The Ullersma model for the damped harmonic oscillator is coupled to the quantised electromagnetic field. All material parameters and interaction strengths are allowed to depend on position. The ensuing Hamiltonian is expressed in terms of canonical fields, and diagonalised by performing a normal-mode expansion. The commutation relations of the diagonalising operators are in agreement with the canonical commutation relations. For the proof we replace all sums of normal modes by complex integrals with the help of the residue theorem. The same technique helps us to explicitly calculate the quantum evolution of all canonical and electromagnetic fields. We identify the dielectric constant and the Green function of the wave equation for the electric field. Both functions are meromorphic in the complex frequency plane. The solution of the extended Ullersma model is in keeping with well-known phenomenological rules for setting up quantum electrodynamics in an absorptive and spatially inhomogeneous dielectric. To establish this fundamental justification, we subject the reservoir of independent harmonic oscillators to a continuum limit. The resonant frequencies of the reservoir are smeared out over the real axis. Consequently, the poles of both the dielectric constant and the Green function unite to form a branch cut. Performing an analytic continuation beyond this branch cut, we find that the long-time behaviour of the quantised electric field is completely determined by the sources of the reservoir. Through a Riemann-Lebesgue argument we demonstrate that the field itself tends to zero, whereas its quantum fluctuations stay alive. We argue that the last feature may have important consequences for application of entanglement and related processes in quantum devices.
The phenomenological Maxwell field is quantized for arbitrarily space- and frequency-dependent complex permittivity. The formalism takes account of the Kramers--Kronig relation and the dissipation-fluctuation theorem and yields the fundamental equal-time commutation relations of QED. Applications to the quantum-state transformation at absorbing and amplifying four-port devices and to the spontaneous decay of an excited atom in the presence of absorbing dielectric bodies are discussed.
Recently a quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive, and absorbing dielectric medium has been developed and applied to a system consisting of two infinite half-spaces with a common planar interface (H.T. Dung, L. Knoell, and D.-G. Welsch, Phys. Rev. A 57, in press). Here we show that the scheme, which is based on the classical Green-tensor integral representation of the electromagnetic field, applies to any inhomogeneous medium. For this purpose we prove that the fundamental equal-time commut…
We investigate the phenomenon of sudden transition between classical and quantum decoherence in the study of quantum discord for a dissipative cavity QED system, which consists of two noninteracting two-level atoms, each trapped in a dissipative cavity. It is found that the quantum discord between two atoms, which are prepared initially in the X-type quantum states, is not destroyed by the dissipation of the cavities for a finite time interval and the stationary quantum discord can arise in the interaction of atoms with cavities as the time approach to infinite. The transition time is sensitiv…
In this paper we give fully analytical description of the dynamics of a collection of $N$-Frenkel excitons in high density regime dispersively coupled to a single mode cavity field, in the presence of both exciton and cavity-field dissipations. By using excitonic operators as q-deformed bosonic operators for the system, we solve analytically the Liouville equation for the density operator at zero temperature and investigate the influence of the number of excitons and the effect of both dissipations on dynamical behavior of the system. We use the solution of master equation to explore the dissi…
We develop a dual description of quantum optics adapted to dielectric systems without magnetic property. Our formalism, which is shown to be equivalent to the standard one within some dipolar approximations discussed in the article, is applied to the description of polaritons in dielectric media. We show that the dual formalism leads to the Huttner-Barnett equations [B. Huttner, S. M. Barnett, Phys. Rev. A \textbf{46}, 4306 (1992)] for QED in dielectric systems. More generally, we discuss the role of electromagnetic duality in the quantization procedure for optical systems and derive the struc…
The spontaneous emission rate of a radiating atom reaches its time-independent equilibrium value after an initial transient regime. In this paper we consider the associated relaxation effects of the spontaneous decay rate of atoms in dispersive and absorbing dielectric media for atomic transition frequencies near material resonances. A quantum mechanical description of such media is furnished by a damped-polariton model, in which absorption is taken into account through coupling to a bath. We show how all field and matter operators in this theory can be expressed in terms of the bath operators…
We present an optical cavity QED configuration that is described by a dissipative version of the Lipkin-Meshkov-Glick model of an infinitely coordinated spin system. This open quantum system exhibits both first- and second-order non-equilibrium quantum phase transitions as a single, effective field parameter is varied. Light emitted from the cavity offers measurable signatures of the critical behavior, including that of the spin-spin entanglement.
