D. P. Caetano, P. H. Souto Ribeiro
We demonstrate theoretical and experimentally how it is possible to manipulate an entangled angular spectrum of twin beams, in order to reconstruct correlated images with coincidence detection. The entangled angular spectrum comes from the pump and the image is obtained only if signal and idler are properly treated.
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We derive a sufficient condition for a set of pure states, each entangled in two remote $N$-dimensional systems, to be transformable to $k$-dimensional-subspace equivalent entangled states ($k\leq N$) by same local operations and classical communication. If $k=N$, the condition is also necessary. This condition reveals the function of the relative marginal density operators of the entangled states in the entanglement manipulation without sufficient information of the initial states.
A silicon quantum photonic circuit was proposed and demonstrated as an integrated quantum light source for telecom band polarization entangled Bell state generation and dynamical manipulation. Biphoton states were firstly generated in four silicon waveguides by spontaneous four wave mixing. They were transformed to polarization entangled Bell states through on-chip quantum interference and quantum superposition, and then coupled to optical fibers. The property of polarization entanglement in generated photon pairs was demonstrated by two-photon interferences under two non-orthogonal polarizati…
When an entangled state is transformed into another one with probability one by local operations and classical communication, the quantity of entanglement decreases. This letter shows that entanglement lost in the manipulation can be partially recovered by an auxiliary entangled pair. As an application, a maximally entangled pair can be obtained from two partially entangled pairs with probability one. Finally, this recovery scheme reveals a fundamental property of entanglement relevant to the existence of incomparable states.
In this thesis, several new procedures for the generation and manipulation of entangled states in quantum optical systems are introduced. Each is evaluated in terms of realistic models of the imperfect apparatus of any real laboratory implementation. The first half of the thesis considers entanglement generation in Cavity QED, introducing several proposals for the creation of maximally entangled two-qubit states. The second half of the thesis focuses on the manipulation of entangled states of light pulses. In particular, an entanglement distillation procedure for Gaussian states is introduced.…
We propose probabilistic controlled-NOT and controlled-phase gates for qubits stored in the polarization of photons. The gates are composed of linear optics and photon detectors, and consume polarization entangled photon pairs. The fraction of the successful operation is only limited by the efficiency of the Bell-state measurement. The gates work correctly under the use of imperfect detectors and lossy transmission of photons. Combined with single-qubit gates, they can be used for producing arbitrary polarization states and for designing various quantum measurements.
We consider the entanglement manipulation capabilities of the universal covariant quantum cloner or quantum processor circuit for quantum bits. We investigate its use for cloning a member of a bipartite or a genuine tripartite entangled state of quantum bits. We find that for bipartite pure entangled states a nontrivial behavior of concurrence appears, while for GHZ entangled states a possibility of the partial extraction of bipartite entanglement can be achieved.
We propose to integrate the electro-optic tuning function into polarization-entangled photon pair generation process in a periodically poled lithium niobate (PPLN). Due to the versatility of PPLN, both the spontaneously parametric down conversion and electro-optic polarization rotation effects could be realized simultaneously. Orthogonally-polarized and parallel-polarized photon pairs thus are instantly switchable by tuning the applied field. The characteristics of the source are investigated showing adjustable bandwidths and high entanglement degrees. Moreover, other kinds of reconfigurable e…
We present the visible entangled states of 4-qubit system which can be observed easily in physical laboratories. This was motivated from the fact that the entangled state of 2-qubit system comes from singlet and triplet states which are constructed through the angular momentum addition formalism. We show that 4-qubit system has the new entangled states different from GHZ or W types entangled states
We introduce a simple, experimentally realisable, entanglement manipulation protocol for exploring mixed state entanglement. We show that for both non-maximally entangled pure, and mixed polarisation-entangled two qubit states, an increase in the degree of entanglement and purity, which we define as concentration, is achievable.
