Viscous fingering of a miscible high viscosity slice of fluid displaced by a lower viscosity fluid is studied in porous media by direct numerical simulations of Darcy's law coupled to the evolution equation for the concentration of a solute controlling the viscosity of miscible solutions. In contrast with fingering between two semi-infinite regions, fingering of finite slices is a transient phenomenon due to the decrease in time of the viscosity ratio across the interface induced by fingering and dispersion processes. We show that fingering contributes transiently to the broadening of the peak in time by increasing its variance. A quantitative analysis of the asymptotic contribution of fingering to this variance is conducted as a function of the four relevant parameters of the problem i.e. the log-mobility ratio R, the length of the slice l, the Peclet number Pe and the ratio between transverse and axial dispersion coefficients $ε$. Relevance of the results is discussed in relation with transport of viscous samples in chromatographic columns and propagation of contaminants in porous media.
A rest fluid displaced by a less viscous fluid in a porous medium triggers the so-called Saffman-Taylor instability at their contact front and hence forms complicated finger-like patterns. When the two fluids are miscible, the surface tension at their contact front vanishes, leaving the variation in viscosity dominant the contribution to the instability. The phenomena, named viscous fingering, can be studied by the analogy of a single-phase flow in the Hele-Shaw cell, a quasi-two-dimensional rectilinear plane. Viscous fingering produces complex geometrical patterns. They are important not only…
We investigate the stability of radial viscous fingering (VF) in miscible fluids. We show that the instability is decided by an interplay between advection and diffusion during initial stages of flow. Using linear stability analysis and nonlinear simulations, we demonstrate that this competition is a function of the radius $r_0$ of the circular region initially occupied by the less viscous fluid in the porous medium. For each $r_0$, we further determine the stability in terms of Péclet number ($Pe$) and log-mobility ratio ($M$). The $Pe-M$ parameter space is divided into stable and unstable zo…
The results from a series of well characterised, unstable, miscible displacement experiments in a Hele Shaw cell with a quarter five-spot source-sink geometry are presented, with comparisons to detailed numerical simulation. We perform repeated experiments at adverse viscosity ratios from 1 - 20 and Peclet numbers from 10$^4$ - 10$^6$ capturing the transition from 2D to 3D radial fingering and experimental uncertainty. The open-access dataset provides time-lapse images of the fingering patterns, transient effluent profiles, and meta-information for use in model validation. We find the complexi…
We perform linear stability analyses (LSA) and direct numerical simulations (DNS) to investigate the influence of the dynamic viscosity on viscous fingering (VF) instability in miscible slices. Selecting the characteristic scales appropriately the importance of the magnitude of the dynamic viscosity of individual fluids on VF in miscible slice has been shown in the context of the transient interfacial tension. Further, we have confirmed this result for immiscible fluids and manifest the similarities between VF in immiscible and miscible slices with transient interfacial tension. In a more gene…
The non-modal linear stability of miscible viscous fingering in a two dimensional homogeneous porous medium has been investigated. The linearized perturbed equations for Darcy's law coupled with a convection-diffusion equation is discretized using finite difference method. The resultant initial value problem is solved by fourth order Runge-Kutta method, followed by a singular value decomposition of the propagator matrix. Particular attention is given to the transient behavior rather than the long-time behavior of eigenmodes predicted by the traditional modal analysis. The transient behaviors o…
We study miscible Rayleigh-Taylor (RT) fingering instability in two-dimensional homogeneous porous media, in which the fluid density varies non-monotonically as a function of the solute concentration such that the maximum density lies in the interior of the domain, thus creating a stable and an unstable density gradients that evolve in time. With the help of linear stability analysis (LSA) as well as nonlinear simulations the effects of density gradients on the stability of RT fingers are investigated. As diffusion relaxes the concentration gradient, a non-monotonic density profile emerges in …
A non-modal linear stability analysis (NMA) of the miscible viscous fingering in a porous medium is studied for a toy model of non-monotonic viscosity variation. The onset of instability and its physical mechanism are captured in terms of the singular values of the propagator matrix corresponding to the non-autonomous linear equations. We discuss two types of non-monotonic viscosity profiles, namely, with unfavorable (when a less viscous fluid displaces a high viscous fluid) and with favorable (when a more viscous fluid displaces a less viscous fluid) end-point viscosities. A linear stability …
The effect of a linear adsorption isotherm on the onset of fingering instability in a miscible displacement in the application of liquid chromatography, pollutant contamination in aquifers etc. is investigated. Such fingering instability on the solute dynamics arise due to the miscible viscus fingering (VF) between the displacing fluid and sample solvent. We use a Fourier pseudo-spectral method to solve the initial value problem appeared in the linear stability analysis. The present linear stability analysis is of generic type and it captures the early time diffusion dominated region which was…
