A novel result concerning Raman coupling schemes in the context of trapped ions is obtained. By means of an operator perturbative approach, it is shown that the complete time evolution of these systems (in the interaction picture) can be expressed, with a high degree of accuracy, as the product of two unitary evolutions. The first one describes the time evolution related to an effective coarse grained dynamics. The second is a suitable correction restoring the {\em fine} dynamics suppressed by the coarse graining performed to adiabatically eliminate the nonresonantly coupled atomic level.
Raman interaction of a trapped ultracold ion with two traveling wave lasers has been used extensively in the ion trap experiments. We solve this interaction in the absence of the rotating wave approximation by a continued fraction, without considering the restriction of the Lamb-Dicke limit and the weak excitation regime. Some interesting characteristics of the ion-trap system, particularly for the ion outside the weak excitation regime are found. Finally, a comparison of our results with the solution under the rotating wave approximation is made.
We demonstrate experimentally how the process of Stimulated Raman Adiabatic Passage (STIRAP) can be utilized for efficient coherent internal state transfer in single trapped and laser-cooled $^{40}$Ca$^+$ ions. The transfer from the D$_{3/2}$ to the D$_{5/2}$ state, is detected by a fluorescence measurement revealing the population not transfered to the D$_{5/2}$ state. A coherent population transfer efficiency at the level of 95 % in a setup allowing for the internal state detection of individual ions in a string has been obtained.
We propose a simple technique for the generation of arbitrary-sized Dicke states in a chain of trapped ions. The method uses global addressing of the entire chain by two pairs of delayed but partially overlapping laser pulses to engineer a collective adiabatic passage along a multi-ion dark state. Our technique, which is a many-particle generalization of stimulated Raman adiabatic passage (STIRAP), is decoherence-free with respect to spontaneous emission and robust against moderate fluctuations in the experimental parameters. Furthermore, because the process is very rapid, the effects of heati…
We present a method of treating the interaction of a single three-level ion with two laser beams. The idea is to apply a unitary transformation such that the exact transformed Hamiltonian has one of the three levels decoupled for all values of the detunings. When one takes into account damping, the evolution of the system is governed by a master equation usually obtained via adiabatic approximation under the assumption of far-detuned lasers. To go around the drawbacks of this technique, we use the same unitary transformation to get an effective master equation.
We study the collective Raman cooling of a polarized trapped Fermi gas in the Festina Lente regime, when the heating effects associated with photon reabsorptions are suppressed. We predict that by adjusting the spontaneous Raman emission rates and using appropriately designed anharmonic traps, temperatures of the order of 2.7% of the Fermi temperature can be achieved in 3D.
We present recent results on the coherent control of an optical transition in a single rubidium atom, trapped in an optical tweezer. We excite the atom using resonant light pulses that are short (4 ns) compared with the lifetime of the excited state (26 ns). By varying the intensity of the laser pulses, we can observe an adjustable number of Rabi oscillations, followed by free decay once the light is switched off. To generate the pulses we have developed a novel laser system based on frequency doubling a telecoms laser diode at 1560 nm. By setting the laser intensity to make a pi-pulse, we use…
We study cooling of the collective vibrational motion of two 138Ba+ ions confined in an electrodynamic trap and irradiated with laser light close to the resonances S_1/2-P_1/2 (493 nm) and P_1/2-D_3/2 (650 nm). The motional state of the ions is monitored by a spatially resolving photo multiplier. Depending on detuning and intensity of the cooling lasers, macroscopically different motional states corresponding to different ion temperatures are observed. We also derive the ions' temperature from detailed analytical calculations of laser cooling taking into account the Zeeman structure of the ene…
We experimentally realize an enhanced Raman control scheme for neutral atoms that features an intrinsic suppression of the two-photon carrier transition, but retains the sidebands which couple to the external degrees of freedom of the trapped atoms. This is achieved by trapping the atom at the node of a blue detuned standing wave dipole trap, that acts as one field for the two-photon Raman coupling. The improved ratio between cooling and heating processes in this configuration enables a five times lower fundamental temperature limit for resolved sideband cooling. We apply this method to perfor…
We present a study of the performance of the trapped-ion driven geometric phase gates introduced in [New J. Phys. 15, 083001 (2013)] when realized in a stimulated Raman transition. We show that the gate can achieve errors below the fault-tolerance threshold in the presence of laser intensity fluctuations. We also find that, in order to reduce the errors due to photon scattering below the fault-tolerance threshold, very intense laser beams are required to allow for large detunings in the Raman configuration without compromising the gate speed.
