We propose and discuss a scheme for robust and efficient generation of many-particle entanglement in an ensemble of Rydberg atoms with resonant dipole-dipole interactions. It is shown that in the limit of complete dipole blocking, the system is isomorphic to a multimode Jaynes-Cummings model. While dark-state population transfer is not capable of creating entanglement, other adiabatic processes are identified that lead to complex, maximally entangled states, such as the N-particle analog of the GHZ state in a few steps. The process is robust, works for even and odd particle numbers and the characteristic time for entanglement generation scales with N^a, with a being less than unity.
We have studied the analytical dynamics of Bell nonlocality as measured by CHSH inequality and entanglement as measured by concurrence for two noisy qubits that have dipole-dipole interaction. The nonlocal entanglement created by the dipole-dipole interaction is found to be protected from sudden death for certain initial states.
The entanglement of two dipole-coupled atoms with nondegenerate two-photon transitions interacting with two-mode field in lossless cavity has been investigated. It shows that the entanglement is dependent on the initial atomic states. The possibility of considerable growth of atomic entanglement due atomic coherence and dipole-dipole interaction is shown in the case of great mean values of thermal photons.
The effect of dipole-dipole interaction, the initial relative phase and the coupling strength with the cavity on the dynamics of three two level atoms in the good and the bad cavity regime are investigated. It is found that the presence of strong dipole-dipole interaction not only ensures avoiding entanglement sudden death but also retains entanglement for long time. The choice of the phase in the initial state is crucial to the operational regime of the cavity. Under specific conditions, the entanglement can be frozen in time to its initial values through strong dipole-dipole interaction. Thi…
We propose a new entanglement switch of qubits consisting of electric dipoles, oriented along or against an external electric field and coupled by the electric dipole-dipole interaction. The pairwise entanglement can be tuned and controlled by the ratio of the Rabi frequency and the dipole-dipole coupling strength. Tuning the entanglement can be achieved for one, two and three-dimensional arrangements of the qubits. The feasibility of building such an entanglement switch is also discussed.
Resonant dipole-dipole interaction (RDDI) is ubiquitous in light-matter interacting systems and is responsible for many fascinating properties of collective radiations. Here we theoretically investigate the role of RDDI in electromagnetically induced transparency (EIT). The resonant dipole-dipole interactions manifest in the cooperative spontaneous emission of the probe light transition, which give rise a broadened linewidth and associated collective frequency shift. This cooperative linewidth originates from the nonlocal and long-range RDDI, which can be determined by the atomic density, opti…
We make a general derivation for the magnetic dipole-dipole interaction based on the mediation of the quantized electro-magnetic field. Due to the interaction with the dipoles, the dynamics of the field is added by a dipole field, which finally gives rise to the dipole-dipole interaction. Different from previous studies, the rotating-wave-approximation is no longer needed throughout this derivation, and our result naturally gives the interaction for non-resonant dipoles. Moreover, our derivation also gives the counter-rotating interaction terms, and even the mixed interaction terms between the…
Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual and real …
We describe a method for generating entanglement between two spatially separated dipoles coupled to optical micro-cavities. The protocol works even when the dipoles have different resonant frequencies and radiative lifetimes. This method is particularly important for solid-state emitters, such as quantum dots, which suffer from large inhomogeneous broadening. We show that high fidelities can be obtained over a large dipole detuning range without significant loss of efficiency. We analyze the impact of higher order photon number states and cavity resonance mismatch on the performance of the pro…
We propose a simple scheme, in which only one atom couples to a cavity field, to entangle two two-level atoms. We connect two atoms with dipole-dipole interaction since one of them can move around the cavity. The results show that the peak entanglment does not depend on dipole-dipole interaction strength but on field density at a certain controlling time. So the field density can act as a switch for maximum entanglement (ME) generation.
We study a possible realization of the position- and momentum-correlated atomic pairs that are confined to adjacent sites of two mutually shifted optical lattices and are entangled via laser-induced dipole-dipole interactions. The Einstein-Podolsky-Rosen (EPR) ``paradox'' [Phys. Rev. 47, 777 (1935)] with translational variables is then modified by lattice-diffraction effects. This ``paradox'' can be verified to a high degree of accuracy in this scheme.
