We demonstrate low-threshold random lasing in random amplifying layered medium via photon localization. Lasing is facilitated by resonant excitation of localized modes at the pump laser wavelength, which are peaked deep within the sample with greatly enhanced intensity. Emission occurs into long-lived localized modes overlapping the localized gain region. This mechanism overcomes a fundamental barrier to reducing lasing thresholds in diffusive random lasers, in which multiple scattering restricts the excitation region to the proximity of the sample surface.
We show that the degree of localization for the modes of a random laser (RL) is affected by the inter mode interaction that is controlled by shaping the spot of the pump laser. By experimentally investigating the spatial properties of the lasing emission we infer that strongly localized modes are activated in the low interacting regime while in the strongly interacting one extended modes are found lasing. Thus we demonstrate that the degree o localization may be finely tuned at the micrometer level.
We prove Anderson localization in a disordered photonic crystal waveguide by measuring the ensemble-averaged localization length which is controlled by the dispersion of the photonic crystal waveguide. In such structures, the localization length shows a 10-fold variation between the fast- and the slow-light regime and, in the latter case, it becomes shorter than the sample length thus giving rise to strongly confined modes. The dispersive behavior of the localization length demonstrates the close relation between Anderson localization and the photon density of states in disordered photonic cry…
The analogue of the paramagnetic to spin-glass phase transition in disordered magnetic systems, leading to the phenomenon of replica symmetry breaking, has been recently demonstrated in a two-dimensional random laser consisting of an organic-based amorphous solid-state thin film. We report here the first demonstration of replica symmetry breaking in a one-dimensional photonic system consisting of an erbium-doped random fiber laser operating in the continuous-wave regime based on a unique random fiber grating system, which plays the role of the random scatterers and operates in the Anderson loc…
Achieving localization with molecular precision has been of great interest for extending fluorescence microscopy to nanoscopy. MINFLUX pioneers this transition through point spread function (PSF) engineering, yet its performance is primarily limited by the signal-to-background ratio. Here we demonstrate that applying two-photon excitation to MINFLUX would double its localization precision through PSF engineering by nonlinear effect. Cramér-Rao Bound (CRB) is studied as the maximum localization precision, and CRB of two-photon MINFLUX is halved compared to single-photon MINFLUX in all three dim…
We experimentally demonstrate that the bandwidth of single photons laser pulse is compressed by a factor of 58 in a periodically poled lithium niobate (PPLN) waveguide chip. A chirped single photons laser pulse and an oppositely chirped classical laser pulse are employed to produce a narrowband single photon pulse with new frequency through sum-frequency generation. In our experiment, the frequency and bandwidth of single photons at 1550 nm are simultaneously converted. Our results mark a critical step towards the realization of coherent photonic interface between quantum communication at 1550…
We present a theoretical study of the wave packet dynamics of the H$_2^+$ molecular ion in plasmon-enhanced laser fields. Such fields may be produced, for instance, when metallic nano-structures are illuminated by a laser pulse of moderated intensity. Their main property is that they vary in space on nanometer scales. We demonstrate that the spatial inhomogeneous character of these plasmonic fields leads to an enhancement of electron localization, an instrumental phenomenon that controls molecular fragmentation. We suggest that the charge-imbalance induced by the surface-plasmon resonance near…
We observe and study the phenomenon of Anderson localization in a system of true quantum kicked rotors. Nitrogen molecules in a supersonic molecular jet are cooled down to 27~K and are rotationally excited by a periodic train of 24~high-intensity femtosecond pulses. Exponential distribution of the molecular angular momentum - the most unambiguous signature of Anderson localization - is measured directly by means of coherent Raman scattering. We demonstrate the suppressed growth of the molecular rotational energy with the number of laser kicks and study the dependence of the localization length…
Unintentional but unavoidable fabrication imperfections in state-of-the-art photonic-crystal waveguides lead to the spontaneous formation of Anderson-localized modes thereby limiting slowlight propagation and its potential applications. On the other hand, disorder-induced cavities offer an approach to cavity-quantum electrodynamics and random lasing at the nanoscale. The key statistical parameter governing the disorder effects is the localization length, which together with the waveguide length determines the statistical transport of light through the waveguide. In a disordered photonic-crysta…
We introduce a method to achieve three-dimensional dynamic localization of light. We consider a dynamically-modulated resonator lattice that has been previously shown to exhibit an effective gauge potential for photons. When such an effective gauge potential varies sinusoidally in time, dynamic localization of light can be achieved. Moreover, while previous works on such effective gauge potential for photons were carried out in the regime where the rotating wave approximation is valid, the effect of dynamic localization persists even when the counter-rotating term is taken into count.
