Electromagnetic forces for an arbitrary optical trapping of a spherical dielectric
Antonio Alvaro Ranha Neves, Adriana Fontes, Liliana de Ysasa Pozzo, Andre Alexandre de Thomaz, Enver Chillce, Eugenio Rodriguez, Luiz Carlos Barbosa, Carlos Lenz Cesar
Analytical solution for optical trapping force on a spherical dielectric particle for an arbitrary positioned focused beam is presented in a generalized Lorenz-Mie and vectorial diffraction theory. In this case the exact electromagnetic field is considered in the focal region. A double tweezers setup was employed to perform ultra sensitive force spectroscopy and observe the forces, demonstrating the selectively couple of the transverse electric (TE), transverse magnetic (TM) modes by means of the beam polarization and positioning, and to observe correspondent morphology-dependent resonances (MDR) as a change in the optical force. The theoretical prediction of the theory agrees well with the experimental results. The algorithm presented here can be easily extended to other beam geometries and scattering particles.
We demonstrate that a single sub-wavelength nanoaperture in a metallic thin film can be used to achieve dynamic optical trapping and control of a single dielectric nanowire. A nanoaperture can trap a nanowire, control its orientation when illuminated by a linearly-polarized incident field, and also rotate the nanowire when illuminated by a circularly-polarized incident field. Compared to other designs, this approach has the advantages of a low-power driving field entailing low heating and photodamage.
The phenomenon of trapping broad spectrum of light is known as `rainbow trapping' and achieved using all-dielectric, hybrid metallo-dielectric or all-metallic configurations. In the latter cases, unavoidable ohmic losses result in sub-picosecond trapped-mode lifetimes. For all practical purposes, novel strategies are required to be devised for trapping and subsequently, releasing broadband electromagnetic (em) field with lifetime > 1 ps. We present a rainbow trapping configuration using the excitation of multiple optical Tamm (OT) modes in an one-dimensional chirped photonic crystal (PC) desig…
We propose a dielectric structure which focuses the laser light well beyond the diffraction limit and thus considerably enhances the exerted optical trapping force upon dielectric nanoparticles. Although the structure supports a Fabry-Perot resonance, it actually acts as a nanoantenna in that the role of the resonance is to funnel the laser light into the structure. In comparison with the lens illuminating the structure, the proposed structure offers roughly a 10000-fold enhancement in the trapping force - part of this enhancement comes from an 80-fold enhancement in the field intensity, and t…
Tuning the near-field using all-dielectric nano-antennae offers a promising approach for trapping atoms, which could enable strong single-atom/photon coupling. Here we report the simulation results of an optical trapping concept, in which a silicon nano-antenna produces a trapping potential for atoms in a chip-scale configuration. Using counter-propagating incident fields, bichromatically detuned from the atomic cesium D-lines, we numerically investigate the dependence of the optical potential on the nano-antenna geometry. We tailor the near-field potential landscape by tuning the evanescent f…
We demonstrate bound states in the first TE and TM diffraction continua (BSC) in a linear periodic array of dielectric spheres in air above the light cone. We classify the BSCs according to the symmetry specified by the azimuthal number $m$, the Bloch wave vector $β$ directed along the array, and polarization. The most simple symmetry protected TE and TM polarized BSCs have $m=0$ and $β=0$ and occur in a wide range of the radius of the spheres and dielectric constant. More complicated BSCs with $m\neq 0$ and $β=0$ exist only for a selected radius of spheres at a fixed dielectric constant. We a…
Optical manipulation in the vicinity of optical micro- and nanofibres has shown potential across several fields in recent years, including microparticle control, and cold atom probing and trapping. To date, most work has focussed on propagation of the fundamental mode through the fibre. However, along the maximum mode intensity axis, higher order modes have a longer evanescent field extension and larger field amplitude at the fibre waist compared to the fundamental mode, opening up new possibilities for optical manipulation and particle trapping. In this work, we demonstrate a microfibre/optic…
We investigate the phenomenon of the transverse breaking of symmetry of Gaussian lasers transmitted through dielectrics, showing for which incidence conditions and beam parameters it can be observed in optical experiments. The numerical analysis, done by using the integral form of the transmitted beam at the lower interface of a dielectric prism, shows, for incidence approaching the critical region, a laser planar trapping. By using an analytic approximation for the intensity of lower transmitted beam, we model the wave front curvature by a closed expression which depends on the refractive ind…
Controlling the transport, trapping, and filtering of nanoparticles is important for many applications. By virtue of their weak response to gravity and their thermal motion, various physical mechanisms can be exploited for such operations on nanoparticles. However, the manipulation based on optical forces is potentially most appealing since it constitutes a highly deterministic approach. Plasmonic nanostructures have been suggested for this purpose, but they possess the disadvantages of locally generating heat and trapping the nanoparticles directly on surface. Here, we propose the use of diel…
