B. A. Cumberland, S. V. Popov, J. R. Taylor, O. I. Medvedkov, S. A. Vasiliev, E. M. Dianov
We report on 33 % efficient generation of the first Stokes in a high concentration GeO2 fiber Raman laser pumped by a 22 W Thulium doped fiber laser. An output power of 4.6 W at 2.105 um is demonstrated.
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The theoretical description of a Raman amplifier based on the vector model of randomly birefringent fibers is proposed and applied to the characterization of Raman polarizers. The Raman polarizer is a special type of Raman amplifier with the property of producing a highly repolarized beam when fed by relatively weak and unpolarized light.
We present a new scheme for a laser cooled Raman optical fiber amplifier. The heat generated in the process of stimulated Raman scattering is compensated for with laser cooling provided by anti-Stokes fluorescence of ytterbium ions doped in the core of the fiber. The device is pumped with two pump sources. One of the pump sources provides Raman amplification of the signal and does not interact with the ytterbium ions in the core of the fiber. The second pump provides laser cooling of the fiber with anti-Stokes fluorescence of the Yb3+ ions. The proper arrangement of Yb3+distribution can provid…
We experimentally demonstrate, for the first time to our knowledge, the generation of correlated photon pairs in a liquid-core photonic crystal fiber. Moreover, we show that, thanks to the specific Raman properties of liquids, the Raman noise (which is the main limitation of the performance of silica-core fiber-based correlated photon pair sources) is highly reduced. With a demonstrated coincident-to-accidental ratio equal to 63 and a pair generation efficiency of about 10$^{-4}$ per pump pulse, this work opens the way for the development of high quality correlated photon pair sources for quan…
We fabricate a fiber coupled ultrahigh-Q resonator from a μdroplet per se; and experimentally measure stimulated Raman emission showing itself at a 160μW threshold. We observe Raman-laser lines that agree with their related calculated molecular-vibrations, as well as with a control-group experiment that uses a Raman-spectrometer. Yet, unlike spectrometers where emission is spontaneous and less directional, our droplet emitter is stimulated, single-mode-fiber coupled, resonantly enhanced with Q of 250 million, confined to a 23 um3 mode volume and has 7 orders of magnitude higher power.
We report the generation of a purely vibrational Raman comb, extending from the vacuum ultraviolet (184 nm) to the visible (478 nm), in hydrogen-filled kagomé-style photonic crystal fiber pumped at 266 nm. Stimulated Raman scattering and molecular modulation processes are enhanced by higher Raman gain in the ultraviolet. Owing to the pressure-tunable normal dispersion landscape of the fiber-gas system in the ultraviolet, higher-order anti-Stokes bands are generated preferentially in higher-order fiber modes. The results pave the way towards tunable fiber-based sources of deep- and vacuum ultra…
Fiber lasers operating via Raman gain or based on rare-earth doped active fibers are widely used as sources of CW radiation. However these lasers are only quasi-CW: their intensity fluctuates strongly on short time-scales. Here the framework of the complex Ginzburg-Landau equations, that are well known as an efficient model of mode-locked fiber lasers, is applied for the description of quasi-CW fiber lasers as well. The first ever vector model of a Raman fiber laser describes the experimentally observed turbulent-like intensity dynamics, as well as polarization rogue waves. Our results open de…
We report on the observation of both stable dissipative solitons and noise-like pulses with the presence of strong Raman scattering in a relatively short all-normal-dispersion Yb-doped fiber laser. We show that Raman scattering can be filtered out by intracavity filter. Furthermore, by appropriate intracavity polarization control, the Raman effect can be utilized to generate broadband noise-like pulses (NLPs) with bandwidth up to 61.4 nm. To the best of our knowledge, this is the broadest NLP achieved in all-normal-dispersion fiber lasers
We demonstrate a new high efficiency architecture for cascaded Raman fiber lasers based on a single pass cascaded amplifier configuration. Conversion is seeded at all intermediate Stokes wavelengths using a multi-wavelength seed source. A lower power Raman laser based on the conventional cascaded Raman resonator architecture provides a convenient seed source providing all the necessary wavelengths simultaneously. In this work we demonstrate a 1480nm laser pumped by an 1117nm Yb-doped fiber laser with maximum output power of 204W and conversion efficiency of 65% (quantum-limited efficiency is ~…
Efficient slow and fast light fiber devices based on narrow band optical parametric amplification require a strict polarization control of the waves involved in the interaction. The use of high birefringence and spun fibers is studied theoretically, possible impairments evaluated, and design parameters determined.
