We propose a novel scheme of solid state realization of a quantum computer based on single spin "enhancement mode" quantum dots as building blocks. In the enhancement quantum dots, just one electron can be brought into initially empty dot, in contrast to depletion mode dots based on expelling of electrons from multi-electron dots by gates. The quantum computer architectures based on depletion dots are confronted by several challenges making scalability difficult. These challenges can be successfully met by the approach based on ehnancement mode, capable of producing square array of dots with versatile functionalities. These functionalities allow transportation of qubits, including teleportation, and error correction based on straightforward one- and two-qubit operations. We describe physical properties and demonstrate experimental characteristics of enhancement quantum dots and single-electron transistors based on InAs/GaSb composite quantum wells. We discuss the materials aspects of quantum dot quantum computing, including the materials with large spin splitting such as InAs, as well as perspectives of enhancement mode approach in materials such as Si.
We show that two electrons confined in a square semiconductor quantum dot have two isolated low-lying energy eigenstates, which have the potential to form the basis of scalable computing elements (qubits). Initialisation, one-qubit and two-qubit universal gates, and readout are performed using electrostatic gates and magnetic fields. Two-qubit transformations are performed via the Coulomb interaction between electrons on adjacent dots. Choice of initial states and subsequent asymmetric tuning of the tunnelling energy parameters on adjacent dots control the effect of this interaction.
Exciton fine-structure splittings within quantum dots introduce phase differences between the two biexciton decay paths that greatly reduce the entanglement of photon pairs generated via biexciton recombination. We analyze this problem in the frequency domain and propose a practicable method to compensate the phase difference by inserting a spatial light modulator, which substantially improves the entanglement of the photon pairs without any loss.
We propose a scheme for realizing the scalable quantum computation based on nonidentical quantum dots trapped in a single-mode waveguide. In this system, the quantum dots simultaneously interact with a large detuned waveguide and classical light fields. During the process, neither the waveguide mode nor the quantum dots are excited, while the sub-system composed of any two quantum dots can acquire phases conditional upon the states of these two quantum dots and the certain detunings between the waveguide mode and corresponding external light fields. Therefore, it can be used to realize selecti…
We report on the control of the spontaneous emission dynamics from InAsP self-assembled quantum dots emitting in the telecommunications C-band and weakly coupled to the mode of a double heterostructure cavity etched on a suspended InP membrane at room temperature. The quality factor of the cavity mode is 44x10^3 with an ultra-low modal volume of the order of 1.2 lambda/n)^3, inducing an enhancement of the spontaneous emission rate of up a factor of 2.8 at 300 K.
Integrated quantum photonic circuits (IQPCs) with deterministically integrated quantum emitters are critical elements for scalable quantum information applications and have attracted significant attention in recent years. However, scaling up them towards fully functional photonic circuits with multiple deterministically integrated quantum emitters to generate photonic input states remains a great challenge. In this work, we report on a monolithic prototype IQPC consisting of two pre-selected quantum dots deterministically integrated into nanobeam cavities at the input ports of a 2x2 multimode …
Scalable Quantum Interference from Indistinguishable Quantum Dots
Institute of Photonics and Quantum Sciences, Heriot-Watt University（赫瑞-瓦特大学光子与量子科学研究所）；Condensed Matter Theory, Technical University of Dortmund（多特蒙德工业大学凝聚态理论系）
Quantum logic gates are the key elements in quantum computing. Here we investigate the possibility of achieving a scalable and compact quantum computing based on stationary electron-spin qubits, by using the giant optical circular birefringence induced by quantum-dot spins in double-sided optical microcavities as a result of cavity quantum electrodynamics. We design the compact quantum circuits for implementing universal and deterministic quantum gates for electron-spin systems, including the two-qubit CNOT gate and the three-qubit Toffoli gate. They are compact and economic, and they do not r…
We introduce a new scalable cavity quantum electrodynamics platform which can be used for quantum computing. This system is composed of coupled photonic crystal (PC) cavities which their modes lie on a Dirac cone in the whole super crystal band structure. Quantum information is stored in quantum dots that are positioned inside the cavities. We show if there is just one quantum dot in the system, energy as photon is exchanged between the quantum dot and the Dirac modes sinusoidally. Meanwhile the quantum dot becomes entangled with Dirac modes. If we insert more quantum dots into the system, the…