A theoretical and experimental investigation of the intensity noise reduction induced by two-photon absorption in a Er,Yb:Glass laser is reported. The time response of the two-photon absorption mechanism is shown to play an important role on the behavior of the intensity noise spectrum of the laser. A model including an additional rate equation for the two-photon-absorption losses is developed and allows the experimental observations to be predicted.
We report on 3D time-domain parallel simulations of Anderson localization of light in inverted disordered opals displaying a complete photonic band-gap. We investigate dynamic diffusion processes induced by femtosecond laser excitations, calculate the diffusion constant and the decay-time distribution versus the strength of the disorder. We report evidence of the transition from delocalized Bloch oscillations to strongly localized resonances in self-starting laser processes.
Self-induced transparency pulses propagating in a random medium embedded in a two-level system can transfer energy to localized Anderson states. This allows the onset of two-level laser-like action.
We theoretically investigate the laser wavelength dependence of asymmetric dissociation of H$_2^+$. It is found that the electron localization in molecular dissociation is significantly manipulated by varying the wavelength of the driving field. Through creating a strong nuclear vibration in the laser-molecular interaction, our simulations demonstrate that the few-cycle mid-infrared pulse can effectively localize the electron at one of the dissociating nuclei with weak ionization. Moreover, we show that the observed phase-shift of the dissociation asymmetry is attributed to the different popul…
We measure the lasing dynamics of single and coupled photonic crystal nanocavity array lasers fabricated in the indium gallium arsenide phosphide material system. Under short optical excitation, single cavity lasers produce pulses as fast as 11 ps (FWHM), while coupled cavity lasers show significantly longer lasing duration which is not explained by a simple rate equations model. A Finite Difference Time Domain simulation including carrier gain and diffusion suggests that asynchronous lasing across the nanocavity array extends the laser's pulse duration.
A Fourier-space based design approach for the systematic control of single and multiple photon localization states in a 1D lattice is presented. Resultant lattices are aperiodic in nature, such that lattice periodicity is not a useful optimization parameter to achieve novel field localization characteristics. Instead, direct control of field localization comes via control of the Parseval strength competition between the different Fourier components characterizing a lattice. This is achieved via an inverse optimization algorithm, tailoring the aperiodic lattice Fourier components to match that …
A photonic crystal (PhC) nanocavity formed in an optically very thick slab can support reasonably high-Q modes for lasing. Experimentally, we demonstrate room-temperature pulsed lasing operation from the PhC dipole mode emitting at 1324 nm, which is fabricated in an InGaAsP slab with thickness (T) of 606 nm. Numerical simulation reveals that, when T > 800 nm, over 90% of the laser output power couples to the PhC slab modes, suggesting a new route towards an efficient in-plane laser for photonic integrated circuits.
Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb technique. Each transition is uniquely identified by the modulation imparted by the interfering comb excitations. The temporal modulation of the spontaneous two-photon fluorescence is monitored with a single photodetector, and the spectrum is revealed by a Fourier transform.
