We propose to create ultracold ground state molecules in an atomic Bose-Einstein condensate by adiabatic crossing of an optical Feshbach resonance. We envision a scheme where the laser intensity and possibly also frequency are linearly ramped over the resonance. Our calculations for $^{87}$Rb show that for sufficiently tight traps it is possible to avoid spontaneous emission while retaining adiabaticity, and conversion efficiencies of up to 50% can be expected.
We derive and discuss the temperature dependance of the condensate and noncondensate density profile of a Bose-Einstein condensate gas with Feshbach resonance in a parabolic trap. These quantities are calculated self-consistently using the generalized Hartree-Fock-Bogoliubov (HFB) equations within the Bogoliubov approximation. At zero temperature, the HFB equation can be solved by means of a variation method that give the low excitation spectrum. Moreover, within the two-body collision theory, we estimate the relationship between the atom number and the external magnetic field $B$, it is in go…
We consider a pair of atoms in an arbitrary trapping potential in the presence of magnetically tunable Feshbach resonance. We find the energy levels and occupation of the bound molecular states taking into account possible coupling between center of mass and relative motion induced by the trap. As a specific example we discuss the case of different atomic species in harmonic potential, where each atom feels different trapping frequency.
Employing a short-range two-channel description we derive an analytic model of atoms in isotropic and anisotropic harmonic traps at a Feshbach resonance. On this basis we obtain a new parameterization of the energy-dependent scattering length which differs from the one previously employed. We validate the model by comparison to full numerical calculations for Li-Rb and explain quantitatively the experimental observation of a resonance shift and trap-induced molecules in exited bands. Finally, we analyze the bound state admixture and Landau-Zener transition probabilities.
We propose a simple idea for realizing a quantum gate with two identical fermions in a double well trap via external optical pulses without addressing the atoms individually. The key components of the scheme are Feshbach resonance and Pauli blocking, which decouple unwanted states from the dynamics. As a physical example we study atoms in the presence of a magnetic Feshbach resonance in a nanoplasmonic trap and discuss the constraints on the operation times for realistic parameters, reaching a fidelity above $99.9\%$ within $42μ$s.
Feshbach resonances are among the essential control tools used in ultracold atom experiments. However, for complex atomic species the theoretical characterization of resonances becomes challenging. For closely spaced resonances, the measurement of three-body losses does not provide sufficient resolution to discriminate them. For this reason, resonance spectroscopy of trapped isolated atoms is becoming the state of the art. Here we show that trapping the atoms in a double well potential such as an optical lattice or a pair of optical tweezers enables precise characterization of not only the res…
We investigate phase separation of Bose-Einstein condensates (BECs) of two-component atoms and one-component molecules with a homonuclear Feshbach resonance. We develop a full model for dilute atomic and molecular gases including correlation of the Feshbach resonance and all kinds of interparticle interactions, and numerically calculate order parameters of the BECs in spherical harmonic oscillator traps at zero temperature with the Bogoliubov's classical field approximation. As a result, we find out that the Feshbach resonance can induce two types of phase separation. The actual phase structur…
We measure chemical reactions between a single trapped $^{174}$Yb$^+$ ion immersed in an ultracold bath of $^6$Li atoms containing trace amounts of Li$_2$ dimers. This produces LiYb$^+$ molecular ions that we detect via mass spectrometry. We explain the reaction rates by modelling the dimer density as a function of the magnetic field and obtain excellent agreement when we assume the reaction to follow the Langevin rate. Our results present a novel approach towards the creation of cold molecular ions and point to the exploration of ultracold chemistry in ion molecule collisions. What is more, w…
We develop a complete theoretical description of photoassociative Stimulated Raman Adiabatic Passage (STIRAP) near a Feshbach resonance in a thermal atomic gas. We show that it is possible to use low intensity laser pulses to directly excite the continuum at a Feshbach resonance and transfer nearly the entire atomic population to the lowest rovibrational level in the molecular ground state. In case of a broad resonance, commonly found in several diatomic alkali molecules, our model predicts a transfer efficiency $η$ up to 97% for a given atom pair, and up to 70% when averaged over an atomic en…
