My previous calculations of the Lamb shift in muonic hydrogen are reviewed and compared with other work. In addition, numerical results for muonic deuterium are presented.
The deuteron charge radius is calculated from the measurement of the Lamb shift in muonic deuterium, taking into account the electron vacuum polarization correction to the nuclear-structure effects. This correction is unexpectedly large and gives a mean-square charge-radii difference $ r_d^2-r_p^2 = 3.81747(346)\, {\rm fm}^2 $, which is now consistent with that obtained from the ordinary H-D isotope shift in the 1$S$-2$S$ transition. This suggests that the long-standing discrepancy in the proton charge radius obtained from electronic and muonic systems is due to an underestimated uncertainty i…
Radiative deexcitation (RD) of the metastable 2S state of muonic protium and deuterium atoms has been observed. In muonic protium, we improve the precision on lifetime and population (formation probability) values for the short-lived μp(2S) component, and give an upper limit for RD of long-lived μp(2S) atoms. In muonic deuterium at 1 hPa, 3.1 +-0.3 % of all stopped muons form μd(2S) atoms. The short-lived 2S component has a population of 1.35 +0.57 -0.33 % and a lifetime of τ_short(μd) = 138 +32 -34 ns. We see evidence for RD of long-lived μd(2S) with a lifetime of τ_long(μd) = 1.15 +0.75 -0.5…
The reduced-mass dependence of relativistic and radiative effects in simple muonic bound systems is investigated. The spin-dependent nuclear recoil correction of order (Zalpha)^4 mu^3/m_N^2 is evaluated for muonic hydrogen and deuterium, and muonic helium ions (mu is the reduced mass and m_N is the nuclear mass). Relativistic corrections to vacuum polarization of order alpha (Zalpha)^4 mu are calculated, with a full account of the reduced-mass dependence. The results shift theoretical predictions. The radiative-recoil correction to vacuum polarization of order alpha (Zα)^5 ln^2(Zalpha) mu^2/m_…
Quantum interference between energetically close states is theoretically investigated, with the state structure being observed via laser spectroscopy. In this work, we focus on hyperfine states of selected hydrogenic muonic isotopes, and on how quantum interference affects the measured Lamb shift. The process of photon excitation and subsequent photon decay is implemented within the framework of nonrelativistic second-order perturbation theory. Due to its experimental interest, calculations are performed for muonic hydrogen, deuterium, and helium-3. We restrict our analysis to the case of phot…
Nuclear structure corrections of orders $Zα\, E_F$ and $(Zα)^2 E_F$ are calculated for the hyperfine splitting of the muonic deuterium. The obtained results disagree with previous calculations and lead to a $5\,σ$ disagreement with the current experimental value of the $2S$ hyperfine splitting in $μ$D.
The non-resonant formation of $ddμ$ molecules in the loosely bound state in collisions of non-thermalized $dμ$ atoms with deuterium molecules D$_2$ has been considered. The process of such a type is possible only for collision energies exceeded the ionization potential of D$_2$. The calculated rates of $ddμ$ formation in the above-threshold energy region are about one order of magnitude higher than obtained earlier. The role of epithermal non-resonant $μ$-molecule formation for the kinetics of $μ$CF processes in D$_2$ gas was studied. It was shown that the non-resonant $ddμ$ formation by $dμ$ …
The muonic hydrogen experiment measuring the $2P-2S$ transition energy [R. Pohl {\em et al.}, Nature {\bf 466}, 213 (2010)] is significantly discrepant with theoretical predictions based on quantum electrodynamics. A possible approach to resolve this conundrum is to compare experimental values with theoretical predictions in another system, muonic deuterium $μ$D. The only correction which might be questioned in $μ$D is that due to the deuteron polarizability. We investigate this effect in detail and observe cancellation with the elastic contribution. The total value obtained for the deuteron s…
The Lamb shift in muonic hydrogen continues to be a subject of experimental and theoretical investigation. Here my older work on the subject is updated to provide a complementary calculation of the energies of the 2p-2s transitions in muonic hydrogen.