Scalable architectures for quantum information technologies require to selectively couple long-distance qubits while suppressing environmental noise and cross-talk. In semiconductor materials, the coherent coupling of a single spin on a quantum dot to a cavity hosting fermionic modes offers a new solution to this technological challenge. Here, we demonstrate coherent coupling between two spatially separated quantum dots using an electronic cavity design that takes advantage of whispering-gallery modes in a two-dimensional electron gas. The cavity-mediated long-distance coupling effectively min…
We show that, Four wave mixing (FWM) processes of grating can be controlled by the presence of interactions with a quantum dot or a molecule made by coupled quantum dots. By choosing the appropriate level spacing for the quantum emitter, one can either suppress or enhance the Four wave mixing process. We revel theoretically the underlying mechanism for this effect. (i) Suppression in FWM intensity occurs simply because induced Electromagnetic Induced Transparency does not allow the excitation at converted FWM frequency. (ii) Enhancement emerges since FWM process can be brought to resonance. Pa…
We show that the two-photon transition rates of quantum dots coupled to nanocavities are enhanced by up to 8 orders of magnitude relative to quantum dots in bulk host. We then propose how to take advantage of this enhancement to implement coherent quantum dot excitation by two-photon absorption, entangled photon pair generation by two-photon spontaneous emission, and single-photon generation at telecommunication wavelengths by two-photon stimulated and spontaneous emission.
A large-scalable quantum computer model, whose qubits are represented by the subspace subtended by the ground state and the single exciton state on semiconductor quantum dots, is proposed. A universal set of quantum gates in this system may be achieved by a mixed approach, composed of dynamic evolution and nonadibatic geometric phase.
A long standing obstacle to realizing highly sought on-chip monolithic solid state quantum optical circuits has been the lack of a starting platform comprising buried (protected) scalable spatially ordered and spectrally uniform arrays of on-demand single photon sources (SPSs). In this paper we report the first realization of such SPS arrays based upon a class of single quantum dots (SQDs) with single photon emission purity > 99.5% and uniformity < 2nm. Such SQD synthesis approach offers rich flexibility in material combinations and thus can cover the emission wavelength regime from long- to m…
The quest for an integrated quantum optics platform has motivated the field of semiconductor quantum dot research for two decades. Demonstrations of quantum light sources, single photon switches, transistors, and spin-photon interfaces have become very advanced. Yet the fundamental problem that every quantum dot is different prevents integration and scaling beyond a few quantum dots. Here, we address this challenge by patterning strain via local phase transitions to selectively tune individual quantum dots that are embedded in a photonic architecture. The patterning is implemented with in oper…
We demonstrate a 12 quantum dot device fabricated on an undoped Si/SiGe heterostructure as a proof-of-concept for a scalable, linear gate architecture for semiconductor quantum dots. The device consists of 9 quantum dots in a linear array and 3 single quantum dot charge sensors. We show reproducible single quantum dot charging and orbital energies, with standard deviations less than 20% relative to the mean across the 9 dot array. The single quantum dot charge sensors have a charge sensitivity of 8.2 x 10^{-4} e/root(Hz) and allow the investigation of real-time charge dynamics. As a demonstrat…
We introduce a silicon metal-oxide-semiconductor quantum dot architecture based on a single polysilicon gate stack. The elementary structure consists of two enhancement gates separated spatially by a gap, one gate forming a reservoir and the other a quantum dot. We demonstrate, in three devices based on two different versions of this elementary structure, that a wide range of tunnel rates is attainable while maintaining single-electron occupation. A characteristic change in slope of the charge transitions as a function of the reservoir gate voltage, attributed to screening from charges in the …
Trion quantum coherence in site-controlled pyramidal InGaAs quantum dots
Department of Physics, University of Strathclyde（斯特拉斯克莱德大学物理系）；Sussex Centre for Quantum Technologies, University of Sussex（苏塞克斯大学苏塞克斯量子技术中心）；Tyndall National Institute, University College Cork（科克大学学院廷德尔国家研究所）
We propose an all-optical implementation of quantum-information processing in semiconductor quantum dots, where electron-hole excitations (excitons) serve as the computational degrees of freedom (qubits). We show that the strong dot confinement leads to an overall enhancement of Coulomb correlations and to a strong renormalization of the excitonic states, which can be exploited for performing conditional and unconditional qubit operations.
