We present a semi-relativistic model for the description of the ionization process of atomic hydrogen by electron impact in the first Born approximation by using the Darwin wave function to describe the bound state of atomic hydrogen and the Sommerfeld-Maue wave function to describe the ejected electron. This model, accurate to first order in $Z/c$ in the relativistic correction, shows that, even at low kinetic energies of the incident electron, spin effects are small but not negligible. These effects become noticeable with increasing incident electron energies. All analytical calculations are exact and our semi-relativistic results are compared with the results obtained in the non relativistic Coulomb Born Approximation both for the coplanar asymmetric and the binary coplanar geometries.
Small Phase Space Structures and their Relevance to Pulsed Quantum Evolution: the Stepwise Ionization of the Excited Hydrogen Atom in a Microwave Pulse
Relativistic strong-field ionization of hydrogen-like atoms or ions in a constant crossed electromagnetic field is studied. The transition amplitude is formulated within the strong-field approximation in Göppert-Mayer gauge, with initial and final electron states being described by the corresponding Dirac-Coulomb and Dirac-Volkov wave functions, respectively. Coulomb corrections to the electron motion during tunneling are taken into account by adjusting an established method to the present situation. Total and energy-differential ionization rates are calculated and compared with predictions fr…
Isotope effect in tunnelling ionization of neutral hydrogen molecules
最近有人从理论上预言,由于原子核运动,暴露在强电场中的轻、重氢分子将表现出明显不同的隧道电离率(O.I.)。Tolstikhin,H. J. Worner和T. Morishita,Phys.Rev.A87,041401(R)(2013)[1])。我们通过测量H2/D2混合气体射流与强飞秒激光脉冲相互作用中每种物质的相对电离产率,实验研究了同位素效应。在反应显微镜装置中,我们检测到离子碎片从所有贡献的渠道(单电离,解离,和顺序双电离),并确定了总单电离产率的比率为H2和D2。测得的比率同意定量与预测的广义弱场渐近理论在一个明显的失败的冻结核近似。
We investigate the strong-field ionization of atomic hydrogen in a few-cycle elliptically polarized infrared pulse by solving the time-dependent Schrödinger equation. The dependence of the photoelectron momentum distribution on the pulse intensity, ellipticity, length, envelope, and carrier envelope phase is analyzed. In particular, we explain the variation of the electron offset angle with asymptotic electron energy through the combined action of the field and the Coulomb potential, and demonstrate that low-ellipticity pulses make it possible to access the electron release time.
Electron's anomalous magnetic moment effects on laser assisted ionization of atomic hydrogen by electronic impact
本文研究了在电子反常磁矩(AMM)作用下氢原子的电子碰撞电离。本文给出了Y. Attaourti和S. Taj [Phys.Rev.A69,063411(2004)]用于检查当异常$κ$取为零时我们的计算的一致性。我们表明,即使在第一玻恩近似中,包含AMM效应的项的贡献也具有重要的贡献,因此必须将其包括在任何可靠的分析中。给出了TDCS的全解析计算。
We present experimental data on the non-adiabatic strong field ionization of atomic hydrogen using elliptically polarized femtosecond laser pulses at a central wavelength of 390 nm. Our measured results are in very good agreement with a numerical solution of the time-dependent Schrödinger equation (TDSE). Experiment and TDSE show four above-threshold ionization (ATI) peaks in the electron's energy spectrum. The most probable emission angle (also known as 'attoclock-offset angle' or 'streaking angle') is found to increase with energy, a trend that is opposite to standard predictions based on Co…
It is generally assumed that for ionization processes, which occur in slow atomic collisions, the coupling of the colliding system to the quantum radiation field is irrelevant. Here we show, however, that -- contrary to expectations -- such a coupling can strongly influence ionization of a beam of atomic species A slowly traversing a gas of atomic species B excited by a weak laser field. Moreover, this coupling becomes even more important when the collision velocity increases, getting comparable or exceeding the typical electron orbiting velocities in A and B. Our results imply furthermore tha…
Wavefunction-splitting or mask method, widely used in the non-relativistic calculations of the photoelectron angular distributions, is extended to the relativistic domain within the dipole approximation. Since the closed-form expressions for the relativistic Volkov states are not available within the dipole approximation, we build such states numerically solving a single second-order differential equation. We calculate the photoelectron energy spectra and angular distributions for highly charged ions under different ionization regimes with both the direct and the relativistic mask methods. We …
Positronium breakup versus hydrogen ionization in collisions with fast charged projectiles: a comparative study
Institute of Modern Physics, Chinese Academy of Sciences(中国科学院近代物理研究所);Heinrich-Heine-University of Düsseldorf(杜塞尔多夫大学);University of Chinese Academy of Sciences(中国科学院大学)
We perform ab initio calculations for the hydrogen atom initially in one of the six circular bound states with the principal quantum numbers n = 2, 3 and 4, irradiated by a short circularly polarized laser pulse of 400 nm. The field propagates in the direction parallel to the z-component of the angular momentum of the atom. We investigate probabilities for the atom to ionize or to get on some bound (excited) state or to remain in the initial state after the end of the laser pulse. In most cases, we find pronounced differences in ionization probabilities for atoms in states having different sig…
Ionization of molecular hydrogen and deuterium by a frequency-doubled Ti:sapphire laser pulses
在$(2-13)\times10^{13} $ W cm $^{-2}$的强度范围内,对平行或垂直于线偏振激光脉冲(400 nm)的氢或氘分子的强场单电离进行了理论研究.该研究是基于非微扰处理,解决了完整的时间依赖的薛定谔方程的相关电子内固定的核和偶极子近似。各种核间分离的结果被用来获得分子氢和氘在其基态振动态的电离产额。一个原子模型是用来识别的影响,内在的双原子两中心字符的问题。