We propose a novel scheme for the lithography of arbitrary, two-dimensional nanostructures via matter-wave interference. The required quantum control is provided by a pi/2-pi-pi/2 atom interferometer with an integrated atom lens system. The lens system is developed such that it allows simultaneous control over atomic wave-packet spatial extent, trajectory, and phase signature. We demonstrate arbitrary pattern formations with two-dimensional 87Rb wavepackets through numerical simulations of the scheme in a practical parameter space. Prospects for experimental realizations of the lithography scheme are also discussed.
The wave-particle duality of massive objects is a cornerstone of quantum physics and a key property of many modern tools such as electron microscopy, neutron diffraction or atom interferometry. Here we report on the first experimental demonstration of quantum interference lithography with complex molecules. Molecular matter-wave interference patterns are deposited onto a reconstructed Si(111) 7x7 surface and imaged using scanning tunneling microscopy. Thereby both the particle and the quantum wave character of the molecules can be visualized in one and the same image. This new approach to nano…
In this paper, we present a brief overview of atom interferometry. This field of research has developed very rapidly since 1991. Atom and light wave interferometers present some similarities but there are very important differences in the tools used to manipulate these two types of waves. Moreover, the sensitivity of atomic waves and light waves to their environment is very different. Atom interferometry has already been used for a large variety of studies: measurements of atomic properties and of inertial effects (accelerations and rotations), new access to some fundamental constants, observa…
Implications of field quantization on Ramsey interferometry are discussed and general conditions for the occurrence of interference are obtained. Interferences do not occur if the fields in two Ramsey zones have precise number of photons. However in this case we show how two atom (like two photon) interferometry can be used to discern a variety of interference effects as the two independent Ramsey zones get entangled by the passage of first atom. Generation of various entangled states like |0,2>+|2,0> are discussed and in far off resonance case generation of entangled state of two coherent sta…
We illustrate how geometric gauge forces and topological phase effects emerge in quantum systems without employing assumptions that rely on adiabaticity. We show how geometric magnetism may be harnessed to engineer novel quantum devices including a velocity sieve, a component in mass spectrometers, for neutral atoms or neutrons. We outline a possible experimental setup that demonstrates topological interferometry for neutral spin 1/2 systems.
It is a commonly stated that the acceleration sensitivity of an atom interferometer is proportional to the space-time area enclosed between the two interfering arms. Here we derive the interferometric phase shift for an extensive class of interferometers, and explore the circumstances in which only the inertial terms contribute. We then analyse various configurations in light of this geometric interpretation of the interferometric phase shift.
We have built an atom interferometer and, by applying an electric field on one of the two interfering beams, we have measured the static electric polarizability of lithium with a 0.66 % uncertainty. Our experiment is similar to an experiment done on sodium in 1995 by D. Pritchard and co-workers, with several improvements: the electric field can be calculated analytically and our phase measurements are very accurate. This experiment illustrates the extreme sensitivity of atom interferometry: when the atom enters the electric field, its velocity increases and the fractional change, equal to 4 x …
We study the preparation and manipulation of states involving a small number of interacting particles. By controlling the splitting and fusing of potential wells, we show how to interconvert Mott-insulator-like and trapped BEC-like states. We also discuss the generation of "Schrödinger cat" states by splitting a microtrap and taking into practical consideration the asymmetry between the resulting wells. These schemes can be used to perform multiparticle interferometry with neutral atoms, where interference effects can be observed only when all the participating particles are measured.
A method for mitigating the readout delay characteristic of Bragg-based atom interferometry is presented, utilizing an asymmetric Mach-Zehnder interferometer sequence to generate spatial fringes that are read out while still overlapped. The time of flight after the final beamsplitter is engineered to facilitate constructive overlap of the fringes on the output states. A noise analysis performed using a precision atom interferometer is presented, comparing the traditional separated symmetric scheme with that of the separated and overlapped asymmetric scheme showing no significant increase in sh…
We report on a novel experiment to generate non-classical atomic states via quantum non-demolition (QND) measurements on cold atomic samples prepared in a high finesse ring cavity. The heterodyne technique developed for the QND detection exhibits an optical shot-noise limited behavior for local oscillator optical power of a few hundred \muW, and a detection bandwidth of several GHz. This detection tool is used in single pass to follow non destructively the internal state evolution of an atomic sample when subjected to Rabi oscillations or a spin-echo interferometric sequence.
