Quantum mechanical calculations are performed of the emission and absorption profiles of the lithium 2s-2p resonance line under the influence of a helium perturbing gas. We use carefully constructed potential energy surfaces and transition dipole moments to compute the emission and absorption coefficients at temperatures from 200 to 3000 K at wavelengths between 500 nm and 1000 nm. Contributions from quasi-bound states are included. The resulting red and blue wing profiles are compared with previous theoretical calculations and with an experiment, carried out at a temperature of 670 K.
We describe an experimental setup comprised of a discharge source for supersonic beams of metastable helium atoms and a magneto-optical trap (MOT) for ultracold lithium atoms that makes it possible to study Penning ionization and associative ionization processes at high ion count rates. The cationic reaction products are analyzed using a novel ion detection scheme which allows for mass selection, a high ion extraction efficiency and a good collision-energy resolution. The influence of elastic He-Li collisions on the steady-state Li atom number in the MOT is described, and the collision data ar…
We have estimated the shift and broadening of the resonance lines in the spectrum of antiprotonic helium atoms $\bar{p}\mathrm{He}^{+}$ implanted in solid helium $^4$He. The application of the response function for crystalline helium has enabled determination of the contributions from the collective degrees of freedom to the shift and broadening. It occurs that the broadening due to the collective motion is negligible compared to the natural line width. The available pair-correlation functions for crystalline $^4$He have been applied for estimating the resonance-line shift due to collisions of…
The precise calculations of blackbody radiation (BBR)-induced Stark shifts and depopulation rates for low-lying states of helium atom with the use of variational approach are presented. An effect of the BBR-induced induced Stark-mixing of energy levels is considered. It is shown that this effect leads to a significant reduction of lifetimes of helium excited states. As a consequence the influence of Stark-mixing effect on the decay rates of metastable states in helium is discussed in context of formation processes of the cosmic microwave background.
We calculate the density shift and broadening of selected dipole transition lines of pionic helium in gaseous helium at low temperatures up to T=12 K and pressure up to a few bar. In the approximation of binary collisions the shift and broadening depend linearly on the density; we evaluate the slope of this linear dependence for a few spectral lines of known experimental interest, and also investigate its temperature dependence. We find a blue shift of the resonance frequencies of the $(n,l)=(16,15) \rightarrow (16,14)$, $(17,16) \rightarrow (17,15)$, and $(16,15)\rightarrow(17,14)$ unfavored …
We demonstrate the control of $^4$He(2$^3$S$_1$)-$^7$Li(2$^2$S$_{1/2}$) chemi-ionization reactions by all-optical electron-spin-state preparation of both atomic species prior to the collision process. Our results demonstrate that chemi-ionization is strongly suppressed (enhanced) for non-spin-conserving (spin-conserving) collisions at thermal energies. These findings are in good agreement with a model based on spin angular momentum coupling of the prepared atomic states to the quasi-molecular states. Small deviations from the model indicate the contribution of the $^4Σ^+$ channel to the reacti…
It is shown that the non-relativistic ground state energy of helium-like and lithium-like ions with static nuclei can be interpolated in full physics range of nuclear charges $Z$ with accuracy of not less than 6 decimal digits (d.d.) or 7-8 significant digits (s.d.) using a meromorphic function in appropriate variable with a few free parameters. It is demonstrated that finite nuclear mass effects do not change 4-5 s.d. for $Z \in [1,50]$ for 2-,3-electron systems and the leading relativistic and QED corrections leave unchanged 3-4 s.d. for $Z \in [1,12]$ in the ground state energy for 2-electr…
Quantum calculation of the collision-induced line-shape effects in antiprotonic helium and the new accurate ab initio $\bar{p}$He$^{+}$-He potential energy surface
The long range interaction between an antiprotonic helium atom $\bar{p}$He$^+$ and helium atom in its ground state is studied. We calculate the dispersion coefficients $C_6$ using the Complex Coordinate Rotation (CCR) formalism in order to comply with the resonant nature of metastable states of the antiprotonic helium. We present as well numerical data on static dipole polarizabilities of antiprotonic helium states. The obtained coefficients $C_6$ may be used to estimate the collisional shift and broadening of transition lines in a low density precision spectroscopy of the antiprotonic helium.
我们推广了Bakalov D.，B.Jeziorski，T.Korona，K.Szalewicz，E.Tchoukova，Phys. Rev. Lett. { \bf 84}（2000）2350，关于单光子电偶极跃迁线移位和加宽到双光子跃迁的情况。作为例子，我们考虑了在氦气靶中产生的反质子氦的激光诱导跃迁。跃迁是在反质子氦态$(n,l)=(33,32)$和$(31,30)$之间。PACS 32.70.Jz、34.20.Gj、36.10.- K
Following detailed analysis of relativistic, QED and mass corrections for helium-like and lithium-like ions with static nuclei for $Z \leq 20$ the domain of applicability of Non-Relativistic QED (NRQED) is localized for ground state energy. It is demonstrated that for both helium-like and lithium-like ions with $Z \leq 20$ the finite nuclear mass effects do not change 4-5 significant digits (s.d.), and the leading relativistic and QED effects leave unchanged 3-4 s.d. in the ground state energy. It is shown that the non-relativistic ground state energy can be interpolated with accuracy not less…
The thermal two-photon level broadening of the excited energy levels in the hydrogen and H-like helium is evaluated via the imaginary part of thermal two-loop self-energy correction for bound electron. All the derivations are presented in the framework of rigorous quantum electrodynamic theory at finite temperatures and are applicable for the H-like ions. On this basis, we found a contribution to the level broadening induced by the blackbody radiation which is fundamentally different from the usual line broadening caused by the stimulated two-photon decay and the Raman scattering of thermal ph…
The collision-induced shift and broadening of selected dipole transition lines of pionic helium in gaseous helium at low temperatures up to $T=12$ K and pressure up to a few bar are calculated within variable phase function approach. We predict blue shift of the resonance frequencies of the $(n,l)=(16,15) \rightarrow (16,14) $ and $(16,15) \rightarrow (17,14)$ unfavored transitions and red shift for the favored transition $(17,16) \rightarrow (16,15)$. The result may be helpful in reducing the systematic error in proposed future experiments for determination of the negatively charged pion mass…
Density effects in precision laser spectroscopy of exotic helium atoms
Nicolaus Copernicus University in Toruń（托伦哥白尼大学）；Radboud University（拉德堡德大学）；Institute for Nuclear Research and Nuclear Energy, Bulgarian Academy of Sciences（保加利亚科学院核研究与核能研究所）；University of Warsaw（华沙大学）
We investigate the absorption line shapes of laser-dressed atoms beyond the single-atom response, by using extreme ultraviolet (XUV) attosecond pulse trains to probe an optically thick helium target under the influence of a strong infrared (IR) field. We study the interplay between the IR-induced phase shift of the microscopic time-dependent dipole moment and the resonant-propagation-induced reshaping of the macroscopic XUV pulse. Our experimental and theoretical results show that as the optical depth increases, this interplay leads initially to a broadening of the IR-modified line shape, and …
We measure the transverse relaxation of the spin state of an ensemble of ground-state rubidium atoms trapped in solid parahydrogen at cryogenic temperatures. We find the spin dephasing time of the ensemble (T$_2^*$) is limited by inhomogeneous broadening. We determine that this broadening is dominated by electrostatic interactions with the host matrix, and can be reduced by preparing nonclassical spin superposition states. Driving these superposition states gives significantly narrower electron paramagnetic resonance lines and the longest reported electron spin $T_2^*$ in any solid-phase syste…