The present knowledge of Lamb shift, fine- and hyperfine structure of the $\mathrm{2S}$ and $\mathrm{2P}$ states in muonic deuterium is reviewed in anticipation of the results of a first measurement of several $\mathrm{2S-2P}$ transition frequencies in muonic deuterium ($μ\mathrm{d}$). A term-by-term comparison of all available sources reveals reliable values and uncertainties of the QED and nuclear structure-dependent contributions to the Lamb shift, which are essential for a determination of the deuteron rms charge radius from $μ\mathrm{d}$. Apparent discrepancies between different sources a…
Contributions to the energy levels in light muonic atoms and, in particular, to the Lamb shift fall into a few well-distinguished classes. The related diagrams are calculated using different approaches. In particular, there is a specific kind of non-relativistic contributions. Here we consider such corrections to the Lamb shift in order $α^5m_μ$. These contributions are due to free vacuum polarization loops as well as to various effects of light-by-light scattering. The closed loop in the related diagrams is an electronic one, which allows a non-relativistic consideration of the muon. Both kin…
We calculate the longitudinal structure function of the deuteron up through next-to-next-to-leading order in the framework of pionless effective field theory. We use these results to compute the two-photon polarizability contribution to Lamb shift in muonic deuterium, which can be utilized to extract the nuclear charge radius of the deuteron. We present analytical expressions order-by-order for the relevant transition matrix elements and the longitudinal structure function, and we give numerical results for the corresponding contributions to the Lamb shift. We also discuss the impact of relati…
Corrections to energy levels in light muonic atoms are investigated in order $α^2(Zα)^4m$. We pay attention to corrections which are specific for muonic atoms and include the electron vacuum polarization loop. In particular, we calculate relativistic and relativistic-recoil two-loop electron vacuum polarization contributions. The results are obtained for the levels with $n=1,2$ and in particular for the Lamb shift ($2p_{1/2}-2s_{1/2}$) and fine-structure intervals ($2p_{3/2}-2p_{1/2}$) in muonic hydrogen, deuterium, and muonic helium ions.
In connection with recent and proposed experiments, and new theoretical results, my previous calculations of the Lamb shift in muonic hydrogen will be reviewed and compared with other work. In addition, numerical results for muonic deuterium and helium will be presented. Some previously neglected (but very small) effects are included.
In the comment we discuss an additional term to the $α^3$ correction to the Lamb shift, which was missed in the calculation by Kinoshita and Nio (Phys. Rev. Lett. 82, 3240 (1999)).
The 7 standard deviations between the proton rms charge radius from muonic hydrogen and the CODATA-10 value from hydrogen spectroscopy and electron-scattering has caused considerable discussions. Here, we review the theory of the 2S-2P Lamb shift and 2S hyperfine splitting in muonic hydrogen combining the published contributions and theoretical approaches. The prediction of these quantities is necessary for the determination of both proton charge and Zemach radii from the two 2S-2P transition frequencies measured in muonic hydrogen.
The largest contributions to the $n=2$ Lamb-shift, fine structure interval and $2s$ hyperfine structure of muonic hydrogen are calculated by exact numerical evaluations of the Dirac equation, rather than by a perturbation expansion in powers of $1/c$, in the framework of non-relativistic quantum electrodynamics. Previous calculations and the validity of the perturbation expansion for light elements are confirmed. The dependence of the various effects on the nuclear size and model are studied
The formation and various disintegration modes of $2s$ states for muonic hydrogen and deuterium atoms at kinetic energies both above and below the $2s-2p$ threshold are studied. The cross sections of the collision-induced radiative quenching, elastic scattering, and Coulomb deexcitation of $(μ^- p)_{2s}$ and $(μ^- d)_{2s}$ atoms in collisions with ordinary hydrogen and deuterium atoms at collision energies below the $2s-2p$ threshold are calculated in the framework of the close-coupling approach. The basis set includes all open and closed channels corresponding to exotic-atom states with princ…