We report continuous Raman sideband cooling (CRSC) of a long ion chain to the motional ground state beyond the Lamb-Dicke (LD) regime. By driving multiple sideband transitions simultaneously, we show that nearly all axial modes of a 24-ion chain are cooled to the ground state, with an LD parameter as large as $η= 1.3$, spanning a frequency bandwidth of 4 MHz. Compared to traditional ground-state cooling methods such as pulsed sideband cooling or electromagnetic-induced-transparency (EIT) cooling, our method offers two key advantages: robustness to timing errors; and an ultra-wide bandwidth unl…
Making use of the Rydberg blockade, we generate entanglement between two atoms individually trapped in two optical tweezers. In this paper we detail the analysis of the data and show that we can determine the amount of entanglement between the atoms in the presence of atom losses during the entangling sequence. Our model takes into account states outside the qubit basis and allows us to perform a partial reconstruction of the density matrix describing the two atom state. With this method we extract the amount of entanglement between pairs of atoms still trapped after the entangling sequence an…
A novel perturbative treatment of the time evolution operator of a quantum system is applied to the model describing a Raman-driven trapped ion in order to obtain a suitable 'effective model'. It is shown that the associated effective Hamiltonian describes the system dynamics up to a certain transformation which may be interpreted as a 'dynamical dressing' of the effective model.
The Raman interaction of a trapped ultracold ion with two travelling wave lasers is studied analytically with series solutions, in the absence of the rotating wave approximation (RWA) and the restriction of both the Lamb-Dicke limit and the weak excitation regime. The comparison is made between our solutions and those under the RWA to demonstrate the validity region of the RWA. As a practical example, the preparation of Schrödinger-cat states with our solutions is proposed beyond the weak excitation regime.
We consider a trapped ion with a quantized center-of-mass motion in 2D trap potential. With external laser fields the effective (non)linear coupling of two orthogonal vibrational modes can be established via stimulated Raman transition. Nonclassical vibrational states such as squeezed states or two-mode entangled states (Schroedinger cat-like states) can be generated. When the vibrational modes are entangled with internal energy levels the Greenberger-Horne-Zeilinger (GHZ) states can be prepared.
The collective Raman cooling of trapped one- and two-component Fermi gases is considered. We obtain the quantum master equation that describes the laser cooling in the festina lente regime, for which the heating due to photon reabsorption can be neglected. For the two-component case the collisional processes are described within the formalism of quantum Boltzmann master equation. The inhibition of the spontaneous emission can be overcome by properly adjusting the spontaneous Raman rate during the cooling. Our numerical results based in Monte Carlo simulations of the corresponding rate equation…
A new optical pumping scheme is presented that uses incoherent Raman transitions to prepare a trapped Cesium atom in a specific Zeeman state within the 6S_{1/2}, F=3 hyperfine manifold. An important advantage of this scheme over existing optical pumping schemes is that the atom can be prepared in any of the F=3 Zeeman states. We demonstrate the scheme in the context of cavity quantum electrodynamics, but the technique is equally applicable to a wide variety of atomic systems with hyperfine ground-state structure.
