arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2603.03214cond-mat.str-elcond-mat.mtrl-sci
收藏

蜂窝状磁体Na$_3$Co$_2$SbO$_6$中的各向异性磁弹性耦合

Anisotropic magnetoelastic coupling in the honeycomb magnet Na$_3$Co$_2$SbO$_6$

University of Augsburg(奥格斯堡大学);Max-Planck-Institute for Solid State Research(马克斯·普朗克固体研究所)
Prashanta K. Mukharjee, Sebastian Erdmann, Lichen Wang, Julian Kaiser, Anton Jesche, Pascal Puphal, Masahiko Isobe, Matthias Hepting, Bernhard Keimer, Philipp G… 展开作者

Prashanta K. Mukharjee, Sebastian Erdmann, Lichen Wang, Julian Kaiser, Anton Jesche, Pascal Puphal, Masahiko Isobe, Matthias Hepting, Bernhard Keimer, Philipp Gegenwart, Alexander A. Tsirlin

AI总结:

通过磁化和膨胀测量,研究了蜂窝状钴酸盐Na$_3$Co$_2$SbO$_6$的相图,发现面内磁场下c*轴晶格响应具有强各向异性,归因于Co-O-Co键角变化,并在低温下观察到磁化台阶和一级相变特征,但未发现场致量子自旋液体态的证据。

摘要:

我们展示了蜂窝状钴酸盐Na$_3$Co$_2$SbO$_6$的磁化和膨胀测量结果,并绘制了其详细的场温相图,温度低至亚开尔文。面内磁场的数据显示c*轴晶格响应具有强各向异性,根据 extit{ab initio}计算,这主要由Co-O-Co键角的变化主导。在$T = 0.4$~K时,磁化强度$M(B)$表现出阶梯状特征,也是高度各向异性的。在$B \parallel b$的情况下,第二个场致磁相变($B_{c2}$)附近观察到的小滞后表明其一级相变特征,而磁Grüneisen参数在$B_{c2}$处的发散在冷却时被抑制,表明进入场极化态时不存在量子临界行为。我们的热力学测量均未提供在$B_{c2}$附近或以上存在场致量子自旋液体态的证据。

英文摘要:

We present magnetization and dilatometry measurements on the honeycomb cobaltate Na$_3$Co$_2$SbO$_6$ and map out its detailed field-temperature phase diagram down to sub-Kelvin temperatures. Our data for in-plane magnetic fields show a strongly anisotropic $c^{*}$-axis lattice response, which is dominated by the variation of Co--O--Co bond angles according to \textit{ab initio} calculations. At $T = 0.4$~K, the magnetization $M(B)$ exhibits step-like features that are also highly anisotropic. In the case of $B \parallel b$, a small hysteresis observed around the second field-induced magnetic transition ($B_{c2}$) indicates its first-order character, whereas divergence of the magnetic Grüneisen parameter at $B_{c2}$ is suppressed upon cooling and signals the absence of quantum critical behavior upon entering the field-polarized state. None of our thermodynamic measurements provide evidence for a field-induced quantum spin liquid state near or above $B_{c2}$.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