In muonic atoms the Uehling potential (an effect of a free electronic vacuum polarization loop) is responsible for the leading contribution to the Lamb shift causing the splitting of states with Delta n = 0 and Delta l \neq 0. Here we consider the Lamb shift in the leading nonrelativistic approximation, i.e., within an approach based on a certain Schrodinger equation. That is valid for low and medium $Z$ as long as (Z alpha)^2 >> 1. The result is a function of a few parameters, including kappa = Z alpha m_ mu/m_e, n and l. We present various asymptotics and in particular we study a region of v…
A recent letter [1] investigated the effects of deuteron polarizability in the mu D atom. The importance of understanding this atom has been heightened because of the possible light it could shed on the proton radius puzzle. Here we confirm, clarify, and emphasize the significance of the result [1] that the effects of the third Zemach moment are canceled by part of the deuteron polarizability effects. 1. K. Pachucki, Phys. Rev. Lett. 106, 193007 (2011)
The ground bound states in the five-body muonic ions $a b μe_2$ (or $(a b μe_2)^{-}$), where $(a, b) = (p, d, t)$, are considered for the first time. As follows from accurate numerical computations of these five-body ions they are similar to the negatively charged hydrogen ion H$^{-}$ with a three-particle central quasi-nucleus $a b μ$ (or $(a b μ)^{+}$). These five-body ions play some role in the muon-catalyzed fusion of nuclear reaction in liquid deuterium and/or deuterium-tritium mixtures. We also discuss the bound states in the six-body $a b c μe_2$ quasi-molecules, where $(a, b, c) = (p, …
We provide a systematic assessment of the order-$α^5$ nuclear contributions to the Lamb shift of muonic deuterium, including the accompanying radiative corrections due to vacuum polarization, up to next-to-next-to-next-to-leading order (N3LO) within the pionless effective field theory (EFT). We also evaluate higher-order corrections due to the single-nucleon structure, which are expected to be the most important corrections beyond N3LO. We find a correlation between the deuteron charge and Friar radii, which can be useful to judge the quality of charge form factor parametrisations. We refine t…
From the comparison between the experimental and theoretical results for the energy difference between 2s1/2 and 2p1/2 states in hydrogen and hydrogen-like ions with different values of Z, we estimate bounds for the presence of an extra fractional dimension. These bounds are higher when we work with muonic hydrogen and muonic deuterium, which open the possibility that future measurements of the Lamb shift in muonic atoms with one electron and higher values of Z may show evidence of the extra dimension.
Non-relativisitic second-order corrections to the wave function at origin in muonic and exotic atoms are considered. The corrections are due to the electronic vacuum polarization. Such corrections are of interest due to various effective approaches, which take into account QED and hadronic effects. The wave function at origin plays a key role in the calculation of the pionium lifetime, various finite nuclear size effects and the hyperfine splitting. The results are obtained for the $1s$ and $2s$ states in pionic and muonic hydrogen and deuterium and in pionium, a bound system of $π^+$ and $π^-…
The proton structure effects, including finite size, polarizability and self-energy is considered and their influence on energy levels of muonic hydrogen is recalculated. A new theoretical prediction for the Lamb shift is presented together with improved values of all known QED contributions.
We provide an up to date summary of the theory contributions to the 2S-2P Lamb shift and the fine structure of the 2P state in the muonic helium ion $(\mathrm{μ^4He})^+$. This summary serves as the basis for the extraction of the alpha particle charge radius from the muonic helium Lamb shift measurements at the Paul Scherrer Institute, Switzerland. Individual theory contributions needed for a charge radius extraction are compared and compiled into a consistent summary. The influence of the alpha particle charge distribution on the elastic two-photon exchange is studied to take into account pos…
Recently the muonic hydrogen lamb shift has been measured with unprecedented accuracy, allowing for a precise determination of the proton radius. This determination is 5 sigma away from the previous CODATA value obtained from (mainly) the hydrogen lamb shift and the electron-proton scattering. Within an effective field theory formalism, I will define the proton radius and briefly review some aspects of the theoretical prediction for the muonic hydrogen lamb shift, studying both the pure QED-like computation and the hadronic effects.
