Caslav Brukner, Vlatko Vedral
We show that macroscopic thermodynamical properties - such as functions of internal energy and magnetization - can detect quantum entanglement in solids at nonzero temperatures in the thermodynamical limit. We identify the parameter regions (critical values of magnetic field and temperature) within which entanglement is witnessed by these thermodynamical quantities.
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We show how the spatial macroscopic entanglement equivalent to the off diagonal long range order (ODLRO) implies the Meissner effect and flux quantisation for a superconductor. It is argued by analogy with superconductors that the Higgs field must also be entangled in the same way. Internal (spin) entanglement is shown to be irrelevant within this context, although it can of course also be computed.
We describe a set of measurement protocols for performing non-classicality tests and the verification of entangled superposition states of macroscopic continuous variable systems, such as nanomechanical resonators. Following earlier works, we first consider a setup where a two-level system is used to indirectly probe the motion of the mechanical system via Ramsey measurements and discuss the application of this methods for detecting non-classical mechanical states. We then show that the generalization of this techniques to multiple resonator modes allows the conditioned preparation and the det…
We show that if the ground state entanglement exceeds the total entropy of a given system, then this system is in an entangled state. This is a universal entanglement witness that applies to any physical system and yields a temperature below which we are certain to find some entanglement. Our witness is then applied to generic bosonic and fermionic many body systems to derive the corresponding "critical" temperatures that have a very broad validity.
Quantum entanglement is a fascinating phenomenon, especially if it is observed at the macroscopic scale. Importantly, macroscopic quantum correlations can be revealed only by accurate measurement outcomes and strategies. Here, we formulate feasible entanglement witnesses for bright squeezed vacuum in the form of the macroscopically populated polarization triplet Bell states. Their testing involves efficient photodetection and the measurement of the Stokes operators variances. We also calculate the measures of entanglement for these states such as the Schmidt number and the logarithmic negativi…
Temporal witnesses of non-classicality in a macroscopic biological system
针对宏观生物系统中激子转移的非经典性验证问题，提出新的非经典性见证方法与通用量子比特转移模型，讨论环境退相干影响，为复杂生物分子量子特性测试提供新方案。
Testing quantum theory on macroscopic scales is a longstanding challenge that might help to revolutionise physics. For example, laboratory tests (such as those anticipated in nanomechanical or biological systems) may look to rule out macroscopic realism: the idea that the properties of macroscopic objects exist objectively and can be non-invasively measured. Such investigations are likely to suffer from i) stringent experimental requirements, ii) marginal statistical significance and iii) logical loopholes. We address all of these problems by refining two tests of macroscopic realism, or `quan…
Detecting entanglement from macroscopic measurements of the electric field and its fluctuations
本文提出基于电场正交分量和总荧光的纠缠见证族，无需态层析即可从几乎任意方向探测大型开放量子系统中的纠缠，适用于冷原子、囚禁离子、色心和超导量子比特等泡利群发射体。
Detecting quantum properties in physical systems using proxy witnesses
本文提出代理见证方法，用于检测宏观量子系统中难以直接观测的微观量子属性，如不可扩展性、相干性等，并在海森堡和J1-J2模型中验证其有效性。
This paper summarises the results of our research on macroscopic entanglement in spin systems and free Bosonic gases. We explain how entanglement can be observed using entanglement witnesses which are themselves constructed within the framework of thermodynamics and thus macroscopic observables. These thermodynamical entanglement witnesses result in bounds on macroscopic parameters of the system, such as the temperature, the energy or the susceptibility, below which entanglement must be present. The derived bounds indicate a relationship between the occurrence of entanglement and the establish…
The entanglement in a general mixed spin chain with arbitrary spin $S$ and 1/2 is investigated in the thermodynamical limit. The entanglement is witnessed by the magnetic susceptibility which decides a characteristic temperature for an entangled thermal state. The characteristic temperature is nearly proportional to the interaction $J$ and the mixed spin $S$. The bound of negativity is obtained on the basis of the magnetic susceptibility. It is found that the macroscopic magnetic properties are affected by the quantum entanglement in the real solids. Meanwhile, the entanglement can be quantita…
Entanglement is a ubiquitous feature of low temperature systems and believed to be highly relevant for the dynamics of condensed matter properties and quantum computation even at higher temperatures. The experimental certification of this paradigmatic quantum effect in macroscopic high temperature systems is constrained by the limited access to the quantum state of the system. In this paper we show how macroscopic observables beyond the energy of the system can be exploited as proxy witnesses for entanglement detection. Using linear and semi-definite relaxations we show that all previous appro…
Here we investigate the impact of temporal entanglement on a system's ability to perform thermodynamical work. We show that while the quantum version of the Jarzynski equality remains satisfied even in the presence of temporal entanglement, the individual thermodynamical work moments in the expansion of the free energy are, in fact, sensitive to the genuine quantum correlations. Therefore, while individual moments of the amount of thermodynamical work can be larger (or smaller) quantumly than classically, when they are all combined together into the (exponential of) free energy, the total effe…