We investigate the behavior of a circuit QED device when the resonator is initially populated with a mesoscopic coherent field. The strong coupling between the cavity and the qubit produces an entangled state involving mesoscopic quasi-pointer states with respect to cavity dissipation. The overlap of the associated field components results in collapse and revivals for the Rabi oscillation. Although qubit relaxation and dephasing do not preserve these states, a simple analytical description of the dissipative dynamics of the circuit QED device including cavity relaxation as well as qubit dissip…
We extend Schwinger's ideas regarding sonoluminescence by explicitly calculating the Bogolubov coefficients relating the QED vacuum states associated with changes in a dielectric bubble. Sudden (non-adiabatic) changes in the refractive index lead to an efficient production of real photons with a broadband spectrum, and a high-frequency cutoff that arises from the asymptotic behaviour of the dielectric constant.
The whispering gallery modes (WGMs) of quartz microspheres are investigated for the purpose of strong coupling between single photons and atoms in cavity quantum electrodynamics (cavity QED). Within our current understanding of the loss mechanisms of the WGMs, the saturation photon number, n, and critical atom number, N, cannot be minimized simultaneously, so that an "optimal" sphere size is taken to be the radius for which the geometric mean, (n x N)^(1/2), is minimized. While a general treatment is given for the dimensionless parameters used to characterize the atom-cavity system, detailed c…
We investigate the influence of temperature and dissipation on the Landau-Zener transition probability in circuit QED. Dissipation is modelled by coupling the transmission line to a bath of harmonic oscillators. The reduced description for the density operator is treated within Bloch-Redfield theory. A phase-space representation allows an efficient numerical implementation of the resulting master equation. It provides reliable results which are valid even for rather low temperatures. We find that the spin-flip probability as a function of temperature and dissipation strength exhibits a non-mon…
Using carefully designed hybrid metal-dielectric resonators, we study molecular optomechanics in the strong coupling regime ($g_{\rm }^2/ω_m {>} κ$), which manifests in anharmonic emission lines in the sideband-resolved region of the cavity-emitted spectrum ($κ{<}ω_m$). This nonlinear optomechanical strong coupling regime is enabled through a metal-dielectric cavity system that yields not only deep sub-wavelength plasmonic confinement, but also dielectric-like confinement times that are more than two orders of magnitude larger than those from typical localized plasmon modes. These hybrid metal…
We examine the routing scheme of single photons in a one-dimensional periodic chain of two-level quantum emitters (QEs) strongly coupled to two waveguides in a ladder configuration. It is known that for a single-emitter chiral waveguide ladder setting, photons can be redirected from one waveguide to another with a $100\%$ probability (deterministically) provided the resonance condition is met and spontaneous emission is completely ignored. However, when the spontaneous emission is included the routing scheme becomes considerably imperfect. In this paper, we present a solution to this issue by …
We discuss the equilibrium and out of equilibrium dynamics of cavity QED in presence of dissipation beyond the standard perturbative treatment of losses. Using the dynamical polaron \emph{ansatz} and Matrix Product State simulations, we discuss the case where both light-matter $g$-coupling and system-bath interaction are in the ultrastrong coupling regime. We provide a critical $g$ for the onset of Rabi oscillations. Besides, we demonstrate that the qubit is \emph{dressed} by the cavity and dissipation. That such dressing governs the dynamics and, thus, it can be measured. Finally, we sketch a…
Condensed matter physics has been driven forward by significant experimental and theoretical progress in the study and understanding of equilibrium phase transitions based on symmetry and topology. However, nonequilibrium phase transitions have remained a challenge, in part due to their complexity in theoretical descriptions and the additional experimental difficulties in systematically controlling systems out of equilibrium. Here, we study a one-dimensional chain of 72 microwave cavities, each coupled to a superconducting qubit, and coherently drive the system into a nonequilibrium steady sta…
We present a theoretical treatment for the dissipative two-resonator circuit quantum electrodynamics setup referred to as quantum switch. There, switchable coupling between two superconducting resonators is mediated by a superconducting qubit operating in the dispersive regime, where the qubit transition frequency is far detuned from those of the resonators. We derive an effective Hamiltonian for the quantum switch beyond the rotating wave approximation and study the dissipative dynamics within a Bloch-Redfield quantum master equation approach. We derive analytically how the qubit affects the …
Here we consider the continuous pumping of a dissipative QED cavity and derive the time-dependent density operator of the cavity field prepared initially as a superposition of mesoscopic coherent states. The control of the coherence of this superposition is analyzed considering the injection of a beam of two-level Rydberg atoms through the cavity. Our treatment is compared to other approaches.