The diffusion radius of the 1S muonic hydrogen atoms in gaseous H_2 targets with various deuterium admixtures has been determined for temperatures T=30 and 300 K. The Monte Carlo calculations have been performed using the partial differential crosssections for $pμ$ and $dμ$ atom scattering from the molecules H$_2$, HD and D$_2$. These cross sections include hyperfine transitions in the muonic atoms, the muon exchange between the nuclei $p$ and $d$, and rotational-vibrational transitions in the target molecules. The Monte Carlo results have been used for preparing the time-projection chamber fo…
We consider one-loop light-by-light-scattering contributions to the Lamb shift of the $1s, 2s, 2p$ states in light muonic hydrogen like atoms at $Z\leq10$. The contributions are of the order $α^5m_μ$ (with diverse dependence on the nuclear charge $Z$). Those include the contributions of the so-called Wichmann-Kroll potential ($α(Zα)^4m_μ$), the virtual Delbrück scattering ($α^2(Zα)^3m_μ$), etc. The results are obtained in a nonrelativistic approximation. For the calculation of the virtual-Delbrück-scattering contribution, we have constructed an effective potential in the coordinate space which…
Recently a high-precision measurement of the Lamb shift in muonic hydrogen has been performed. An accurate value of the proton charge radius can be extracted from this datum with a high accuracy. To do that a sufficient accuracy should be achieved also on the theoretical side, including an appropriate treatment of higher-order proton-structure effects. Here we consider a higher-order contribution of the finite size of the proton to the Lamb shift in muonic hydrogen. Only model-dependent results for this correction have been known up to date. Meantime, the involved models are not consistent eit…
The relativistic recoil contributions to the Uehling corrections are revisited. We consider a controversy in recent calculations based on different approaches including Breit-type and Grotch-type calculations. We have found that calculations of those authors were in fact done in different gauges and in some of those gauges contributions the retardation and two-photon-exchange effects were missed. We have evaluated such effects and obtained a consistent result from those approaches. We present a correct expression for the Grotch-type approach which produces a correct gauge-invariant result. We …
The Lamb shift in muonic hydrogen was measured some time ago to a high accuracy. The theoretical prediction of this value is very sensitive to the proton-finite-size effects. The proton radius extracted from muonic hydrogen is in contradiction with the results extracted from elastic electron-proton scattering. That creates a certain problem for the interpretation of the results from the muonic hydrogen Lamb shift. For the latter we need also to take into account the two-photon-exchange contribution with the proton finite size involved. The only way to describe it relies on the data from the sc…
Weak interaction contributions to hyperfine splitting and Lamb shift in light electronic and muonic atoms are calculated. We notice that correction to hyperfine splitting turns into zero for deuterium. Weak correction to the Lamb shift in hydrogen is additionally suppressed in comparison with other cases by a small factor $(1-4\sin^2θ_W)$.
We present a precise calculation of the Lamb shift $(2P_{1/2}-2S_{1/2})$ in muonic ions $(μ^6_3Li)^{2+},~(μ^7_3Li)^{2+}$, $(μ^9_4Be)^{3+},~(μ^{10}_4Be)^{3+}$, $(μ^{10}_5B)^{4+},~(μ^{11}_5B)^{4+}$. The contributions of orders $α^3\divα^6$ to the vacuum polarization, nuclear structure and recoil, relativistic effects are taken into account. Our numerical results are consistent with previous calculations and improve them due to account of new corrections. The obtained results can be used for the comparison with future experimental data, and extraction more accurate values of nuclear charge radii.
On the basis of quasipotential method in quantum electrodynamics we calculate nuclear finite size radiative corrections of order $α(Z α)^5$ to the Lamb shift in muonic hydrogen and helium. To construct the interaction potential of particles, which gives the necessary contributions to the energy spectrum, we use the method of projection operators to states with a definite spin. Separate analytic expressions for the contributions of the muon self-energy, the muon vertex operator and the amplitude with spanning photon are obtained. We present also numerical results for these contributions using m…
The measurement of the Lamb shift in muonic hydrogen and the subsequent emergence of the proton-radius puzzle have motivated an experimental campaign devoted to measuring the Lamb shift in other light muonic atoms, such as muonic deuterium and helium. For these systems it has been shown that two-photon exchange nuclear structure corrections are the largest source of uncertainty and consequently the bottleneck for exploiting the experimental precision to extract the nuclear charge radius. Utilizing techniques and methods developed to study electromagnetic reactions in light nuclei, recent calcu…
We report the first direct observation of excited state muon transfer in hydrogen/deuterium mixtures by direct measurement of q_1s, the probability that a mu-p atom, which is initially formed in an excited state, reaches the 1s ground state. The dependence of q_1s on deuterium concentration c_d was measured for two different densities at cryogenic temperatures using charge coupled devices (CCDs) to detect the muonic X rays. First results based on the analysis of the K_alpha-lines of the two isotopes are presented.