Indistinguishability of photonic qubits emitted from trapped $^{40}$Ca$^+$ ions via pulsed excitation
Fachrichtung Physik, Universität des Saarlandes（萨尔兰州立大学物理系）；Zentrum für Quantentechnologien (QuTe), Universität des Saarlandes（萨尔兰州立大学量子技术中心）；Luxembourg Institute of Science and Technology (LIST)（卢森堡科学与技术研究所）
We present two schemes for driving Raman transitions between the ground state hyperfine manifolds of a single atom trapped within a high-finesse optical cavity. In both schemes, the Raman coupling is generated by standing-wave fields inside the cavity, thus circumventing the optical access limitations that free-space Raman schemes must face in a cavity system. These cavity-based Raman schemes can be used to coherently manipulate both the internal and the motional degrees of freedom of the atom, and thus provide powerful tools for studying cavity quantum electrodynamics. We give a detailed theo…
We demonstrate the initialisation, read-out and high-speed manipulation of a qubit stored in a single 87 Rb atom trapped in a submicron-size optical tweezer. Single qubit rotations are performed on a sub-100 ns time scale using two-photon Raman transitions. Using the ``spin-echo'' technique, we measure an irreversible dephasing time of 34 ms. The read-out of the single atom qubit is at the quantum projection noise limit when averaging up to 1000 individual events.
Efficient preparation and detection of the motional state of trapped ions is important in many experiments ranging from quantum computation to precision spectroscopy. We investigate the stimulated Raman adiabatic passage (STIRAP) technique for the manipulation of motional states in a trapped ion system. The presented technique uses a Raman coupling between two hyperfine ground states in $^{25}$Mg$^+$, implemented with delayed pulses, which removes a single phonon independent of the initial motional state. We show that for a thermal state the STIRAP population transfer is more efficient than a …
We theoretically study a pulsed stimulated two-photon Raman outcoupler for an atom laser using a full three-dimensional description. A finite-temperature trapped Bose-condensed atomic gas is treated self-consistently by the Hartree-Fock-Bogoliubov equations. The model is closely related to a recent experiment on optical outcoupling [E.W. Hagley et al., Science 283, 1706 (1999)]. We analyze the momentum distribution of the output atoms and show how the output beam may be used as a probe of the quantum state for the trapped atomic gas and how it could be engineered and controlled in a nonlinear …
We investigate the collective excitations of a Raman-induced spin-orbit coupled Bose-Einstein condensate confined in a quasi one-dimension harmonic trap using the Bogoliubov method. By tuning the Raman coupling strength, three phases of the system can be identified. By calculating the transition strength, we are able to classify various excitation modes that are experimentally relevant. We show that the three quantum phases possess distinct features in their collective excitation properties. In particular, the spin dipole and the spin breathing modes can be used to clearly map out the phase bo…
We propose a geometric phase gate in a decoherence-free subspace with trapped ions. The quantum information is encoded in the Zeeman sublevels of the ground-state and two physical qubits to make up one logical qubit with ultra long coherence time. Single- and two-qubit operations together with the transport and splitting of linear ion crystals allow for a robust and decoherence-free scalable quantum processor. For the ease of the phase gate realization we employ one Raman laser field on four ions simultaneously, i.e. no tight focus for addressing. The decoherence-free subspace is left neither …
We analyze the error in trapped-ion, hyperfine qubit, quantum gates due to spontaneous scattering of photons from the gate laser beams. We investigate single-qubit rotations that are based on stimulated Raman transitions and two-qubit entangling phase-gates that are based on spin-dependent optical dipole forces. This error is compared between different ion species currently being investigated as possible quantum information carriers. For both gate types we show that with realistic laser powers the scattering error can be reduced to below current estimates of the fault-tolerance error threshold…
We report new techniques for driving high-fidelity stimulated Raman transitions in trapped ion qubits. An electro-optic modulator induces sidebands on an optical source, and interference between the sidebands allows coherent Rabi transitions to be efficiently driven between hyperfine ground states separated by 14.53 GHz in a single trapped 111Cd+ ion.