We demonstrated sub-wavelength (~111 nm diameter) single nanowire (NW) continuous wave (CW) lasers on silicon photonic crystal in the telecom-band with direct modulation at 10 Gb/s by optical pumping at cryogenic temperatures. To estimate the small signal response and pseudo-random bit sequence (PRBS) modulation of our CW lasers, we employed a new signal detection technique that employs a superconducting single photon detector and a time-correlated single photon counting module. The results showed that our NW laser was unambiguously modulated at above 10 Gb/s and an open eye pattern was obtain…
Current quantum cascade lasers based upon conduction band electron transitions are predominantly TM (electrical field normal to the epitaxial direction) polarized. Here we present a study of localized defect modes, with the requisite TM polarization, in connected square and hexagonal lattice two-dimensional (2D) photonic crystals for application as quantum cascade laser resonators. A simple group-theory based analysis is used to produce an approximate description of the resonant modes supported by defects situated at different high symmetry points within the host photonic lattice. The results …
The threshold properties of photonic crystal quantum dot lasers operating in the slow-light regime are investigated experimentally and theoretically. Measurements show that, in contrast to conventional lasers, the threshold gain attains a minimum value for a specific cavity length. The experimental results are explained by an analytical theory for the laser threshold that takes into account the effects of slow-light and random disorder due to unavoidable fabrication imperfections. Longer lasers are found to operate deeper into the slow-light region, leading to a trade-off between slow-light in…
Photoelectric effect in a Ge-on-Si single-photon avalanche detector (SPAD) at a sub-photon energy in incident pulsed laser radiation is considered in frames of classical electrodynamics of continuous media. It is shown that the energy of incident laser radiation, which is shared among a huge number of electrons in Ge matrix, can concentrate on only one of these through the effect of the constructive interference of the fields re-emitted by surrounding electrons. Conservation of energy in this case is upheld because of a substantial narrowing of the effective bandgap in heavily doped p-Ge, whic…
We studied numerically and experimentally the effects of structural disorder on the performance of ultraviolet photonic crystal slab lasers. Optical gain selectively amplifies the high-quality modes of the passive system. For these modes, the in-plane and out-of-plane leakage rates may be automatically balanced in the presence of disorder. The spontaneous optimization of in-plane and out-of-plane confinement of light in a photonic crystal slab may lead to a reduction of the lasing threshold.
We report on femtosecond laser writing of single mode optical waveguides in chalcogenide Gallium Lanthanum Sulphide (GLS) glass. A multiscan fabrication process was employed to create waveguides with symmetric single mode guidance and low insertion losses at 800 nm wavelength, compatible with Ti:Sapphire ultrafast lasers. μRaman and X-Ray microanalysis were used to elucidate the origin of the laser-induced refractive index change in GLS. Nonlinear refractive index measurements of the waveguides were performed by finding the optical switching parameters of a directional coupler, demonstrating t…
We develop an analytical theory for diffusive random lasers by coupling the transport theory of the disordered medium to the semiclassical laser rate equations, accounting for (coherent) stimulated and (incoherent) spontaneous emission. From the causality of wave propagation in an amplifying, diffusive medium we derive a novel length scale which we identify with the average mode radius of the lasing quasi-modes. We show further that loss at the surface of the laser-active medium is crucial in order to stabilize a stationary lasing state. The solution of the transport theory of random lasers fo…
We demonstrate experimentally that structural perturbations imposed on highly-dispersive photonic crystal-based waveguides give rise to spectral features that bear signatures of Anderson localization. Sharp resonances with the effective Qs of over 30,000 are found in scattering spectra of disordered waveguides. The resonances are observed in a ~20-nm bandwidth centered at the cutoff of slowly-guided Bloch-modes. Their origin can be explained with interference of coherently scattered electromagnetic waves which results in the formation of a narrow impurity (or localization) band populated with …
We demonstrate three-photon excitation in quantum dots with a mode-locked fiber laser operating in the telecommunications band. We compare spectra and intensity dependence of fluorescence from one- and three-photon excitation of commercially available 640 nm quantum dots, using a 372 nm diode laser for one-photon excitation and 116 fs pulses from a mode-locked fiber laser with a center wavelength of 1575 nm for three-photon excitation.
