Realistic linear quantum information processing necessitates the ability to synchronously generate entangled photon pairs either at the same or at distant locations. Here, we report the experimental realization of synchronized generation of independent entangled photon pairs. The quality of synchronization is confirmed by observing a violation of Bell's inequality with 3.2 standard deviations in an entanglement swapping experiment. The techniques developed in our experiment will be of great importance for future linear optical realization of quantum repeaters and quantum computation.
We report a proof-of-principle experiment on distant clock synchronization. Besides the achievement of picosecond resolution at 3 kilometer distance, this experiment demonstrated a novel concept for high accuracy non-local timing and positioning based on the quantum feature of entangled states.
We present an algorithm for synchronizing two clocks based on second-order quantum interference between entangled photons generated by parametric down-conversion. The procedure is distinct from the standard Einstein two-way clock synchronization method in that photon correlations are used to define simultaneous events in the frame of reference of a Hong-Ou-Mandel (HOM) interferometer. Once the HOM interferometer is balanced, by use of an adjustable optical delay in one arm, arrival times of simultaneously generated photons are recorded by each clock. Classical information on the arrival times …
High-precision nonlocal temporal correlation identification in the entangled photon pairs is critical to measure the time offset between remote independent time scales for many quantum information applications. The first nonlocal correlation identification was reported in 2009, which extracts the time offset via the algorithm of iterative fast Fourier transformations (FFTs) and their inverse. The least identification resolution is restricted by the peak identification threshold of the algorithm, and thus the time offset calculation precision is limited. In this paper, an improvement for the id…
A method is proposed to employ entangled and squeezed light for determining the position of a party and for synchronizing distant clocks. An accuracy gain over analogous protocols that employ classical resources is demonstrated and a quantum-cryptographic positioning application is given, which allows only trusted parties to learn the position of whatever must be localized. The presence of a lossy channel and imperfect photodetection is considered. The advantages in using partially entangled states is discussed.
Entangled states of light exhibit measurable correlations between light detections at separated locations. These correlations are exploited in entangled-state quantum key distribution. To do so involves setting up and maintaining a rhythm of communication among clocks at separated locations. Here, we try to disentangle our thinking about clocks as used in actual experiments from theories of time, such as special relativity or general relativity, which already differ between each other. Special relativity intertwines the concept of time with a particular definition of the synchronization of clo…
We propose a multi party quantum clock synchronization protocol that makes optimal use of the maximal multipartite entanglement of GHZ-type states. To realize the protocol, different versions of maximally entangled eigenstates of collective energy are generated by local transformations that distinguish between different groupings of the parties. The maximal sensitivity of the entangled states to time differences between the local clocks can then be accessed if all parties share the results of their local time dependent measurements. The efficiency of the protocol is evaluated in terms of the s…
We begin with the simple model of phase sychronization in open classical nonlinear system which is represented in the language of angular momentum variables. After that we propose the relevant quantum counterpart of this system. Using the appropriate Lindblad master equation for the density matrix of two qubit realization of such system we have revealed that stationary state of this composite system is pure and entangled with small dispersion of phase observable. We believe that such curious connection between entangled stationary states of quantum composite system and phase sychronization bet…
We present a scheme to produce an entangled four-photon state from two pairs of entangled two-photon states. Such entangled four-photon states are equivalent to the quantum state of two maximally entangled spin-1 particles. The scheme can also be generated to prepare an entangled 2N-photon state from N pairs of entangled two-photon states. Such multi-photon states play a crucial role in fundamental tests of quantum mechanics versus local realism and in many quantum information and quantum computation schemes.
We study two quantum versions of the Eddington clock-synchronization protocol in the presence of decoherence. The first protocol uses maximally entangled states to achieve the Heisenberg limit for clock synchronization. The second protocol achieves the limit without using entanglement. We show the equivalence of the two protocols under any single-qubit decoherence model that does not itself provide synchronization information.
A scheme to distinguish entangled two-photon-polarization states (ETP) from two independent entangled one-photon-polarization states (EOP) is proposed. Using this scheme, the experimental generation of ETP by parametric down-conversion is confirmed through the anti-correlations between three orthogonal two-photon-polarization states. The estimated fraction of ETP among the correlated photon pairs is 37% in the present experimental setup.