Scaling law for optimal excitation storage and superradiant release in waveguide QED systems
National Taiwan University（台湾大学）；Institute of Atomic and Molecular Sciences, Academia Sinica（中央研究院原子与分子科学研究所）；Center for Quantum Science and Engineering, National Taiwan University（台湾大学量子科学与工程中心）；Trapped-Ion Quantum Computing Laboratory, Hon Hai Research Institute（鸿海研究院会离子阱量子计算实验室）；Physics Division, National Center for Theoretical Sciences（国家理论科学中心物理组）；Department of Physics, National Central University（中央大学物理系）
We investigate a two-level atom coupled to a cavity with a strong classical driving field in a dissipative environment and find an analytical expression of the time evolution density matrix for the system. The analytical density operator is then used to study the entanglement between the atom and cavity by considering the competing process between the atom-field interactions and the field-environment interactions. It is shown that there is an optimal interaction time for generating atom-cavity entanglement.
In spite of decades of effort, it has not yet been possible to create single-mode multiphoton states of light with high success probability and near unity fidelity. Complex quantum states of propagating optical photons would be an enabling resource for diverse protocols in quantum information science, including for interconnecting quantum nodes in quantum networks. Here, we propose several methods to generate heralded mutipartite entangled atomic and photonic states by using the strong and long-range dissipative couplings between atoms emerging in waveguide QED setups. Our theoretical analysis…
After giving an outline of the quantization scheme based on the microscopic Hopfield model of a dielectric bulk material, we show how the classical phenomenological Maxwell equations of the electromagnetic field in the presence of dielectric matter of given space- and frequency-dependent complex permittivity can be transferred to quantum theory. Including in the theory the interaction of the medium-assisted field with atomic systems, we present both the minimal-coupling Hamiltonian and the multipolar-coupling Hamiltonian in the Coulomb gauge. To illustrate the concept, we discuss the input--ou…
We introduce a second quantization scheme based on quasinormal modes, which are the dissipative modes of leaky optical cavities and plasmonic resonators with complex eigenfrequencies. The theory enables the construction of multi-plasmon/photon Fock states for arbitrary three-dimensional dissipative resonators and gives a solid understanding to the limits of phenomenological dissipative Jaynes-Cummings models. In the general case, we show how different quasinormal modes interfere through an off-diagonal mode coupling and demonstrate how these results affect cavity-modified spontaneous emission.…
By exploiting the nonlinear nature of the Jaynes Cumming's interaction, one can get photon population trapping in cavity-QED arrays. However, the unavoidable dissipative effects in a realistic system would destroy the self-trapped state by continuous photon leakage. To circumvent this issue, we show that a careful engineering of drive, dissipation and Hamiltonian results in achieving indefinitely sustained self-trapping. We show that the intricate interplay between drive, dissipation, and light-matter interaction results in requiring an optimal window of drive strengths in order to achieve suc…
We propose an experiment with two coupled microwave cavities and a "tunneling" photon observed by the passage of Rydberg atoms. We model the coupled cavities as in Ref. \cite{art1} and include dissipative effects as well as limited detection efficiency. We also consider realistic finite atom-field interaction times and provide for a simple analytical expression for the photon "tunneling" probability including all these effects. We show that for sufficiently small dissipation constants the effect can be observed with current experimental facilities.
We calculate the transmission spectra of a flux qubit coupled to a dissipative resonator in the ultrastrong coupling regime. Such a qubit-oscillator system constitutes the building block of superconducting circuit QED platforms. The calculated transmission of a weak probe field quantifies the response of the qubit, in frequency domain, under the sole influence of the oscillator and of its dissipative environment, an Ohmic heat bath. We find the distinctive features of the qubit-resonator system, namely two-dip structures in the calculated transmission, modified by the presence of the dissipati…
We study photon condensation phenomena in a driven and dissipative array of superconducting microwave resonators. Specifically, we show that by using an appropriately designed coupling of microwave photons to superconducting qubits, an effective dissipative mechanism can be engineered, which scatters photons towards low-momentum states while conserving their number. This mimics a tunable coupling of bosons to a low temperature bath, and leads to the formation of a stationary photon condensate in the presence of losses and under continuous-driving conditions. Here we propose a realistic experim…
In recent years, a rigorous quantum mechanical model for the interaction between light and macroscopic dispersive, lossy dielectrics has emerged -macroscopic QED- allowing the application of the usual methods of quantum field theory. Here, we apply time dependent perturbation theory to a general class of problems involving time dependent lossy, dispersive dielectrics. The model is used to derive polariton excitation rates in three illustrative cases, including that of a travelling Gaussian perturbation to the susceptibility of an otherwise infinite homogeneous dielectric, motivated by recent e…
A quantum damped-polariton model is constructed for an inhomogeneous anisotropic linear dielectric with arbitrary dispersion in space and time. The model Hamiltonian is completely diagonalized by determining the creation and annihilation operators for the fundamental polariton modes as specific linear combinations of the basic dynamical variables. Explicit expressions are derived for the time-dependent operators describing the electromagnetic field, the dielectric polarization and the noise term in the latter. It is shown how to identify bath variables that generate the dissipative dynamics of…
We derive expressions for the quantum electromagnetic field in a dispersive and dissipative dielectric medium, treating the medium as a continuum. We compare the Langevin approach with the Fano diagonalization procedure for the coupled system composed of the electromagnetic field, the dielectric medium, and the reservoir. In particular, we show that the quantized electric and magnetic fields obtained in both methods have exactly the same form. More generally, in thermal equilibrium, correlation functions computed in both methods are identical.
