Self-similar propagation of ultrashort, parabolic pulses in a laser resonator is observed theoretically and experimentally. This constitutes a new type of pulse-shaping in modelocked lasers: in contrast to the well-known static (soliton-like) and breathing (dispersion-managed soliton) pulse evolutions, asymptotic solutions to the nonlinear wave equation that governs pulse propagation in most of the laser cavity are observed. Stable self-similar pulses exist with energies much greater than can be tolerated in soliton-like pulse shaping, and this will have implications for practical lasers.
In this paper, we investigate for the first time, the spatiotemporal dynamics of self-similar parabolic pulse evolution in multimode fibers (MMFs). We present numerical predictions of the existence of parabolic pulse in a graded and step index MMFs and demonstrate that the parabolic pulse formation process could have a prominent effect on the spatiotemporal behavior in both fibers. We study the effect of the input pulse energy and its initial modal composition on the resulting parabolic pulse and the corresponding spatial beam profile. When the fundamental mode is mostly excited, the pulse evo…
We expand our previous analysis of nonlinear pulse shaping in optical fibres using machine learning [Opt. Laser Technol., 131 (2020) 106439] to the case of pulse propagation in the presence of gain/loss, with a special focus on the generation of self-similar parabolic pulses. We use a supervised feedforward neural network paradigm to solve the direct and inverse problems relating to the pulse shaping, bypassing the need for direct numerical solution of the governing propagation model.
We explore parabolic pre-shaping as a means of generating and amplifying ultrashort pulses. We develop a theoretical framework for modeling the technique and use its conclusions to design a femtosecond fiber amplifier. Starting from 9 ps pulses, we obtain 4.3 $μ$J, nearly transform-limited pulses 275 fs in duration, simultaneously achieving over 40 dB gain and 33-fold compression. Finally, we show that this amplification scheme is limited by Raman scattering, and outline a method by which the pulse duration and energy may be further improved and tailored for a given application.
We demonstrate gain-switched fiber laser with bias pumping plays an important role in regulating chaotic relaxation spikes. Under certain conditions the profile of output pulse from gain-switched fiber laser can keep the same shape as that of pump pulse. Bias pumping technique may have significance in increasing output stable pulse energy in gain-switched fiber laser. Gain-switched fiber laser with bias pumping may be interesting for some applications in micro-processing and thin film removal.
Ultrafast optical excitation with intense mid-infrared and terahertz pulses has emerged as a new tool to control materials dynamically. As most experiments are performed with femtosecond pulse excitation, typical lifetimes of most light-induced phenomena in solids are of only few picoseconds. Yet, many scientific applications require longer drive pulses and lifetimes. Here, we describe a mid-infrared pump - terahertz-probe setup based on a CO$\mathrm{_2}$ laser seeded with 10.6 $\mathrmμ$m wavelength pulses from an optical parametric amplifier, itself pumped by a Ti:Al$\mathrm{_2}$O$\mathrm{_3…
Spatiotemporal control refers to a class of optical techniques for structuring a laser pulse with coupled space-time dependent properties, including moving focal points, dynamic spot sizes, and evolving orbital angular momenta. Here we introduce the concept of arbitrarily structured laser (ASTRL) pulses which generalizes these techniques. The ASTRL formalism employs a superposition of prescribed pulses to create a desired electromagnetic field structure. Several examples illustrate the versatility of ASTRL pulses to address a range of laser-based applications.
