We report a new calculation of the parity non-conserving E1 amplitude for the 6p_{1/2} -> 6p_{3/2} transition in Tl. Our result for the reduced matrix element is $E1_{PNC}=-(66.7 \pm 1.7) i 10^{-11} (-Q_W/N)$ a.u. Comparison with the experiment of Vetter et al [PRL,{\bf 74},2658 (1995)] gives the following result for the weak charge of $^{205}$Tl: $Q_W/Q_W^{SM} = 0.97 (\pm 0.01)_{expt} (\pm 0.03)_{theor}$, where $Q_W^{SM}=-116.7$ is the standard model prediction. This result confirms an earlier conclusion based on the analysis of a Cs experiment that atomic PNC experiments are in agreement with the standard model.
We calculate nuclear spin-dependent parity non-conserving $E1$-amplitudes for optical transition $6p_{1/2,F} -> 6p_{3/2,F'}$ and for hyperfine transition $6p_{1/2,F} -> 6p_{1/2,F'}$ in Tl. Experimental limit on the former amplitude placed by Vetter et al. [PRL, 74, 2658 (1995)] corresponds to the anapole moment constant $κ_a = -0.26 \pm 0.27$. Experiment on the hyperfine transition can give direct measurement of the spin-dependent amplitude, because spin-independent amplitude turns to zero.
Parity and time invariance violating electric dipole moment of $^{205}$Tl is calculated using the relativistic Hartree-Fock and configuration interaction methods and the many-body perturbation theory. Contributions from the interaction of the electron electric dipole moments with internal electric field and scalar-pseudoscalar electron-nucleon (T,P)-odd interaction are considered. The results are $d(^{205}{\rm Tl})=-582(20) d_e$ or $d(^{205}{\rm Tl})=-7.0(2)\times 10^{-18}C^{SP} e {\rm cm}$. Interpretation of the measurements are discussed. The results of similar calculations for $^{133}$Cs ar…
In a recent Comment [arXiv:1108.3399], Dzuba and Flambaum have referred to the disagreement of the results of our latest calculations of Tl electron and scalar-pseudoscalar (S-PS) electric dipole moments (EDMs) and Cs parity non-conservation (PNC) with some other calculations. We have responded to all their points and also discussed the larger issues related to them. We have attempted to find the reasons for the disagreement between the results of our calculations and those of others. In particular, we have found that the two important reasons for the discrepancies between the Tl EDM calculati…
We present accurate {\em ab initio} non-perturbative calculations of the Breit correction to the parity non-conserving (PNC) amplitudes of the $6s-7s$ and $6s-5d_{3/2}$ transitions in Cs, $7s-8s$ and $7s-6d_{3/2}$ transitions in Fr, $6s-5d_{3/2}$ transition in Ba$^+$, $7s-6d_{3/2}$ transition in Ra$^+$, and $6p_{1/2} - 6p_{3/2}$ transition in Tl. The results for the $6s-7s$ transition in Cs and $7s-8s$ transition in Fr are in good agreement with other calculations while calculations for other atoms/transitions are presented for the first time. We demonstrate that higher-orders many-body correc…
We use configuration interaction technique to calculate parity non-conservation (PNC) in metastable Xe and Hg [proposal of the experiment in L. Bougas et al, Phys. Rev. Lett. 108, 210801 (2012)]. Both, nuclear spin-independent and nuclear spin-dependent (dominated by the nuclear anapole moment) parts of the amplitude are considered. The amplitudes are strongly enhanced by proximity of the states of opposite parity.
We calculate magnetic dipole transition amplitudes in s-s and s-d transitions of Rb, Cs, Ba+, Fr, Ra+, Yb+, Ac2+ and Th3+. These transitions were used or considered to be used for the measurements of parity non-conservation (PNC). We also calculate the magnetic g-factor anomalies for a selection of states, along with electric quadrupole transition amplitudes for s-d transitions in these systems.