We propose and investigate a realization of the position- and momentum-correlated Einstein-Podolsky-Rosen (EPR) states [Phys. Rev. 47, 777 (1935)] that have hitherto eluded detection. The realization involves atom pairs that are confined to adjacent sites of two mutually shifted optical lattices and are entangled via laser-induced dipole-dipole interactions. The EPR "paradox" with translational variables is then modified by lattice-diffraction effects, and can be verified to a high degree of accuracy in this scheme.
Single--photon which is initially uncorrelated with atom, will evolve to be entangled with the atom on their continuous kinetic variables in the process of resonant scattering. We find the relations between the entanglement and their physical control parameters, which indicates that high entanglement can be reached by broadening the scale of the atomic wave or squeezing the linewidth of the incident single--photon pulse.
The influence of dipole-dipole interaction on the entanglement between two atoms with different initial entangled W-like states in Tavis-Cummings model with degenerate two-photon transitions has been investigated. The results show that the entanglement between two atoms can be increased by means of dipole-dipole interaction and for some initial states the entanglement sudden death effect can be weakened.
A scheme for the extraction of entanglement in two noninteracting qubits (spins) is proposed. The idea is to make use of resonant transmission of ancilla qubit through the two fixed qubits, controlled by the entanglement in the scatterers. Repetition of the resonant transmission extracts the singlet state in the target qubits from their arbitrary given state. Neither the preparation nor the post-selection of the ancilla spin is required, in contrast to the previously proposed schemes.
Generation of entanglement between two qubits by scattering an entanglement mediator is discussed. The mediator bounces between the two qubits and exhibits a resonant scattering. It is clarified how the degree of the entanglement is enhanced by the constructive interference of such bouncing processes. Maximally entangled states are available via adjusting the incident momentum of the mediator or the distance between the two qubits, but their fine tunings are not necessarily required to gain highly entangled states and a robust generation of entanglement is possible.
Using the nonperturbative method, we study the exact entanglement dynamics of two two-level dipole-dipole interacting atoms coupled to a common non-Markovian reservoir with different coupling strengths. Besides analyzing the conditions for the existence of steady state, we find, though the dipole-dipole interaction could destroy the stationary entanglement, that relatively strong dipole-dipole interaction does suppress the disentanglement in the initial period of time. These results are helpful for the practical engineering of the entanglement in the future.
While the Rydberg-blockade regime provides the natural setting for creating $W$-type entanglement with cold neutral atoms, it is demonstrated here that a scalable entanglement resource of this type can even be obtained under completely different physical circumstances. To be more precise, a special instance of twisted $W$ states -- namely, $π$-twisted ones -- can be engineered in one-dimensional arrays of cold neutral atoms with Rydberg-dressed resonant dipole-dipole interaction. In particular, it is shown here that this is possible even when a (dressed) Rydberg excitation is coupled to the mo…
We report a model that makes it possible to analyze quantitatively the dipole blockade effect on the dynamical evolution of a two two-level atom system driven by an external laser field. The multiple excitations of the atomic sample are taken into account. We find very large concurrence in the dipole blockade regime. We further find that entanglement can be tuned by changing the intensity of the exciting laser. We also report a way to lift the dipole blockade paving the way to manipulate in a controllable way the blockade effects. We finally report how a continuous monitoring of the dipole blo…
We use a versatile model to evaluate the multipartite entanglement and the nonclassical light generation in optical parametric oscillators, exploring the differences between doubly and triply resonant cavity configurations. We demonstrate the entanglement of the pump mode with converted fields in both situations, and the fundamental differences of oscillators using parametric down conversion and four wave mixing processes as the intracavity amplification technique. The strong correlations involving the sidebands of the pump and converted fields gives the signatures of a rich dynamic of multipa…
It is commonly believed that photon polarisation entanglement can only be obtained via pair creation within the same source or via postselective measurements on photons that overlapped within their coherence time inside a linear optics setup. In contrast to this, we show here that polarisation entanglement can also be produced by distant single photon sources in free space and without the photons ever having to meet, if the detection of a photon does not reveal its origin -- the which way information. In the case of two sources, the entanglement arises under the condition of two emissions in c…
We use the quantum jump approach to study the entanglement dynamics of a quantum register, which is composed of two or three dipole-dipole coupled two-level atoms, interacting with a common environment. Our investigation of entanglement dynamics reflects that the environment has dual actions on the entanglement of the qubits in the model. While the environment destroys the entanglement induced by the coherent dipole-dipole interactions, it can produce stable entanglement between the qubits prepared initially in a separable state. The analysis shows that it is the entangled decoherence-free sta…
We explore the possibilities of creating radiatively stable entangled states of two three-level dipole-interacting atoms in a $Λ$ configuration by means of laser biharmonic continuous driving or pulses. We propose three schemes for generation of entangled states which involve only the lower states of the $Λ$ system, not vulnerable to radiative decay. Two of them employ coherent dynamics to achieve entanglement in the system, whereas the third one uses optical pumping, i.e., an essentially incoherent process.