We analyze approximate transformations of pure entangled quantum states by local operations and classical communication, finding explicit conversion strategies which optimize the fidelity of transformation. These results allow us to determine the most faithful teleportation strategy via an initially shared partially entangled pure state. They also show that procedures for entanglement manipulation such as entanglement catalysis [Jonathan and Plenio, Phys. Rev. Lett. 83, 3566 (1999)] are robust against perturbation of the states involved, and motivate the notion of non-local fidelity, which qua…
Hybrid entangled states exhibit entanglement between different degrees of freedom of a particle pair and thus could be useful for asymmetric optical quantum network where the communication channels are characterized by different properties. We report the first experimental realization of hybrid polarization-orbital angular momentum (OAM) entangled states by adopting a spontaneous parametric down conversion source of polarization entangled states and a polarization-OAM transferrer. The generated quantum states have been characterized through quantum state tomography. Finally, the violation of B…
We have observed the stationary interference oscillations of a triple-entangled neutron state in an interferometric experiment. Time-dependent interaction with two radio-frequency (rf) fields enables coherent manipulation of an energy degree of freedom in a single neutron. The system is characterized by a multiply entangled state governed by a Jaynes-Cummings Hamiltonian. The experimental results confirm coherence of the manipulation as well as the validity of the description.
Starting from the standard Hamiltonian describing the optical non-linear process of spontaneous parametric down-conversion, we theoretically show that the generated entangled photon-pairs carry non-negligible orbital angular momentum in the degrees of freedom of relative movement in the type-II cases due to spatial symmetry breaking. We also show that the orbital angular momentum carried by photon-pairs in these degrees of freedom escapes detection in the traditional measurement scheme, which demands development of new techniques for further experimental investigations.
What are the orbital angular momentum correlations between spatially entangled photon pairs generated in spontaneous parametric down-conversion? We show that the answer to this question can be given in two alternative, although complementary, ways. The answer posed in this letter explains satisfactorily the seemingly contradictory results obtained in different experiments, and theoretical approaches.
Orbital angular momentum (OAM) multiplexed entangled state is an important quantum resource for high dimensional quantum information processing. In this paper, we experimentally quantify quantum coherence of OAM multiplexed continuous-variable (CV) entangled state and characterize its evolution in a noisy environment. We show that the quantum coherence of the OAM multiplexed CV entangled state carrying topological charges $l=1$ and $l=2$ are the same as that of the Gaussian mode with $l=0$ in a noisy channel. Furthermore, we show that the quantum coherence of OAM multiplexed entangled state is…
We present an experimental evidence that high dimensional orbital angular momentum entanglement of a pair of photons can be survived after a photon-plasmon-photon conversion. The information of spatial modes can be coherently transmitted by surface plasmons. This experiment primarily studies the high dimensional entangled systems based on surface plasmon with subwavelength structures. It maybe useful in the investigation of spatial mode properties of surface plasmon assisted transmission through subwavelength hole arrays.
We analyze the effect of atmospheric Kolmogorov turbulence on entangled orbital angular momentum states generated by parametric down-conversion. We calculate joint and signal photon detection probabilities and obtain numerically their dependence on the mode-width-to-Fried-parameter ratio. We demonstrate that entangled photons are less robust to the effects of Kolmogorov turbulence compared to single photons. In contrast, signal photons are more robust than single photons in the lowest-order mode. We also obtain numerically a scaling relation between the value of the mode-width-to-Fried-paramet…
In this thesis, we report the theoretical and experimental investigations towards the creation, characterization, and manipulation of quantum entanglement in a photonic system. We examine two different aspects of quantum entanglement: In the first part, we discuss the experimental method for the preparation and characterization of SPDC-based polarization-entangled photon source. We provide a review study comparing different Entanglement Measures for non-maximally entangled two-qubit pure states and extend this analysis to higher-dimensional systems. In the second part, we study the entanglemen…
The non-classical spectral and temporal features of entangled photons offer new possibilities to investigate the interactions of excitons in photosynthetic complexes, and to target the excitation of specific states. Simulations of fluorescence in the bacterial reaction center induced by entangled light demonstrate a selectivity of double-exciton states which is not possible using classical stochastic light with the same power spectrum.