We demonstrate a point-to-point clock synchronization protocol based on bidirectionally propagating photons generated in a single spontaneous parametric down-conversion (SPDC) source. Tight timing correlations between photon pairs are used to determine the single and round-trip times measured by two separate clocks, providing sufficient information for distance-independent absolute synchronization secure against symmetric delay attacks. We show that the coincidence signature useful for determining the round-trip time of a synchronization channel, established using a 10\,km telecommunications f…
The generation and storage of entangled photons play important roles in quantum information technique. Spontaneous Raman scattering (SRS) in atomic ensembles provides a promising method to generate entangled photons capable of storage. In the past experiments, a spin-wave-photon entangled state is produced via SRS in an atomic ensemble, with which a pair of entangled photons is obtained. Here, we report a scheme of simultaneously generating two spin-wave-photon entangled states in an atomic ensemble by collecting Stokes photons at two different directions. Based on the obtained two atom-photon…
We demonstrate a point-to-point clock synchronization protocol based on bidirectionally exchanging photons produced in spontaneous parametric down conversion (SPDC). The technique exploits tight timing correlations between photon pairs to achieve a precision of 51ps in 100s with count rates of order 200s$^{-1}$. The protocol is distance independent, secure against symmetric delay attacks and provides a natural complement to techniques based on Global Navigation Satellite Systems (GNSS). The protocol works with mobile parties and can be augmented to provide authentication of the timing signal v…
Based on the second-order quantum interference between frequency entangled photons that are generated by parametric down conversion, a quantum strategic algorithm for synchronizing two spatially separated clocks has been recently presented. In the reference frame of a Hong-Ou-Mandel (HOM) interferometer, photon correlations are used to define simultaneous events. Once the HOM interferometer is balanced by use of an adjustable optical delay in one arm, arrival times of simultaneously generated photons are recorded by each clock. The clock offset is determined by correlation measurement of the r…
An essential requirement for the future of quantum communication is the capability to create undistinguishable photons at distant locations. The main challenge is to control the various sources of timing jitter in order to conserve temporal undistinguishability. We report on a system that enables a large tolerance against such jitter by using synchronized sources of photons with coherence lengths on the order of centimeters.
We extend entangled coincidence (ghost) imaging to fluorescent samples. Given the entangled photon correlation, one photon of the pair carries information on where the other photon has been absorbed and has produced fluorescence in a sample. Fluorescent molecules serve as ''detectors breaking'' the entanglement.
Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that allows the spectral shaping of entangled photons with high resolution. We evaluate its performances by detecting sum frequency generation in a non-linear crystal. The efficiency of the process is compared when performed with classical or entangled light.
The general concept of entangled photon holes is based on a correlated absence of photon pairs in an otherwise constant optical background. Here we consider the specialized case when this background is confined to two well-defined time bins, which allows the formation of time-bin entangled photon holes. We show that when the typical coherent state background is replaced by a true single-photon (Fock state) background, the basic time-bin entangled photon-hole state becomes equivalent to one of the time-bin entangled photon-pair states. We experimentally demonstrate these ideas using a parametri…
We present a concentration and purification scheme for nonmaximally entangled pure and mixed porization entangled state. We firstly show that two distant parties Alice and Bob first start with two shared but less entangled photon pure states to produce a four photon GHZ state, and then perform a 45 polarization measurement onto one of the two photons at each location such that the remaining two photon are projected onto a maximally entangled state. We further show the scheme also can be used to purify a class of mixed polarization-entangled state.
In addition to photon pairs entangled in polarization or other variables, quantum mechanics also allows optical beams that are entangled through the absence of the photons themselves. These correlated absences, or ``entangled photon holes'', can lead to counter-intuitive nonlocal effects analogous to those of the more familiar entangled photon pairs. Here we report an experimental observation of photon holes generated using quantum interference effects to suppress the probability that two photons in a weak laser pulse will separate at an optical beam splitter.
I show that the photon pairs used in experimental tests of quantum non-locality based on Bell's theorem are not in the entangled quantum state. The correct quantum state of the ``entangled'' photon pairs is suggested. Two experiments for testing this quantum state are proposed.
The quantum interference of entangled photons forms a key phenomenon underlying various quantum-optical technologies. It is known that the quantum interference patterns of entangled photon pairs can be reconstructed classically by the time-reversal method; however, the time-reversal method has been applied only to time-frequency-entangled two-photon systems in previous experiments. Here, for the first time, we apply the time-reversal method to the position-wavevector-entangled two-photon systems: the two-photon Young interferometer and the two-photon beam focusing system. We experimentally dem…
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single…
An experimental scheme for concentrating entanglement in partially entangled photon pairs is proposed. In this scheme, two separated parties obtain one maximally entangled photon pair from previously shared two partially entangled photon pairs by local operations and classical communication. A practical realization of the proposed scheme is discussed, which uses imperfect photon detectors and spontaneous parametric down-conversion as a photon source. This scheme also works for purifying a class of mixed states.