We present nuclear spin-independent and dependent parity non-conservation amplitudes for the $[4f^{14}]6s\;^2S_{1/2}-[4f^{14}]5d\;^2D_{3/2}$ transition of $^{171}$Yb$^+$, calculated using perturbed relativistic coupled-cluster theory. As a proxy to estimate theoretical uncertainty of these results we calculate the excitation energies, hyperfine structure constants and E1 transition amplitudes for the important low lying states. The PNC results presented in paper shall be useful in the propose PNC experiments.
We calculate the binding energy, charge radii in $^{126}$Ba--$^{140}$Ba and $^{214}$Ra--$^{228}$Ra using the relativistic mean field theory which includes scalar and vector mesons. We then evaluate the nuclear structure corrections to the weak charges for a series of isotopes of these atoms using different parameters and estimate their uncertainty in the framework of this model. Our results will have important implication for the ongoing and planned parity non-conservation experiments and atomic structure calculations on Ba$^+$ and Ra$^+$.
Currently the theoretical uncertainty limits the interpretation of the atomic parity non-conservation (PNC) measurements. We calculate the PNC $5s$ - $6s$ electric dipole transition amplitude in rubidium and demonstrate that rubidium is a good candidate to search for new physics beyond the standard model since accuracy of the atomic calculations in rubidium can be higher than in cesium. PNC in cesium is currently the best low-energy test of the standard model, therefore, similar measurements for rubidium present a good option for further progress in the field. We also calculate nuclear spin-de…
We have developed a relativistic coupled-cluster theory to incorporate nuclear spin-dependent interaction Hamiltonians perturbatively. This theory is ideal to calculate parity violating nuclear spin-dependent electric dipole transition amplitudes, $E1_{\rm PNC}^{\rm NSD}$, of heavy atoms. Experimental observation of which is a clear signature of nuclear anapole moment, the dominant source of nuclear spin-dependent parity violation in atoms and ions. We apply the theory to calculate $E1_{\rm PNC}^{\rm NSD}$ of Cs, which to date has provided the best atomic parity violation measurements. We also…
The contribution of the axial triangle anomalous graph to the parity non-conservation effect in atoms is evaluated. The final answer looks like the emission of the electric photon by the magnetic dipole. The relative contribution to the parity non-conservation effect in neutral atoms appears to be negligible but is essentially larger in case of multicharged ions.
We have developed a relativistic coupled-cluster theory to incorporate nuclear spin-dependent interaction Hamiltonians perturbatively. In this theory, the coupled-cluster operators in the electronic sector are defined as tensor operators of rank one and we introduce suitable diagrammatic representations. For properties calculations, the electronic part is first calculated and later coupled to the nuclear spin part. The method is ideal to calculate parity violating nuclear spin-dependent electric dipole transition amplitudes, $E1_{\rm PNC}^{\rm NSD}$, of heavy atoms. To validate the proposed me…
Using recent high-precision measurements of electric dipole matrix elements of atomic cesium, we make an improved determination of the scalar ($α$) and vector ($β$) polarizabilities of the cesium $6s \ ^2S_{1/2} \rightarrow 7s \ ^2S_{1/2} $ transition calculated through a sum-over-states method. We report values of $α= -268.82 \ (30) \ a_0^3$ and $β= 27.139 \ (42) \ a_0^3$ with the highest precision to date. We find a discrepancy between our value of $β$ and the past preferred value, resulting in a significant shift in the value of the weak charge $Q_w$ of the cesium nucleus. Future work to re…
We discuss the prospects for parity non-conservation experiments with highly charged heavy ions. Energy levels and parity mixing for heavy ions with two to five electrons are calculated. We investigate two-photon-transitions and the possibility to observe interference effects between weak-matrix elements and Stark matrix elements for periodic electric field configurations.