Since the advent of atom laser-cooling, trapping or cooling natural molecules has been a long standing and challenging goal. Here, we demonstrate a method for laser-trapping molecules that is radically novel in its configuration, in its underlined physical dynamics and in its outcomes. It is based on self-optically spatially-nanostructured high pressure molecular hydrogen confined in hollow-core photonic-crystal-fibre. An accelerating molecular-lattice is formed by a periodic potential associated with Raman saturation except for a 1-dimentional array of nanometer wide and strongly-localizing s…
We propose and demonstrate a protocol for high-fidelity indirect readout of trapped ion hyperfine qubits, where the state of a $^9\text{Be}^+$ qubit ion is mapped to a $^{25}\text{Mg}^+$ readout ion using laser-driven Raman transitions. By partitioning the $^9\text{Be}^+$ ground state hyperfine manifold into two subspaces representing the two qubit states and choosing appropriate laser parameters, the protocol can be made robust to spontaneous photon scattering errors on the Raman transitions, enabling repetition for increased readout fidelity. We demonstrate combined readout and back-action e…
We construct a connection of the ultracold atomic system in a harmonic trap with Raman-induced spin-orbit coupling to the quantum Rabi-like model. By mapping the trapped atomic system to a Rabi-like model, we can get the exact solution of the Rabi-like model following the methods to solve the quantum Rabi model. The existence of such a mapping implies that we can study the basic model in quantum optics by using trapped atomic gases with spin-orbit coupling.
We propose an efficient scheme for the implementation of quantum information transfer in a onedimensional coupled resonator waveguide. We show that, based on the effective long-range dipole-dipole interactions between the atoms mediated by the cavity modes, Raman transitions between the atoms trapped in different nodes can take place. Quantum information could be transferred directly between the opposite ends of the coupled waveguide without involving the intermediate nodes via either Raman transitions or the stimulated Raman adiabatic passages. Since this scheme, in principle, is a one-step p…
A protocol is proposed to generate atomic entangled states in a cavity QED system. It utilizes Raman transitions or stimulated Raman adiabatic passages between two systems to entangle the ground states of two three-state $Λ$-type atoms trapped in a single mode cavity. It does not need the measurements on cavity field nor atomic detection and can be implemented in a deterministic fashion. Since the present protocol is insensitive to both cavity decay and atomic spontaneous emission, the produced entangled states may have some interesting applications in quantum information processing.
We propose a scheme involving cold atoms trapped in optical lattices to observe different phenomena traditionally linked to quantum-optical systems. The basic idea consists of connecting the trapped atomic state to a non-trapped state through a Raman scheme. The coupling between these two types of atoms (trapped and free) turns out to be similar to that describing light-matter interaction within the rotating-wave approximation, the role of matter and photons being played by the trapped and free atoms, respectively. We explain in particular how to observe phenomena arising from the collective s…
We propose an optical scheme to generate an entangled state between a trapped ion and a solid state donor qubit through which-path erasure of identical photons emitted from the two systems. The proposed scheme leverages the similar transition frequencies between In donor bound excitons in ZnO and the $^2P_{1/2}$ to $^2S_{1/2}$ transition in Yb$^+$. The lifetime of the relevant ionic state is longer than that of the ZnO system by a factor of 6, leading to a mismatch in the temporal profiles of emitted photons. A detuned cavity-assisted Raman scheme weakly excites the donor with a shaped laser p…
We present a quantum computing scheme with atomic Josephson junction arrays. The system consists of a small number of atoms with three internal states and trapped in a far-off resonant optical lattice. Raman lasers provide the "Josephson" tunneling, and the collision interaction between atoms represent the "capacitive" couplings between the modes. The qubit states are collective states of the atoms with opposite persistent currents. This system is closely analogous to the superconducting flux qubit. Single qubit quantum logic gates are performed by modulating the Raman couplings, while two-qub…
We study harmonically trapped one-dimensional atoms subjected to an equal combination of Rashba and Dresselhaus spin-orbit coupling induced by Raman transition. We first examine the wave function and the degeneracy of the single-particle ground state, followed by a study of two weakly interacting bosons or fermions. For the two-particle ground state, we focus on the effects of the interaction on the degeneracy, the spin density profiles, and the density-density correlation functions. Finally we show how these studies help us to understand the many-body properties of the system.