The complete contribution of diagrams with the light-by-light scattering to the Lamb shift is found for muonic hydrogen, deuterium and helium ion. The results are obtained in the static muon approximation and a part of the paper is devoted to the verification of this approximation and analysis of its uncertainty.
We present a study of the two-photon-exchange ($2γ$-exchange) corrections to the $S$-levels in muonic ($μ$D) and ordinary (D) deuterium within the pionless effective field theory (pionless EFT). Our calculation proceeds up to next-to-next-to-next-to-leading order (N3LO) in the pionless EFT expansion. The only unknown low-energy constant entering the calculation at this order corresponds to the coupling of a longitudinal photon to the nucleon-nucleon system. To minimise its correlation with the deuteron charge radius, it is extracted using the information about the hydrogen-deuterium isotope sh…
The recent conundrum with the proton charge radius inspires reconsideration of the corrections that enter into determinations of the proton size. We study the two-photon proton-structure corrections, with special consideration of the non-pole subtraction term in the dispersion relation, and using fits to modern data to evaluate the energy contributions. We find that individual contributions change more than the total, and present results with error estimates.
We calculate the amplitude T_1 for forward doubly-virtual Compton scattering in heavy-baryon chiral perturbation theory, to fourth order in the chiral expansion and with the leading contribution of the gammaNDelta form factor. This provides a model-independent expression for the amplitude in the low-momentum region, which is the dominant one for its contribution to the Lamb shift. It allows us to significantly reduce the theoretical uncertainty in the proton polarisability contributions to the Lamb shift in muonic hydrogen. We also stress the importance of consistency between the definitions o…
The proton-polarizability contribution to the muonic-hydrogen Lamb shift is a major source of theoretical uncertainty in the extraction of the proton charge radius. An empirical evaluation of this effect, based on the proton structure functions, requires a systematically improvable calculation of the "subtraction function", possibly using lattice QCD. We consider a different subtraction point, with the aim of accessing the subtraction function directly in lattice calculations. A useful feature of this subtraction point is that the corresponding contribution of the structure functions to the La…
We comprehensively analyse the theoretical prediction for the Lamb shift in muonic hydrogen, and the associated determination of the proton radius. We use effective field theories. This allows us to relate the proton radius with well-defined objects in quantum field theory, eliminating unnecessary model dependence. The use of effective field theories also helps us to organize the computation so that we can clearly state the parametric accuracy of the result. In this paper we review all (and check several of) the contributions to the energy shift of order $α^5$, as well as those that scale like…
The proton polarizability effect in the muonic-hydrogen Lamb shift comes out as a prediction of baryon chiral perturbation theory at leading order and our calculation yields for it: $ΔE^{(\mathrm{pol})} (2P-2S) = 8^{+3}_{-1}\, μ$eV. This result is consistent with most of evaluations based on dispersive sum rules, but is about a factor of two smaller than the recent result obtained in {\em heavy-baryon} chiral perturbation theory. We also find that the effect of $Δ(1232)$-resonance excitation on the Lamb-shift is suppressed, as is the entire contribution of the magnetic polarizability; the elec…
We obtain a model independent expression for the muonic hydrogen Lamb shift. This expression includes the leading logarithmic ${\cal O}(m_μα^6)$ terms, as well as the leading ${\cal O}(m_μα^5 \frac{m_μ^2}{m_ρ^2})$ hadronic effects. The latter are controlled by the chiral theory, which allows for their model independent determination. In this paper we give the missing piece for their complete expression including the pion and Delta particles. Out of this analysis and the experimental measurement of the muonic hydrogen Lamb shift we determine the electromagnetic proton radius: $r_p=0.8412(15)$ f…
The extraction of nuclear charge radii from spectroscopy experiments in muonic atoms is currently limited by the large uncertainties associated with the theoretical evaluation of the nuclear polarizability effects. To facilitate calculations, these polarizability corrections are conventionally expressed as an expansion in a dimensionless parameter $η$, which has been argued in previous literature to hold an approximate value of 0.33 in light-nuclear systems. In this work, we check this claim by doing a Bayesian analysis of the nuclear-polarizability corrections to the Lamb shift in $μ^2$H and …
We present calculations of nuclear structure effects to the Lamb shift in light muonic atoms. We adopt a modern ab-initio approach by combining state-of-the-art nuclear potentials with the hyperspherical harmonics method. Our calculations are instrumental to the determination of nuclear charge radii in the Lamb shift measurements, which will shed light on the proton radius puzzle.