Raman sensing and Raman microscopy are amongst the most specific optical technologies to identify the chemical compounds of unknown samples, and to enable label-free biomedical imaging with molecular contrast. However, the high cost and complexity, low speed, and incomplete spectral information provided by current technology are major challenges preventing more widespread application of Raman systems. To overcome these limitations, we developed a new method for stimulated Raman spectroscopy and Raman imaging using continuous wave (CW), rapidly wavelength swept lasers. Our all-fiber, time-encod…
High power fiber lasers operating at the 1.5micron wavelength region have attractive features like eye-safety and atmospheric transparency, and cascaded Raman fiber lasers offer a convenient method to obtain high power sources at these wavelengths. A limitation to power scaling however has been the lower conversion efficiency of these lasers. We recently introduced a high efficiency architecture for high power cascaded Raman fiber lasers applicable for 1.5micron fiber lasers. Here we demonstrate further power scaling using this new architecture. Using numerical simulations we identify the idea…
Kilowatt-level high efficiency all-fiberized Raman fiber amplifier based on pure passive fiber is proposed for the first time in this paper. The laser system is established on master oscillator power amplification configuration while a piece of graded-index passive fiber is utilized as stokes shifting as well as gain medium, which is entirely irrelevant to rare-earth-doped gain mechanism. When the pump power is 1368.8 W, we obtained 1002.3 W continuous-wave laser power at 1060 nm with the corresponding optical-to-optical efficiency of 84%. The beam parameter M2 improves from 9.17 of the pump l…
Spontaneous Raman scattering in SDM fibers
本研究将单模光纤中的自发拉曼散射模型扩展至多模光纤，用于评估光链路中的散射噪声，并通过实验验证其有效性。
We demonstrate sensitive high-resolution stimulated Raman measurements of hydrogen using a hollow-core photonic crystal fiber (HC-PCF). The Raman transition is pumped by a narrow linewidth (<50 kHz) 1064 nm continuous-wave (CW) fiber laser. The probe light is produced by a homebuilt CW optical parametric oscillator (OPO), tunable from around 800 nm to 1300 nm (linewidth ~ 5 MHz). These narrow linewidth lasers allow for an excellent spectral resolution of approximately 10^-4 cm^(-1). The setup employs a differential measurement technique for noise rejection in the probe beam, which also elimina…
Hydrogen detection is of great importance in chemical and energy industries. Optical fiber hydrogen sensors show flexibility and compactness and have the potential for distributed analysis. However, traditional fiber sensors encounter a challenge for light to interact with hydrogen directly since hydrogen only display weak quadrupole absorption, and metallic palladium and platinum thin-film coatings are typically used as an optically detectable label. Here, based on stimulated Raman spectroscopy in hollow-core photonic crystal fibers, we investigate the label-free optical fiber distributed hyd…
We experimentally study the competition between Kerr beam self-cleaning and Raman beam cleanup in a multimode air-silica microstructure optical fiber. Kerr beam self-cleaning of the pump is observed for a certain range of input powers only. Raman Stokes beam generation and cleanup lead to both depletion and degradation of beam quality for the pump. The interplay of modal four-wave mixing and Raman scattering in the infrared domain lead to the generation of a multimode supercontinuum ranging from 500 nm up to 1800 nm.