Optical energy flow inside a dielectric microsphere exposed to an optical wave is usually codirected with its wave vector. At the same time, if the optical field in a microparticle is in resonance with a high-quality spatial eigenmode, referred to as the whispering-gallery mode (WGM), at least two regions of reverse energy flow emerge in the illuminated and shadow particle hemispheres. These areas are of considerable practical interest due to their enhanced optical trapping potential provided they should be previously cleared from particle material. In this paper, we consider a perforated micr…
Enantioselective optical trapping and characterization of all dielectric disorder-enabled chiral particles
Instituto de Física, Universidade Federal do Rio de Janeiro（里约热内卢联邦大学物理研究所）；Laboratoire Kastler Brossel, Sorbonne Université, CNRS, ENS-PSL, Collège de France（巴黎高等师范学院-PSL研究大学、法兰西公学院、法国国家科学研究中心和索邦大学卡斯特勒·布罗塞尔实验室）
Slow light and rainbow trapping attract many attentions in last twenty years, and in most of the previous works, the researchers achieve the slow light and rainbow trapping with complicate configurations or techniques, for example, metamaterial techniques. In this paper, we propose a simple waveguide consisted with semiconductor and dielectric layers, and we find that the slow-light peaks appear in the dispersion curves. Besides, the cutoff frequency with $v_g = 0$ ($v_g$ is the group velocity) in the slow-light peaks is depending on the thicknesses of the semiconductor and dielectric. Then, w…
We numerically investigate the propagation of a spatially localized and quasi-monochromatic electromagnetic pulse through a slab with Lorentz dielectric response in the epsilon-near-zero regime, where the real part of the permittivity vanishes at the pulse carrier frequency. We show that the pulse is able to excite a set of virtual polariton modes supported by the slab, the excitation undergoing a generally slow damping due to absorption and radiation leakage. Our numerical and analytical approaches indicate that in its transient dynamics the electromagnetic field displays the very same enhanc…
Optical trapping, where microscopic particles are trapped and manipulated by light is a powerful and widespread technique, with the single-beam gradient trap (also known as optical tweezers) in use for a large number of biological and other applications. The forces and torques acting on a trapped particle result from the transfer of momentum and angular momentum from the trapping beam to the particle. Despite the apparent simplicity of a laser trap, with a single particle in a single beam, exact calculation of the optical forces and torques acting on particles is difficult. Calculations can be…
While various nanophotonic structures applicable to relatively thin crystalline silicon-based solar cells were proposed to ensure effective light in-coupling and light trapping in the absorber, it is of great importance to evaluate their performance on the solar module level under realistic irradiation conditions. Here, we analyze the annual energy yield of relatively thin heterojunction (HJT) solar module architectures when optimized anti-reflective and light trapping titanium dioxide (TiO$_2$) nanodisk square arrays are applied on the front and rear cell interfaces. Our numerical study shows…
Vector spherical wavefunctions were derived in closed-form to represent time-harmonic electromagnetic fields in an orthorhombic dielectric-magnetic material with gyrotropic-like magnetoelectric properties. These wavefunctions were used to formulate the T matrix for scattering by a three-dimensional object composed of the chosen material. Furthermore, a closed-form, coordinate-free expression of the dyadic Green function for the chosen material was derived. Expressions ascertained for the singularity behavior will be useful for formulating volume integral equations for scattering inside the cho…
High-refractive index dielectric nanoparticles may exhibit strong directional forward light scattering at visible and near-infrared wavelengths due to interference of simultaneously excited electric and magnetic dipole resonances. For a spherical high-index dielectric, the so-called first Kerker's condition can be realized, at which the backward scattering practically vanishes for some combination of refractive index and particle size. However, Kerker's condition for spherical particles is only possible at the tail of the scattering resonances, when the particle scatters light weakly. Here we …
A technique to levitate and measure the three-dimensional position of micrometer-sized dielectric spheres with heterodyne detection is presented. The two radial degrees of freedom are measured by interfering light transmitted through the microsphere with a reference wavefront, while the axial degree of freedom is measured from the phase of the light reflected from the surface of the microsphere. This method pairs the simplicity and accessibility of single beam optical traps to a measurement of displacement that is intrinsically calibrated by the wavelength of the trapping light and has excepti…
We discuss the statistical properties of lifetimes of electromagnetic eigenmodes in dielectric microresonators with fully chaotic ray dynamics. Using the example of a resonator of stadium geometry, we find that a recently proposed random-matrix model very well describes the lifetime statistics of long-lived resonances, provided that two effective parameters are appropriately renormalized. This renormalization is linked to the formation of anomalously short-lived resonances, a mechanism also known from the fractal Weyl law and the resonance trapping phenomenon.
