumed to be controllable only with its total spin. Using a repeated sequence of random basis rotations followed by squeezing, we show that the probability distribution of the final measurements quickly approaches a Porter-Thomas distribution. We show that the sampling probability can be related to a #P-hard problem with a complexity scaling as $(N+1)^M$, where $N$ is the number of qubits in an ensemble and $ M $ is the number of…
Large optical nonlinearities can have numerous applications, ranging from the generation of cat-states for optical quantum computation, through to quantum sensing where the sensitivity exceeds Heisenberg scaling in the resources. However, the generation of ultra-large optical nonlinearities has proved immensely challenging experimentally. We describe a novel protocol where one can effectively generate large optical nonlinearities via the conditional application of a linear operation on an optical mode by an ancilla mode, followed by a measurement of the ancilla and corrective operation on the …
Broadband quantum noise reduction can be achieved in gravitational wave detectors by injecting frequency dependent squeezed light into the the dark port of the interferometer. This frequency dependent squeezing can be generated by combining squeezed light with external filter cavities. However, in future long baseline interferometers (LBIs), the filter cavity required to achieve the broadband squeezing has a low bandwidth -- necessitating a very long cavity to mitigate the issue from optical loss. It has been shown recently that by taking advantage of Einstein-Podolsky-Rosen (EPR) entanglement…
We have studied the intensity correlations between two orthogonally linearly polarized components of a laser field propagating through a resonant atomic medium. These experiments have been performed in a Rubidium atomic vapor. We observe that the correlations between the orthogonally polarized components of the laser beam are maximal in the absence of a magnetic field. The magnitude of the correlations depends on the applied magnetic field, and the magnitude first decreases and then increases with increasing magnetic field. Minimal correlations and maximal rotation angles are observed at the s…
Cavities with extremely narrow linewidth of 10-100 Hz are required for realizing frequency dependent squeezing to enable gravitational wave detectors to surpass the free mass standard quantum limit over a broad frequency range. Hundred-meter-scale high finesse cavities have been proposed for this purpose. Optomechanically induced transparency (OMIT) enables the creation of optomechanical cavities in which the linewidth limit is set by the extremely narrow linewidth of a high Q factor mechanical resonator. Using an 85mm OMIT cavity with a silicon nitride membrane, we demonstrate a tunable linew…
We study a squeezed vacuum field generated in hot Rb vapor via the polarization self-rotation effect. Our previous experiments showed that the amount of observed squeezing may be limited by the contamination of the squeezed vacuum output with higher-order spatial modes, also generated inside the cell. Here, we demonstrate that the squeezing can be improved by making the light interact several times with a less dense atomic ensemble. With optimization of some parameters we can achieve up to -2.6 dB of squeezing in the multi-pass case, which is 0.6 dB improvement compared to the single-pass expe…
Phonon heat transport with squeezing-based symmetry breaking
Institute of Quantum Science and Precision Measurement, School of Physics, East China Normal University（华东师范大学物理学院量子科学与精密测量研究所）；Collaborative Innovation Center of Extreme Optics, Shanxi University（山西大学极端光学协同创新中心）；Shanghai Branch, Hefei National Laboratory（合肥微尺度物质科学国家研究中心上海分部）；Shanghai Research Center for Quantum Sciences（上海量子科学研究与发展中心）
We propose to simulate bosonic pair creation using large arrays of long-lived dipoles with multilevel internal structure coupled to an undriven optical cavity. Entanglement between the atoms, generated by the exchange of virtual photons through a common cavity mode, grows exponentially fast and is described by two-mode squeezing of effective bosonic quadratures. The mapping between an effective bosonic model and the natural spin description of the dipoles allows us to realize the analog of optical homodyne measurements via straightforward global rotations and population measurements of the ele…
With our all-atomic squeezing and filtering setup, we demonstrate control over the noise amplitudes and manipulation of the frequency-dependent squeezing angle of a squeezed vacuum quantum state by passing it through an atomic medium with electromagnetically induced transparency (EIT). We generate low sideband frequency squeezed vacuum using the polarization self-rotation effect in a hot Rb vapor cell, and input it into a second atomic vapor subject to EIT conditions. We use the frequency-dependent absorption of the EIT window to demonstrate an example of squeeze amplitude attenuation and sque…
Quantum entanglement can provide enhanced precision beyond standard quantum limit (SQL), the highest precision achievable with classical means. It remains challenging, however, to observe large enhancement limited by the experimental abilities to prepare, maintain, manipulate and detect entanglement. Here, we present nonlinear interferometry protocols based on echoing spin-nematic squeezing to achieve record high enhancement factors in atomic Bose-Einstein condensate. The echo is realized by a state-flip of the spin-nematic squeezed vacuum, which serves as the probe state and is refocused back…
We report on the generation of pulses of a low-frequency squeezed vacuum with noise suppression >2 dB below the standard quantum limit in a hot resonant 87 Rb vapor with polarization self-rotation. We demonstrate the possibility to precisely control the temporal profile of the squeezed noise quadrature by applying a calibrated longitudinal magnetic field, without degrading the maximum amount of squeezing.