Raman fiber lasers (RFLs) are currently promising and versatile light sources for a variety of applications. So far, operations of high power and brightness-enhanced RFLs have absorbed enormous interests along with rapid progress. Nevertheless, the stable Raman lasing at high power levels remains challenged by the thermal effects. In an effort to realize more effective thermal management in high power RFLs, here we demonstrate, for the first time, an all-fiberized RFA employing metal-coated passive fiber enabling high power lasing. By employing aluminum to the cladding of graded-index (GRIN) p…
This letter is to pave the way towards the demonstration of spatiotemporal similariton pulses evolution in passive multimode fibers with Raman amplification. We present numerically these issues in a graded-index and step-index multimode fibers and provide a first look at the complex spatiotemporal dynamics of similariton pulses. The results showed that the similariton pulses can be generated in both multimode fibers. The temporal and the spectral evolution of the pulses can be characterized as parabolic shapes with linear chirp and kW peak power. By compressed these, high energy femtoseconds p…
Raman-Accelerated Power Depletion of Fundamental Mode in a Few-Mode Fiber in the Visible Spectral Range
本文实验和数值研究可见光超短脉冲在少模光纤基模中由拉曼散射引起的功率耗尽，发现能量向高阶模式显著转移，对高功率激光传输和光通信有重要意义。
In this paper we consider mid-infrared Raman lasers based on gas-filled hollow-core silica fibers and provide theoretical and experimental analysis of factors that limit the efficiency and output power of these lasers. As a result, we realized an efficient ns-pulsed 4.42 μm Raman laser based on an 1H2-filled revolver silica fiber. Quantum efficiency as high as 36 % is achieved, and output average power as high as 250 mW is demonstrated. The possibilities of further improving the laser efficiency are discussed.
In this letter, we present a high pulse energy Raman laser at 1946 nm wavelength directly pumped with a 1533 nm custom-made fiber laser. The Raman laser is based on the stimulated Raman scattering (SRS) in an 8-meter carbon dioxide (CO2) filled nested anti-resonant hollow-core fiber (ARHCF). The low energy phonon emission combined with the inherent SRS process along the low-loss fiber allows the generation of high pulse energy up to 15.4 μJ at atmospheric CO2 pressure. The Raman laser exhibits good long-term stability and low relative intensity noise (RIN) of less than 4%. We also investigate …
We demonstrate a route to supercontinuum generation in gas-filled hollow-core anti-resonant fibers through the creation of a broad vibrational Raman frequency comb followed by continuous broadening and merging of the comb lines through either rotational Raman scattering or the optical Kerr effect. Our demonstration experiments, utilizing a single pump pulse with 20 ps duration at 532 nm in a nitrogen-filled fiber, produce a supercontinuum spanning from 440 nm to 1200 nm, with an additional deep ultraviolet continuum from 250 nm to 360 nm. Numerical results suggest that this approach can produc…
The theory of two counter-propagating polarized beams interacting in a randomly birefringent fiber via the Kerr and Raman effects is developed and applied to the quantitative description of Raman polarizers in the undepleted regime. Here Raman polarizers, first reported by Martinelli et. al. [Opt. Express. 17, 947 (2009)], are understood as Raman amplifiers operating in the regime in which an initially weak unpolarized beam is converted into an amplified fully polarized beam towards the fiber output. Three parameters are selected for the characterization of a Raman polarizer: the degree of pol…
In this letter, the characteristics of noise and long-term stability of near- and mid-infrared (near-IR and mid-IR) gas-filled fiber Raman lasers have been investigated for the first time. The results reveal that an increase in Raman pulse energy is associated with a decrease in noise, and that the relative pulse peak intensity noise (RIN) is always lower than the relative pulse energy noise (REN). We also demonstrate that long-term drift of the pulse energy and peak power are directly linked with the high amount of heat release during the Raman Stokes generation. The demonstrated noise and lo…
We report on trapped pulse generation in birefringent microstructured optical fiber. Linearly polarized fs pulses are injected into the microstructured fiber in anomalous dispersion regime. We observed experimentally that soliton pulse polarized along the fast fiber axis partially transfers its energy to the orthogonal polarization. The generated pulse is amplified through the orthogonal Raman gain. The two polarization components are located at group-velocity matched wavelengths. The experimental works are supported with numerical simulations. The obtained results are important for the light …