We propose a method for generation of entangled photonic states in high dimensions, the so-called qudits, by exploiting quantum correlations of Orbital Angular Momentum (OAM) entangled photons, produced via Spontaneous Parametric Down Conversion. Diffraction masks containing $N$ angular slits placed in the path of twin photons define a qudit space of dimension $N^2$, spanned by the alternative pathways of OAM-entangled photons. We quantify the high-dimensional entanglement of path-entangled photons by the Concurrence, using an analytic expression valid for pure states. We report numerical resu…
Parallelization of frequency domain quantum gates: manipulation and distribution of frequency-entangled photon pairs generated by a 21 GHz silicon micro-resonator
本研究研发出小尺寸硅环形谐振器，利用其窄间隔多频率信道，通过现成电光器件并行控制单量子比特门，实现纠缠对表征并首次演示频域全连接5用户量子网络，推动可扩展硅基量子电路发展。
Maximally entangled photon pairs with a spatial degree of freedom is a potential way for realizing high-capacity quantum computing and communication. However, methods to generate such entangled states with high quality, high brightness, and good controllability are needed. Here, a scheme is experimentally demonstrated that generates spatially maximally entangled photon pairs with an orbital angular momentum degree of freedom via spontaneous parametric down-conversion in a nonlinear crystal. Compared with existing methods using post-selection, the technique can directly modulate the spatial spe…
Entangled spin states are created by implanting muons into single crystal LiY0.95Ho0.05F4 to form a cluster of correlated, dipole-coupled local magnetic moments. The resulting states have well-defined energy levels allowing experimental manipulation of the state populations by electromagnetic excitation. Experimental control of the evolution of the muon spin polarization is demonstrated through application of continuous, radio-frequency magnetic excitation fields. A semiclassical model of quantum, dipole-coupled spins interacting with a classical, oscillating magnetic field accounts for the mu…
High-dimensional entangled quantum states improve the performance of quantum technologies compared to qubit-based approaches. In particular, they enable quantum communications with higher information capacities or enhanced imaging protocols. However, the presence of optical disorder such as atmospheric turbulence or biological tissue perturb quantum state propagation and hinder their practical use. Here, we demonstrate a wavefront shaping approach to transmit high-dimensional spatially entangled photon pairs through scattering media. Using a transmission matrix approach, we perform wavefront c…
Catalytic and asymptotic equivalence for quantum entanglement
本文研究量子纠缠的催化与渐近操作，证明两者对所有可蒸馏态完全等价，并发现使用纠缠催化剂无法提升渐近单态蒸馏率，突出了多拷贝相关性的关键作用。
The orbital angular momentum of light, unlike spin, is an infinite-dimensional discrete variable and may hence offer enhanced performances for encoding, transmitting, and processing information in the quantum regime. Hitherto, this degree of freedom of light has been studied mainly in the context of quantum states with definite number of photons. On the other hand, field-quadrature continuous-variable quantum states of light allow implementing many important quantum protocols not accessible with photon-number states. Here, we present the first generation and complete experimental characterizat…
In order to cope with the fact that there exists no single maximally entangled state (up to local unitaries) in the multipartite setting, we introduced in [J. I. de Vicente, C. Spee and B. Kraus, Phys. Rev. Lett. 111, 110502 (2013)] the maximally entangled set of n-partite quantum states. This set consists of the states that are most useful under conversion of pure states via Local Operations assisted by Classical Communication (LOCC). We will review our results here on the maximally entangled set of three- and generic four-qubit states. Moreover, we will discuss the preparation of arbitrary (…