We present an scheme to generate entangled state between two traveling modes for fixed number of photon, which is based on beam splitter transformation and conditional zero photon counters.
We discuss the possibility of synchronising two atomic clocks exchanging entangled photon pairs through a quantum channel. A proposal for implementing practically such a scheme is discussed.
We report on the the experimental realization of hyper-entangled two photon states, entangled in polarization and momentum. These states are produced by a high brilliance parametric source of entangled photon pairs with peculiar characteristics of flexibility in terms of state generation. The quality of the entanglement in the two degrees of freedom has been tested by multimode Hong-Ou-Mandel interferometry.
Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources. Therefore, a worldwide effort has focused in overcoming the limitation of probabilistic emission by generating two-photon entangled states conditioned on the detection of auxiliary photons. Here we present the first heralded generation of photon states that are maximally entangled in polarization with linear optics and standard photon detection from spontaneous p…
Recently a protocol for Quantum Clock Synchronization (QCS) of remote clocks using quantum entanglement was proposed by Jozsa et al. This method has the goal of eliminating the random noise present in classical synchronization techniques. However, as stated QCS depends on the two members of each entangled pair undergoing the same unitary evolution even while being transported to different locations. This is essentially equivalent to a perfect Eddington Slow Clock Transfer protocol and thus, not an improvement over classical techniques. We will discuss this and suggest ways in which QCS may sti…
Entangled photons are crucial for quantum technologies, but generating arbitrary entangled photon states deterministically, efficiently, and with high fidelity remains a challenge. Here, we demonstrate how hybridization and dipole-dipole interactions -- potentially simultaneously available in colloidal quantum dots and molecular aggregates -- leveraged in conjunction can couple simple, well understood emitters into composite emitters with flexible control over the level structure. We show that cascade decay through carefully designed level structures can result in emission of frequency-entangl…
We construct an entangled photon polarimeter capable of monitoring a two-qubit quantum state in real time. Using this polarimeter, we record a nine frames-per-second video of a two-photon state's transition from separability to entanglement.
We present detailed instructions for constructing and operating an apparatus to produce and detect polarization-entangled photons. The source operates by type-I spontaneous parametric downconversion in a two-crystal geometry. Photons are detected in coincidence by single-photon counting modules and show strong angular and polarization correlations. We observe more than 100 entangled photon pairs per second. A test of a Bell inequality can be performed in an afternoon.
We present a feasible scheme to produce a polarization-entangled photon states $\frac{1}{\sqrt{2}}(|H>|V>+|V>|H>)$ in a controllable way. This scheme requires single-photon sources, linear optical elements and photon detectors. It generates the entanglement of spatially separated photons. The interaction takes place in the photon detectors. We also show that the same idea can be used to produce the entangled $N$-photon state $\frac{1}{\sqrt{2}}(|0,N>+|N,0>)$
We propose a simple scheme to produce the polarization entangled photon pairs without the type II phase match. The same scheme can also be used to produce the macroscopic entangled photon states in both photon number space and the polarization space(A. Lamas-Linares, J.C. Howell and D. Bouwmeester, Nature, 412887(2001)). Advantages and applications of our scheme in quantum key distribution are discussed.
We report on a method for optimizing the collection of entangled photon pairs in type-II parametric fluorescence. With this technique, we detected 360000 polarization-entangled photon pairs per second in the near-IR region in single-mode optical fibers. The entanglement of the photon pairs was verified by measuring polarization correlations in different bases of at least 96%.
We consider ramifications of the use of high speed light modulators to questions of correlation and measurement of time-energy entangled photons. Using phase modulators, we find that temporal modulation of one photon of an entangled pair, as measured by correlation in the frequency domain, may be negated or enhanced by modulation of the second photon. Using amplitude modulators we describe a Fourier technique for measurement of biphoton wave functions with slow detectors.
When basic tools of quantum information are applied to the quantum tomography data presented in Nature 439, 179 (2006), none of their devices appears to be a source of entangled photons.
