We report on experimental evidences of the preservation of energy-time entanglement for extraordinary plasmonic light transmission through sub-wavelength metallic hole arrays, and for long range surface plasmon polaritons. Plasmons are shown to coherently exist at two different times separated by much more than the plasmons lifetime. This kind of entanglement involving light and matter is expected to be useful for future processing and storing of quantum information.
We experimentally study two-photon coherence in plasmon-assisted transmission with a two-photon Mach-Zehnder (MZ) interferometer. Two collinear photons of identical or orthogonal polarization are simultaneously incident on one optically thick metal film, perforated with a periodic array of subwavelength holes. The de Broglie wavelength of plasmon-assisted transmitted photons is measured, which shows that two photons are re-eradiated by the plasmons and the quantum coherence of biphoton is preserved in the conversion process of transforming biphoton to plasmons and then back to biphoton.
Orbital angular momentum of photons is explored to study the spatial mode properties of plasmon assisted transmission process. We found that photons carrying different orbital angular momentums have different transmission efficiencies, while the coherence between these spatial modes can be preserved.
We present an experimental evidence that high dimensional orbital angular momentum entanglement of a pair of photons can be survived after a photon-plasmon-photon conversion. The information of spatial modes can be coherently transmitted by surface plasmons. This experiment primarily studies the high dimensional entangled systems based on surface plasmon with subwavelength structures. It maybe useful in the investigation of spatial mode properties of surface plasmon assisted transmission through subwavelength hole arrays.
We show how to generate and control the correlations in a set of two distant quantum emitters coupled to a one-dimensional dissipative plasmonic waveguide. An external laser field enhances the dimer's steady-state correlations and allows an active control (switching on/off) of nonclassical correlations. The plasmon-assisted dipolar-interacting qubits exhibit persistent correlations, which in turn can be decoupled and made to evolve independently from each other. The setup enables long-distance ($\sim 1\, μ$m) qubit control that works for both resonant and detuned emitters. For suitable emitter…
The recent surface plasmon entanglement experiment [E. Altewischer et al., Nature (London) 418, 304 (2002)] is theoretically analyzed. The entanglement preservation upon transmission in the non-focused case is found to provide information about the interaction of the biphoton and the metallic film. The entanglement degradation in the focused case is explained in the framework of a fully multimode model. This phenomenon is a consequence of the polarization-selective filtering behavior of the metallic nanostructured film.
The state of a two-particle system is called entangled when its quantum mechanical wave function cannot be factorized in two single-particle wave functions. Entanglement leads to the strongest counter-intuitive feature of quantum mechanics, namely nonlocality. Experimental realization of quantum entanglement is relatively easy for the case of photons; a pump photon can spontaneously split into a pair of entangled photons inside a nonlinear crystal. In this paper we combine quantum entanglement with nanostructured metal optics in the form of optically thick metal films perforated with a periodi…
In this paper, the following scenario is considered: there are two qubits possessed by two parties at different locations. Qubits have been prepared in one of a maximum of four, mutually-orthogonal, entangled states and the parties wish to distinguish between the states by using local operations and classical communication. Although in general it is not possible to distinguish between four arbitrary states, the parties can spend some pre-shared entanglement to achieve perfect discrimination between four qubit states and can also preserve the entanglement of the states after discrimination. Thi…
We analyse the quantum mechanical limits to the plasmon-assisted entanglement transfer observed by E. Altewischer, M.P. van Exter, and J.P. Woerdman [Nature, 418, 304 (2002)]. The maximal violation S of Bell's inequality at the photodetectors behind two linear media (such as the perforated metal films in the experiment) can be described by two ratio's tau_1, tau_2 of polarization-dependent transmission probabilities. A fully entangled incident state is transferred without degradation for tau_1=tau_2, but a relatively large mismatch of tau_1 and tau_2 can be tolerated with a small reduction of …
We theoretically demonstrate coherent control over propagation of surface plasmon polaritons(SPP), at both telecommunication and visible wavelengths, on a metallic surface adjacent to quantum coherence (phaseonium) medium composed of three-level quantum emitters (semiconductor quantum dots, atoms, rare-earth ions, etc.) embedded in a dielectric host. The coherent drive allows us to provide sufficient gain for lossless SPP propagation and also lowers the pumping requirements. In case of lossy propagation, an order of magnitude enhancement in propagation length can be achieved. Optical control o…
We report on the efficient generation, propagation, and re-emission of squeezed long-range surface-plasmon polaritons (SPPs) in a gold waveguide. Squeezed light is used to excite the non-classical SPPs and the re-emitted quantum state is fully quantum characterized by complete tomographic reconstruction of the density matrix. We find that the plasmon-assisted transmission of non-classical light in metallic waveguides can be described by a Hamiltonian analogue to a beam splitter. This result is explained theoretically.