Interferometric characterization of pulse front tilt of spatiotemporally focused femtosecond laser pulses for three-dimensional micromachining application
An all-optical pulse power editing (PPE) technique is reported. Using the PPE technique, pulses with different peak powers are output and directed to the positive or reverse saturable absorption (SA) range of the saturable absorber. Further, under the combined action of the PPE technique and SA, four pulse patterns including dissipative soliton (DS), DS molecules, soliton compounds composed of DS and noise-like pulse (NLP), and pure NLP are controllably generated in fiber lasers. The results are conducive for developing advanced DS lasers and can further clarify the onset of pulse dynamic patt…
Stable 30 fs pulses centered at 1068 nm (less than 10 optical cycles) are demonstrated in a diode pumped Yb:CaYAlO4 laser by using high-quality chemical vapor deposited monolayer graphene as the saturable absorber. The mode locked 8.43 optical-cycle pulses have a spectral bandwidth of ~ 50 nm and a pulse repetition frequency of ~ 113.5 MHz. To our knowledge, this is the shortest pulse ever reported for graphene mode-locked lasers and mode-locked Yb-doped bulk lasers. Our experimental results demonstrate that graphene mode locking is a very promising practical technique to generate few-cycle op…
We experimentally demonstrate that the bandwidth of single photons laser pulse is compressed by a factor of 58 in a periodically poled lithium niobate (PPLN) waveguide chip. A chirped single photons laser pulse and an oppositely chirped classical laser pulse are employed to produce a narrowband single photon pulse with new frequency through sum-frequency generation. In our experiment, the frequency and bandwidth of single photons at 1550 nm are simultaneously converted. Our results mark a critical step towards the realization of coherent photonic interface between quantum communication at 1550…
Femtosecond laser micromachining provides high precision and less thermal diffusion in surface structuring as a result of the ultrashort temporal duration and ultrahigh peak intensity of the femtosecond laser pulses. To increase the throughput of surface patterning, the focal spot size can be expanded with loose focusing, which, however, could lead to nonlinear self-focusing of the pulses when the pulses propagate in air. We solve the problem by use of spatiotemporally focused femtosecond laser pulses for ablation of metal surfaces, which gives rise to improved surface quality as compared with…
A dual color, frequency and pulse duration agile laser system, capable of delivering laser pulses in arbitrary temporal profiles with ~1 ns to ~1 us pulse duration, chirping rates of ~27 MHz/ns with an achievable chirping range of several GHz across the pulse duration, and with energies ranging from a few nJ to hundreds of mJ per pulse has been developed. The flexibility and capability of this laser system provide a wide range of laser parameters that can be exploited to optimize operational conditions in various experiments ranging from laser diagnostics to spectroscopy and optical manipulati…
In this paper, we studied the optimal alignment and anti-alignment of O2 molecules by femtosecond laser pulse under different input energy. The results show that there is an energy limit in molecular alignment. The optimal molecular alignment and anti-alignment degree will never increase with the increase of laser energy when the input laser energy exceeds the energy limit. Besides, under the energy limit, the molecular optimal alignment (or anti-alignment) degree by using a shorter pulse duration (under 100 fs) will be about same when the input laser energy remained constant (different pulse …
Pulse generation often requires a stabilized cavity and its corresponding mode structure for initial phase-locking. Contrastingly, modeless cavity-free random lasers provide new possibilities for high quantum efficiency lasing that could potentially be widely tunable spectrally and temporally. Pulse generation in random lasers, however, has remained elusive since the discovery of modeless gain lasing. Here we report coherent pulse generation with modeless random lasers based on the unique polarization selectivity and broadband saturable absorption of monolayer graphene. Simultaneous temporal c…
Laser Induced Incandescence (LII) is an experimental technique that has been extensively used for in-flame measurement of soot properties. The traditional laser used for LII has been Nd:YAG laser with 5-10 ns pulse durations. The present study investigates an unexpected LII signal behaviour in the form of a secondary peak observed when using long laser pulse duration in the range of hundreds of ns. Temporal LII signals at varying fluences (up to 4.5 J/cm2) and pulse durations are presented and discussed. Although an explanation based on theoretical grounds has not been found, the study shows t…
We report mode-locked ~1550 nm output of transform-limited ~180 fs pulses from a large mode-area (diameter ~ 50 μm) guided-wave erbium fluorozirconate glass laser. The passively mode-locked oscillator generates pulses with 25 nm bandwidth at 156 MHz repetition rate and peak-power of 260 W. Scalability to higher repetition rate is demonstrated by transform-limited 410 fs pulse output at 1.3 GHz. To understand the origins of the broad spectral output, the laser cavity is simulated by using a numerical solution to the Ginzburg-Landau equation. This paper reports the widest bandwidth and shortest …
Evolution of dissipative-soliton-resonance (DSR) pulses in an all-normal-dispersion fiber laser with pump power under various operation conditions are experimentally studied. The fiber laser is mode-locked by using a nonlinear fiber loop mirror. Apart from the typical pulse broadening due to the peak power clamping effect, pulse breaking was observed. In addition, pulse narrowing with pump power increasing was observed. All the incompatible evolution of DSR pulses could be attributed to the multiple parameters change due to pump power increasing under specific operation conditions.