Viscous fingering patterns can form at the interface between two immiscible fluids confined in the gap between a pair of flat plates; whenever the fluid with lower viscosity displaces the one of higher viscosity the interface is unstable. For miscible fluids the situation is more complicated due to the formation of interfacial structure in the thin dimension spanning the gap. Here we study the effect of the inherent diffusion between the two miscible fluids on this structure and on the viscous fingering patterns that emerge. We discover an unexpected transition separating two distinct regimes …
Viscous and gravitational fingering refer to flow instabilities in porous media that are triggered by adverse mobility or density ratios, respectively. These instabilities have been studied extensively in the past for 1) single-phase flow (e.g., contaminant transport in groundwater, first-contact-miscible displacement of oil by gas in hydrocarbon production), and 2) multi-phase immiscible and incompressible flow (e.g., water-alternating-gas (WAG) injection in oil reservoirs). Fingering in multiphase compositional and compressible flow has received much less attention, perhaps due to its high c…
Viscous fingering is a well-known hydrodynamic instability that sets in when a less viscous fluid displaces a more viscous fluid. When the two fluids are miscible, viscous fingering introduces disorder in the velocity field and exerts a fundamental control on the rate at which the fluids mix. We present a fluid dynamics video of the mixing process in a viscously unstable flow, generated from a high-resolution numerical simulation using a computational strategy that is stable for arbitrary viscosity ratios. We develop a two-equation dynamic model of concentration variance and mean dissipation r…
Viscous fingering patterns form in confined geometries at the interface between two fluids as the lower-viscosity fluid displaces the one with higher viscosity. Previous studies have examined the most unstable wavelength of the patterns that form using both linear-stability analysis and the dynamics of finger growth in the nonlinear regime. Interesting differences in dynamics have been seen between rectilinear and radial geometries as well as between fluid pairs that are immiscible (with interfacial tension) or miscible (with negligible interfacial tension). This paper reports measurements of …
The hydrodynamic viscous fingering instability can be influenced by a simple viscosity changing chemical reaction of type A+B --> C, when a solution of reactant A is injected into a solution of B and a product C of different viscosity is formed. We investigate here numerically such reactive viscous fingering in the case of a reaction decreasing the viscosity to define the optimal conditions on the chemical and hydrodynamic parameters for controlling fingering. In particular, we analyze the influence of the injection flow rate or equivalently of the Peclet number (Pe) of the problem on the effi…
The invasion of one fluid into another of higher viscosity in a quasi-two dimensional geometry typically produces complex fingering patterns. Because interfacial tension suppresses short-wavelength fluctuations, its elimination by using pairs of miscible fluids would suggest an instability producing highly ramified singular structures. Previous studies focused on wavelength selection at the instability onset and overlooked the striking features appearing more globally. Here we investigate the non-linear growth that occurs after the instability has been fully established. We find a rich variety…
The dynamics of $A + B \rightarrow C$ fronts is analyzed numerically in a radial geometry. We are interested to understand miscible fingering instabilities when the simple chemical reaction changes the viscosity of the fluid locally and a non-monotonic viscosity profile with a global maximum or minimum is formed. We consider viscosity-matched reactants $A$ and $B$ generating a product $C$ having different viscosity than the reactants. Depending on the effect of $C$ on the viscosity relative to the reactants, different viscous fingering (VF) patterns are captured which are in good qualitative a…
We examine the transport in a homogeneous porous medium of a finite slice of a solute which adsorbs on the porous matrix following a Langmuir adsorption isotherm and can influence the dynamic viscosity of the solution. In the absence of any viscosity variation, the Langmuir adsorption induces the formation of a shock layer wave at the frontal interface and of a rarefaction wave at the rear interface of the sample. For a finite width sample, these waves interact after a given time that varies nonlinearly with the adsorption properties to give a triangle-like concentration profile in which the m…
We present a theoretical study on pattern formation occurring in miscible fluids reacting by a second-order reaction $A + B \to S$ in a vertical Hele-Shaw cell under constant gravity. We have recently reported that concentration-dependent diffusion of species coupled with a frontal neutralization reaction can produce a multi-layer system where low density depleted zones could be embedded between the denser layers. This leads to the excitation of chemoconvective modes spatially separated from each other by a motionless fluid. In this paper, we show that the layers can interact via a diffusion m…