Nonmagnetic and spherically symmetric dielectric material media are investigated in their generality as analogue models, in the domains of geometrical optics, for a few relevant static and spherically symmetric solutions of gravitation, including black holes and wormholes. Typic and desirable gravitational features are systematically linked to the nonlinear properties of the phenomenological dielectric permittivity of the medium. From this, the limitations of such analogies are explored in terms of their corresponding geometric flexibility, dielectric configurations and causal structure.
Two point charges are placed in a spherical dielectric core-shell embedded in a dielectric environment, one of the charges being located in the core and the other in the shell. The core, shell, and environment are characterized by different dielectric constants. Analytical solutions for the electrostatic energy of the system and the polarization charge density at the core-shell and shell-environment interfaces are obtained by a classical approach.
A simple yet effective achiral platform using elliptical nanoholes for chiroptical analysis is demonstrated. Under linearly polarized excitation, an elliptical nanohole in a thin gold film can generate a localized chiral optical field for chiroptical analysis and simultaneously serve as a near-field optical trap to capture dielectric and plasmonic nanospheres. In particular, the trapping potential is enantioselective for dielectric nanospheres, i.e., the hole traps or repels the dielectric nanoparticles depending on the sample chirality. For plasmonic nanospheres, the trapping potential well i…
We fabricate a miniature spherical mirror for tightly focusing an optical dipole trap for neutral atoms. The mirror formation process is modelled to predict the dimensions for particular fabrication parameters. We integrate the spherical mirror with a neutral atom experiment to trap and detect a single atom with high efficiency. The mirror serves the dual purpose of focusing the dipole trap as well as collection of the atomic fluorescence into an optical fibre.
Low-dimensional ordered arrays of optical elements can possess bound modes having an extremely high quality factor. Typically, these arrays consist of metal elements which have significantly high light absorption thus restricting performance. In this paper we address the following question: can bound modes be formed in dielectric systems where the absorption of light is negligible? Our investigation of circular arrays of spherical particles shows that (1) high quality modes in an array of 10 or more particles can be attained at least for a refractive index $n_{r}>2$, so optical materials like …
Optical trapping can be used to manipulate the three-dimensional (3-D) motion of spherical particles based on the simple prediction of optical forces and the responding motion of samples. However, controlling the 3-D behaviour of non-spherical particles with arbitrary orientations is extremely challenging, due to experimental difficulties and the extensive computations. Here, we achieved the real-time optical control of arbitrarily shaped particles by combining the wavefront shaping of a trapping beam and measurements of the 3-D refractive index (RI) distribution of samples. Engineering the 3-…
The superposition of a Gaussian mode and a Laguerre-Gauss mode with $\ell=0,p\neq0$ generates the so-called bottle beam: a dark focus surrounded by a bright region. In this paper, we theoretically explore the use of bottle beams as an optical trap for dielectric spheres with a refractive index smaller than that of their surrounding medium. The forces acting on a small particle are derived within the dipole approximation and used to simulate the Brownian motion of the particle in the trap. The intermediate regime of particle size is studied numerically and it is found that stable trapping of la…
Dynamic control of compact chip-scale contactless manipulation of particles for bioscience applications remains a challenging endeavor, which is restrained by the balance between trapping efficiency and scalable apparatus. Metasurfaces offer the implementation of feasible optical tweezers on a planar platform for shaping the exerted optical force by a microscale-integrated device. Here, we design and experimentally demonstrate a highly efficient silicon-based metalens for two-dimensional optical trapping in the near-infrared. Our metalens concept is based on the Pancharatnam-Berry phase, which…
Small form-factor, narrowband, and highly directive antennas are of critical importance in a variety of applications spanning wireless communications, remote sensing, Raman spectroscopy, and single photon emission enhancement. Surprisingly, we show that the classical directivity limit can be appreciably surpassed for electrically small multilayer spherical antennas excited by a point electric dipole even if limiting ourselves to purely dielectric materials. Experimentally feasible designs of superdirective antennas are established by using a stochastic optimization algorithm combined with a ri…