We have fabricated an atom chip device which combines the circuitry for magnetic trapping of cold atoms with high-finesse optical resonators suitable for cavity QED in the single-atom strong coupling regime. Fabry-Perot optical resonators with finesse F > 2 X 10^5 were formed between a micropatterned on-chip planar mirror with lateral dimension of < 100 um and a curved mirror suspended above the chip. The strong and rapid thermal coupling between on-chip electrical and optical elements was utilized to stabilize the cavity mirror separation with servo bandwidth exceeding 100 kHz during simulate…
A quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive and absorbing dielectric medium is developed. The classical Maxwell equations with spatially varying and Kramers-Kronig consistent permittivity are regarded as operator-valued field equations, introducing additional current- and charge-density operator fields in order to take into account the noise associated with the dissipation in the medium. It is shown that the equal-time commutation relations between the fundamental electromagnetic fields $\hat …
Discrete time crystals are a recently proposed and experimentally observed out-of-equilibrium dynamical phase of Floquet systems, where the stroboscopic evolution of a local observable repeats itself at an integer multiple of the driving period. We address this issue in a driven-dissipative setup, focusing on the modulated open Dicke model, which can be implemented by cavity or circuit QED systems. In the thermodynamic limit, we employ semiclassical approaches and find rich dynamical phases on top of the discrete time-crystalline order. In a deep quantum regime with few qubits, we find clear s…
We describe the transfer of quantum information and entanglement from three flying (radiation) to three localized (atomic) qubits via cavity modes resonantly coupled to the atoms, in the presence of a common reservoir. Upon addressing the full dynamics of the resulting nine-qubit open system, we find that once the cavities are fed, fidelity and transferred entanglement are optimal, while their peak values exponentially decrease due to dissipative processes. The external radiation is then turned off and quantum correlations oscillate between atomic and cavity qubits. For a class of mixtures of …
The interaction of quantum emitters with one-dimensional photon-like reservoirs induces strong and long-range dissipative couplings that give rise to the emergence of so-called Decoherence Free Subspaces (DFS) which are decoupled from dissipation. When introducing weak perturbations on the emitters, e.g., driving, the strong collective dissipation enforces an effective coherent evolution within the DFS. In this work, we show explicitly how by introducing single-site resolved drivings, we can use the effective dynamics within the DFS to design a universal set of one and two-qubit gates within t…
We present a fully analytical solution of the dynamics of two strongly-driven atoms resonantly coupled to a dissipative cavity field mode. We show that an initial atom-atom entanglement cannot be increased. In fact, the atomic Hilbert space divides into two subspaces, one of which is decoherence free so that the initial atomic entanglement remains available for applications, even in presence of a low enough atomic decay rate. In the other subspace a measure of entanglement, decoherence, and also purity, are described by a similar functional behavior that can be monitored by joint atomic measur…
Optical cavity QED provides a platform with which to explore quantum many-body physics in driven-dissipative systems. Single-mode cavities provide strong, infinite-range photon-mediated interactions among intracavity atoms. However, these global all-to-all couplings are limiting from the perspective of exploring quantum many-body physics beyond the mean-field approximation. The present work demonstrates that local couplings can be created using multimode cavity QED. This is established through measurements of the threshold of a superradiant, self-organization phase transition versus atomic pos…
We study dynamical phase transitions (DPT) in the driven and damped Dicke model, realizable for example by a driven atomic ensemble collectively coupled to a damped cavity mode. These DPTs are characterized by non-analyticities of certain observables, primarily the overlap of time evolved and initial state. Even though the dynamics is dissipative, this phenomenon occurs for a wide range of parameters and no fine-tuning is required. Focusing on the state of the 'atoms' in the limit of a bad cavity, we are able to asymptotically evaluate an exact path integral representation of the relevant over…