We show how a spin interaction between electrons localized in neighboring quantum dots can be induced and controlled optically. The coupling is generated via virtual excitation of delocalized excitons and provides an efficient coherent control of the spins. This quantum manipulation can be realized in the adiabatic limit and is robust against decoherence by spontaneous emission. Applications to the realization of quantum gates, scalable quantum computers, and to the control of magnetization in an array of charged dots are proposed.
Sources of non-classical light are of paramount importance for future applications in quantum science and technology such as quantum communication, quantum computation and simulation, quantum sensing and quantum metrology. In this review we discuss the fundamentals and recent progress in the generation of single photons, entangled photon pairs and photonic cluster states using semiconductor quantum dots. Specific fundamentals which are discussed are a detailed quantum description of light, properties of semiconductor quantum dots and light-matter interactions. This includes a framework for the…
A theoretical investigation on slow light propagation based on eletromagnetically induced transparency in a three-level quantum-dot system is performed including non-Markovian effects and correlated dephasing reservoirs. It is demonstraonated that the non-Markovian nature of the process is quite essential even for conventional dephasing typical of quantum dots leading to significant enhancement or inhibition of the group velocity slow-down factor as well as to the shifting and distortion of the transmission window. Furthermore, the correlation between dephasing reservoirs may also either enhan…
Measurements provide a novel mechanism for generating the entanglement resource necessary for performing scalable quantum computation. Recently, we proposed a method for performing parity measurements in a coupled quantum dot system. In this paper we generalise this scheme and perform a comprehensive analytic and numerical study of environmental factors. We calculate the effects of possible error sources including non-ideal photon detectors, ineffective spin-selective excitation and dot distinguishability (both spatial and spectral). Furthermore, we present an experimental approach for verifyi…
We present time-resolved spontaneous emission measurements of single quantum dots embedded in photonic crystal waveguides. Quantum dots that couple to the photonic crystal waveguide are found to decay up to 27 times faster than uncoupled quantum dots. From these measurements $β$-factors of up to 0.89 are derived, and an unprecedented large bandwidth of 20 nm is demonstrated. This shows the promising potential of photonic crystal waveguides for efficient single-photon sources. The scaled frequency where the enhancement is observed is in excellent agreement with theory taking into account that t…
In this paper we investigate the coherence properties of a quantum dot under two-photon resonant excitation in combination with an additional photo-neutralization laser. The photo-neutralization increases the efficiency of the excitation process and thus, the brightness of the source, by a factor of approximately 1.5 for biexciton-exciton pairs. This enhancement does not degrade the relevant coherences in the system; neither the single photon coherence time, nor the coherence of the excitation process.
Solid-state systems such as P donors in Si have considerable potential for realization of scalable quantum computation. Recent experimental work in this area has focused on implanted Si:P double quantum dots (DQDs) that represent a preliminary step towards the realization of single donor charge-based qubits. This paper focuses on the techniques involved in analyzing the charge transfer within such DQD devices and understanding the impact of fabrication parameters on this process. We show that misalignment between the buried dots and surface gates affects the charge transfer behavior and identi…
The coupling between single photon emitters and integrated photonic circuits is an emerging topic relevant for quantum information science and other nanophotonic applications. We investigate the coupling between a hybrid system of colloidal quantum dots and propagating gap modes of a silicon nitride waveguide system. We furthermore explore the density of optical states of the system by using a scanning probe technique and find that the quantum dots couple significantly to the photonic circuit. Our results indicate that a scalable slot-waveguide might serve as a promising platform in future dev…
We present evidence of cavity quantum electrodynamics from a sparse density of strongly quantum-confined Pb-chalcogenide nanocrystals (between 1 and 10) approaching single-dot levels on moderately high-Q mesoscopic silicon optical cavities. Operating at important near-infrared (1500-nm) wavelengths, large enhancements are observed from devices and strong modifications of the QD emission are achieved. Saturation spectroscopy of coupled QDs is observed at 77K, highlighting the modified nanocrystal dynamics for quantum information processing.