We propose a Ramsey interferometry experiment using an entangled state of N atoms to reach the Heisenberg limit for the estimation of an atomic phase shift if the atom number parity is perfectly determined. In a more realistic situation, due to statistical fluctuations of the atom source and the finite detection efficiency, the parity is unknown. We then achieve about half the Heisenberg limit. The scheme involves an ensemble of circular Rydberg atoms which dispersively interact successively with two initially empty microwave cavities. The scheme does not require very high-Q cavities. An exper…
A quantum gravity-gradiometer consists of two spatially separated ensembles of atoms interrogated by pulses of a common laser beam. Laser pulses cause the probability amplitudes of atomic ground-state hyperfine levels to interfere, producing two motion-sensitive phase shifts which allow the measurement of the average acceleration of each ensemble, and, via simple differencing, of the acceleration gradient. Here I propose entangling the quantum states of the two ensembles prior to the pulse sequence, and show that entanglement encodes their relative acceleration in a single interference phase w…
A new technique for maintaining high contrast in an atom interferometer is used to measure large de Broglie wave phase shifts. Dependence of an interaction induced phase on the atoms' velocity is compensated by applying an engineered \emph{counter phase}. The counter phase is equivalent to a rotation and precisely determined by a frequency, and can be used to measure phase shifts due to interactions of unknown strength. Phase shifts of 150 radians (5 times larger than previously possible) have now been measured in an atom beam interferometer and we suggest that this technique can enable compar…
Quantum non-locality based on the well-known Bell inequality is of kinematic nature. A different type of quantum non-locality, the non-locality of the quantum equation of motion, is recently put forward with connection to the Aharonov-Bohm effect [Nature Phys. 6, 151 (2010)]. Evolution of the displacement operator provides an example to manifest such dynamic quantum non-locality. We propose an experiment using single-atom interferometry to test such dynamic quantum non-locality. We show how to measure evolution of the displacement operator with clod atoms in a spin-dependent optical lattice po…
A novel atomic beam splitter, using reflection of atoms off an evanescent light wave, is investigated theoretically. The intensity or frequency of the light is modulated in order to create sidebands on the reflected de Broglie wave. The weights and phases of the various sidebands are calculated using three different approaches: the Born approximation, a semiclassical path integral approach, and a numerical solution of the time-dependent Schrödinger equation. We show how this modulated mirror could be used to build practical atomic interferometers.
Atom matterwave interferometry requires mirror and beamsplitter pulses that are robust to inhomogeneities in field intensity, magnetic environment, atom velocity and Zeeman sub-state. Pulse shapes determined using quantum control methods offer significantly improved interferometer performance by allowing broader atom distributions, larger interferometer areas and higher contrast. We have applied gradient ascent pulse engineering (GRAPE) to optimise the design of phase-modulated mirror pulses for a Mach-Zehnder light-pulse atom interferometer, with the aim of increasing fringe contrast when ave…
Bragg diffraction is comparable to a hard-wall reflection if the Bragg condition is exactly fulfilled. However, in a neutron interferometer in the gravitational field (COW experiment) this is not the case and the momentum transfers should not be described by hard wall reflection, as it has been done in the commented article. Instead, and quite similar to the atom case, each mirror or beam splitter creates a constant momentum transfer given by the reciprocal lattice vector of the Bragg crystal. To lowest order there are no differences between the atom and the neutron case.
We examine the passage of ultracold two-level atoms through two separated laser fields for the nonresonant case. We show that implications of the atomic quantized motion change dramatically the behavior of the interference fringes compared to the semiclassical description of this optical Ramsey interferometer. Using two-channel recurrence relations we are able to express the double-laser scattering amplitudes by means of the single-laser ones and to give explicit analytical results. When considering slower and slower atoms, the transmission probability of the system changes considerably from a…
Recent progress in generating entangled spin states of neutral atoms provides opportunities to advance quantum sensing technology. In particular, entanglement can enhance the performance of accelerometers and gravimeters based on light-pulse atom interferometry. We study the effects of error sources that may limit the sensitivity of such devices, including errors in the preparation of the initial entangled state, imperfections in the laser pulses, momentum spread of the initial atomic wave packet, measurement errors, spontaneous emission, and atom loss. We determine that, for each of these err…
The advantages of light and matter-wave Sagnac interferometers -- large area on one hand and high rotational sensitivity per unit area on the other -- can be combined utilizing ultra-slow light in cold atomic gases. While a group-velocity reduction alone does not affect the Sagnac phase shift, the associated momentum transfer from light to atoms generates a coherent matter-wave component which gives rise to a substantially enhanced rotational signal. It is shown that matter-wave sensitivity in a large-area interferometer can be achieved if an optically dense vapor at sub-recoil temperatures is…
We apply the new constraints from atom-interferometry searches for screening mechanisms to the symmetron model, finding that these experiments exclude a previously unexplored region of parameter space. We discuss the possibility of networks of domain walls forming in the vacuum chamber, and how this could be used to discriminate between models of screening.