We demonstrate a high power, all-fiber, tunable laser source that can operate in the L-band region. A low power, tunable input laser is amplified with a recently proposed, high efficiency, 6th order cascaded Raman amplifier. The proposed system is scalable and overcomes the limitations of Erbium and Erbium-Ytterbium co-doped fiber lasers for power scaling. A tunable Erbium-Ytterbium co-doped fiber ring laser generating ~0.5W of power and tunable in the 1560-1590 nm wavelength range is utilized as the seed source. The output from the seed laser is amplified to ~24 W using 6th order cascaded Ram…
In this work, we present a high pulse energy multi-wavelength Raman laser spanning from 1.53 um up to 2.4 um by employing the cascaded rotational stimulated Raman scattering (SRS) effect in a 5-m hydrogen (H2) -filled nested anti-resonant fiber (NARF), pumped by a linearly polarized Er/Yb fiber laser with a peak power of ~13 kW and pulse duration of ~7 ns in the C-band. The developed Raman laser has distinct lines at 1683 nm, 1868 nm, 2100 nm, and 2400 nm, with pulse energies as high as 18.25 uJ, 14.4 uJ, 14.1 uJ, and 8.2 uJ, respectively. We demonstrate how the energy in the Raman lines can b…
We report Raman lasing and the optical analog of electromagnetically-induced-transparency (EIT) in a whispering-gallerymode (WGM) microtoroid resonator embedded in a low refractive index polymer matrix together with a tapered fiber coupler. The Raman laser supports both single and multimode operation with low power thresholds. Observations of Fano and EIT-like pheonomena in a packaged microresonator will enable high resolution sensors and can be used in networks where slow light process is needed. These results open the way for portable, robust, and stable WGM microlasers and laserbased sensor…
A novel method for efficient generation of high power, equalized continuous-wave supercontinuum source in an all conventional silica fiber architecture is demonstrated. Highly nonlinear fiber (HNLF) is pumped in its anomalous dispersion region using a novel, high power, L-band laser. The L-band laser encompasses a 6th order cascaded Raman amplifier which is pumped with a high power Ytterbium doped fiber laser and amplifies a low-power, tunable L-band seed source. The supercontinuum generated 35W of power with ~40% efficiency. The Supercontinuum spectrum was measured to have a high degree of fl…
In this paper, we demonstrate that it is possible to combine both Raman amplification and polarization attraction of a signal wave in a single optical fiber by means of a counterpropagating scheme. Experiments were performed near 1550 nm in a continuous wave regime and by means of a 10 Gbit / s return-to-zero signal injected in a 20 kmlong low polarization mode dispersion optical fiber. Complete repolarization and 6.7 dB amplification of the signal wave was achieved by injecting a 850 mW, 1480 nm counterpropagating polarized pump wave.
Optical properties of hollow-core revolver fibers are numerically investigated depending on various parameters: the hollow-core diameter, the capillary wall thickness, the values of the minimum gap between the capillaries, the number of capillaries in the cladding and the type of glass (silica and chalcogenide). Preliminary, similar calculations are made for simple models of hollow-core fibers. Based on the obtained results, the optimal design of the revolver fiber for Raman laser frequency conversion (1560 nm to 4420 nm in H2) was determined. As a result, efficient ns-pulsed 4420 nm Raman las…
The interplay of such cornerstones of modern nonlinear fiber optics as a nonlinearity, stochasticity and polarization leads to variety of the noise induced instabilities including polarization attraction and escape phenomena harnessing of which is a key to unlocking the fiber optic systems specifications required in high resolution spectroscopy, metrology, biomedicine and telecommunications. Here, by using direct stochastic modeling, the mapping of interplay of the Raman scattering-based nonlinearity, the random birefringence of a fiber, and the pump-to-signal intensity noise transfer has been…
We have developed an analytical model based on the perturbation theory in order to study the optical propagation of two successive intense solitons in hollow-core photonic crystal fibers filled with Raman-active gases. Based on the time delay between the two solitons, we have found that the trailing soliton dynamics can experience unusual nonlinear phenomena such as spectral and temporal soliton oscillations and transport towards the leading soliton. The overall dynamics can lead to a spatiotemporal modulation of the refractive index with a uniform temporal period and a uniform or chirped spat…