Methods for distilling maximally entangled tripartite (GHZ) states from arbitrary entangled tripartite pure states are described. These techniques work for virtually any input state. Each technique has two stages which we call primary and secondary distillation. Primary distillation produces a GHZ state with some probability, so that when applied to an ensemble of systems, a certain percentage is discarded. Secondary distillation produces further GHZs from the discarded systems. These protocols are developed with the help of an approach to quantum information theory based on absolutely selecti…
Generation of polarization-entangled counter-propagating photons with high orbital angular momentum
提出一种基于光纤的高阶OAM偏振纠缠光子源，通过四波混频产生纠缠光子对，并利用helical gratings转换为高OAM模式，实现了对联合光谱幅度的鲁棒控制。
Generation of subnatural-linewidth orbital angular momentum entangled biphotons using a single driving laser in hot atoms
本文提出在热铷原子蒸气中仅用单一驱动激光，通过自发四波混频和OAM守恒直接产生亚自然线宽轨道角动量纠缠双光子，实验测得保真度95.7%、并发度0.926，方案显著简化并首次在热原子系统中实现。
We present the novel embodiment of a photonic qubit that makes use of one continuous spatial degree of freedom of a single photon and relies on the the parity of the photon's transverse spatial distribution. Using optical spontaneous parametric downconversion to produce photon pairs, we demonstrate the controlled generation of entangled-photon states in this new space. Specifically, two Bell states, and a continuum of their superpositions, are generated by simple manipulation of a classical parameter, the optical-pump spatial parity, and not by manipulation of the entangled photons themselves.…
Hong-Ou-Mandel (HOM) effect was long believed to be a two-photon interference phenomenon. It describes the fact that two indistinguishable photons mixed at a beam splitter will bunch together to one of the two output modes. Considering the two single-photon emitters such as trapped ions, we explore a hidden scenario of the HOM effect, where entanglement can be generated between the two ions when a single photon is detected by one of the detectors. A second photon emitted by the entangled photon sources will be subsequently detected by the same detector. However, we can also control the fate of…
Phase manipulation is essential to quantum information processing, for which the orbital angular momentum (OAM) of photon is a promising high-dimensional resource. Dove prism (DP) is one of the most important element to realize the nondestructive phase manipulation of OAM photons. DP usually changes the polarization of light and thus increases the manipulation error for a spin-OAM hybrid state. DP in a Sagnac interferometer also introduces a mode-dependent global phase to the OAM mode. In this work, we implemented a high-dimensional controlled-phase manipulation module (PMM), which can compens…
Polarized light passing through twisted special wave plates show entangled state of both SAM and OAM. The variable circular and linear retarders (VCR and VLR) are studied here from the view point of quantum processing of entangled states. Interestingly the geometric phase in association with twist dependent gain of OAM has been discussed here. As an application of VLR, the origin of gradual flattened shape of wave fronts through successive array of antennas (QHQ) has been explained through new physical approach of the concurrence of entangled states.
We show that the use of entangled photons having non-zero orbital angular momentum (OAM) increases the resolution and sensitivity of angular-displacement measurements performed using an interferometer. By employing a 4$\times$4 matrix formulation to study the propagation of entangled OAM modes, we analyze measurement schemes for two and four entangled photons and obtain explicit expressions for the resolution and sensitivity in these schemes. We find that the resolution of angular-displacement measurements scales as $Nl$ while the angular sensitivity increases as $1/(2Nl)$, where $N$ is the nu…
Engineering of maximally entangled orbital angular momentum states via path identity
针对基于轨道角动量的路径身份纠缠缺乏态分布工程化设计研究的空白，结合泵浦光空间工程与路径身份方法确定最大纠缠态最优维度，揭示高维目标态保真度限制并证明两类双光子纠缠态等价，助力高维最大纠缠态优化制备。
We investigate how quantum coincidence interferometry is affected by a controllable manipulation of transverse wave-vectors in type-II parametric down conversion using adaptive optics techniques. In particular, we discuss the possibility of spatial walk-off compensation in quantum interferometry and a new effect of even-order spatial aberration cancellation.