In proposals for quantum computers using arrays of trapped ultracold polar molecules as qubits, a strong external field with appreciable gradient is imposed in order to prevent quenching of the dipole moments by rotation and to distinguish among the qubit sites. That field induces the molecular dipoles to undergo pendular oscillations, which markedly affect the qubit states and the dipole-dipole interaction. We evaluate entanglement of the pendular qubit states for two linear dipoles, characterized by pairwise concurrence, as a function of the molecular dipole moment and rotational constant, s…
We investigate numerically the time dependence of the multiple quantum coherences and entanglement in linear chains up to nine nuclear spins of 1/2 coupled by the dipole-dipole interactions. Two models are considered: (1) a spin chain with nearest-neighbor dipole -dipole interactions; (2) a more realistic model with interactions between all spins. It is shown that the entangled states appear between remote particles which do not interact directly (model 1), while the interaction between all spins (model 2) not always results in entanglement between remote spins.
We propose a scheme of generating and verifying mesoscopic-level entanglement between two atomic ensembles using non-resonant stimulated Raman scattering. Entanglement can be generated by direct detection or balanced homodyne detection of the Stokes fields from the two cells, after they interfere on a beam splitter. The entanglement of the collective atomic fields can be transferred to the anti-Stokes fields in a readout process. By measuring the operator moments of the anti-Stokes fields, we can verify the presence of entanglement. We model the effects of practical factors such as Stokes fiel…
We present the differences between Input-Output formalism (IOF) and Incoherent Pumping Mechanism (IPM) derived from Lindblad Master Equation approach in terms of the transmission spectrum of Coupled high-Q Cavity with Quantum Dot system in the strong coupling regime. Fullwidth- half-maximum (FWHM) and the peak transmission of Dipole Induced Transparency (DIT) are inquired for detailed comparison in on-resonant and off-resonant conditions. We have found that DIT phenomenon in off-resonant case cannot be explained entirely by IPM although both methods can exhibit the same Vacuum Rabi splitting i…
Effectiveness of using laser field to produce entanglement between two dipole-interacting identical two-level atoms is considered in detail. The entanglement is achieved by driving the system with a carefully designed laser pulse transferring the system's population to one of the maximally entangled Dicke states in a way analogous to population inversion by a resonant $π$-pulse in a two-level atom. It is shown that for the optimally chosen pulse frequency, power and duration, the fidelity of generating a maximally entangled state approaches unity as the distance between the atoms goes to zero.
We provide an exact and complete characterization of the entanglement dynamics of two qubits coupled to a common structured reservoir at zero temperature. We derive the conditions to maximize reservoir-induced entanglement for an initially factorized state of the two-qubit system. In particular, when the two qubits are placed inside a lossy cavity, we show that high values of entanglement can be obtained, even in the bad cavity limit, in the dispersive regime. Finally we show that, under certain conditions, the entanglement dynamics exhibits quantum beats and we explain their physical origin i…
Entanglement of dipole-dipole interacting spins 1/2 is usually investigated when the energy of interaction with an external magnetic field (the Zeeman energy) is greater than the energy of dipole interactions by three orders. Under this condition only a non-equilibrium state of the spin system, realized by pulse radiofrequence irradiations, results in entanglement. The present paper deals with the opposite case: the dipolar interaction energy is the order of magnitude or even larger than the Zeeman one. It was shown that entanglement appears under the thermodynamic equilibrium conditions and t…
In this chapter we review the use of semiconductor quantum dots as sources of quantum light. Principally, we focus on resonant two-photon excitation, which is a method that allows for on-demand generation of photon pairs. We explore the advantages of resonant excitation and present a number of measurements that were made in this excitation regime. In particular, we cover the following topics: photon statistics, coherent manipulation of the ground-excited state superposition, and generation of time-bin entangled photon pairs.
