氧化物异质结构中的涡旋隧道效应与临界态

Superconductivity in epitaxially grown LaVO3/KTaO3(111) heterostructures

Complex oxide heterointerfaces can host a rich of emergent phenomena, and epitaxial growth is usually at the heart of forming these interfaces. Recently, a strong crystalline-orientation-dependent two-dimensional superconductivity was discovered at interfaces between KTaO3 single-crystal substrates and films of other oxides. Unexpectedly, rare of these oxide films was epitaxially grown. Here, we report the existence of superconductivity in epitaxially grown LaVO3/KTaO3(111) heterostructures, with a superconducting transition temperature of ~0.5 K. Meanwhile, no superconductivity was detected i…

Evidence for spin-triplet superconducting correlations in metal-oxide heterostructures with non-collinear magnetization

Heterostructures composed of ferromagnetic La0.7Sr0.3MnO3, ferromagnetic SrRuO3, and superconducting YBa2Cu3Ox were studied experimentally. Structures of composition Au/La0.7Sr0.3MnO3/SrRuO3/YBa2Cu3Ox were prepared by pulsed laser deposition, and their high quality was confirmed by X-ray diffraction and reflectometry. A non-collinear magnetic state of the heterostructures was revealed by means of SQUID magnetometry and polarized neutron reflectometry. We have further observed superconducting currents in mesa-structures fabricated by deposition of a second superconducting Nb layer on top of the…

Correlation of Fe-based Superconductivity and Electron-Phonon Coupling in an FeAs/Oxide Heterostructure

Interfacial phonons between iron-based superconductors (FeSCs) and perovskite substrates have received considerable attention due to the possibility of enhancing preexisting superconductivity. Using scanning tunneling spectroscopy, we studied the correlation between superconductivity and e-ph interaction with interfacial-phonons in an iron-based superconductor Sr$_2$VO$_3$FeAs ($T_c \approx$ 33 K) made of alternating FeSC and oxide layers. The quasiparticle interference measurement over regions with systematically different average superconducting gaps due to the e-ph coupling locally modulate…

Proximity effect and electron transport in the oxide hybrid heterostructures with superconducting/magnetic interfaces

We report on the study of electron transport in the oxide heterostructures with superconductor/magnetic matter (S/M) interfaces where anomaly large penetration of superconducting correlations in magnetic matter (proximity effect) is realized. The developed theoretical model based on multilayer magnetic structure of M-interlayer and experiment show presence of the long-range proximity effect at S/M-interface with antiferromagnetic (AF) ordering of the interlayer magnetization. The investigated hybrid heterostructures include cuprate superconductor, the AF-cuprate interlayer and conventional sup…

Factors limiting ferroelectric field-effect doping in complex-oxide heterostructures

Ferroelectric field-effect doping has emerged as a powerful approach to manipulate the ground state of correlated oxides, opening the door to a new class of field-effect devices. However, this potential is not fully exploited so far, since the size of the field-effect doping is generally much smaller than expected. Here we study the limiting factors through magneto-transport, scanning transmission electron and piezo-response force microscopy in ferroelectric/superconductor (YBa2Cu3O7-δ /BiFeO3) heterostructures, a model system showing very strong field-effects. Still, we find that they are lim…

Interface controlled electronic charge inhomogeneities in correlated heterostructures

For heterostructures of ultrathin, strongly correlated copper-oxide films and dielectric perovskite layers, we predict inhomogeneous electronic interface states. Our study is based on an extended Hubbard model for the cuprate film. The interface is implemented by a coupling to the electron and phonon degrees of freedom of the dielectric oxide layer. We find that electronic ordering in the film is associated with a strongly inhomogeneous polaron effect. We propose to consider the interfacial tuning as a powerful mechanism to control the charge ordering in correlated electronic systems.

Topological superconductivity from transverse optical phonons in oxide heterostructures

A topological superconductor features at its boundaries and vortices Majorana fermions, which are potentially applicable for topological quantum computations. The scarcity of the known experimentally verified physical systems with topological superconductivity, time-reversal invariant ones in particular, is giving rise to a strong demand for identifying new candidate materials. In this research, we study a heterostructure consisting of a transition metal oxide two-dimensional electron gas (2DEG) sandwiched by insulators near the paraelectric (PE) / ferroelectric (FE) phase transition. Its rele…

Universality of transition temperatures in families of copper-oxide superconductors: interlayer tunneling redux

We revisit the interlayer tunneling theory of high temperature superconductors and formulate it as a mechanism by which the striking systematics of the transition temperature within a given homologous series can be understood. We pay attention not only to the enhancement of pairing, as was originally suggested, but also to the role of competing order parameters that tend to suppress superconductivity, and to the charge imbalance between inequivalent outer and inner CuO2 planes in a unit cell. Calculations based on a generalized Ginzburg-Landau theory yield results that bear robust and remarkab…

从头计算识别Nb₂O₅和Ta₂O₅中的氢隧穿作为双态系统

From Atomistic Impurity Landscapes to Two-Level-System Distributions and Microwave Loss: Hydrogen-Induced Losses in Nb$_2$O$_{5-δ}$ and Ta$_2$O$_{5-δ}$

研究通过机器学习加速氢配置采样和扩散路径分析，结合从头计算验证，揭示氢隧穿是Nb₂O₅和Ta₂O₅中双态系统的主要来源，解释了实验观测到的Nb氧化物损耗高于Ta氧化物的现象。