We study the inverse problem of localization (imaging) of a laser beam from measurements of the intensity of light scattered off-axis by a Poisson cloud of small particles. Starting from the wave equation, we analyze the microscopic coherence of the scattered intensity and show that it is possible to determine the laser beam from the speckle pattern captured by a group of CCD cameras. Two groups of cameras are sufficient when the particles are either small or large with respect to the wavelength. For general particle sizes the accuracy of the laser localization with two groups of cameras is su…
Ultrafast all-optical control of spins with femtosecond laser pulses is one of the hot topics at the crossroads of photonics and magnetism with a direct impact on future magnetic recording. Unveiling light-assisted recording mechanisms for an increase of the bit density beyond the diffraction limit without excessive heating of the recording medium is an open challenge. Here we show that surface plasmon-polaritons in hybrid metal-dielectric structures can provide spatial confinement of the inverse Faraday effect, mediating the excitation of localized coherent spin precession with 0.41 THz frequ…
Laser-driven radiation sources are attracting increasing attention for several materials science applications. While laser-driven ions, electrons and neutrons have already been considered to carry out the elemental characterization of materials, the possibility to exploit high energy photons remains unexplored. Indeed, the electrons generated by the interaction of an ultra-intense laser pulse with a near-critical material can be turned into high energy photons via bremsstrahlung emission when shot into a high-Z converter. These photons could be effectively exploited to perform Photon Activatio…
Lasing transition is known to be analogous to the second-order phase transition. Furthermore, for some cases, it is possible to define the Ginzburg-Landau (GL) potential, and the GL theory predicts the photon statistical properties of lasers. However, the GL potential for lasers is surprising, because lasers are operating far from equilibrium. In this paper, we theoretically examine the validity of the GL theory for lasers in terms of various parameters, particularly, the ratio between photon and carrier lifetimes. For this purpose, we use stochastic rate equations and higher-order photon corr…
This paper looks at a potentially unique measurable due to photon-axion coupling in an external magnetic field. Simulations indicate that probing couplings significantly lower than seen by previous cavity experiments is possible.
An extraordinarily efficient mechanism, operating at high laser intensities and powers, is identified for spectral transferring huge laser energies to shorter ultraviolet and x-ray wavelengths. With megajoule laser energies currently available at near-optical wavelengths, this transfer would enable megajoule x-ray lasers, a huge advance over the millijoules x-ray pulses produced now.
We detail a method to produce a GeV-photon source with polarisation purity exceeding $96\%$ and $89\%$ for linear and circular polarisation respectively and with a brilliance of the order of $10^{21}\,\textrm{photons}/(\textrm{s}~\textrm{mm}^2~\textrm{mrad}^2~0.1\%~\textrm{BW})$. Using currently available multi-GeV electron bunches and laser pulses of moderately relativistic intensities, we show how the weakly nonlinear regime can produce photons polarised mainly parallel to the laser field. We demonstrate the robustness of this scheme by considering electron bunches of various emissivities co…
Non-linear Compton scattering in ultra-short intense laser pulses is discussed with the focus on angular distributions of the emitted photon energy. This is an observable which is accessible easily experimentally. Asymmetries of the azimuthal distributions are predicted for both linear and circular polarization. We present a systematic survey of the influence of the laser intensity, the carrier envelope phase and the laser polarization on the emission spectra for single-cycle and few-cycle laser pulses. For linear polarization, the dominant direction of the emission changes from a perpendicula…
The second-order temporal interference between two independent single-mode continuous-wave lasers is discussed by employing two-photon interference in Feynman's path integral theory. It is concluded that whether the second-order temporal interference pattern can be retrieved via two-photon coincidence counting measurement is dependent on the relationship between the resolution time of the detection system and the frequency difference between these two lasers. Two identical and tunable single-mode diode lasers are employed to verify the predictions experimentally. The experimental results are c…
We predict the existence of a novel interaction-induced spatial localization in a periodic array of qubits coupled to a waveguide. This localization can be described as a quantum analogue of a self-induced optical lattice between two indistinguishable photons, where one photon creates a standing wave that traps the other photon. The localization is caused by the interplay between on-site repulsion due to the photon blockade and the waveguide-mediated long-range coupling between the qubits.