Tho-photon Rabi oscillations hold potential for quantum computing and quantum information processing, because during a Rabi cycle a pair of entangled photons may be created. We theoretically investigate the onset of this phenomenon in a heterodimer comprising a semiconductor quantum dot strongly coupled to a metal nanoparticle. Two-photon Rabi oscillations in this system occur due to a coherent two-photon process involving the ground-to-biexciton transition in the quantum dot. The presence of a metal nanoparticle nearby the quantum dot results in a self-action of the quantum dot via the metal …
We investigate the time-dependent Casimir-Polder potential of a polarizable two-level atom placed near a surface of arbitrary material, after a sudden change in the parameters of the system. Different initial conditions are taken into account. For an initially bare ground-state atom, the time-dependent Casimir-Polder energy reveals how the atom is "being dressed" by virtual, matter-assisted photons. We also study the transient behavior of the Casimir-Polder interaction between the atom and the surface starting from a partially dressed state, after an externally induced change in the atomic lev…
Surface plasmon polaritons (SPPs) are collective excitations of free electrons propagating along a metal-dielectric interface. Although some basic quantum properties of SPPs, such as the preservation of entanglement, the wave-particle duality of a single plasmon, the quantum interference of two plasmons, and the verification of entanglement generation, have been shown, more advanced quantum information protocols have yet to be demonstrated with SPPs. Here, we experimentally realize quantum state teleportation between single photons and SPPs. To achieve this, we use polarization-entangled photo…
Graphene plasmons provide a suitable alternative to noble-metal plasmons because they exhibit much larger confinement and relatively long propagation distances, with the advantage of being highly tunable via electrostatic gating. We report strong light- matter interaction assisted by graphene plasmons, and in particular, we predict unprecedented high decay rates of quantum emitters in the proximity of a carbon sheet, large vacuum Rabi splitting and Purcell factors, and extinction cross sections exceeding the geometrical area in graphene ribbons and nanometer-sized disks. Our results provide th…
Quantum plasmonics experiments have on multiple occasions reported the observation of quantum coherence of discrete plasmons, which exhibit remarkable preservation of quantum interference visibility, a seemingly surprising feature for systems mixing light and matter with high ohmic losses during propagation. However, most experiments to date used essentially weakly-confined plasmons, which experience limited light-matter hybridization, thus limiting the potential for decoherence. Here, we report quantum coherence of plasmons near the surface plasmon polariton (SPP) resonance frequency, where p…
Strong-coupling between light and matter produces hybridized states (polaritons) whose delocalization and electromagnetic character allow for novel modifications in spectroscopy and chemical reactivity of molecular systems. Recent experiments have demonstrated remarkable distance-independent long-range energy transfer between molecules strongly coupled to optical microcavity modes. To shed light on the mechanism of this phenomenon, we present the first comprehensive theory of polariton-assisted remote energy transfer (PARET) based on strong-coupling of donor and/or acceptor chromophores to sur…