We demonstrate several building blocks for an ion-photon interface based on a trapped Ca ion in an optical cavity. We identify a favorable experimental configuration and measure system parameters, including relative motion of the trapped ion and the resonator mode. A complete spectrum of cavity-assisted Raman transitions between the $4^{2}S_{1/2}$ and $3^{2}D_{5/2}$ manifolds is obtained. On two of these transitions, we generate orthogonally polarized cavity photons, and we demonstrate coherent manipulation of the corresponding pair of atomic states. Possible implementations of atom-photon ent…
Decoupling of the STIRAP and Microwave-Dressing paths in Trapped Rydberg Ion Gates
Center for Quantum Technologies, Department of Physics, Sofia University（索非亚大学量子技术中心物理系）；Georgi Nadjakov Institute of Solid State Physics, Bulgarian Academy of Sciences（保加利亚科学院格奥尔基·纳德贾科夫固体物理研究所）；Department of Physics, Stockholm University（斯德哥尔摩大学物理系）
We present a new and efficient implementation of Raman cooling of trapped atoms. It uses Raman pulses with an appropriate frequency chirp to realize a velocity selective excitation through a rapid adiabatic passage. This method allows to address in a single pulse a large number of non zero atomic velocity classes and it produces a nearly unity transfer efficiency. We demonstrate this cooling method using cesium atoms in a far-detuned crossed dipole trap. Three-dimensional cooling of $1 \times 10^{5}$ atoms down to $2 μ$K is performed in 100 ms. In this preliminary experiment the final atomic d…
Fidelity bounds for spin-dependent kicks with pulsed lasers
Universidad Carlos III de Madrid（马德里卡洛斯三世大学）；IonQ, Inc.（IonQ公司）；Instituto de Física Fundamental, Consejo Superior de Investigaciones Científicas (IFF-CSIC)（西班牙高等科学研究所基础物理研究所）
Quantum-optical techniques allow for generating controllable spin-spin interactions between ions, making trapped ions an ideal quantum simulator of Heisenberg chains. A single parameter, the detuning of the Raman coupling, allows to switch between ferromagnetic and antiferromagnetic chains, and to modify the range of the interactions. On the antiferromagnetic side, the system can be tuned from an extreme long-range limit, in which any pair of ions interacts with almost equal strength, to interactions with a $1/r^3$ decay. By exact diagonalization, we study how a system of up to 20 ions behaves…
Molecules are the most demanding quantum systems to be simulated by quantum computers because of their complexity and the emergent role of quantum nature. The recent theoretical proposal of Huh et al. (Nature Photon., 9, 615 (2015)) showed that a multi-photon network with a Gaussian input state can simulate a molecular spectroscopic process. Here, we report the first experimental demonstration of molecular vibrational spectroscopy of SO$_{2}$ with a trapped-ion system. In our realization, the molecular scattering operation is decomposed to a series of elementary quantum optical operations, whi…
Protein folding on a 64 qubit trapped-ion hardware via counterdiabatic quantum optimization
Kipu Quantum GmbH（Kipu Quantum有限公司）；University of the Basque Country EHU（巴斯克大学）；Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC)（马德里材料科学研究所）；Universidad Autónoma de Madrid（马德里自治大学）；University of Valencia（瓦伦西亚大学）；IonQ Inc.（IonQ公司）
We demonstrate simple and robust methods for Doppler cooling and obtaining high fluorescence from trapped 43Ca+ ions at a magnetic field of 146 Gauss. This field gives access to a magnetic-field-independent "atomic clock" qubit transition within the ground level hyperfine structure of the ion, but also causes the complex internal structure of the 64 states relevant to Doppler cooling to be spread over many times the atomic transition line-width. Using a time-dependent optical Bloch equation simulation of the system we develop a simple scheme to Doppler-cool the ion on a two-photon dark resonan…
One can think of some physical evolutions as being the emergent-effective result of a microscopic discrete model. Inspired by classical coarse-graining procedures, we provide a simple procedure to coarse-grain color-blind quantum cellular automata that follow Goldilocks rules. The procedure consists in (i) space-time grouping the quantum cellular automaton (QCA) in cells of size $N$; (ii) projecting the states of a cell onto its borders, connecting them with the fine dynamics; (iii) describing the overall dynamics by the border states, that we call signals; and (iv) constructing the coarse-gra…