A fundamental element of quantum information processing with photonic qubits is the nonclassical quantum interference between two photons when they bunch together via the Hong-Ou-Mandel (HOM) effect. Ultimately, many such pure photons must be processed in complex interferometric networks, and for this it is essential to synchronize the arrival times of the flying photons preserving their purity. Here we demonstrate for the first time the HOM interference of two heralded, pure optical photons synchronized through two independent quantum memories. Controlled storage times up to 1.8 microseconds …
Using the process of cavity-enhanced spontaneous parametric down-conversion (SPDC), we generate a narrow-band polarization-entangled photon pair resonant on the rubidium (Rb) D1 line (795 nm). The degenerate single-mode photon pair is selected by multiple temperature controlled etalons. The linewidth of generated polarization-entangled photon pairs is 15 MHz which matches the typical atomic memory bandwidth. The measured Bell parameter for the polarization-entangled photons S=2.73+-0.04 which violates the Bell-CHSH inequality by ~18 standard deviations. The presented entangled photon pair sour…
We present an algorithm to detect the time and frequency difference of independent clocks based on observation of time-correlated photon pairs. This enables remote coincidence identification in entanglement-based quantum key distribution schemes without dedicated coincidence hardware, pulsed sources with a timing structure or very stable reference clocks. We discuss the method for typical operating conditions, and show that the requirement in reference clock accuracy can be relaxed by about 5 orders of magnitude in comparison with previous schemes.
In this paper, an experiment of quantum diffraction of position-momentum entangled photons from a straight sharp edge is presented. Path of a single photon of an entangled pair is partially blocked by a sharp edge whereas the other photon is detected at a stationary location without revealing the which-path information of the other photon. Quantum diffraction pattern of the sharp edge is revealed only in the correlated conditional detection of spatially separated photons and no diffraction pattern is formed in local detections of individual photons. Theoretical analysis of the quantum diffract…
A novel method for preparation of a single photon in temporally-delocalized entangled modes is proposed and analyzed. We show that two single-photon pulses propagating in a driven nonabsorbing medium with different group velocities are temporally split under parametric interaction into well-separated pulses. In consequence, the single-photon "time-bin-entangled" states are generated with a programmable entanglement easily controlled by driving field intensity. The experimental study of nonclassical features and nonlocality of generated states by means of balanced homodyne tomography is discuss…
Remote state preparation (RSP) provides an indirect way of manipulating quantum information based on the nonlocal effect of quantum measurement. Although RSP has been demonstrated in recent years to remotely prepare multi-photon states, quantum measurement on the same number of photons was required, i.e., to prepare N-photon states via RSP, quantum measurement on the other N-photons was required, hence significantly limiting practicality and applicability of RSP. Here we report the first experimental demonstration of remote preparation of three-photon entangled states by measuring only a singl…
High quality factors, strong nonlinearities, and extensive design flexibility make superconducting circuits an ideal platform to investigate synchronization phenomena deep in the quantum regime. Recently~\cite{Loerch-2017}, it was predicted that energy quantization and conservation can block the synchronization of two identical, weakly coupled nonlinear self-oscillators. Here we propose a Josephson junction circuit realization of such a system along with a simple homodyne measurement scheme to observe this effect. We also show that at finite detuning, where phase synchronization takes place, t…
The properties of an entangled two-photon state antisymmetric in frequencies are studied. At a beam-splitter, two entangled photons are perfectly anti-correlated. In addition, they cannot be detected at the same time instant despite the fact that their detection times are confined to a narrow time window, i.e. they are temporally anti-bunched. Using nonlinear photonic-band-gap structures made of GaN/AlN, two schemes for generating such states are described.
Multi-dimensional entangled states have been proven to be more powerful in some quantum information process. In this paper, down-converted photons from spontaneous parametric down conversion(SPDC) are used to engineer multi-dimensional entangled states. A kind of multi-degree multi-dimensional Greenberger-Horne-Zeilinger(GHZ) state can also be generated. The hyper-entangled photons, which are entangled in energy-time, polarization and orbital angular momentum (OAM), is proved to be useful to increase the dimension of systems and investigate higher-dimensional entangled states.
The dispersion cancellation feature of pulses which are entangled in frequency is employed to synchronize clocks of distant parties. The proposed protocol is insensitive to the pulse distortion caused by transit through a dispersive medium. Since there is cancellation to all orders, also the effects of slowly fluctuating dispersive media are compensated. The experimental setup can be realized with currently available technology, at least for a proof of principle.
A photon source based on postselection from entangled photon pairs produced by parametric frequency down-conversion is suggested. Its ability to provide good approximations of single-photon states is examined. Application of this source in quantum cryptography for quantum key distribution is discussed. Advantages of the source compared to other currently used sources are clarified. Future prospects of the photon source are outlined.
We report measurements of time-frequency entangled photon pairs and heralded single photons at telecommunications wavelengths, generated using a periodically-poled, lithium niobate on insulator (LNOI) waveguide pumped optically by a diode laser. We achieve a high Coincidences-to-Accidentals Ratio (CAR) at high pair brightness, a low value of the conditional self-correlation function [$g^{(2)}$(0)], and high two-photon energy-time Franson interferometric visibility, which demonstrate the high quality of the entangled photon pairs and heralded single photons.