We provide an introduction into the field of atom optics and review our work on interferometry with cold atoms, and in particular with Bose-Einstein condensates. Here we emphasize applications of atom interferometry with sources of this kind. We discuss tests of the equivalence principle, a quantum tiltmeter, and a gravimeter.
We theoretically investigate the use of quantum non-demolition measurement to enhance the sensitivity of atom interferometry with Bose-condensed atoms. In particular, we are concerned with enhancing existing high-precision atom interferometry apparatuses, so restrict ourselves to dilute atomic samples, and the use of free-propagating light, or optical cavities in the weak-coupling regime. We find the optimum parameter regime that balances between spin squeezing and atomic loss, and find that significant improvements in sensitivity are possible. Finally, we consider the use of squeezed light, a…
We propose a scheme to significantly enhance the sensitivity of atom-interferometry performed with Bose-Einstein condensates. When a two-photon Raman transition is used to split the condensate into two modes, some information about the number of atoms in one of the modes is transferred to one of the optical modes. We introduce a simple model to describe this process, and find that by processing this information in an appropriate way, the sensitivity of atom interferometry can be enhanced by more than a factor of 10 for realistic parameters.
We demonstrate matterwave interference in a warm vapor of rubidium atoms. Established approaches to light pulse atom interferometry rely on laser cooling to concentrate a large ensemble of atoms into a velocity class resonant with the atom optical light pulse. In our experiment, we show that clear interference signals may be obtained without laser cooling. This effect relies on the Doppler selectivity of the atom interferometer resonance. This interferometer may be configured to measure accelerations, and we demonstrate that multiple interferometers may be operated simultaneously by addressing…
Inertial sensors based on cold atoms have great potential for navigation, geodesy, or fundamental physics. Similar to the Sagnac effect, their sensitivity increases with the space-time area enclosed by the interferometer. Here, we introduce twin-lattice atom interferometry exploiting Bose-Einstein condensates. Our method provides symmetric momentum transfer and large areas in palm-sized sensor heads with a performance similar to present meter-scale Sagnac devices.
Optics and interferometry with matter waves is the art of coherently manipulating the translational motion of particles like neutrons, atoms and molecules. Coherent atom optics is an extension of techniques that were developed for manipulating \emph{internal} quantum states. Applying these ideas to translational motion required the development of techniques to localize atoms and transfer population coherently between distant localities. In this view position and momentum are (continuouse) quantum mechanical degree of freedom analogous to discrete internal quantum states. In our contribution we…
We show that light-pulse atom interferometry with atomic point sources and spatially resolved detection enables multi-axis (two rotation, one acceleration) precision inertial sensing at long interrogation times. Using this method, we demonstrate a light-pulse atom interferometer for Rb-87 with 1.4 cm peak wavepacket separation and a duration of 2T = 2.3 seconds. The inferred acceleration sensitivity of each shot is 6.7 * 10^(-12) g, which improves on previous limits by more than two orders of magnitude. We also measure the Earth's rotation rate with a precision of 200 nrad/s.
