We demonstrate a standing wave light pulse sequence that places atoms into a superposition of displaced wavepackets with precisely controlled displacements that remain constant for times as long as 1 s. The separated wavepackets are subsequently recombined resulting in atom interference patterns that probe energy differences of approximately 10^-34 J, and can provide acceleration measurements that are insensitive to platform vibrations.
Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain both high temporal and spectral resolution by stimulating Raman interferences with one light pulse and monitoring the differential changes in the electron yield in a separate step. Applying this spectroscopic approach to the autoionizing states of argon, we experimentally resolved its electronic composition and time-evolution in exquisite detail. Theoretical ca…
A Ramsey-type interferometer is suggested, employing a cold trapped ion and two time-delayed off-resonant femtosecond laser pulses. The laser light couples to the molecular polarization anisotropy, inducing rotational wavepacket dynamics. An interferogram is obtained from the delay dependent populations of the final field-free rotational states. Current experimental capabilities for cooling and preparation of the initial state are found to yield an interferogram visibility of more than 80\%. The interferograms can be used to determine the polarizability anisotropy with an accuracy of about $\p…
We propose a marginally stable optical resonator suitable for atom interferometry. The resonator geometry is based on two flat mirrors at the focal planes of a lens that produces the large beam waist required to coherently manipulate cold atomic ensembles. Optical gains of about 100 are achievable using optics with part-per-thousand losses. The resulting power build-up will allow for enhanced coherent manipulation of the atomic wavepackets such as large separation beamsplitters. We study the effect of longitudinal misalignments and assess the robustness of the resonator in terms of intensity a…
We present designs for the augmentation 'mirror' pulses of large-momentum-transfer atom interferometers that maintain their fidelity as the wavepacket momentum difference is increased. These bi-selective pulses, tailored using optimal control methods to the evolving bi-modal momentum distribution, should allow greater interferometer areas and hence increased inertial measurement sensitivity, without requiring elevated Rabi frequencies or extended frequency chirps. Using an experimentally validated model, we have simulated the application of our pulse designs to large-momentum-transfer atom int…
Atom interferometry relies on the separation and recombination of atom wavepackets. When the two paths overlap perfectly at the end of the interferometer, the phase is insensitive to the atomic velocity distribution. Here, we show that, when the separation and recombination is performed using a Raman transition there is a displacement of the atomic wavepacket due to a phase shift during light pulses. Because of the variation of the laser intensity seen by the atoms, there is an imperfect cancellation of these displacements. The observation of a velocity-dependent phase shift on the interferome…
We show that light-pulse atom interferometry with atomic point sources and spatially resolved detection enables multi-axis (two rotation, one acceleration) precision inertial sensing at long interrogation times. Using this method, we demonstrate a light-pulse atom interferometer for Rb-87 with 1.4 cm peak wavepacket separation and a duration of 2T = 2.3 seconds. The inferred acceleration sensitivity of each shot is 6.7 * 10^(-12) g, which improves on previous limits by more than two orders of magnitude. We also measure the Earth's rotation rate with a precision of 200 nrad/s.