Integrated modelocked lasers with high power are of utmost importance for next generation optical systems that can be field-deployable and mass produced. Here we study fully integrated modelocked laser designs that have the potential to generate ultrashort, high power, and high quality pulses. We explore a large mode area laser for high power pulse generation and study the various mode-locking regimes of dispersion managed soliton pulses in net anomalous and net normal dispersion cavities. Furthermore, we study numerically and experimentally general properties and tunability of a fast integrat…
The question of electromagnetic field intensification towards the values typical for strong field Quantum Electrodynamics is of fundamental importance. One of the most promising intensification schemes is based on the relativistic-flying mirror concept, which shows that the electromagnetic radiation reflected by the mirror will be frequency up-shifted by a factor of 4 gamma^2 (gamma: the Lorentz factor of the mirror). In laser-plasma interactions, such a mirror travels with relativistic velocities and typically has a parabolic form, which is advantageous for light intensification. Thus, a rela…
The efficient excitation of quantum sources such as quantum dots or single molecules requires high NA optics which is often a challenge in cryogenics, or in ultrafast optics. Here we propose a 3.2 um wide parabolic mirror, with a 0.8 um focal length, fabricated by direct laser writing on CdSe/CdS colloidal quantum dots, capable of focusing the excitation light to a sub-wavelength spot and to extract the generated emission by collimating it into a narrow beam. This mirror is fabricated via in-situ volumetric optical lithography, which can be aligned to individual emitters, and it can be easily …
Propagation of a tightly focused high-power ultrashort laser pulse in an optical medium is usually substantially influenced by the medium optical nonlinearity that can noticeably affect the laser pulse parameters around the nonlinear focus and lead to unavoidable and often undesirable spatial distortions of the focal waist. We present the results of our experimental study and numerical simulations on a femtosecond Ti-Sapphire laser pulse propagation in air under different spatial focusing. We concentrated our study on spectral-angular and spatial pulse transformations under different focusing …
We propose a laser-controlled plasma shutter technique to generate sharp laser pulses using a process analogous to electromagnetically-induced transparency in atoms. The shutter is controlled by a laser with moderately strong intensity, which induces a transparency window below the cutoff frequency, and hence enables propagation of a low frequency laser pulse. Numerical simulations demonstrate it is possible to generate a sharp pulse wavefront (sub-ps) using two broad pulses in high density plasma. The technique can work in a regime that is not accessible by plasma mirrors when the pulse pedes…
We propose a new method for laser pulse compression that uses the spatially varying dispersion of a plasma plume with a density gradient. This novel scheme can be used to compress ultrahigh power lasers. A long, negatively frequency-chirped, laser pulse reflects off the plasma ramp of an over-dense plasma. As the density increases longitudinally the high frequency photons at the leading part of the laser pulse propagates more deeply than low frequency photons, the pulse is compressed in a similar way to compression off a chirped mirror. Proof-of-principle simulations, using a one-dimensional (…
We report a novel optical pulse generation method for high-speed wavelength switching of amplified nanosecond (ns) laser pulses resonant to atomic transitions.Under free-running condition, a slave laser diode is blue-detuned with tens of GHz relative to the master laser. A ns pulse chain generated by modulating the continuous-wave master laser with a fiber-pigtailed electro-optical intensity modulator is injected into the slave laser diode to fast switch the slave laser's wavelength back and forth. The output beam of slave laser is filtered by a temperature-controlled etalon to get the amplifi…