Why we do not see large macroscopic objects in entangled states? There are two ways to approach this question. The first is dynamic: the coupling of a large object to its environment cause any entanglement to decrease considerably. The second approach, which is discussed in this paper, puts the stress on the difficulty to observe a large scale entanglement. As the number of particles n grows we need an ever more precise knowledge of the state, and an ever more carefully designed experiment, in order to recognize entanglement. To develop this point we consider a family of observables, called wi…
Thermodynamics is a macroscopic physical theory whose two very general laws are independent of any underlying dynamical laws and structures. Nevertheless, its generality enables us to understand a broad spectrum of phenomena in physics, information science and biology. Recently, it has been realised that information storage and processing based on quantum mechanics can be much more efficient than their classical counterpart. What general bound on storage of quantum information does thermodynamics imply? We show that thermodynamics implies a weaker bound than the quantum mechanical one (the Hol…
Macroscopic realism, the classical world view that macroscopic objects exist independently of and are not influenced by measurements, is usually tested using Leggett-Garg inequalities. Recently, another necessary condition called no-signaling in time (NSIT) has been proposed as a witness for non-classical behavior. In this paper, we show that a combination of NSIT conditions is not only necessary but also sufficient for a macrorealistic description of a physical system. Any violation of macroscopic realism must therefore be witnessed by a suitable NSIT condition. Subsequently, we derive an ope…
We present a general argument showing that the temperature as well as other thermodynamical state variables can qualify as entanglement witnesses for spatial entanglement. This holds for a variety of systems and we exemplify our ideas using a simple free non-interacting Bosonic gas. We find that entanglement can exist at arbitrarily high temperatures, provided that we can probe smaller and smaller regions of space. We then discuss the relationship between the occurrence of Bose-Einstein condensation and our conditions for the presence of entanglement and compare the respective critical tempera…
The task of testing whether quantum theory applies to all physical systems and all scales requires considering situations where a quantum probe interacts with another system that need not obey quantum theory in full. Important examples include the cases where a quantum mass probes the gravitational field, for which a unique quantum theory of gravity does not yet exist, or a quantum field, such as light, interacts with a macroscopic system, such as a biological molecule, which may or may not obey unitary quantum theory. In this context a class of experiments has recently been proposed, where th…
The canonical quantization of macroscopic electromagnetism was recently presented in New J. Phys. 12 (2010) 123008. This theory is here used to derive the Casimir effect, by considering the special case of thermal and zero-point fields. The stress-energy-momentum tensor of the canonical theory follows from Noether's theorem, and its electromagnetic part in thermal equilibrium gives the Casimir energy density and stress tensor. The results hold for arbitrary inhomogeneous magnetodielectrics and are obtained from a rigorous quantization of electromagnetism in dispersive, dissipative media. Conti…
Evidencing Quantum Gravity with Thermodynamical Observables
通过测量玻色气体的比热，研究引力相互作用的量子化特征，区分经典与量子引力相互作用。
We review experiments and theoretical models about the possible mutual interplay between the gravitational field and materials in the superconducting state or other macroscopic quantum states. More generally, we focus on the possibility for quantum macrosystems in a coherent state to produce local alterations of the gravitational field in which they are immersed. This fully interdisciplinary research field has witnessed a conspicuous progress in the last decades, with hundreds of published papers, and yet several questions are still completely open.
The current-carrying steady-state that arises in the middle of a metallic wire connected to macroscopic leads is characterized regarding its response functions, correlations and entanglement entropy. The spectral function and the dynamical structure factor show clear non-equilibrium signatures accessible by state-of-the-art techniques. In contrast with the equilibrium case, the entanglement entropy is extensive with logarithmic corrections at zero-temperature that depend on the wire-leads coupling and, in a non-analytic way, on voltage. This shows that some robust universal quantities found in…
We demonstrate that the presence of entanglement in macroscopic bodies (e.g. solids) in thermodynamical equilibrium could be revealed by measuring heat-capacity. The idea is that if the system were in a separable state, then for certain Hamiltonians heat capacity would not tend asymptotically to zero as the temperature approaches absolute zero. Since this would contradict the third law of thermodynamics, one concludes that the system must contain entanglement. The separable bounds are obtained by minimization of the heat capacity over separable states and using its universal low-temperature be…
In this paper I intend to show that macroscopic entanglement is possible at high temperatures. I analyze multipartite entanglement produced by the $η$ pairing mechanism which features strongly in the fermionic lattice models of high $T_c$ superconductivity. This problem is shown to be equivalent to calculating multipartite entanglement in totally symmetric states of qubits. I demonstrate that we can conclusively calculate the relative entropy of entanglement within any subset of qubits in an overall symmetric state. Three main results then follow. First, I show that the condition for supercond…