We identify a pair of near-degenerate states of opposite parity in atomic Xe, the $5p^5 10s \,\, ^2[3/2]_2^o$ at $\rm{E}=94759.927$ cm$^{-1}$ and $5p^5 6f \,\, ^2[5/2]_2$ at $\rm{E}= 94759.935$ cm$^{-1}$, for which parity- and time-odd effects are expected to be enhanced by the small energy separation. We present theoretical calculations which indicate narrow widths for both states and we report a calculated value for the weak matrix element, arising from configuration mixing, of $|W|=2.1$ Hz for $^{132}$Xe. In addition, we measured the Stark effect of the $5p^5\,6f$ $^2[5/2]_{2}$ and $5p^5 \,…
A dynamic blue-detuned optical dipole trap with stable $^{87}Rb$ atoms produces a differential ac Stark shift of 18 Hz in the ground state hyperfine transition, and it preserves the ground state hyperfine superpositions for a long coherence time of 180 ms. The trapped atoms undergoing microwave Rabi oscillations are sensitive to a small signal, artificially generated with a second microwave source, phase locked to the first allow- ing a simple and effective method for determining signal-to-noise ratio limits through interference techniques. This provides an excellent means of calibrating sensi…
Due to electron-nucleus weak interaction, atomic bound states with different parities turn out to be mixed. We discuss a prospect for measuring the mixing parameter between the nearly degenerate metastable states 1s_{1/2} 2s_{1/2} : J = 0 and 1s_{1/2} 2p_{1/2} : J = 0 in heliumlike Uranium. Our analysis is based on the polarization properties of the photons emitted in the two-photon decays of such states.
We apply the sum-over-states approach to calculate partial contributions to the parity non-conservation (PNC) in cesium [Porsev {\em et al}, Phys. Rev. D {\bf 82}, 036008 (2010)]. We have found significant corrections to two non-dominating terms coming from the contribution of the core and highly excited states ($n>9$, the so called {\em tail}). When these differences are taken into account the result of Porsev {\em et al}, $E_{\rm PNC} = 0.8906\,(24) \times 10^{-11}i(-Q_W/N)$ changes to $0.8977\,(40)$, coming into good agreement with our previous calculations, $0.8980\,(45)$. The interpretati…
Fock-space perturbed relativistic coupled-cluster calculations of electric dipole polarizability and nuclear spin-dependent parity non-conservation in Cs
Recent progress in calculations of QED radiative corrections to parity nonconservation in atoms is reviewed. The QED vacuum polarization, the self-energy corrections and the vertex corrections are shown to be described very reliably by different methods used by different groups. All new calculations have recently converged to very close final values. Each separate radiative correction is very large, above 1 % for heavy atoms, but having different signs they partly compensate each other. Our results for the radiative corrections for all atoms are presented. The corrections are -0.54 % for 133 C…
We have performed relativistic many-body calculations of the hyperfine interaction in the $6s$ and $7s$ states of Cs, including the off-diagonal matrix element. The calculations were used to determine the accuracy of the semi-empirical formula for the electromagnetic transition amplitude $<6s|M1|7s>$ induced by the hyperfine interaction. We have found that even though the contribution of the many-body effects into the matrix elements is very large, the square root formula $<6s|H_{hfs}|7s > = \sqrt{< 6s|H_{hfs}|6s > < 7s|H_{hfs}|7s >}$ remains valid to the accuracy of a fraction of $10^{-3}$. T…
A semi-empirical calculation of the 6s - 7s Stark amplitude $α$ in Cs has been performed using the most accurate measurements and calculations of the electromagnetic amplitudes available. This is then used to extract the parameters of the electroweak theory from experimental data. The results are: $α= 269.0 (1.3) a_0^3$, weak charge of Cs $Q_W = -72.41(25)_{exp} (80)_{theor}$, deviation from the Standard model $S = -1.0(.3)_{exp} (1.0)_{theor}$ and limit on the mass of the extra Z-boson in SO(10) model $M_{Z_x} > 550 GeV$.