We report the coherent generation and detection of terahertz (THz) pulses covering the bandwidth of 0.1-9 THz in a high repetition rate, low pulse energy laser system. In this work we demonstrate the application and evaluation of solid-state biased coherent detection in combination with a spintronic emitter. This combination was used to generate and detect THz pulses in a time-domain spectroscopy (TDS) setup and tested on bulk nonlinear crystals. These results establish a new promising candidate to extend the possibilities for compact, broadband THz TDS systems driven by high repetition rate l…
We propose a novel measurement technique capable of determining the temporal duration of an intense laser pulse directly in its focus at full intensity. We show that the electromagnetic radiation pattern emitted by an electron bunch with a temporal energy chirp colliding perpendicularly with the laser pulse exhibits a distinct dependence on the pulse's duration. As the electrons emit radiation into an angular region determined by the ratio of their instantaneous energy to the laser's local field strength, the temporal change of the electrons' energy imprints information about the laser's pulse…
The measurement of weak temporal phase for picosecond and nanosecond laser pulses is important but quite difficult. We propose a simple iterative algorithm, which is based on a temporally movable phase modulation process, to retrieve the weak temporal phase of laser pulses. This unambiguous method can achieve a high accuracy and simultaneously measure the weak temporal phase and temporal profile of pulses, which are almost transform-limited. Detailed analysis shows that this iterative method has valuable potential applications in the characterization of pulses with weak temporal phase.
Understanding the mechanisms and controlling the possibilities of surface nanostructuring is of crucial interest from fundamental and practical perspectives. Here we report a direct experimental observation of laser-induced periodic surface structures (LIPSS) formed near a predesigned gold step edge following single-pulse femtosecond laser irradiation. A hybrid atomistic-continuum model fully supports experimental observations. We identify two key components of single-pulse LIPSS formation: excitation of surface plasmon polaritons and material reorganization. Our results lay the foundation tow…
Advances of high intensity lasers have opened up the field of strong field physics and led to a broad range of technological applications. Recent x ray laser sources and optics development makes it possible to obtain extremely high intensity and brightness at x ray wavelengths. In this paper, we present a system design that implements chirped pulse amplification for hard x ray free electron lasers. Numerical modeling with realistic experimental parameters show that near-transform-limit single-femtosecond hard x ray laser pulses with peak power exceeding 1 TW and brightness exceeding $4\times10…
The pressing need for the detailed wavefront properties of ultra-bright and ultra-short pulses produced by free-electron lasers (FELs) has spurred the development of several complementary characterization approaches. Here we present a method based on ptychography that can retrieve full high-resolution complex-valued wave functions of individual pulses. Our technique is demonstrated within experimental conditions suited for diffraction experiments in their native imaging state. This lensless technique, applicable to many other short-pulse instruments, can achieve diffraction-limited resolution.
We demonstrate laser driven acceleration of electrons to MeV-scale energies at 1kHz repetition rate using <10mJ pulses focused on near-critical density He and H2 gas jets. Using the H2 gas jet, electron acceleration to ~0.5MeV in ~10fC bunches was observed with laser pulse energy as low as 1.3mJ. Increasing the pulse energy to 10mJ, we measure ~1pC charge bunches with >1MeV energy for both He and H2 gas jets.
The critical power of self-focusing in the air for ultrashort UV laser pulses stretched due to dispersion from 90 up to 730 fs was experimentally measured. It was shown that the pulse duration enhancement due to its propagation in condensed media within above mentioned time-range leads to almost linear decrease of self-focusing critical power. It was also observed that when the pulse peak power exceeds the critical one, the maximum of linear plasma distribution along the UV laser filament does not shifted in the direction opposite to the laser pulse propagation as in the case of IR laser filam…