Creation of entanglement is considered theoretically and numerically in an ensemble of spin chains with dipole-dipole interaction between the spins. The unwanted effect of the long-range dipole interaction is compensated by the optimal choice of the parameters of radio-frequency pulses implementing the protocol. The errors caused by (i) the influence of the environment,(ii) non-selective excitations, (iii) influence of different spin chains on each other, (iv) displacements of qubits from their perfect locations, and (v) fluctuations of the external magnetic field are estimated analytically an…
Influence of environment on quantum correlations in two-spin systems with dipole-dipole interactions
Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry of Russian Academy of Sciences（俄罗斯科学院化学物理与药物化学问题联邦研究中心）；Lomonosov Moscow State University（莫斯科国立罗蒙诺索夫大学）
The entanglement character including the so-called sudden death effect between atoms in the non-degenerate two photons Tavis-Cummings model is studied by means of concurrence. The results show that the so-called sudden death effect occurs only for some kind of initial states. In other words, the phenomenon is sensitive to the initial conditions. One can expect the resurrection of the original entanglement to occur in a periodic way following each sudden death event. The length of the time interval for the zero entanglement is dependent on not only the degree of entanglement of the initial stat…
We investigate the time evolution and asymptotic behavior of a system of two two-level atoms (qubits) interacting off-resonance with a single mode radiation field. The two atoms are coupled to each other through dipole-dipole as well as Ising interactions. An exact analytic solution for the system dynamics that spans the entire phase space is provided. We focus on initial states that cause the system to evolve to entanglement sudden death (ESD) between the two atoms. We find that combining the Ising and dipole-dipole interactions is very powerful in controlling the entanglement dynamics and ES…
We theoretically investigate the super- and sub-radiance from the resonant dipole-dipole interactions (RDDI) in a confined two-dimensional (2D) reservoir. The distinctive feature of 2D RDDI shows qualitatively and quantitatively different long-range behavior from RDDI in free space. We investigate the superradiant properties of the singly-excited symmetric state under this 2D RDDI. This state also allows subradiant decays in much longer distances than the transition wavelength, showing long-range atom-atom correlations. We further study the dynamics of the subradiant states which can be access…
In this paper we show that three cavity fields can be entangled when they are tuned on resonance with an ensemble of dressed three-level atoms. The master equation for the three cavity modes is derived by using atomic dressed states and the inseparability of the three output cavity modes is described by using a sufficient criterion proposed by van Loock and Furusawa. The physical cause is the atomic coherence effects, by which the quantum correlations are created in the field dynamics.
We study the output entanglement in a three-mode optomechanical system via reservoir engineering by shifting the center frequency of filter function away from resonant frequency. We find the bandwidth of the filter function can suppress the entanglement in the vicinity of resonant frequency of the system, while the entanglement will become prosperous if the center frequency departs from the resonant frequency. We obtain the approximate analytical expressions of the output entanglement, and from which we give the optimal center frequency at which the entanglement takes the maximum. Furthermore,…
We show that initially localized and uncorrelated two-particles quantum wavepackets evolving in a one-dimensional discrete lattice become strongly entangled while drifting under the action of an harmonic AC field resonant with doubled Bloch oscillations promoted by a static DC field. Although partial entanglement is achieved when the AC field is resonant with the single-particle Bloch oscillations, it is strongly limited by the survival of anti-correlated unbounded states. We further show that the phase dependence of the wavepacket centroid velocity is similar to the semiclassical behavior dep…
Multiparticle entangled states generated via interaction between narrow-band light and an ensemble of identical two-level atoms are considered. Depending on the initial photon statistics, correlation between atoms and photons can give rise to entangled states of these systems. It is found that the state of any pair of atoms interacting with weak single-mode squeezed light is inseparable and robust against decay. Optical schemes for preparing entangled states of atomic ensembles by projective measurement are described.
We have observed resonant energy transfer between cold Rydberg atoms in spatially separated cylinders. Resonant dipole-dipole coupling excites the 49s atoms in one cylinder to the 49p state while the 41d atoms in the second cylinder are transferred down to the 42p state. We have measured the production of the 49p state as a function of separation of the cylinders (0 - 80 um) and the interaction time (0 - 25 us). In addition we measured the width of the electric field resonances. A full many-body quantum calculation reproduces the main features of the experiments.