Entanglement is a resource in quantum information theory when state manipulation is restricted to Local Operations assisted by Classical Communication (LOCC). It is therefore of paramount importance to decide which LOCC transformations are possible and, particularly, which states are maximally useful under this restriction. While the bipartite maximally entangled state is well known (it is the only state that cannot be obtained from any other and, at the same time, it can be transformed to any other by LOCC), no such state exists in the multipartite case. In order to cope with this fact, we in…
Entangled quantum states play an important role in quantum information science and also in quantum mechanics fundamental investigations. Implementation and characterization of techniques allowing for easy preparation of entangled states are important steps in such fields. Here we generated entangled quantum states encoded in photons transversal paths, obtained by pumping a non-linear crystal with multiple transversal Gaussian beams. Such approach allows us to generate entangled states of two qubits and two qutrits encoded in Gaussian transversal path of twin photons. We make a theoretical anal…
We derive an exact formula for the angular Schmidt spectrum of the orbital angular momentum (OAM)-entangled states produced by parametric down-conversion (PDC). We show that our formula yields true theoretical spectrum without any convergence issue as has been the case with the previously derived formulas. Furthermore, we use this formula to experimentally characterize the angular Schmidt spectrum for non-collinear PDC. We report the measurements of very broad angular Schmidt spectra corresponding to angular Schmidt numbers up to 233, which, to the best of our knowledge, is the highest number …
We show that the process of entanglement distillation is irreversible by showing that the entanglement cost of a bound entangled state is finite. Such irreversibility remains even if extra pure entanglement is loaned to assist the distillation process.
Deterministic extraction of Bell pairs from a finite number of partially entangled pairs is discussed. We derive the maximum number of Bell pairs that can be obtained with probability 1 by local operations and classical communication. It is proved that the optimal deterministic concentration needs only a two-pair collective manipulation in each step, and that a collective manipulation of all entangled pairs is not necessary. Finally, this scheme reveals an entanglement measure for the deterministic concentration.
A class of centrosymmetric molecules support excitons with a well-defined quasi-angular momentum. Cofacial arrangements of these molecules can be engineered so that quantum cutting produces a pair of excitons with angular momenta that are maximally entangled. The Bell state constituents can subsequently travel in opposite directions down molecular chains as ballistic wave packets. This is a direct excitonic analog to the entangled polarization states produced by the spontaneous parametric downconversion of light. As in optical settings, the ability to produce Bell states should enable foundati…
Entanglement manipulation through multicore fibres
本文提出利用多芯光纤中纤芯间串扰作为量子信道，生成两个 qudit 的束缚纠缠态，从而将多芯光纤的应用从量子通信扩展到纠缠态制备。
We consider a system of two particles, each with large angular momentum $j$, in the singlet state. The probabilities of finding projections of the angular momenta on selected axes are determined. The generalized Bell inequalities involve these probabilities and we study them using statistical methods. We show that most of Bells inequalities cannot be violated, or are violated only marginally, in the limit $j\to \infinity$. The precision required to confirm a violation appears to be difficult to achieve. In practice, the quantum system, in spite of being entangled, becomes indistinguishable fro…
We investigate two-photon entangled states using two important degrees of freedom of the electromagnetic field, namely orbital angular momentum (OAM) and spin angular momentum. For photons propagating in the same direction we apply the idea of $\textit{entanglement duality}$ and develop schemes to do $\textit{entanglement sorting}$ based either on OAM or polarization. In each case the entanglement is tested using appropriate witnesses. We finally present generalizations of these ideas to three- and four-photon entangled states.
Constructing a quantum memory for a photonic entanglement is vital for realizing quantum communication and network. Besides enabling the realization of high channel capacity communication, entangled photons of high-dimensional space are of great interest because of many extended applications in quantum information and fundamental physics fields. Photons entangled in a two-dimensional space had been stored in different system, but there have been no any report on the storage of a photon pair entangled in a high-dimensional space. Here, we report the first experimental realization of storing an …
Quantum protocols will be more efficient with high-dimensional entangled states. Photons carrying orbital angular momenta can be used to create a high-dimensional entangled state. In this paper we experimentally demonstrate the entanglement of the orbital angular momentum between the Stokes and anti-Stokes photons generated in a hot atomic ensemble using spontaneous four-wave-mixing. This experiment also suggests the existence of the entanglement concerned with spatial degrees of freedom between the hot atomic ensemble and the Stokes photon.
