Accurate characterization of coherent and non-Markovian errors remains a central challenge in quantum information processing, as conventional benchmarking techniques typically rely on Markovian and time-independent noise assumptions. In practice, however, quantum devices exhibit both systematic coherent miscalibrations and temporally correlated fluctuations, which complicate error diagnosis and mitigation. Here, we apply a technique based on tangent-space decomposition to characterize such error in single-qubit quantum gates implemented on a trapped ion platform. Small imperfections in a quantum operation are treated as perturbations of the target quantum map, represented as tangent vectors in the space of quantum channels. This formulations enables a natural decomposition of the deviation into three components corresponding to coherent, Markovian and non-Markovian processes.The relative weights of these components provide a quantitative measure of the contribution from each type of error mechanism, directly from a single tomographic snapshot. We experimentally validate this method on a single-qubit gates implemented on a trapped $^{40}$Ca$^+$ ion, where control is achieved through laser-driven optical transitions. By analyzing experimentally reconstructed process matrices, expressed in the Pauli Transfer Matrix and Choi representations, we identify and quantify non-Markovian effects arising from controlled injection of slow fluctuations in the experimental environment. We also characterize deterministic coherent miscalibrations using the same technique. This approach provides a physically transparent and experimentally accessible tool for diagnosing complex error sources in quantum control systems.
We examine the properties of open quantum systems with respect to their time evolution in different regimes, Markovian and non-Markovian. We analyze their behaviour with respect to their coherent or decoherent time evolution by means of different models and try to gain some insight into the possible correlations between Markovianity and coherence.
We derive the explicit commutation relations for the generators of quantum dynamical semigroup - Markovian superoperator evolution, allowing the extension of Baker-Campbell-Hausdorff-type relations to general Lindblad-type evolutions. This provides a novel tool for exploring the interaction of time-dependent coherent and Markovian evolutions - a surprisingly rich set of behaviors which include deformation by coherent driving of Markovian terms, generation of new Lindblad terms from time-dependent noise and even a coherent driving term generated by the interaction of time-separated Markovian no…
We study the unitary time evolution of photons interacting with a dielectric resonator using coherent control pulses. We show that non-Markovianity of transient photon dynamics in the resonator subsystem may be controlled to within a photon-resonator transit time. In general, appropriate use of coherent pulses and choice of spatial subregion may be used to create and control a wide range of non-Markovian transient dynamics in photon resonator systems.
We microscopically model the decoherence dynamics of entangled coherent states under the influence of vacuum fluctuation. We derive an exact master equation with time-dependent coefficients reflecting the memory effect of the environment, by using the Feynman-Vernon influence functional theory in the coherent-state representation. Under the Markovian approximation, our master equation recovers the widely used Lindblad equation in quantum optics. We then investigate the non-Markovian entanglement dynamics of the quantum channel in terms of the entangled coherent states under noise. Compared wit…
This paper presents a non-Markovian coherent feedback scheme to control single quantum dot systems. The feedback loop is closed via a quantum tunneling junction between the natural source and drain baths of the quantum dot. The exact feedback-controlled non-Markovian Langevin equation is derived for describing the dynamics of the quantum dot. To deal with the nonlinear memory function in the Langevin equation, we analyze the Green's function-based root locus, from which we show that the decoherence of the quantum dot can be suppressed via increasing the feedback coupling strength. This effecti…
We critically evaluate the most widespread assumption in the theoretical description of coherent control strategies for open quantum systems. We show that, for non-Markovian open systems dynamics, this fixed-dissipator assumption leads to a serious pitfall causing insurmountable difficulties in the effective modelling of the controlled system. We show that the only way to avoid these problems is a full microscopic description of the controlled system in presence of noise. We illustrate our findings with a paradigmatic example.
We study the interaction between several fields initially in coherent states. The solution allows us to explain why coherent states remain coherent states when subject to non-Markovian dissipation. We first study the interaction between two fields and show that this is the building block of the total interaction. We give a completely algebraic solution of this system.
We develop a notion of stochastic quantum trajectories. First, we construct a basis set of trajectories, called elementary trajectories, and go on to show that any quantum dynamical process, including those that are non-Markovian, can be expressed as a linear combination of this set. We then show that the set of processes divide into two natural classes: those that can be expressed as convex mixture of elementary trajectories and those that cannot be. The former are shown to be entanglement breaking processes (in each step), while the latter are dubbed coherent processes. This division of proc…
Based on tensor network realizations of path integrals reducing exponential memory scaling to polynomial efficiency and a Liouville space implementation of a time-discrete quantum memory, we investigate a quantum system simultaneously exposed to two structured reservoirs. For this purpose, we employ a numerically exact quasi-2D tensor network combining both diagonal and off-diagonal system-reservoir interactions with a twofold memory for continuous and discrete retardation effects. As a possible example, we study the non-Markovian dynamical interplay between discrete photonic feedback and stru…
Unveiling coherent dynamics in non-Markovian open quantum systems: exact expression and recursive perturbation expansion
Università degli Studi di Milano（米兰大学）；INFN, Sezione di Milano（意大利国家核物理研究所米兰分部）；Institute of Physics, University of Freiburg（弗赖堡大学物理研究所）；EUCOR Centre for Quantum Science and Quantum Computing, University of Freiburg（弗赖堡大学EUCOR量子科学与量子计算中心）；Naturwissenschaftlich-Technische Fakultät, Universität Siegen（锡根大学自然科学与技术学院）；Física Teòrica: Informació i Fenòmens Quàntics, Department de Física, Universitat Autònoma de Barcelona（巴塞罗那自治大学物理系理论物理：信息与量子现象部门）