The dynamics of entanglement between three - level atoms coupled to the common vacuum is investigated. We show that the collective effects such as collective damping, dipole - dipole interaction and the cross coupling between orthogonal dipoles, play a crucial role in the process of creation of entanglement. In particular, the additional cross coupling enhances the production of entanglement. For the specific initial states we find that the effect of delayed sudden birth of entanglement, recently invented by Ficek and Tanas [Phys. Rev. A 77, o54301(2008)] in the case of two - level atoms, can …
Entanglement between two electrons belonging to an auto-ionization system and a neighbor two-level atom produced by the dipole-dipole interaction is studied. The entanglement is quantified using the quadratic negativity of a bipartite system including the continuum of states. Suitable conditions for the generation of highly entangled states of two electrons are revealed. Internal structure of the entanglement is elucidated using the spectral density of quadratic negativity.
By properly considering the propagation dynamics of the dipole field, we obtain the full magnetic dipolar interaction between two quantum dipoles for general situations. With the help the Maxwell equation and the corresponding Green function, this result applies for general boundary conditions, and naturally unifies all the interaction terms between permanent dipoles, resonant or non-resonant transition dipoles, and even the counter-rotating interaction terms altogether. In particular, we study the dipolar interaction in a rectangular 3D cavity with discrete field modes. When the two dipoles a…
We discuss the creation of entanglement between two two-level atoms in the dissipative process of spontaneous emission. It is shown that spontaneous emission can lead to a transient entanglement between the atoms even if the atoms were prepared initially in an unentangled state. The amount of entanglement created in the system is quantified by using two different measures: concurrence and negativity. We find analytical formulas for the evolution of concurrence and negativity in the system. We also find the analytical relation between the two measures of entanglement. The system consists of two…
We study a special two-atom entanglement case in assumed Cavity QED experiment in which only one atom effectively exchanges a single photon with a cavity mode. We compute diatom entanglement under position-dependent atomic resonant dipole-dipole interaction (RDDI) for large interatomic separation limit. We show that the RDDI, even which is much smaller than the maximal atomic Rabi frequency, can induce distinct diatom entanglement. The peak entanglement (PE) reaches a maximum when RDDI strength can compare with the Rabi frequency of an atom.
In this paper, we have investigated the entanglement between two dipole coupled two-level atoms. The model, in which only one atom is trapped in an lossless cavity and interacts with single-mode thermal field, and the other one can be spatially moved freely outside the cavity has been carried out. We have considered the effect of the atomic coherence on the entanglement behavior. We have shown that a thermal field might cause high entanglement between the atoms both for coherent and incoherent initial atomic states only for small values of the cavity mean photon number. In the considered model…
Studying the physics of quantum correlations has gained new interest after it has become possible to measure entanglement entropies of few body systems in experiments with ultracold atomic gases. Apart from investigating trapped atom systems, research on correlation effects in other artificially fabricated few-body systems, such as quantum dots or electromagnetically trapped ions, is currently underway or in planning. Generally, the systems studied in these experiments may be considered as composed of a small number of interacting elements with controllable and highly tunable parameters, effec…
The pairwise entanglement of an arbitrary atomic pair randomly extracted from a laser-driven dense multiqubit sample in the presence of quantum dissipation due to spontaneous emission is considered. The dipole-dipole interaction between the particles shifts the laser-qubit resonance frequency and consequently modifies the quantum entanglement. By means of an appropriate tuning of the laser frequency, one can optimize the entanglement in this system. For large ensembles, the maximum entanglement occurs near the laser parameters where the steady-state sample exhibits phase transition phenomena.
We propose a scheme that employs dissipation to deterministically generate entanglement in an ensemble of strongly interacting Rydberg atoms. With a combination of microwave driving between different Rydberg levels and a resonant laser coupling to a short lived atomic state, the ensemble can be driven towards a dark steady state that entangles all atoms. The long-range resonant dipole-dipole interaction between different Rydberg states extends the entanglement beyond the van der Walls interaction range with perspectives for entangling large and distant ensembles.
Two efficient and isotope-selective resonant two-photon ionization techniques for loading barium ions into radio-frequency (RF)-traps are demonstrated. The scheme of using a strong dipole-allowed transition at λ=553 nm as a first step towards ionization is compared to the established technique of using a weak intercombination line (λ=413 nm). An increase of two orders of magnitude in the ionization efficiency is found favoring the transition at 553 nm. This technique can be implemented using commercial all-solid-state laser systems and is expected to be advantageous compared to other narrowban…