We report the first realization of large momentum transfer (LMT) clock atom interferometry. Using single-photon interactions on the strontium ${}^1S_0 - {}^3P_1$ transition, we demonstrate Mach-Zehnder interferometers with state-of-the-art momentum separation of up to $141\,\hbar k$ and gradiometers of up to $81\,\hbar k$. Moreover, we circumvent excited state decay limitations and extend the gradiometer duration to 50 times the excited state lifetime. Because of the broad velocity acceptance of the interferometry pulses, all experiments are performed with laser-cooled atoms at a temperature o…
In quantum interferometry, it is vital to control and utilize nonlinear interactions for achieving high-precision measurements. Attribute to their long coherent time and high controllability, ultracold atoms including Bose condensed atoms have been widely used for implementing quantum interferometry. Here, we review the recent progresses in theoretical studies of quantum interferometry with Bose condensed atoms. In particular, we focus on the nonlinear phenomena induced by the atom-atom interaction and how to control and utilize these nonlinear phenomena. Under the mean-field description, due …
In Paris, we are using an atom interferometer to precisely measure the recoil velocity of an atom that absorbs a photon. In order to reach a high sensitivity, many recoils are transferred to atoms using the Bloch oscillations technique. In this lecture, I will present in details this technique and its application to high precision measurement. I will especially describe in details how this method allows us to perform an atom recoil measurement at the level of $1.3 \times 10^{-9}$. This measurement is used in the most precise determination of the fine structure constant that is independent of q…
We present a source engineering concept for a binary quantum mixture suitable as input for differential, precision atom interferometry with drift times of several seconds. To solve the non-linear dynamics of the mixture, we develop a set of scaling approach equations and verify their validity contrasting it to the one of a system of coupled Gross-Pitaevskii equations. This scaling approach is a generalization of the standard approach commonly used for single species. Its validity range is discussed with respect to intra- and inter-species interaction regimes. We propose a multi-stage, non-line…
We propose and demonstrate a new scheme for atom interferometry, using light pulses inside an optical cavity as matter wave beamsplitters. The cavity provides power enhancement, spatial filtering, and a precise beam geometry, enabling new techniques such as low power beamsplitters ($<100 \mathrm{μW}$), large momentum transfer beamsplitters with modest power, or new self-aligned interferometer geometries utilizing the transverse modes of the optical cavity. As a first demonstration, we obtain Ramsey-Raman fringes with $>75\%$ contrast and measure the acceleration due to gravity, $\mathit{g}$, t…
Hypothetical models have been proposed in which explicit collapse mechanisms prevent the superposition principle to hold at large scales. In particular, the model introduced by Ellis and co-workers [Phys. Lett. B ${\bf 221}$, 113 (1989)] suggests that quantum gravity might be responsible for the collapse of the wavefunction of massive objects in spatial superpositions. We here consider a recent experiment reporting on interferometry with atoms delocalized over half a meter for timescale of a second [Nature ${\bf 528}$, 530 (2015)] and show that the corresponding data strongly bound quantum gra…
Quantum interferometers are generally set so that phase differences between paths in coordinate space combine constructive or destructively. Indeed, the interfering paths can also meet in momentum space leading to momentum-space fringes. We propose and analyze a method to produce interference in momentum space by phase-imprinting part of a trapped atomic cloud with a detuned laser. For one-particle wave functions analytical expressions are found for the fringe width and shift versus the phase imprinted. The effects of unsharpness or displacement of the phase jump are also studied, as well as m…
We present mirror and beamsplitter pulse designs that improve the fidelity of atom interferometry and increase its tolerance of systematic inhomogeneities. These designs are demonstrated experimentally with a cold thermal sample of $^{85}$Rb atoms. We first show a stimulated Raman inversion pulse design that achieves a ground hyperfine state transfer efficiency of 99.8(3)%, compared with a conventional $π$ pulse efficiency of 75(3)%. This inversion pulse is robust to variations in laser intensity and detuning, maintaining a transfer efficiency of 90% at detunings for which the $π$ pulse fideli…
Every measurement of the population in an uncorrelated ensemble of two-level systems is limited by what is known as the quantum projection noise limit. Here, we present quantum projection noise limited performance of a Ramsey type interferometer using freely propagating coherent atoms. The experimental setup is based on an electro-optic modulator in an inherently stable Sagnac interferometer, optically coupling the two interfering atomic states via a two-photon Raman transition. Going beyond the quantum projection noise limit requires the use of reduced quantum uncertainty (squeezed) states. T…
We present here a new type of cold atom interferometry gravimeter based on Bragg diffraction, which is able to increase the gravity measurement sensitivity and stability of common Raman atom gravimeters significantly. By comparing with Raman transition, the principles and advantages of Bragg diffraction-based atom gravimeters have been introduced. The theoretical model for a time-domain Bragg atom gravimeter with atomic incident direction parallels to the wave vector of Bragg lasers has been constructed. Some key technical requirements for an nth-order Bragg diffraction-based atom gravimeter h…
In a light-pulse atom interferometer, we use a tip-tilt mirror to remove the influence of the Coriolis force from Earth's rotation and to characterize configuration space wave packets. For interferometers with large momentum transfer and large pulse separation time, we improve the contrast by up to 350% and suppress systematic effects. We also reach what is to our knowledge the largest spacetime area enclosed in any atom interferometer to date. We discuss implications for future high performance instruments.