Cascaded Raman lasers enable high powers at various wavelength bands inaccessible with conventional rare-earth doped lasers. The input and output wavelengths of conventional implementations are fixed by the constituent fiber gratings necessary for cascaded Raman conversion. We demonstrate here, a simple architecture for high power, fixed and wavelength tunable, grating-free, cascaded Raman conversion between different wavelength bands. The architecture is based on the recently proposed distributed feedback Raman lasers. Here, we implement a module which converts the Ytterbium band to the eye-s…
The main subject of this contribution is the all-optical control over the state of polarization (SOP) of light, understood as the control over the SOP of a signal beam by the SOP of a pump beam. We will show how the possibility of such control arises naturally from a vectorial study of pump-probe Raman interactions in optical fibers. Most studies on the Raman effect in optical fibers assume a scalar model, which is only valid for high-PMD fibers (here, PMD stands for the polarization-mode dispersion). Modern technology enables manufacturing of low-PMD fibers, the description of which requires …
In this work, the spectral evolution properties in single-frequency Raman fiber amplifier (RFA) with different pump manners are analyzed theoretically for the first time based on the gain dynamics. The analysis of gain dynamics reveals that the walk-off effect in counter-pumped manner produces a natural low-pass filter in single-frequency RFA. When applying rare-earth doped fiber lasers as the pump source, the strong temporal fluctuations in the pump source lead to spectral broadening in co-pumped manner, while the natural low-pass filter in countered-pumped case can still ensure single-freque…
As shown in the early 1960s, the gain in stimulated Raman scattering (SRS) is drastically suppressed when the rate of creation of phonons (via pump-to-Stokes conversion) is exactly balanced by the rate of phonon annihilation (via pump-to-anti-Stokes conversion). This occurs when the phonon coherence waves synchronized vibrations of a large population of molecules have identical propagation constants for both processes, i.e., they are phase-velocity matched. As recently demonstrated, hydrogen-filled photonic crystal fiber pumped in the vicinity of its zero dispersion wavelength provides an idea…
The red shifted solitonic resonant radiation is a fascinating phase matching phenomenon that occurs when an optical pulse, launched in the normal dispersion regime of photonic crystal fiber, radiates across the zero dispersion wavelength. The formation of such phase-matched radiation is independent of the generation of any optical soliton and mainly governed by the leading edge of input pump which forms a shock front. The radiation is generated at the anomalous dispersion regime and found to be confined both in time and frequency domain. We experimentally investigate the formation of such radi…
Experimental observation of self-frequency-shifting Raman quasi-solitons in a fiber Fabry-Perot resonator
本文实验观测了脉冲泵浦高Q值光纤法布里-珀罗谐振腔中由四阶色散调制不稳定性诱发的自频移拉曼准孤子，首次用色散傅里叶变换识别该过程，并通过同步失配抑制实现标准耗散克尔孤子。
Four-wave mixing in the form of Bragg scattering (BS) has been predicted to enable quantum noise less frequency conversion by analytic quantum approaches. Using a semi-classical description of quantum noise that accounts for loss and stimulated and spontaneous Raman scattering, which are not currently described in existing quantum approaches, we quantify the impacts of these effects on the conversion efficiency and on the quantum noise properties of BS in terms of an induced noise figure (NF). We give an approximate closed-form expression for the BS conversion efficiency that includes loss and…
Broadband-tunable sources of circularly-polarized light are crucial in fields such as laser science, biomedicine and spectroscopy. Conventional sources rely on nonlinear wavelength conversion and polarization control using standard optical components, and are limited by the availability of suitably transparent crystals and glasses. Although gas-filled hollow-core photonic crystal fiber provides pressure-tunable dispersion, long well-controlled optical path-lengths, and high Raman conversion efficiency, it is unable to preserve circular polarization state, typically exhibiting weak linear biref…
We propose supercritical xenon in a hollow-core photonic bandgap fiber as a highly nonlinear medium, and demonstrate 200 nm control over the guidance window of the fiber as the xenon goes through its supercritical phase transition. The large optical polarizability and monoatomic nature of xenon are predicted to allow large optical nonlinearity, on the same order as that of fused silica, while maintaining greatly reduced Raman scattering, offering benefits for nonlinear and quantum optics.