In this work, we demonstrate the on-chip two-photon interference between single photons emitted by a single self-assembled InGaAs quantum dot and an external laser. The quantum dot is embedded within one arm of an air-clad directional coupler which acts as a beam-splitter for incoming light. Photons originating from an attenuated external laser are coupled to the second arm of the beam-splitter and then combined with the quantum dot photons, giving rise to two-photon quantum interference between dissimilar sources. We verify the occurrence of on-chip Hong-Ou-Mandel interference by cross-correl…
A femtosecond frequency-doubled Erbium-doped fiber laser with adjustable pulse repetition rate is developed and applied in two-photon excited fluorescence microscopy. The all-fiber laser system provides the fundamental pulse at 1560 nm wavelength with 22 fs duration for the second harmonic generation, resulting in 1.35 nJ, 60 fs pulses at 780 nm. The repetition rate is adjusted by a pulse picker unit built-in within the amplifier chain, directly providing transform-limited pulses for any chosen repetition rate between 1 and 12 MHz. We employed the laser source to drive a scanning two-photon ex…
The simplest model of a single-emitter laser generating in the regime of small number of photons in the cavity is theoretically investigated. Based on a system of equations for different moments of the field operators the analytical expressions for mean number of photons and its dispersion are obtained. Using the master equation approach the differential equation for the phase-averaged quasi-probability Q is derived. For some limiting cases the exact solutions of this equation are found.
Recently, intensely driven laser-matter interactions have been used to connect the fields of strong laser field physics with quantum optics by generating non-classical states of light. Here, we make a further key step and show the potential of strong laser fields for generating controllable high-photon-number coherent-state superpositions. This has been achieved by using two of the most prominent strong-laser induced processes: high-harmonic generation and above-threshold ionization. We show how the obtained coherent-state superpositions change from an optical Schrödinger "cat" state to a "kit…
We report a time-resolved study of the thermalization dynamics and the lasing to photon Bose-Einstein condensation crossover by in-\textit{situ} monitoring the photon kinetics in a dye microcavity. When the equilibration of the light to the dye temperature by absorption and re-emission is faster than photon loss in the cavity, the optical spectrum becomes Bose-Einstein distributed and photons accumulate at low-energy states, forming a Bose-Einstein condensate. The thermalization of the photon gas and its evolution from nonequilibrium initial distributions to condensation is monitored in real-t…
Modulational excitation of longitudinal photons (photonikos) and electron Langmuir waves, as well as ion sound waves by an incoherent strong and superstrong radiation (high-power short pulse lasers, non-thermal equilibrium cosmic field radiation, etc.) in plasmas are investigated. A simultaneous generation of photonikos and plasmons are demonstrated. Furthermore, the kinetic instability is considered when a low frequency photonikos are generated alone. Growth rates of these new modes are obtained.