A wide variety of dissipative and fluctuation problems involving a quantum system in a heat bath can be described by the independent-oscillator (IO) model Hamiltonian. Using Heisenberg equations of motion, this leads to a generalized quantum Langevin equation (QLE) for the quantum system involving two quantities which encapsulate the properties of the heat bath. Applications include: atomic energy shifts in a blackbody radiation heat bath; solution of the problem of runaway solutions in QED; electrical circuits (resistively shunted Josephson barrier, microscopic tunnel junction, etc.); conduct…
Microscopic theory of exciton-polariton model involving multiple molecules: Macroscopic quantum electrodynamics formulation and essence of direct intermolecular interactions
In a companion paper [quant-ph/9904013] we have investigated several variations of Schwinger's proposed mechanism for sonoluminescence. We demonstrated that any realistic version of Schwinger's mechanism must depend on extremely rapid (femtosecond) changes in refractive index, and discussed ways in which this might be physically plausible. To keep that discussion tractable, the technical computations in that paper were limited to the case of a homogeneous dielectric medium. In this paper we investigate the additional complications introduced by finite-volume effects. The basic physical scenari…
We propose a cavity QED setup which implements a dissipative Lipkin-Meshkov-Glick model -- an interacting collective spin system. By varying the external model parameters the system can be made to undergo both first-and second-order quantum phase transitions, which are signified by dramatic changes in cavity output field properties, such as the probe laser transmission spectrum. The steady-state entanglement between pairs of atoms is shown to peak at the critical points and can be experimentally determined by suitable measurements on the cavity output field. The entanglement dynamics also exhi…
We present theoretical transmission spectra of a strongly driven, damped, flux qubit coupled to a dissipative resonator in the ultrastrong coupling regime. Such a qubit-oscillator system, described within a dissipative Rabi model, constitutes the building block of superconducting circuit QED platforms. The addition of a strong drive allows one to characterize the system properties and study novel phenomena, leading to a better understanding and control of the qubit-oscillator system. In this work, the calculated transmission of a weak probe field quantifies the response of the qubit, in freque…
Various aspects of dissipative and nondissipative decoherence of Rabi oscillations are discussed in the context of field quantization in alternative representations of CCR. Theory is confronted with experiment, and a possibility of more conclusive tests is analyzed.
We propose a scheme for the quantum non-demolition (QND) measurement of Fock states of a nanomechanical resonator via feedback control of a coupled circuit QED system. A Cooper pair box (CPB) is coupled to both the nanoresonator and microwave cavity. The CPB is read-out via homodyne detection on the cavity and feedback control is used to effect a non-dissipative measurement of the CPB. This realizes an indirect QND measurement of the nanoresonator via a second-order coupling of the CPB to the nanoresonator number operator. The phonon number of the Fock state may be determined by integrating th…
By numerically calculating the time-evolved Wigner functions, we investigate the dynamics of a few-photon superposed (e.g., up to two ones) state in a dissipating cavity. It is shown that, the negativity of the Wigner function of the photonic state unquestionably vanishes with the cavity's dissipation. As a consequence, the nonclassical effects related to the negativity of the Wigner function should be weakened gradually. However, it is found that the value of the second-order correlation function $g^{(2)}(0)$ (which serves usually as the standard criterion of a typical nonclassical effect, i.…
Within the framework of exact quantization of the electromagnetic field in dispersing and absorbing media the input-output problem of a high-$Q$ cavity is studied, with special emphasis on the absorption losses in the coupling mirror. As expected, the cavity modes are found to obey quantum Langevin equations, which could be also obtained from quantum noise theories, by appropriately coupling the cavity modes to dissipative systems, including the effect of the mirror-assisted absorption losses. On the contrary, the operator input-output relations obtained in this way would be incomplete in gene…
We propose a quantum metrology scheme in a cavity QED setup to achieve the Heisenberg limit. In our scheme, a series of identical two-level atoms randomly pass through and interact with a dissipative single-mode cavity. Different from the entanglement based Heisenberg limit metrology scheme, we do not need to prepare the atomic entangled states before they enter into the cavity. We show that the initial atomic coherence will induce an effective driving to the cavity field, whose steady state is an incoherent superposition of orthogonal states, with the superposition probabilities being depende…
