There are several factors which lead to a huge enhancement of parity and time invariance violating effects in the Ra atom: very close electronic levels of opposite parity, the large nuclear charge Z and the collective nature of T,P-odd nuclear moments. Experiments with Radium may be used to measure it's nuclear anapole, magnetic quadrupole and Schiff moments. Such measurements provide information about parity and time invariance violating nuclear forces and electron-nucleon interactions.
Parity (P) and time (T) invariance violating effects in the Ra atom are strongly enhanced due to close states of opposite parity, the large nuclear charge Z and the collective nature of P,T-odd nuclear moments. We have performed calculations of the atomic electric dipole moments (EDM) produced by the electron EDM and the nuclear magnetic quadrupole and Schiff moments. We have also calculated the effects of parity non-conservation produced by the nuclear anapole moment and the weak charge. Our results show that as a rule the values of these effects are much larger than those considered so far i…
Single trapped and laser cooled Radium ion as a possible candidate for measuring the parity violation induced frequency shift has been discussed here. Even though the technique to be used is similar to that proposed by Fortson [1], Radium has its own advantages and disadvantages. The most attractive part of Radium ion as compared to that of Barium ion is its mass which comes along with added complexity of instability as well as other issues which are discussed here
The radium atom is a promising system for studying parity and time invariance violating weak interactions. However, available experimental spectroscopic data for radium is insufficient for designing an optimal experimental setup. We calculate the energy levels and transition amplitudes for radium states of significant interest. Forty states corresponding to all possible configurations consisting of the $7s$, $7p$ and $6d$ single-electron states as well as the states of the $7s8s$, $7s8p$ and $7s7d$ configurations have been calculated. The energies of ten of these states corresponding to the $6…
We explore the possibilities for a next-generation electron-electric-dipole-moment experiment using ultracold heteronuclear diatomic molecules assembled from a combination of radium and another laser-coolable atom. In particular, we calculate their ground state structure and their sensitivity to parity- and time-reversal (${\cal{P,T}}$) violating physics arising from flavor-diagonal charge-parity (${\cal{CP}}$) violation. Among these species, the largest ${\cal{P,T}}$-violating molecular interaction constants -- associated for example with the electron electric dipole moment -- are obtained fo…
The particular advantages of using the diatomic molecule radium monofluoride (RaF) as a versatile molecular probe for physics beyond the Standard Model are highlighted. i) RaF was previously suggested as being potentially amenable to direct cooling with lasers. As shown in the present work, RaF's energetically lowest electronically excited state is of ${}^{2}Π$ symmetry (in contrast to BaF), such that no low-lying ${}^{2}Δ$ state prevents efficient optical cooling cycles. ii) The effective electric field acting on the unpaired electron in the electronic ground state of RaF is estimated larger …
We report on a theoretical analysis of the suitability of the 7s 2S1/2 <-> 6d 2D3/2 transition in singly ionized radium to measure parity nonconservation, in the light of an experiment planned at the KVI of the University of Groningen. Relativistic coupled-cluster theory has been employed to perform an ab initio calculation of the parity nonconserving electric dipole amplitude of this transition, including single, double, and leading triple excitations. We discuss the prospects for a sub-1% precision test of the electroweak theory of particle physics.