We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the ionization. The phase of the photoelectron wavepackets is measured by an attosecond interferometric technique, using the 17$^\mathrm{th}$ harmonic. We perform experiments with angular resolution using a velocity map imaging spectrometer and with high energy resolution using a magnetic bottle electron spectrometer. Our results are compared to calculations using th…
We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic orders with a sufficient degree of alignment. This results from molecular-scale quantum interferences between the molecular electronic wave function and the recolliding electron as it recombines with the molecule, and is consistent with a two-center model. Furthermore, using the combined harmonic intensity and phase information, we extract accurate information…
Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be described as a coherent sum of waves of given angular momentum, called partial waves, each characterized by an amplitude and a phase. The complete characterization of the individual angular momentum components is experimentally challenging, requiring the analysis of the interference between partial waves both in energy and angle. Using a two-photon interferometry …
We propose new multi-dimensional atom optics that can create coherent superpositions of atomic wavepackets along three spatial directions. These tools can be used to generate light-pulse atom interferometers that are simultaneously sensitive to the three components of acceleration and rotation, and we discuss how to isolate these inertial components in a single experimental shot. We also present a new type of atomic gyroscope that is insensitive to parasitic accelerations and initial velocities. The ability to measure the full acceleration and rotation vectors with a compact, high-precision, l…
We simulate ultracold Sagnac atom interferometers using quantum-mechanical matter wavepackets, e.g. Bose-Einstein condensates, that counter-propagate within a rotating ring-trap. We find that the accumulation of the relative phase difference between wavepackets, i.e. the matter wave Sagnac effect, is manifested as discrete phase jumps. These plateaus result from three effects; that the atoms should be initially trapped at rest with respect to the rotating frame, that they counter-propagate with the same group velocities in the rotating frame, and that the imaging is performed in the rotating f…
We propose a tractor atom interferometer (TAI) based on three-dimensional (3D) confinement and transport of split atomic wavefunction components in potential wells that follow programmed paths. The paths are programmed to split and recombine atomic wavefunctions at well-defined space-time points, guaranteeing closure of the interferometer. Uninterrupted 3D confinement of the interfering wavefunction components in the tractor wells eliminates coherence loss due to wavepacket dispersion. Using Crank-Nicolson simulation of the time-dependent Schrödinger equation, we compute the quantum evolution …
We report entanglement of a single atom's hyperfine spin state with its motional state in a timescale of less than 3 ns. We engineer a short train of intense laser pulses to impart a spin-dependent momentum transfer of +/- 2 hbar k. Using pairs of momentum kicks, we create an atomic interferometer and demonstrate collapse and revival of spin coherence as the motional wavepacket is split and recombined. The revival after a pair of kicks occurs only when the second kick is delayed by an integer multiple of the harmonic trap period, a signature of entanglement and disentanglement of the spin with…
Leibniz University Hannover（汉诺威莱布尼茨大学）；University Innsbruck（因斯布鲁克大学）；Institute for Quantum Optics and Quantum Information, Austrian Academy of Sciences（奥地利科学院量子光学与量子信息研究所）
A new generation of atomic sensors using ultra-narrow optical clock transitions and composite pulses are pushing quantum engineering control to a very high level of precision for applied and fundamental physics. Here, we propose a new version of Ramsey-Bordé interferometry introducing arbitrary composite laser pulses with tailored pulse duration, Rabi field, detuning and phase-steps. We explore quantum metrology below the $10^{-18}$ level of fractional accuracy by a fine tuning control of light excitation parameters protecting ultra-narrow optical clock transitions against residual light-shift…
We describe an atom interferometric gravitational wave detector design that can operate in a resonant mode for increased sensitivity. By oscillating the positions of the atomic wavepackets, this resonant detection mode allows for coherently enhanced, narrow-band sensitivity at target frequencies. The proposed detector is flexible and can be rapidly switched between broadband and narrow-band detection modes. For instance, a binary discovered in broadband mode can subsequently be studied further as the inspiral evolves by using a tailored narrow-band detector response. In addition to functioning…
In an atomic interferometer, the phase shift due to rotation is proportional to the area enclosed by the split components of the atom. However, this model is unclear for an atomic interferometer demonstrated recently by Shahriar et al., for which the atom simply passes through a single-zone optical beam, consisting of a pair of bichromatic counter-propagating beams. During the passage, the atomic wave packets in two distinct internal states couple to each other continuously. The two internal states trace out a complicated trajectory, guided by the optical beams, with the amplitude and spread o…
Long-time atom interferometry is instrumental to various high-precision measurements of fundamental physical properties, including tests of the equivalence principle. Due to rotations and gravity gradients, the classical trajectories characterizing the motion of the wave packets for the two branches of the interferometer do not close in phase space, an effect which increases significantly with the interferometer time. The relative displacement between the interfering wave packets in such open interferometers leads to a fringe pattern in the density profile at each exit port and a loss of contr…