We present coherent reflection spectroscopy on a charge and DC Stark tunable quantum dot embedded in a high-quality and externally mode-matched microcavity. The addition of an exciton to a single-electron charged quantum dot forms a trion that interacts with the microcavity just below strong coupling regime of cavity quantum electrodynamics. Such an integrated, monolithic system is a crucial step towards the implementation of scalable hybrid quantum information schemes that are based on an efficient interaction between a single photon and a confined electron spin.
Several recently proposed implementations of scalable quantum computation rely on the ability to manipulate the spin polarization of individual electrons in semiconductors. The most rapid single-spin-manipulation technique to date relies on the generation of an effective magnetic field via a spin-sensitive optical Stark effect. This approach has been used to split spin states in colloidal CdSe quantum dots and to manipulate ensembles of spins in ZnMnSe quantum wells with femtosecond optical pulses. Here we report that the process will produce a coherent rotation of spin in quantum dots contain…
Spin qubit gates via phonon buses in electron nanowires
Blackett Laboratory, Imperial College London（帝国理工学院布莱克特实验室）；Department of Physics and Astronomy, University College London（伦敦大学学院物理与天文系）；School of Basic Sciences, Indian Institute of Technology, Bhubaneswar（印度理工学院布巴内斯瓦尔基础科学系）；Department of Electronic and Electrical Engineering, University College London（伦敦大学学院电子电气工程系）；London Centre for Nanotechnology, University College London（伦敦大学学院纳米技术研究中心）；Cavendish Laboratory, Department of Physics, University of Cambridge（剑桥大学卡文迪许物理学实验室）；CPHT, CNRS, École Polytechnique, Institut Polytechnique de Paris（巴黎综合理工学院高等应用物理中心，法国国家科学研究中心）
One of the key challenges for the implementation of scalable quantum information processing is the design of scalable architectures that support coherent interaction and entanglement generation between distant quantum systems. We propose a nanotube double quantum dot spin transducer that allows to achieve steady-state entanglement between nitrogen-vacancy center spins in diamond with spatial separations over micrometers. The distant spin entanglement further enables us to design a scalable architecture for solid-state quantum information processing based on a hybrid platform consisting of nitr…
We analyze the decoherence of charge states in double quantum dots due to cotunneling. The system is treated using the Bloch-Redfield generalized master equation for the Schrieffer-Wolff transformed Hamiltonian. We show that the decoherence, characterized through a relaxation $τ_{r}$ and a dephasing time $τ_ϕ$, can be controlled through the external voltage and that the optimum point, where these times are maximum, is not necessarily in equilibrium. We outline the mechanism of this nonequilibrium-induced enhancement of lifetime and coherence. We discuss the relevance of our results for recent …
Realization of controllable interaction between distant qubits is one of the major problems in scalable solid state quantum computing. We study a superconducting transmission line resonator (TLR) as a tunable dispersive coupler for the double-dot molecules. A general interaction Hamiltonian of $n$ two-electron spin-based qubits and the TLR is presented, where the double-dot qubits are biased at the large detuning region and the TLR is always empty and virtually excited. Our analysis o the main decoherence sources indicates that various major quantum operations can be reliably implemented with …
Parity measurements on qubits can generate the entanglement resource necessary for scalable quantum computation. Here we describe a method for fast optical parity measurements on electron spin qubits within coupled quantum dots. The measurement scheme, which can be realised with existing technology, consists of the optical excitation of excitonic states followed by monitored relaxation. Conditional on the observation of a photon, the system is projected into the odd/even parity subspaces. Our model incorporates all the primary sources of error, including detector inefficiency, effects of spati…
Studying quantum properties in solid-state systems is a significant avenue for research. In this scenario, double quantum dots (DQDs) appear as a versatile platform for technological breakthroughs in quantum computation and nanotechnology. This work inspects the thermal entanglement and quantum coherence in two-coupled DODs, where the system is exposed to an external stimulus that induces an electronic transition within each subsystem. The results show that the introduction of external stimulus induces a quantum level crossing that relies upon the Coulomb potential changing the degree of quant…
Single photons produced by fundamentally dissimilar physical processes will in general not be indistinguishable. We show how photons produced from a quantum dot and by parametric down-conversion in a nonlinear crystal can be manipulated to be indistinguishable. The measured two-photon coalescence probability is 16%, and is limited by quantum-dot decoherence. Temporal filtering to the quantum dot coherence time and accounting for detector time response increases this to 61% while retaining 25% of the events. This technique can connect different elements in a scalable quantum network.