We explore the possibility that a new interaction between muons and protons is responsible for the discrepancy between the CODATA value of the proton radius and the value deduced from the measurement of the Lamb shift in muonic hydrogen. We show that a new force carrier with roughly MeV mass can account for the observed energy shift as well as the discrepancy in the muon anomalous magnetic moment. However, measurements in other systems constrain the couplings to electrons and neutrons to be suppressed relative to the couplings to muons and protons, which seems challenging from a theoretical po…
The correction to the hydrogen Lamb shift due to the proton electric and magnetic polarizabilities is expressed analytically through their static values, which are known from experiment. The numerical value of the correction to the hydrogen 1S state is $ - 71 \pm 11 \pm 7$ Hz. Correction to the H-D 1S-2S -- isotope shift due to the proton and neutron polarizabilities is estimated as $ 53 \pm 9 \pm 11$ Hz.
The uncertainty in the contribution to the Lamb shift in muonic hydrogen, $ΔE^{subt}$ arising from proton polarizability effects in the two-photon exchange diagram at large virtual photon momenta is shown large enough to account for the proton radius puzzle. This is because $ΔE^{subt}$ is determined by an integrand that falls very slowly with very large virtual photon momenta. We evaluate the necessary integral using a set of chosen form factors and also a dimensional regularization procedure which makes explicit the need for a low energy constant. The consequences of our two-photon exchange i…
Laser spectroscopy of the Lamb shift (2S-2P energy difference) in light muonic atoms or ions, in which one negative muon $μ^-$ is bound to a nucleus, has been performed. The measurements yield significantly improved values of the root-mean-square charge radii of the nuclei, owing to the large muon mass, which results in a vastly increased muon wave function overlap with the nucleus. The values of the proton and deuteron radii are 10 and 3 times more accurate than the respective CODATA values, but 7 standard deviations smaller. Data on muonic helium-3 and -4 ions is being analyzed and will give…
The measurement of the 2P^{F=2}_{3/2} to 2S^{F=1}_{1/2} transition in muonic hydrogen by Pohl et al. and subsequent analysis has led to the conclusion that the rms radius of the proton differs from the accepted (CODATA) value by approximately 4%, corresponding to a 4.9 sigma discrepancy. We investigate the finite-size effects - in particular the dependence on the shape of the proton electric form-factor - relevant to this transition using bound-state QED with nonperturbative, relativistic Dirac wave-functions for a wide range of idealised charge-distributions and a parameterization of experime…
The current discrepancy of theory and experiment observed recently in muonic hydrogen necessitates a reinvestigation of all corrections to contribute to the Lamb shift in muonic hydrogen muH, muonic deuterium muD, the muonic 3He ion, as well as in the muonic 4He ion. Here, we choose a semi-analytic approach and evaluate a number of higher-order corrections to vacuum polarization (VP) semi-analytically, while remaining integrals over the spectral density of VP are performed numerically. We obtain semi-analytic results for the second-order correction, and for the relativistic correction to VP. T…
Reference Quadrupole Moments of Transition Elements from Lamb Shifts in Muonic Atoms
Technion-Israel Institute of Technology(以色列理工学院);ETH Zürich(苏黎世联邦理工学院);Sorbonne Université, CNRS, ENS-PSL Research University, Collège de France(索邦大学、法国国家科学研究中心、巴黎文理研究大学、法兰西公学院)