Investigation of states with a periodic time dependence of physical quantities attracts a considerable interest now. Although it has been proposed initially that such states (coined Quantum Time Crystals) might be macroscopic and thermodynamically stable, results of a more careful study of the problem seemed to indicate that quantum time crystals could be realized only in systems out of equilibrium. Here we show that, in contrast to the general belief, thermodynamically stable macroscopic quantum time crystals can exist. The order parameter of this new state of matter is periodic in both real …
Precision bounds for bosonic quantum batteries
研究通过非高斯性提升玻色量子电池的充电精度，提出线性光电检测模型并验证非高斯性作为资源的可行性。
Entanglement is a vital property of multipartite quantum systems, characterised by the inseparability of quantum states of objects regardless of their spatial separation. Generation of entanglement between increasingly macroscopic and disparate systems is an ongoing effort in quantum science which enables hybrid quantum networks, quantum-enhanced sensing, and probing the fundamental limits of quantum theory. The disparity of hybrid systems and the vulnerability of quantum correlations have thus far hampered the generation of macroscopic hybrid entanglement. Here we demonstrate, for the first t…
Genuine Hybrid Number-Polarization Entanglement
本文通过自发参量下转换产生的宏观贝尔态，提出并验证了一种操作性的判据，用于检测超越连续-离散变量分类的真正混合数-偏振纠缠。
Operational entanglement of collective quantum modes at room temperature
该研究在室温下展示了集体量子模式的操作纠缠，通过推导纠缠边界并验证稳态纠缠的维持条件，建立了连接动力学、噪声和宏观纠缠认证的理论框架。
We consider two non-interacting infinite quantum spin chains immersed in a common thermal environment and undergoing a local dissipative dynamics of Lindblad type. We study the time evolution of collective mesoscopic quantum spin fluctuations that, unlike macroscopic mean-field observables, retain a quantum character in the thermodynamical limit. We show that the microscopic dissipative dynamics is able to entangle these mesoscopic degrees of freedom, through a purely mixing mechanism. Further, the behaviour of the dissipatively generated quantum correlations between the two chains is studied …
The relationship between the mean-field approximations in various interacting models of statistical physics and measures of classical and quantum correlations is explored. We present a method that allows us to bound the total amount of correlations (and hence entanglement) in a physical system in thermal equilibrium at some temperature in terms of its free energy and internal energy. This method is first illustrated using two qubits interacting through the Heisenberg coupling, where entanglement and correlations can be computed exactly. It is then applied to the one dimensional Ising model in …
A mesoscopic system of a few particles exhibits behaviors that strongly differ from those of a macroscopic system. While in a macroscopic system phase transitions are universal, a change in the state of a mesoscopic system depends on its specific properties, like the number of particles, to the point that changes of state can be disfavored for specific magic numbers. A transition that has no counterpart in the macroscopic world is orientational melting, in which localized particles with long-range repulsive interactions forming a two-dimensional crystal become delocalized in common circular or…
A theory recently proposed by the author aims to explain decoherence and the thermodynamical behaviour of closed systems within a conservative, unitary, framework for quantum gravity by assuming that the operators tied to the gravitational degrees of freedom are unobservable and equating physical entropy with matter-gravity entanglement entropy. Here we obtain preliminary results on the extent of decoherence this theory predicts. We treat first a static state which, if one were to ignore quantum gravitational effects, would be a quantum superposition of two spatially displaced states of a sing…
Descriptions of molecular systems usually refer to two distinct theoretical frameworks. On the one hand the quantum pure state, i.e. the wavefunction, of an isolated system which is determined to calculate molecular properties and to consider the time evolution according to the unitary Schrödinger equation. On the other hand a mixed state, i.e. a statistical density matrix, is the standard formalism to account for thermal equilibrium, as postulated in the microcanonical quantum statistics. In the present paper an alternative treatment relying on a statistical analysis of the possible wavefunct…
Witnessing Spin-Orbital Entanglement using Resonant Inelastic X-Ray Scattering
提出基于共振非弹性X射线散射（RIXS）谱构建厄米生成元，计算量子Fisher信息（QFI）以检测自旋-轨道纠缠，并扩展至有限偏振分辨的松弛QFI界。
Witnessing Light-Driven Entanglement using Time-Resolved Resonant Inelastic X-Ray Scattering
提出利用时间分辨共振非弹性X射线散射量化量子材料瞬态的量子Fisher信息和纠缠深度，以扩展Hubbard模型验证效率并预测光增强多体纠缠，为实验观测和控制光驱动纠缠奠定基础。
Phase transitions are commonly held to occur only in the thermodynamical limit of large number of system components. Here we exemplify at the hand of the exactly solvable Jaynes-Cummings (JC) model and its generalization to finite JC-lattices that finite component systems of coupled spins and bosons may exhibit quantum phase transitions (QPT). For the JC-model we find a continuous symmetry-breaking QPT, a photonic condensate with a macroscopic occupation as the ground state and a Goldstone mode as a low-energy excitation. For the two site JC-lattice we show analytically that it undergoes a Mot…
Why is thermalisation a universal phenomenon? How does a quantum system reach thermodynamical equilibrium? These questions are not new, dating even from the very birth of quantum theory and have been the subject of a renewed interest over the two last decades (see for instance the review in Eisert et al, Nature Physics 2015). In this work, we propose a universal model demonstrating that thermalisation of a small quantum system is an emergent property of the unitary evolution under a Schrödinger equation of a larger composite system, whose initial state can be arbitrary. We show that the origin…
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