We report on experimental realization of impulsive rotational Raman scattering from neutral nitrogen molecules in a femtosecond laser filament using an intense self-induced white-light seeding "air laser" generated during the filamentation of an 800 nm Ti: Sapphire laser in nitrogen gas. The impulsive rotational Raman fingerprint signals are observed with a maximum conversion efficiency of ~0.8%. Our observation provides a promising way of remote identification and location of chemical species in atmosphere by rotational Raman scattering of molecules.
Ultrafast broadband ultraviolet radiation is of importance in spectroscopy and photochemistry, since high photon energies enable single-photon excitations and ultrashort pulses allow time-resolved studies. Here we report the use of gas-filled hollow-core photonic crystal fibers (HC-PCFs) for efficient ultrafast nonlinear optics in the ultraviolet. Soliton self-compression of 400 nm pulses of (unprecedentedly low) ~500 nJ energies down to sub-6-fs durations is achieved, as well as resonant emission of tunable dispersive waves from these solitons. In addition, we discuss the generation of a flat…
We present the design and anticipated performance of an optically pumped monolithic all-silicon mid-IR (MIR) Raman laser. For the proposed 3.15 um cw laser design pumped at a 2.71 um pump wavelength, we estimate a threshold pump power of < 10 mW and an estimated output laser linewidth of <50 MHz. This design may pave the road toward demonstration of the first mid-IR silicon Raman laser.
By focusing on a typical emitting wavelength of 1120 nm as an example, we present the first demonstration of a high-efficiency, narrow-linewidth kilowatt-level all-fiber amplifier based on hybrid ytterbium-Raman (Yb-Raman) gains. Notably, two temporally stable, phase-modulated single-frequency lasers operating at 1064 nm and 1120nm, respectively, were applied in the fiber amplifier, to alleviate the spectral broadening of the 1120 signal laser and suppress the stimulated Brillouin scattering (SBS) effect simultaneously. Over 1 kW narrow-linewidth 1120 nm signal laser was obtained with a slope …
We present a technique for simultaneous power-combining and wavelength-conversion of multiple fiber lasers into a single, lower wavelength in a different band through Raman-based, nonlinear power combining. We illustrate this by power combining of two independent Ytterbium lasers into a single wavelength around 1.5micron with high output powers of upto 99W. A high conversion efficiency of ~64% of the quantum limited efficiency and a high level of wavelength conversion with >85% of the output power in the final wavelength is demonstrated. The proposed method enables power-scaling in various wav…
High-Polarization-Extinction Raman Conversion in Gas-Filled Polarization-Maintaining Hollow-Core Fibers
通过偏振维持空芯光纤实现高偏振纯度的拉曼转换，为气体光子学中的偏振可控光源提供新方案。
We describe the application of Raman Optical-fiber Amplification (ROA) for the phase coherent transfer of optical frequencies in an optical fiber link. ROA uses the transmission fiber itself as a gain medium for bi-directional coherent amplification. In a test setup we evaluated the ROA in terms of on-off gain, signal-to-noise ratio, and phase noise added to the carrier. We transferred a laser frequency in a 200 km optical fiber link with an additional 16 dB fixed attenuator (equivalent to 275 km of fiber on a single span), and evaluated both co-propagating and counter-propagating amplificatio…
A scheme for an X-ray free electron laser is proposed, based on a Raman process occurring during the interaction between a moderately relativistic bunch of free electrons, and twin intense short pulse lasers interfering to form a transverse standing wave along the electron trajectories. In the high intensity regime of the Kapitza-Dirac effect, the laser ponderomotive potential forces the electrons into a lateral oscillatory motion, resulting in a Raman scattering process. I show how a parametric process is triggered, resulting in the amplification of the Stokes component of the Raman-scattered…
We report on the generation of a Raman cascade spanning the wavelength range of 523 to 1750 nm wavelength range, in a standard telecommunication graded-index multimode optical fiber. Despite the highly multimode nature of the pump, the Raman peaks are generated in specific modes of the fiber, confirming substantial beam cleanup during the stimulated Raman scattering process.