We study a range of radio-frequency ion trap geometries and investigate the effect of integrating dielectric cavity mirrors on their trapping potential. We aim to identify ion trap and cavity configurations that are best suited for achieving small cavity volumes and thus large ion-photon coupling as required for scalable quantum information networks. In particular, we investigate the trapping potential distortions caused by the dielectric material of the cavity mirrors for different mirror orientations with respect to the trapping electrodes, as well as for mirror misalignment. We also analyze…
It was theoretically proposed and experimentally demonstrated that anti-reflection coating allows one to trap a high dielectric sphere, at the same time enhancing the transverse optical force. Here, by explicitly calculating the gradient force and the scattering force, we rigorously show that these were mainly consequences of the reduction in scattering force due to the suppression of backward scattering, and enhancement in gradient force due to the increased in overall particle size. The reduction of scattering force can be understood within a ray optics theory and also the Mie theory. The co…
We reveal peculiarities of the trapped (dark) mode excitation in a polarization-insensitive all-dielectric metasurface, whose unit super-cell is constructed by particularly arranging four cylindrical dielectric particles. Involving group-theoretical description we discuss in detail the effect of different orientations of particles within the super-cell on characteristics of the trapped mode. The theoretical predictions are confirmed by numerical simulations and experimental investigations. Since the metasurface is realized from simple dielectric particles without the use of any metallic compon…
Developing angular trapping methods, which will enable optical tweezers to rotate a micronized bead, is of great importance for the studies of biomacromolecules during a wide range of torque-generation processes. Here we report a novel controlled angular trapping method based on composite Janus particles. We used a chemically synthesized Janus particle, which consists of two hemispheres made of polystyrene (PS) and poly(methyl methacrylate) (PMMA) respectively, as a model system to demonstrate this method. Through computational and experimental studies, we demonstrated the feasibility to contr…
We have studied the effective response of composites of spherical particles with a dielectric profile which varies along the radius of the particles. We developed a differential effective dipole theory to compute the dipole moment of individual spherical particle and hence the effective dielectric response of a dilute suspension. The theory has been applied to two model dielectric profiles. Moreover, we compare the approximate results with the exact results of the power-law profile and the agreement is excellent.
We investigate the dynamic evolution of the radiation forces produced by the pulsed Gaussian beams acting on a Rayleigh dielectric sphere. We derive the analytical expressions for the scattering force and all components of the ponderomotive force induced by the pulsed Gaussian beams. Our analysis shows that the radiation force, for both the transverse and longitudinal components, can be greatly enhanced as the pulse duration decreases. It is further found that for the pulse with long pulse duration, it can be used for the stable trapping and manipulating the particle, while for the pulse with …
The interference of polariton guiding modes propagating through "traffic circle" waveguides composed of dielectric spherical particles is investigated. The dependence of intensity of the wave on the position of the particle was studied using the multisphere the Mie scattering formalism. We show that if the frequency of light belongs to the passband of the waveguide, electromagnetic waves may be considered as two optical beams running along a circle in opposite directions and interfering with each other. Indeed, the obtained intensity behavior can be represented as a simple superposition of two…
We report the development of quantum microscopic theory of quasi-resonant dipole-dipole interaction in the ensembles of impurity atoms imbedded into transparent dielectric and located into Fabry-Perot cavity. On the basis of the general approach we study the simultaneous influence of the cavity and resonant dipole-dipole interaction on the shape of the line of atomic transition as well as on light trapping in dense impurity ensembles. We analyze this influence depending on the size of the ensemble, its density, as well as on r.m.s. deviation of the transition frequency shifts caused by the sym…
We show that dielectric spheres can be cloaked by a shell of amorphously arranged metallic nanoparticles. The shell represents an artificial medium with tunable effective properties that can be adjusted such that the scattered signals of shell and sphere almost cancel each other. We provide an analytical model for the cloak design and prove numerically that the cloak operates as desired. We show that more than 70% of the scattered signal of the sphere can be suppressed at the design wavelength. Advantages and disadvantages of such a cloak when compared to other implementations are disclosed.