The parameter $W_\mathrm{a}$, which characterizes nuclear spin-dependent parity violation effects within the effective molecular spin-rotational Hamiltonian, was computed for the electronic ground state of radium fluoride (RaF) and found to be one of the largest absolute values predicted so far. These calculations were performed with the complex generalised Hartree-Fock method within a two-component (quasi-relativistic) zeroth-order regular approximation framework. Peculiarities of the molecular electronic structure of RaF lead to highly diagonal Franck-Condon matrices between vibrational stat…
The scaling of nuclear spin-dependent parity violating effects with increasing nuclear charge $Z$ is discussed in two series of isovalent open-shell diatomic molecules. The parameter $W_\mathrm{a}$ characterising the strength of parity violation in diatomic molecules is calculated in the framework of the zeroth-order regular approximation (ZORA) and found to be in good agreement with the $R(Z) Z^k$ scaling law derived for atoms in which $R(Z)$ represents a relativistic enhancement factor. The influence of electron correlation is studied on the molecular level, with spin-polarisation effects be…
The radioactive radium-225 ($^{225}$Ra) atom is a favorable case to search for a permanent electric dipole moment (EDM). Due to its strong nuclear octupole deformation and large atomic mass, $^{225}$Ra is particularly sensitive to interactions in the nuclear medium that violate both time-reversal symmetry and parity. We have developed a cold-atom technique to study the spin precession of $^{225}$Ra atoms held in an optical dipole trap, and demonstrated the principle of this method by completing the first measurement of its atomic EDM, reaching an upper limit of $|$$d$($^{225}$Ra)$|$ $<$ $5.0\!…
The existence of a nuclear electric octupole moment (EOM) requires both parity and time invariance violation. The EOMs of odd $Z$ nuclei that are induced by a particular T- and P-odd interaction are calculated. We compare such octupole moments with the collective EOMs that can occur in nuclei having a static octupole deformation. A nuclear EOM can induce a parity and time invariance violating atomic electric dipole moment, and the magnitude of this effect is calculated. The contribution of a nuclear EOM to such a dipole moment is found, in most cases, to be smaller than that of other mechanism…
Studying the violation of parity and time-reversal invariance in atomic systems has proven to be a very effective means for testing the electroweak theory at low energy and searching for physics beyond it. Recent developments in both atomic theory and experimental methods have led to the ability to make extremely precise theoretical calculations and experimental measurements of these effects. Such studies are complementary to direct high-energy searches, and can be performed for just a fraction of the cost. We review the recent progress in the field of parity and time-reversal violation in ato…
We show that the present experimental limits on electron-nucleon interactions that violate both parity and time reversal invariance provide new stringent bounds on the imaginary parts of some of the products of the R-parity violating coupling constants in the R-parity violating Minimal Supersymmetric Standard Model.
We review the current status of the study of parity and time invariance violation in atoms, nuclei and molecules. We focus on parity non-conservation in cesium and three of the most promising areas of research: (i) parity non-conservation in a chain of isotopes, (ii) search for nuclear anapole moments, and (iii) search for permanent electric dipole moments (EDMs) of atoms and molecules, which in turn are caused by either an electron EDM or nuclear $T,P$-odd moments such as a nuclear EDM or nuclear Schiff moment.
Pseudoscalar or pseudovector cosmic fields, that serve as a source of parity ($\mathcal{P}$) violation, are invoked in different models for cold dark matter or in the standard model extension that allows for Lorentz invariance violation. A direct detection of the timelike-component of such fields requires a direct measurement of $\mathcal{P}$-odd potentials or their evolution over time. Herein, advantageous properties of chiral molecules, in which $\mathcal{P}$-odd potentials lead to resonance frequency differences between enantiomers, for direct detection of such $\mathcal{P}$-odd cosmic fiel…
We review current status of the study of parity and time invariance phenomena in atoms, nuclei and molecules. We focus on three most promising areas of research: (i) parity non-conservation in a chain of isotopes, (ii) search for nuclear anapole moments, and (iii) search for permanent electric dipole moments (EDM) of atoms and molecules which are caused by either, electron EDM or nuclear $T,P$-odd moments such as nuclear EDM and nuclear Schiff moment.
Parity and time invariance violating (P,T-odd) nuclear forces produce P,T-odd nuclear moments. In turn, these moments can induce electric dipole moments (EDMs) in atoms through the mixing of electron wavefunctions of opposite parity. The nuclear EDM is screened by atomic electrons. The EDM of an atom with closed electron subshells is induced by the nuclear Schiff moment. Previously the interaction with the Schiff moment has been defined for a point-like nucleus. No problems arise with the calculation of the electron matrix element of this interaction as long as the electrons are considered to …
We consider a mechanism by which dyons (electrically charged magnetic monopoles) can produce both a T- and P-odd (i.e. time reversal invariance and parity violating) mixed polarizability beta [defined by Delta E = -beta E.B, where Delta E is the energy change when electric (E) and magnetic (B) fields are applied to a system] and a T- and P-odd interaction between two particles: psi_1-bar gamma_5 psi_1 psi_2-bar psi_2, where the psi_i are electron and quark spinors. The latter can create atomic and neutron electric dipole moments (EDMs). From experimental bounds on these we find limits on the p…
Planning and interpretation of the experiments searching for the time reversal (T) and parity (P) violation in neutron reactions require values of the matrix elements of the T,P-violating nuclear forces between nuclear compound states. We calculate the root mean square values and the ratio of the matrix elements of the T,P-violating and P-violating interactions using statistical theory based on the properties of chaotic compound states and present the results in terms of the fundamental parameters in four different forms: in terms of the constants of the contact nuclear interaction, meson exch…