We show that, in multimode Raman lasers, cascaded light scattering (CLS) not only extends the optical frequency range, but could also modulate the laser dynamics. The origin of this phenomenon is based on the fact that many Raman lasing modes are directly correlated through CLS. The coupled-mode equations only describe single-mode cascaded Raman lasers and are insufficient for describing the multimode case. In this work, we introduce additional terms to account for intermodal interaction and, thence, reveal the physical mechanism behind the mode-switching phenomenon. Additionally, mode-switchi…
The unique ring-shaped intensity patterns and helical phase fronts of optical vortices make them useful in many applications. Here we report for the first time efficient Raman frequency conversion between vortex modes in twisted hydrogen-filled single-ring hollow core photonic crystal fiber (SR-PCF). High fidelity transmission of optical vortices in untwisted SR-PCF becomes more and more difficult as the orbital angular momentum (OAM) order increases, due to scattering at structural imperfections in the fiber microstructure. In helically twisted SR-PCF, however, the degeneracy between left- an…
In this work, we derive and present the coupled amplitude equations to describe the evolutions of different spectral components in different transverse modes for Raman fiber amplifiers (RFAs). Both the effects of the four-wave-mixing in the fundamental mode (FM FWM) and the inter-modal four-wave-mixing (IM FWM) on high-power RFAs are demonstrated through numerical simulations. Specifically, effective FM FWM interactions could occur and lead to a drop of the Raman threshold for RFAs by over 50%, despite that the corresponding wave-vector mismatch is rather big. In addition, the IM FWM could als…
We show that coherent anti-Stokes Raman lineshapes do not follow known spectral profiles if the time asymmetry of realistic laser pulses is taken into account. Examples are given for nanosecond and picosecond laser pulses commonly employed in frequency-resolved coherent anti-Stokes Raman scattering. More remarkably, the analysis suggests an effect of line narrowing in comparison to the customary approach, based primarily on the Voigt lineshape.
Backward stimulated Raman scattering in gases provides a promising route to compression and amplification of a Stokes seed-pulse by counter-propagating against a pump-pulse, as has been already demonstrated in various platforms, mainly in free-space. However, the dynamics governing this process when seeded by noise has not yet been investigated in a fully controllable collinear environment. Here we report the first unambiguous observation of efficient noise-seeded backward stimulated Raman scattering in a hydrogen-filled hollow-core photonic crystal fiber. At high gas pressures, when the backw…
In 1964 Bloembergen and Shen predicted that Raman gain could be suppressed if the rates of phonon creation and annihilation (by inelastic scattering) exactly balance. This is only possible if the momentum required for each process is identical, i.e., phonon coherence waves created by pump-to-Stokes scattering are identical to those annihilated in pump-to-anti-Stokes scattering. In bulk gas cells, this can only be achieved over limited interaction lengths at an oblique angle to the pump axis. Here we report a simple system that provides dramatic Raman gain suppression over long collinear path-l…
Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies and laser power. Here we report efficient generation of deep and vacuum UV light using hydrogen-filled hollow-core photonic crystal fiber (HC-PCF). Pumping above the stimulated Raman threshold at 532 nm, coherent molecular vibrations are excited in the gas, permitting highly efficient thresholdless wavelength conversion in the UV. The system is uniquely press…
We report on the observation of a novel mode locked optical comb generated at the Raman offset (Raman comb) in an optically pumped crystalline whispering gallery mode resonator. Mode locking is confirmed via measurement of the radio-frequency beat note produced by the optical comb on a fast photodiode. Neither the conventional Kerr comb nor hyper-parametric oscillation is observed when the Raman comb is present.
We study coherent anti-Stokes Raman spectroscopy in air-filled anti-resonance hollow-core photonic crystal fiber, otherwise known as 'revolver' fiber. We compare the vibrational coherent anti-Stokes Raman signal of N$_2$, at 2331 cm$^{-1}$, generated in ambient air (no fiber present), with the one generated in a 2.96 cm of a revolver fiber. We show a 170 times enhancement for the signal produced in the fiber, due to an increased interaction path. Remarkably, the N$_2$ signal obtained in the revolver fiber shows near-zero non-resonant background, due to near-zero overlap between the laser field…
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