The Compton scattering of X-ray photons, assisted by a short intense optical laser pulse, is discussed. The differential scattering cross section reveals the interesting feature that the main Klein-Nishina line is accompanied by a series of side-lines forming a broad plateau where up to ${\cal O} (10^3)$ laser photons participate simultaneously in a single scattering event. An analytic formula for the width of the plateau is given. Due to the non-linear mixing of X-ray and laser photons a frequency dependent rotation of the polarization of the final state X-ray photons relative to the scatteri…
We propose a framework that unifies the description of light transport in three-dimensional amorphous dielectric materials that exhibit both localization and a photonic bandgap. To this end, we argue that coherent reflection near and in the bandgap attenuates the generation of diffuse or localized photons. Using the self-consistent theory of localization and considering the density of states of photons, we can quantitatively describe all transport regimes: Transparency, light diffusion, localization, and bandgap. Comparing the model with numerical data on optical transport in hyperuniform diel…
We show that the reduction in photon number fluctuations at laser threshold often cited as a fundamental laser property does not occur in typical semiconductor lasers such as the ones commonly used in modern technological applications today. Indeed, such lasers may still exhibit thermal intensity fluctuations far above threshold. We therefore conclude that sub-thermal intensity fluctuations cannot be regarded as a necessary property of laser light. Rather, one should distinguish betwen a thermal laser regime and a sub-thermal laser regime.
Exact four-photon resonance of collinear planar laser pulses is known to be prohibited by the classical dispersion law of electromagnetic waves in plasma. We show here that the renormalization produced by an arbitrarily small relativistic electron nonlinearity removes this prohibition. The laser frequency shifts in collinear resonant four-photon scattering increase with laser intensities. For laser pulses of frequencies much greater than the electron plasma frequency, the shifts can also be much greater than the plasma frequency and even nearly double the input laser frequency at still small r…
We demonstrate a \SI{650}{\mW} \SI{243}{\nm} continuous-wave laser coupled to a linear optical enhancement cavity. The enhancement cavity can maintain $>$\SI{30}{\W} of intracavity power for \SI{1}{\hour} of continuous operation without degradation. This system has sufficient power for a demonstration of two-photon laser cooling of hydrogen and may be useful for experiments on other simple two-body atomic systems.
A midinfrared quantum cascade laser with high wall-plug efficiency is analyzed by means of an ensemble Monte Carlo method. Both the carrier transport and the cavity field dynamics are included in the simulation, offering a self-consistent approach for analyzing and optimizing the laser operation. It is shown that at low temperatures, photon emission and absorption can govern the carrier transport in such devices. Furthermore, we find that photon-induced scattering can strongly affect the kinetic electron distributions within the subbands. Our results are validated against available experimenta…
The Formation of metastable molecules (Feshbach resonances) at the collision of two atoms and subsequent stimulated transition to a lower unbound electronic molecular state, with emission of a photon of the laser radiation has been investigated. This can develop, in particular, for $Rb_2$ molecules due to resonance scattering of two $Rb$ atoms. The considered process is a basis for the creation of excimer lasers. Expressions for the cross sections of elastic and inelastic resonance scattering and the intensity of the stimulated emission of the photons have been obtained.
We derive an analytical expression for the count probability of a single photon detector for a wide range of input optical power that includes afterpulsing effects. We confirm the validity of the expression by fitting it to the data obtained from a saturated commercial Single Photon Detector by illuminating it with a cw laser. Detector efficiency and afterpulsing probability extracted from the fits agree with the manufacture specs for low repetition frequencies.
The marriage of two vibrant fields---photonics and neuromorphic processing---is fundamentally enabled by the strong analogies within the underlying physics between the dynamics of biological neurons and lasers, both of which can be understood within the framework of nonlinear dynamical systems theory. Whereas neuromorphic engineering exploits the biophysics of neuronal computation algorithms to provide a wide range of computing and signal processing applications, photonics offer an alternative approach to neuromorphic systems by exploiting the high speed, high bandwidth, and low crosstalk avai…
We demonstrate laser oscillation in a hexagonal-lattice photonic crystal nanocavity using an InGaAs quantum dot gain material by optical pumping at 5 K. The cavity comprises a defect created by shifting several air holes in a two-dimensional photonic crystal slab structure without removing any air holes to achieve both small mode volume and a high cavity quality factor. The measured cavity quality factors and estimated mode volume for the nanocavity are ~33,000 and ~0.004 um^3. The laser threshold is compared between the zero-cell and L3-type nanocavity lasers, and the zero-cell nanolasers are…
