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arXiv 2602.20747cond-mat.mtrl-sci
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InSiTe3中接近孤立爱因斯坦模式的声子频率梳

Phonon frequency comb close to an isolated Einstein mode in InSiTe3

Center for Solid State Physics and New Materials, Institute of Physics Belgrade(贝尔格莱德物理研究所固态物理与新材料中心);Departamento de Física de Materiales, Facultad de Ciencias, Universidad Autónoma de Madrid(马德里自治大学理学院材料物理系);Department of Condensed Matter Physics, Jozef Stefan Institute(约泽夫·斯特凡研究所凝聚态物理系);Shanghai Advanced Research in Physical Sciences (SHARPS)(上海物理科学研究院);Center for Correlated Matter and School of Physics, Zhejiang University(浙江大学物理学院相关物质研究中心)
Tea Belojica, Jovan Blagojević, Sanja Djurdjić Mijin, Andrijana Šolajić, Jelena Pešić, Emil S. Božin, Bojana Višić, Yu Liu, Cedomir Petrovic, Zoran V. Popović, … 展开作者

Tea Belojica, Jovan Blagojević, Sanja Djurdjić Mijin, Andrijana Šolajić, Jelena Pešić, Emil S. Božin, Bojana Višić, Yu Liu, Cedomir Petrovic, Zoran V. Popović, Rudi Hackl, Ana Milosavljević, Nenad Lazarević

AI总结:

InSiTe3中发现接近孤立爱因斯坦模式的声子频率梳,揭示了该材料中高结构化声子光谱相关性和强非谐效应的共存,为低维材料中的振动现象研究提供了新途径。

摘要:

声子频率梳的出现体现了量子固体中一种罕见而引人入胜的现象。具有独特声子带结构的材料尤其有希望承载此类状态,因为它们的振动色散景观在整个布里渊区中可以促进长寿命、集体晶格激发的形成。在层状范德瓦尔化合物InSiTe3中,偏振分辨拉曼光谱揭示了在对称预测模式中表现出显著的非谐性,并在约500 cm⁻¹的局部高能A₁g声子模式附近形成了自组织的频率域结构(相干态)。这种强声子-声子耦合表现为在约200 K附近出现异常的温度依赖性,恰好对应于声子密度态间隙内的高阶激发出现。这些发现将InSiTe3定位为一种非常规平台,其中内在的高结构化声子光谱相关性和异常强的非谐效应共存,为探索低维材料中的新兴振动现象开辟了新途径。

英文摘要:

The emergence of phonon frequency combs exemplifies a rare and intriguing phenomenon in quantum solids. Materials with distinctive phonon band structures are especially promising for hosting such states, as their vibrational dispersion landscape across the Brillouin zone can facilitate the formation of long-lived, collective lattice excitations. In the layered Van der Waals compound InSiTe$_3$, polarization-resolved Raman spectroscopy reveals a pronounced anharmonicity in symmetry-predicted modes and the formation of a self-organized frequency domain structure (coherent-like state), in the range of a localized highenergy A$_{1g}$ phonon mode near 500 cm$^{-1}$. This strong phonon-phonon coupling manifests itself as an anomalous temperature dependence around 200 K, coinciding with the appearance of higher-order excitations within the phonon density of states gap. These findings position InSiTe$_3$ as an unconventional platform where intrinsic highly structured phonon spectral correlations and unusually strong anharmonic effects coexist, opening new avenues for exploring emergent vibrational phenomena in low-dimensional materials.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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