An ideal source of entangled photon pairs combines the perfect symmetry of an atom with the convenient electrical trigger of light sources based on semiconductor quantum dots. We create a naturally symmetric quantum dot cascade that emits highly entangled photon pairs on demand. Our source consists of strain-free GaAs dots self-assembled on a triangular symmetric (111)A surface. The emitted photons strongly violate Bell's inequality and reveal a fidelity to the Bell state as high as 86 (+-2) % without postselection. This result is an important step towards scalable quantum-communication applic…
Quantum scars are enhancements of quantum probability density along classical periodic orbits. We study the recently discovered phenomenon of strong, perturbation-induced quantum scarring in the two-dimensional harmonic oscillator exposed to a homogeneous magnetic field. We demonstrate that both the geometry and the orientation of the scars are fully controllable with a magnetic field and a focused perturbative potential, respectively. These properties may open a path into an experimental scheme to manipulate electric currents in nanostructures fabricated in a two-dimensional electron gas.
We develop an architecture for distributed quantum computation using quantum bus of plasmonic circuits and spin qubits in self-assembled quantum dots. Deterministic quantum gates between two distant spin qubits can be reached by using an adiabatic approach in which quantum dots couple with highly detuned plasmon modes in a metallic nanowire. Plasmonic quantum bus offers a robust and scalable platform for quantum optics experiments and the development of on-chip quantum networks composed of various quantum nodes, such as quantum dots, molecules and nanoparticles.
Solid-state single-photon emitters are key components for integrated quantum photonic devices. However, they can suffer from poor extraction efficiencies, caused by the large refractive index contrast between the bulk material they are embedded in and air: this results in a small fraction (that can be as low as <1%) of the emitted photons reaching free-space collection optics. To overcome this issue, we present a device that combines a metallic nano-ring, positioned on the sample surface and centered around the emitter, and an epoxy-based super-solid immersion lens, deterministically deposited…
The generation and long-haul transmission of highly entangled photon pairs is a cornerstone of emerging photonic quantum technologies, with key applications such as quantum key distribution and distributed quantum computing. However, a natural limit for the maximum transmission distance is inevitably set by attenuation in the medium. A network of quantum repeaters containing multiple sources of entangled photons would allow to overcome this limit. For this purpose, the requirements on the source's brightness and the photon pairs' degree of entanglement and indistinguishability are stringent. D…
A high-quality quantum dot (QD) single-photon source is a key resource for quantum information processing. Exciting a QD emitter resonantly can greatly suppress decoherence processes and lead to highly indistinguishable single-photon generation. It has, however, remained a challenge to implement strict resonant excitation in a stable and scalable way, without compromising any of the key specs of the source (efficiency, purity, and indistinguishability). In this work, we propose a novel dual-mode photonic-crystal waveguide that realizes direct in-plane resonant excitation of the embedded QDs. T…
Solution processible colloidal quantum dots hold great promise for realizing single-photon sources embedded into scalable quantum technology platforms. However, the high-yield integration of large numbers of individually addressable colloidal quantum dots in a photonic circuit has remained an outstanding challenge. Here, we report on integrating individual colloidal core-shell quantum dots (CQDs) into a nanophotonic network that allows for excitation and efficient collection of single-photons via separate waveguide channels. An iterative electron beam lithography process provides a viable meth…
We propose a quantum computer architecture based on quantum dots both for short distance and for long distance communication/computation. Our scheme exploits the natural characteristics of self-assembled quantum dots and it is scalable. It is centered on the idea of a quantum bus based on semiconductor self-assembled quantum dots. This allows for transmission of qubits between the different quantum registers, and could be integrated in most of the present proposal for semiconductor quantum dot-based quantum computation. Our proposal exploits the peculiar properties of {\it relatively short} sp…
We present a method to enact a deterministic, measurement-free, optically generated controlled-phase gate on two qubits defined by single electrons trapped in large-area quantum dots in a planar microcavity. This method is robust to optical quantum dot inhomogeneity, requires only a modest-$Q$ planar cavity, employs only a single laser pulse, and allows the integration of many entangled qubits on one semiconductor chip. We present the gate in the contexts of both adiabatic evolution and geometric phases, and calculate the degradation of performance in the presence of both spontaneous emission …