The nuclear spin of a He$^3$ quasiparticle dissolved in superfluid He$^4$ sees an apparent magnetic field proportional to the Fermi coupling constant, the superfluid condensate density, and the electron current at the He$^3$ nucleus. Whereas the direction of the current must be parallel to the quasiparticle momentum, calculating its magnitude presents an interesting theoretical challenge because it vanishes in the Born-Oppenheimer approximation. We find the effect is too small to be observed and present our results in the hope others will be inspired to look for similar effects in other system…
We propose the effective simulation of light-matter ultrastrong-coupling phenomena with strong-coupling systems. Recent theory and experiments have shown that the quantum Rabi Hamiltonian can be simulated by a Jaynes--Cummings system with the addition of two classical drives. This allows to implement nonlinear processes that do not conserve the total number of excitations. However, parity is still a conserved quantity in the quantum Rabi Hamiltonian, which forbids a wide family of processes involving virtual transitions that break this conservation. Here, we show that these parity-non-conservi…
We review the current status of the study of parity and time invariance violation in atoms, nuclei and molecules. We focus on parity non-conservation in cesium and three of the most promising areas of research: (i) parity non-conservation in a chain of isotopes, (ii) search for nuclear anapole moments, and (iii) search for permanent electric dipole moments (EDMs) of atoms and molecules, which in turn are caused by either an electron EDM or nuclear $T,P$-odd moments such as a nuclear EDM or nuclear Schiff moment.
The atomic parity non-conservation(PNC) experiments has reached accuracies which have important implications for physics beyond the standard model. An optical rotation experiment to measure the atomic PNC of the 3P1(6s6p)--1P1(6s6p) in Yb was proposed recently. Our screened electron-electron coulomb potential multi-configuration Dirac-Fock calculation of th PNC induced E1 transition amplitude of this transition E1_PNC = -96.0 x 10^{-11}iea_0(-Q_W/N) of 171Yb is more than two orders of magnitude larger than E1_PNC(6s-7s) = -0.8991 x 10^{-11}iea_0(-Q_W/N) of 133Cs.
Parity (P) and time (T) invariance violating effects in the Ra atom are strongly enhanced due to close states of opposite parity, the large nuclear charge Z and the collective nature of P,T-odd nuclear moments. We have performed calculations of the atomic electric dipole moments (EDM) produced by the electron EDM and the nuclear magnetic quadrupole and Schiff moments. We have also calculated the effects of parity non-conservation produced by the nuclear anapole moment and the weak charge. Our results show that as a rule the values of these effects are much larger than those considered so far i…
Accurately calibrated effective field theories are used to compute atomic parity non-conserving (APNC) observables. Although accurately calibrated, these effective field theories predict a large spread in the neutron skin of heavy nuclei. While the neutron skin is strongly correlated to a large number of physical observables, in this contribution we focus on its impact on new physics through APNC observables. The addition of an isoscalar-isovector coupling constant to the effective Lagrangian generates a wide range of values for the neutron skin of heavy nuclei without compromising the success…
Employing the relativistic coupled-cluster method, comparative studies of the parity non-conserving electric dipole amplitudes for the $7s \ ^2S_{1/2} \rightarrow 6d \ ^2D_{5/2}$ transitions in $^{210}$Fr and $^{211}$Fr isotopes have been carried out. It is found that these transition amplitudes, sensitive only to the nuclear spin dependent effects, are enhanced by more than 3 orders compared to the low-lying $S-D_{5/2}$ transitions in Ba$^+$ and Ra$^+$ owing to the very large contributions from the electron core-polarization effects in Fr. This translates to a relatively large and, in princip…
We perform calculations for the neutron skin of nuclei and its contribution to atomic parity non-conservation (PNC) in many isotopes of Cs, Ba, Sm, Dy, Yb, Tl, Pb, Bi, Fr, Ra. Three problems are addressed: i) Neutron-skin induced errors to single-isotope PNC, ii) Possibility to measure neutron skin using atomic PNC, iii) Neutron-skin induced errors for ratios of PNC effects in different isotopes. In the latter case the correlations in the neutron skin values for different isotopes lead to cancelations of the errors; this makes the isotopic ratio method a competitive tool in a search for new ph…