The momentum- and frequency-dependent T-matrix operator for the scattering of electromagnetic waves by a dielectric/conducting and para- or diamagnetic sphere is derived as a Mie-type series, and presented in a compact form emphasizing various symmetry properties, notably the unitarity identity. This result extends to magnetic properties one previously obtained for purely dielectric contrasts by other authors. Several situations useful to spatially-dispersive effective-medium approximations to one-body order are examined. Partial summation of the Mie series is achieved in the case of elastic s…
We review recent works on optomechanics of optically trapped microspheres and nanoparticles in vacuum, which provide an ideal system for studying macroscopic quantum mechanics and ultrasensitive force detection. An optically trapped particle in vacuum has an ultrahigh mechanical quality factor as it is well-isolated from the thermal environment. Its oscillation frequency can be tuned in real time by changing the power of the trapping laser. Furthermore, an optically trapped particle in vacuum may rotate freely, a unique property that does not exist in clamped mechanical oscillators. In this re…
Dielectric spheres of various sizes may sustain electromagnetic whispering-gallery modes resonating at optical frequencies with very narrow linewidths. Arbitrary small deviations from the spherical shape typically shift and broaden such resonances. Our goal is to determine these shifted and broadened resonances. A boundary-condition perturbation theory for the acoustic vibrations of nearly circular membranes was developed by Rayleigh more than a century ago. We extend this theory to describe the electromagnetic excitations of nearly spherical dielectric cavities. This approach permits us to av…
For homogenous isotropic dielectric nanospheres with incident plane waves, Cartesian electric and toroidal dipoles can be tunned to cancel each other in terms of far-field scattering, leading to the effective anopole excitation. At the same time however, other multipoles such as magnetic dipoles with comparable scattered power are simultanesouly excited, mixing with the anopole and leading to a non-negligible total scattering cross section. Here we show that for homogenous dielectric nanospheres, radial anisotropy can be employed to significantly suppress the other multipole excitation, which …
Experimental observations suggest that there are differences between the behavior of particles optically trapped in air and trapped in a liquid phase. We present a modified version of Mie Debye Spherical Aberration theory to numerically simulate such optical system in attempt to explain and predict these effects. The model incorporates Mie scattering and focussing of the trapping beam through media of stratified refractive index. Our results show a geometrical optics approach cannot correctly describe our system and that spherical aberration must be included. We successfully qualitatively expl…
Tailored multipolar optical trapping with higher-order structured light
The Institute of Optics, University of Rochester（罗切斯特大学光学研究所）；Department of Physics, University of Rochester（罗切斯特大学物理系）；Center for Coherence and Quantum Optics, University of Rochester（罗切斯特大学相干与量子光学中心）
A new strategy for trapping quantum particles is presented, which behaves like an effective harmonic oscillator potential trap wherever is desired. The approach is based on harmonic contraction and expansion of the system around a fixed point (trapping point) at high frequencies. Analytical results are presented for an arbitrary potential and contrasted with numerical calculations for a quantum particle between two impenetrable walls. Similarly, making use of the analogy between quantum mechanics and optics, it is shown that an harmonically breathing waveguide lattice can be used to trap optic…
Optical trapping and manipulation using laser beams play a key role in many areas including biology, atomic science, and nanofabrication. Here, we propose and experimentally demonstrate the first use of a vortex-pair beam in optical trapping and manipulation. We successfully trap two spherical microparticles simultaneously by a single vortex-pair beam. Precisely position-controllable manipulation of the trapped spherical microparticles is realized by adjusting the off-axis distance of the vortices on the initial phase plane of the vortex-pair beam. Based on the feature of the vortex-pair beam,…
High-index spherical nanoparticles with low material losses support sharp high-Q electric and magnetic resonances and exhibit a number of interesting optical phenomena. Developments in fabrication techniques have enabled the further study of their properties and the investigation of related optical effects. After deposition on a substrate, the optical properties of a particle change dramatically due to mutual interaction. Here, we consider a silicon spherical nanoparticle on a dielectric one-layered substrate. At the normal incidence of light, the layer thickness controls the contribution of t…
Light forces induced by scattering and absorption in elastic dielectrics lead to local density modulations and deformations. These perturbations in turn modify light propagation in the medium and generate an intricate nonlinear response. We generalise an analytic approach where light propagation in one-dimensional media of inhomogeneous density is modelled as a result of multiple scattering between polarizable slices. Using the Maxwell stress tensor formalism we compute the local optical forces and iteratively approach self-consistent density distributions where the elastic back-action balance…
Multipolar plasmon oscillation frequencies and corresponding damping rates for nanospheres formed of the simplest free-electron metals are studied. The possibility of controlling plasmon features by choosing the size and dielectric properties of the sphere surroundings is discussed. Optical properties of the studied metals are described within the Drude-Sommerfeld model of the dielectric function with effective parameters acounting for the contribution of conduction electrons and of interband transitions. No approximation is made in respect of the size of a particle; plasmon size characteristi…
Light injected into a spherical dielectric body may be confined very efficiently via the mechanism of total internal reflection. The frequencies that are most confined are called resonances. If the shape of the body deviates from the perfect spherical form the resonances change accordingly. In this thesis, a perturbation theory for the optical resonances of such a deformed sphere is developed. The optical resonances of such an open system are characterized by complex eigenvalues, where the real part relates to the frequency of the resonant light and the imaginary part to the energy leakage out…