Bose-Einstein condensates can be used to produce work by tuning the strength of the interparticle interactions with the help of Feshbach resonances. In inhomogeneous potentials, these interaction ramps change the volume of the trapped gas allowing one to create a thermodynamic cycle known as the Feshbach engine. However, in order to obtain a large power output, the engine strokes must be performed on a short timescale, which is in contrast with the fact that the efficiency of the engine is reduced by irreversible work if the strokes are done in a non-adiabatic fashion. Here we investigate how …
We consider the stability of an ultracold trapped Bose-Einstein condensate near a Feshbach resonance. Using a modified Gross-Pitaevskii equation that includes higher-order terms and a multi-channel model of Feshbach resonances, we find regions where stability can be enhanced or suppressed around experimentally measured resonances. We suggest a number of ways to probe the stability diagram. Using scattering length zero-crossings huge deviations are founds for the critical particle number. Effects are enhanced for narrow resonances or tighter traps. Macroscopic tunneling of the condensate is ano…
Nuclear spin exchange occurs in ultracold collisions of fermionic alkaline-earth-like atoms due to a difference between s- and p-wave phase shifts. We study the use of an optical Feshbach resonance, excited on the ${}^1S_0 \to {}^3P_1$ intercombination line of ${}^{171}$Yb, to affect a large modification of the s-wave scattering phase shift, and thereby optically mediate nuclear exchange forces. We perform a full multichannel calculation of the photoassociation resonances and wave functions and from these calculate the real and imaginary parts of the scattering length. As a figure of merit of …
Large anomalous shifts of potassium-39 Feshbach resonances
Swinburne University of Technology（斯威本科技大学）；CSIRO（联邦科学与工业研究组织）；Instytut Fizyki Teoretycznej, Uniwersytet Jagielloński（雅盖隆大学理论物理研究所）；Österreichische Academie der Wissenschaften（奥地利科学院）；Institut für Quantenoptik und Quanteninformation (IQOQI)（量子光学与量子信息研究所）；Universität Innsbruck（因斯布鲁克大学）
We present a detailed analysis of the production efficiency of weakly bound heteronuclear KRb-Feshbach molecules using radio frequency association in a harmonic trap. The efficiency was measured in a wide range of temperatures, binding energies and radio frequencies. A comprehensive analytical model is presented, explaining the observed asymmetric spectra and achieving good quantitative agreement with the measured production rates. This model provides a deep understanding of the molecule association process and paves the way for future experiments which rely on Feshbach molecules e.g. for the …
The present paper aims at finding optimal parameters for trapping of Cs$_2$ molecules in optical lattices, with the perspective of creating a quantum degenerate gas of ground-state molecules. We have calculated dynamic polarizabilities of Cs$_2$ molecules subject to an oscillating electric field, using accurate potential curves and electronic transition dipole moments. We show that for some particular wavelengths of the optical lattice, called "magic wavelengths", the polarizability of the ground-state molecules is equal to the one of a Feshbach molecule. As the creation of the sample of groun…
By including the effect of a trap with characteristic energy given by the Fermi temperature $T_F$ in a two-body two-channel model for Feshbach resonances, we reproduce the experimental closed-channel fraction $Z$ across the BEC-BCS crossover and into the BCS regime of a $^6$Li atomic Fermi gas. We obtain the expected behavior $Z \propto \sqrt{T_F}$ at unitarity, together with the recently measured proportionality constant. Our results are also in agreement with recent measurements of the $Z$ dependency on $T_F$ on the BCS side, where a significant discrepancy between experiments and theory has…
We present two simple designs of matter-wave beam splitters in a trapped Bose-Einstein Condensate (BEC). In our scheme, identical pairs of atomic solitons are produced by an adequate control --- in time and/or space --- of the scattering length. Our analysis is performed by numerical integration of the Gross-Pitaevskii equation and supported by several analytic estimates. Our results show that these devices can be implemented in the frame of current BEC experiments. The system has potential applications for the construction of a soliton interferometer.
Controlling physical systems and their dynamics on the level of individual quanta propels both fundamental science and quantum technologies. Trapped atomic and molecular systems, neutral and charged, are at the forefront of quantum science. Their extraordinary level of control is evidenced by numerous applications in quantum information processing and quantum metrology. Studying the long-range interactions between these systems when combined in a hybrid atom-ion trap has lead to landmark results. Reaching the ultracold regime, however, where quantum mechanics dominates the interaction, e.g., g…
Using an optically-trapped mixture of the two lowest hyperfine states of a $^6$Li Fermi gas, we observe two-field optical tuning of the narrow Feshbach resonance by up to 3 G and an increase in spontaneous lifetime near the broad resonance from $0.5$ ms to $0.4$ s. We present a new model of light-induced loss spectra, employing continuum-dressed basis states, that agrees in shape and magnitude with measurements for both broad and narrow resonances.