We demonstrated that by using a pump field with non-zero orbital angular momentum (OAM) in the polarization self-rotation squeezing process it is possible to generate a squeezed vacuum optical field with the matching OAM. We found a similar level of maximum quantum noise reduction for a first-order Laguerre-Gaussian pump beam and a regular Gaussian pump beam, even though the optimal operational conditions differed in these two cases. Also, we investigated the effect of self-defocusing on the level of the vacuum squeezing by simultaneously monitoring the minimum quantum noise level and the outp…
We report the generation of a squeezed vacuum state of light whose noise ellipse rotates as a function of the detection frequency. The squeezed state is generated via a four-wave mixing process in a vapor of 85Rb. We observe that rotation varies with experimental parameters such as pump power and laser detunings. We use a theoretical model based on the Heisenberg-Langevin formalism to describe this effect. Our model can be used to investigate the parameter space and to tailor the ellipse rotation in order to obtain an optimum squeezing angle, for example, for coupling to an interferometer whos…
We study the strong coupling between photons and atoms that can be achieved in an optical nanofiber geometry when the interaction is dispersive. While the Purcell enhancement factor for spontaneous emission into the guided mode does not reach the strong-coupling regime for individual atoms, one can obtain high cooperativity for ensembles of a few thousand atoms due to the tight confinement of the guided modes and constructive interference over the entire chain of trapped atoms. We calculate the dyadic Green's function, which determines the scattering of light by atoms in the presence of the fi…
We report quantum enhancement of Faraday rotation spin noise spectroscopy by polarization squeezing of the probe beam. Using natural abundance Rb in 100 Torr of N_2 buffer gas, and squeezed light from a sub-threshold optical parametric oscillator stabilized 20 GHz to the blue of the D_1 resonance, we observe that an input squeezing of 3.0 dB improves the signal-to-noise ratio by 1.5 dB to 2.6 dB over the combined (power)$\otimes$(number density) ranges (0.5 mW to 4.0 mW )$\otimes$(1.5 x 10^{12} cm^{-3} to 1.3 x 10^{13} cm^{-3}), covering the ranges used in optimized spin noise spectroscopy exp…
We study the effect of optical polarization squeezing on the performance of a sensitive, quantum-noise-limited optically pumped magnetometer. We use Bell-Bloom (BB) optical pumping to excite a $^{87}$Rb vapor containing $8.2 \cdot 10^{12} \mathrm{atoms/cm^3}$ and Faraday rotation to detect spin precession. The sub-$\mathrm{pT}/\sqrt{\mathrm{Hz}}$ sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases measurement bandwidth, with no loss of sensitivity at any frequency, a d…
We investigated the propagation of a squeezed optical field, generated via the polarization self-rotation (PSR) effect, with a sinusoidally-modulated degree of squeezing through an atomic medium with anomalous dispersion. We observed the advancement of the signal propagating through a resonant Rb vapor compared to the reference signal, propagating in air. The measured advancement time grew linearly with atomic density, reaching a maximum of $11 \pm 1~μ$s, which corresponded to a negative group velocity of $v_g\approx - 7,000~$m/s. We also confirmed that the increasing advancement was accompani…
We reported a compact squeezed light source consisting of an diode laser near resonant on 87Rb optical D1 transition and an warm Rubidium vapor cell. The -4dB vacuum squeezing at 795 nm via nonlinear magneto-optical rotation was observed when applying the magnetic field orthogonal to the propagation direction of the light beam. This compact squeezed light source can be potentially utilized in the quantum information protocols such as quantum repeater and memory, and quantum metrology such as atomic magnetometer.
Transition to the semiclassical behaviour and the decoherence process for inhomogeneous perturbations generated from the vacuum state during an inflationary stage in the early Universe are considered both in the Heisenberg and the Schrödinger representations to show explicitly that both approaches lead to the same prediction: the equivalence of these quantum perturbations to classical perturbations having stochastic Gaussian amplitudes and belonging to the quasi-isotropic mode. This equivalence and the decoherence are achieved once the exponentially small (in terms of the squeezing parameter $…
We measure the sensitivity of a broadband atomic magnetometer using quantum non-demolition spin measurements. A cold, dipole-trapped sample of rubidium atoms provides a long-lived spin system in a non-magnetic environment, and is probed non-destructively by paramagnetic Faraday rotation. The calibration procedure employs a known reference state, the maximum-entropy or 'thermal' spin state and quantitative imaging-based atom counting to identify electronic, quantum, and technical noise in both the probe and spin system. The measurement achieves sensitivity 2.8 dB better than the projection nois…
With the help of Stokes operator S2 squeezed state (also called polarization squeezed state (PSS)) of 795-nm light, rubidium-87 (87Rb) atomic magnetometer based on Faraday rotation has been implemented and characterized.The PSS of Stokes operator S2 of 795-nm light has been prepared by means of coherently combining the polarization coherent state (PCS) of a linearly p-polarized bright 795-nm light beam and a linearly s-polarized squeezed vacuum state (SVS) generated by a 397.5-nm ultraviolet laser pumped sub-threshold optical parametric oscillator (OPO) with a PPKTP bulk crystal inside the OPO…