We propose a scalable neutral atom quantum computer with an on-demand interaction through a selective two-qubit gate operation. Atoms are trapped by a lattice of near field Fresnel diffraction lights so that each trap captures a single atom. One-qubit gate operation is implemented by a gate control laser beam which is applied to an individual atom. Two-qubit gate operation between an arbitrary pair of atoms is implemented by sending these atoms to a state-dependent optical lattice and making them collide so that a particular two-qubit state acquires a dynamical phase. We give numerical evaluat…
We sense the motion of a trapped atomic ion using a sequence of state-dependent ultrafast momentum kicks. We use this atom interferometer to characterize a nearly-pure quantum state with $n=1$ phonon and accurately measure thermal states ranging from near the zero-point energy to $\bar{n}\sim 10^4$, with the possibility of extending at least 100 times higher in energy. The complete energy range of this method spans from the ground state to far outside of the Lamb-Dicke regime, where atomic motion is greater than the optical wavelength. Apart from thermometry, these interferometric techniques a…
We theoretically investigate the dynamics of a gas of strongly interacting Rydberg atoms subject to a time-domain Ramsey interferometry protocol. The many-body dynamics is governed by an Ising-type Hamiltonian with long range interactions of tunable strength. We analyze and model the contrast degradation and phase accumulation of the Ramsey signal and identify scaling laws for varying interrogation times, ensemble densities, and ensemble dimensionalities.
We show that entanglement monotones can characterize the pronounced enhancement of entanglement at a quantum phase transition if they are sensitive to long-range high order correlations. These monotones are found to develop a sharp peak at the critical point and to exhibit universal scaling. We demonstrate that similar features are shared by noise correlations and verify that these experimentally accessible quantities indeed encode entanglement information and probe separability.
We present new techniques for inertial-sensing atom interferometers which produce multiple phase measurements per experimental cycle. With these techniques, we realize two types of multiport measurements, namely quadrature phase detection and real-time systematic phase cancellation, which address challenges in operating high-sensitivity cold-atom sensors in mobile and field applications. We confirm experimentally the increase in sensitivity due to quadrature phase detection in the presence of large phase uncertainty, and demonstrate suppression of systematic phases on a single shot basis.
We demonstrate the operation of an atom interferometer based on a weakly interacting Bose-Einstein condensate. We strongly reduce the interaction induced decoherence that usually limits interferometers based on trapped condensates by tuning the s-wave scattering length almost to zero via a magnetic Feshbach resonance. We employ a $^{39}$K condensate trapped in an optical lattice, where Bloch oscillations are forced by gravity. With a control of the scattering length better that 0.1 $a_0$ we achieve coherence times of several hundreds of ms. The micrometric sizes of the atomic sample make our s…
We theoretically discuss an implementation of a Sagnac interferometer with cold atoms. In contrast to currently existing schemes our protocol does not rely on any free propagation of atoms. Instead it is based on superpositions of fully confined atoms and state-dependent transport along a closed path. Using Ramsey sequences for an atomic clock, the accumulated Sagnac phase is encoded in the resulting population imbalance between two internal (clock) states. Using minimal models for the above protocol we analytically quantify limitations arising from atomic dynamics and finite temperature. We d…
Floquet engineering offers a compelling approach for designing the time evolution of periodically driven systems. We implement a periodic atom-light coupling to realize Floquet atom optics on the strontium ${}^1\!S_0\,\text{-}\, {}^3\!P_1$ transition. These atom optics reach pulse efficiencies above $99.4\%$ over a wide range of frequency offsets between light and atomic resonance, even under strong driving where this detuning is on the order of the Rabi frequency. Moreover, we use Floquet atom optics to compensate for differential Doppler shifts in large momentum transfer atom interferometers…
An accurate measurement of the bunching of photons in the fluorescent emission from an ultracold ensemble of thermal 87Rb atoms in a steady-state magneto-optical trap is presented. Time-delayed-intensity-interferometry (TDII) performed with a 5-nanosecond time resolution yielded a second-order intensity correlation function that has the ideal value of 2 at zero delay, and that shows coherent Rabi oscillations of upto 5 full periods - much longer than the spontaneous emission lifetime of the excited state of Rb. The oscillations are damped out by ~150ns, and thereafter, as expected from a therm…
We present a single-source dual atom interferometer and utilize it as a gradiometer for precise gravitational measurements. The macroscopic separation between interfering atomic wave packets (as large as 16 cm) reveals the interplay of recoil effects and gravitational curvature from a nearby Pb source mass. The gradiometer baseline is set by the laser wavelength and pulse timings, which can be measured to high precision. Using a long drift time and large momentum transfer atom optics, the gradiometer reaches a resolution of $3 \times 10^{-9}$ s$^{-2}$ per shot and measures a 1 rad phase shift …