Dynamics of atomic and molecular bright solitons in a hybrid atom-molecular BEC (Bose Einstein Condensate) system of 85Rb coupled through Magnetic Feshbach Resonance (MFR) has been investigated. By solving the time independent atom-molecular coupled equations, the initial atomic and molecular wavefunctions were obtained and the dynamics of the initial atomic and molecular waves in a spherical one-dimensional trap were studied by solving the time-dependent atom-molecular coupled equations. During evolution two types of induced or stimulated decays of the feshbach molecules were switched on. The…
We report the observation of resonance-like loss in the trap population of ultracold dysprosium as a function of magnetic field, which we attribute to anisotropy-induced Fano-Feshbach resonances arising from Dy's large magnetic dipole moment and nonzero electronic orbital angular momentum. We recorded these resonances for four different isotopes, three bosonic and one fermionic, over a field range of 0-6 G and show that the number of resonances changes significantly as a function of temperature, even in the nK regime. Most of the observed resonances are of very narrow width. The fermionic isot…
We optimize a collision-induced cooling process for ultracold atoms in the nondegenerate regime. It makes use of a Feshbach resonance, instead of rf radiation in evaporative cooling, to selectively expel hot atoms from a trap. Using functional minimization we analytically show that for the optimal cooling process the resonance energy must be tuned such that it linearly follows the temperature. Here, optimal cooling is defined as maximizing the phase-space density after a fixed cooling duration. The analytical results are confirmed by numerical Monte-Carlo simulations. In order to simulate more…
We demonstrate the production of large $^7$Li Bose-Einstein condensates in an optical dipole trap using $D_1$ gray molasses. The sub-Doppler cooling technique reduces the temperature of $4\times10^9$ atoms to $25~μ$K in 3~ms. After microwave evaporation cooling in a magnetic quadrupole trap, we transfer the atoms to a crossed optical dipole trap, where we employ a magnetic Feshbach resonance on the $|F=1,m_F=1\rangle$ state. Fast evaporation cooling is achieved by tilting the optical potential using a magnetic field gradient on the top of the Feshbach field. Our setup produces pure condensates…
We consider a fully polarized ultracold Fermi gas interacting through a p-wave Feshbach resonance. Using a two-channel model, we find the effective potential at the point where the p-wave scattering length goes to zero. Here the effective interaction provides attraction and one can therefore ask about the stability of the system. We calculate the energy density of the system in the Thomas-Fermi approximation, determine the profile of the gas, and the critical number of particle in the system as function of the relevant interaction parameters. The instability can be deduced from a simple breath…
The goal of adiabatic ground-state preparation is to start a simple quantum system in its ground state and adiabatically evolve the Hamiltonian to a complex one, maintaining the ground state throughout the evolution. In ion-trap-based quantum simulations, coherence times are too short to allow for adiabatic evolution for large chains, so the system evolves diabatically, creating excitations to higher energy states. Because the probability for diabatic excitation depends exponentially on the excitation energy and because the thermal distribution also depends exponentially on the excitation ener…
Decay of bound states due to coupling with free particle states is a general phenomenon occurring at energy scales from MeV in nuclear physics to peV in ultracold atomic gases. Such a coupling gives rise to Fano-Feshbach resonances (FFR) that have become key to understanding and controlling interactions - in ultracold atomic gases, but also between quasiparticles such as microcavity polaritons. The energy positions of FFR were shown to follow quantum chaotic statistics. In contrast, lifetimes which are the fundamental property of a decaying state, have so far escaped a similarly comprehensive …
We investigate the prospects of controlling charge-exchange in ultracold collisions of heteroisotopic combinations of atoms and ions of the same element. The treatment, readily applicable to alkali or alkanine-earth metals, is illustrated in the process $^9$Be$^{+}$ + $^{10}$Be $\leftrightarrow$ $^{9}$Be + $^{10}$Be$^{+}$, which exhibits favorable electronic, nuclear, and hyperfine structure. Feshbach resonances are obtained from quantum scattering calculations in a standard coupled-channel formalism with non-BO terms originating from the nuclear kinetic operator. Near a narrow resonance predi…
Collisional resonances are an important tool which has been used to modify interactions in ultracold gases, for realizing novel Hamiltonians in quantum simulations, for creating molecules from atomic gases and for controlling chemical reactions. So far, such resonances have been observed for atom-atom collisions, atom-molecule collisions and collisions between Feshbach molecules which are very weakly bound. Whether such resonances exist for ultracold ground state molecules has been debated due to the possibly high density of states and/or rapid decay of the resonant complex. Here we report a v…
Overlapping Feshbach resonances are commonly observed in experiments with ultracold atoms and can influence the molecule production process. We derive an effective approach to describe magnetoassociation in an external trap in the presence of multiple overlapping resonances. We study how the strength and shape of the trap affects the energy level structure and demonstrate the existence of a regime in which the conventional two-channel Landau-Zener description of the molecule production process breaks down.
We consider controlled collisions between two ultracold atoms guided by external harmonic potentials. We derive analytical solutions of the Schroedinger equation for this system, and investigate the properties of eigenergies and eigenstates for different trap geometries as a function of a trap separation and of the scattering length. When varying the trap separation the energy spectrum exhibits avoided crossings, corresponding to trap-induced shape resonances. Introducing an energy-dependent scattering length we investigate the behavior of the system in the vicinity of a magnetic Feshbach reso…
Ultracold potassium is an interesting candidate for quantum technology applications and fundamental research as it allows controlling intra-atomic interactions via low-field magnetic Feshbach resonances. However, the realization of high-flux sources of Bose-Einstein condensates remains challenging due to the necessity of optical trapping to use magnetic fields as free parameter. We investigate the production of all-optical $^{39}$K Bose-Einstein condensates with different scattering lengths using a Feshbach resonance near $33$ G. By tuning the scattering length in a range between $75\, a_0$ an…
Ultracold atoms placed in a tight cigar-shaped trap are usually described in terms of the Lieb-Liniger model. We study the extensions of this model which arise when van der Waals interaction between atoms is taken into account. We find that the corrections induced by the finite range of interactions can become especially important in the vicinity of narrow Feshbach resonances and suggest realistic schemes of their experimental detection. The interplay of confinement and interactions can lead to effective transparency where the one-dimensional interactions are weak in a wide range of parameters…