Methods for, and limitations to, the generation of entangled states of trapped atomic ions are examined. As much as possible, state manipulations are described in terms of quantum logic operations since the conditional dynamics implicit in quantum logic is central to the creation of entanglement. Keeping with current interest, some experimental issues in the proposal for trapped-ion quantum computation by I. Cirac and P. Zoller (University of Innsbruck) are discussed. Several possible decoherence mechanisms are examined and what may be the more important of these are identified. Some potential…
We report the first quantum entanglement experiment in South Africa. The spatial modes of the entangled photon pair are investigated with their potential for high-dimensional entanglement. The generation, measurement and characterisation of the entangled states are examined in detail, where we show high-dimensional entanglement in a Hilbert space of dimension 25. We highlight the experimental challenges contained within each step and provide practical techniques for future experiments in the quantum regime.
Postselection-free controlled generation of a high-dimensional orbital-angular-momentum entangled state
本文提出并实验演示了一种完全无后选择且可控的高维轨道角动量纠缠态产生技术，实现了约150维的纠缠态，产生精度超过98%，最大纠缠态精度达90%。
The measurement of high-dimensional entangled states of orbital angular momentum prepared by spontaneous parametric down-conversion can be considered in two separate stages: a generation stage and a detection stage. Given a certain number of generated modes, the number of measured modes is determined by the measurement apparatus. We derive a simple relationship between the generation and detection parameters and the number of measured entangled modes.
We study how to efficiently manipulate and store quantum information between optical fields and atomic ensembles. We show how various non-dissipative transfer schemes can be used to transfer and store quantum states such as squeezed vacuum states or entangled states into the long-lived ground state spins of atomic ensembles.
The Einstein Podolsky Rosen (EPR) entangled quantum state is of special importance not only for fundamental research in quantum mechanics, but also for information processing in the field of quantum information. Previous EPR entangled state demonstrations were constructed with photons of equal phase wave fronts. More complex scenarios with structured wave fronts have not been investigated. Here, we report the first experimental demonstration of EPR entanglement for photon pairs carrying orbital angular momentum (OAM) information, resulting in an OAM embedded EPR entangled state. We measured th…
Local discrimination of orbital angular momentum in entangled states
本文提出利用方解石晶体及受控空间位移对局域判别参量下转换量子辐射的轨道角动量，并指出其在长距离量子通信中的应用潜力。
We demonstrate that local transformations on a composite quantum system can be enhanced in the presence of certain entangled states. These extra states act much like catalysts in a chemical reaction: they allow otherwise impossible local transformations to be realised, without being consumed in any way. In particular, we show that this effect can considerably improve the efficiency of entanglement concentration procedures for finite states.
The unavoidable and irreversible interaction between an entangled quantum system and its environment causes decoherence of the individual qubits as well as degradation of the entanglement between them. Entanglement sudden death (ESD) is the phenomenon wherein disentanglement happens in finite time even when individual qubits decohere only asymptotically in time due to noise. Prolonging the entanglement is essential for the practical realization of entanglement-based quantum information and computation protocols. For this purpose, the local NOT operation in the computational basis on one or bot…
The experimental realization of multidimensional quantum states may lead to unexplored and interesting physics, as well as advanced quantum communication protocols. The orbital angular momentum of photons is a well suitable discrete degree of freedom for implementing high-dimensional quantum systems. The standard method to generate and manipulate such photon modes is to use bulk and fixed optics. Here the authors demonstrate the utilization of a spatial light modulator to manipulate the orbital angular momentum of entangled photons generated in spontaneous parametric downconversion. They show …
Spontaneous parametric down conversion has been shown to be a reliable source of entangled photons. Amongst the wide range of properties that have been shown to be entangled, it is the orbital angular momentum that is the focus of our study. We investigate, in particular, the bi-photon state generated using a Gaussian pump beam. We derive an expression for the simultaneous correlations in the orbital angular momentum and radial momentum of the down-converted Laguerre-Gaussian beams. Our result allows us, for example, to calculate the spiral bandwidth with no restriction on the geometry of the …
We investigate the decay properties of the quantumness including quantum entanglement, quantum discord and quantum coherence for two photonic qubits, which are partially entangled in their orbital angular momenta, through Kolmogorov turbulent atmosphere. It is found that the decay of quantum coherence and quantum discord may be qualitatively different from that of quantum entanglement when the initial state of two photons is not maximally entangled. We also derive two universal decay laws for quantum coherence and quantum discord, respectively, and show that the decay of quantum coherence is m…
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