We study the dynamics of a macroscopic superconducting qubit coupled to two independent non-stationary reservoirs by using time-dependent perturbation theory. We show that an equilibrium environment surpasses the coherent evolution of the macroscopic qubit completely. When the qubit couples to two different reservoirs, exemplifying a non-equilibrium environment, the short-time dynamics is affected by the interference between two reservoirs, implying the non-additivity of effects of two reservoirs. The non-additivity can be traced back to a non-Markovian effect, even though two reservoirs are i…
Given any two quantum states $ρ$ and $σ$ in Hilbert spaces of equal dimension satisfying the majorization condition $ρ\succ σ$, it is always possible to transform $ρ\mapsto σ$ by a unital quantum map. In fact, any such transformation can be achieved just by means of noisy operations, i.e., by access to maximally mixed ancillary states and unitary transformations that act jointly in the system-ancilla space. Here, we investigate the possible transitions between states (i.e., the induced preorder of states) when one restricts the unitary control to the quantum system alone and replaces the maxim…
We present the non-Markovian generalization of the widely used stochastic Schrodinger equation. Our result allows to describe open quantum systems in terms of stochastic state vectors rather than density operators, without approximation. Moreover, it unifies two recent independent attempts towards a stochastic description of non-Markovian open systems, based on path integrals on the one hand and coherent states on the other. The latter approach utilizes the analytical properties of coherent states and enables a microscopic interpretation of the stochastic states. The alternative first approach…
We investigate the coherence and non-Markovianity of a quantum tunneling system whose barrier is fluctuated by a telegraph noise, and its energy gap is modulated by Gaussian noise. With the help of averaging method, the system dynamics are analytically derived, and the analytical expression for coherence measure and non-Markovianity for the very limited parameter regimes for both initially coherent and non-coherent states are obtained. We observe non-Markovian dynamics in a situation where the Kubo number is high. It is also found that there is no strong relation between the coherence of the s…
We investigate the non-Markovian dynamics of a qubit-oscillator system embedded in a noisy environment by employing the hierarchical equations of motion approach. It is found that the decoherence rate of the whole qubit-oscillator-bath system can be significantly suppressed by enhancing the coupling strength between the qubit and the harmonic oscillator. Moreover, we find that the non-Markovian memory character of the bath is able to facilitate a robust quantum coherent dynamics in this qubit-oscillator-bath system. Our findings may be used to engineer some tunable coherent manipulations in me…
We propose the generalized stochastic Liouville equation to investigate the coherent dynamics in single molecule systems coupled to environments which exhibit both nonstationary and non-Markovian features. The generalized stochastic Liouville equation contains a generalized memory kernel associated with both the intrinsic system Hamiltonian and the non-Markovian features of the environmental noise, which returns to the well-known framework established by Kubo in the limit case that the environmental noise is stationary and memoryless. The coherence of the quantum system can be derived by means…
We study the coexistence of the quantum Zeno effect and non-Markovianity for a system decaying in a structured bosonic environment and subject to a control field. The interaction with the environment induces decay from the excited to the ground level, which, in turn, is coherently coupled to another meta-stable state. The control of the strength of the coherent coupling between the stable levels allows the engineering of both the dissipation and of the memory effects, without modifying neither the system-reservoir interaction, nor environmental properties. We use this framework in two differen…
We address continuous variable quantum key distribution (QKD) in non-Markovian lossy channels and show how the non-Markovian features may be exploited to enhance security and/or to detect the presence and the position of an eavesdropper along the transmission line. In particular, we suggest a coherent states QKD protocol which is secure against individual attacks for arbitrarily low values of the overall transmission line. Our scheme relies on specific non-Markovian properties, and cannot be implemented in ordinary Markovian channels characterized by uniform losses.
Excitation energy transfer (EET) and electron transfer (ET) are crucially involved in photosynthetic processes. In reality, the photosynthetic reaction center constitutes an open quantum system of EET and ET, which manifests an interplay of pigments, solar light and phonon baths. So far theoretical studies have been mainly based on master equation approaches in the Markovian condition. The non-Markovian environmental effect, which may play a crucial role, has not been sufficiently considered. In this work, we propose a mixed dynamic approach to investigate this open system. The influence of ph…
Established methods for characterizing quantum information processes do not capture non-Markovian (history-dependent) behaviors that occur in real systems. These methods model a quantum process as a fixed map on the state space of a predefined system of interest. Such a map averages over the system's environment, which may retain some effect of its past interactions with the system and thus have a history-dependent influence on the system. Although the theory of non-Markovian quantum dynamics is currently an active area of research, a systematic characterization method based on a general repre…
We investigate the single-photon scattering spectra of a giant atom coupled to a one dimensional waveguide via multiple connection points or a continuous coupling region. Using a full quantum mechanical method, we obtain the general analytic expressions for the single-photon scattering coefficients, which are valid in both the Markovian and the non-arkovian regimes. We summarize the influences of the non-dipole effects, mainly caused by the phases accumulated by photons traveling between coupling points, on the scattering spectra. We find that under the Markovian limit, the phase decay is detu…
On the non-Markovian quantum stochastic network dynamics
The Chinese University of Hong Kong（香港中文大学）；The Hong Kong Polytechnic University（香港理工大学）；The Hong Kong Polytechnic University Shenzhen Research Institute（香港理工大学深圳研究院）
In this paper we present a method to derive an exact master equation for a bosonic system coupled to a set of other bosonic systems, which plays the role of the reservoir, under the strong coupling regime, i.e., without resorting to either the rotating-wave or secular approximations. Working with phase-space distribution functions, we verify that the dynamics are separated in the evolution of its center, which follows classical mechanics, and its shape, which becomes distorted. This is the generalization of a result by Glauber, who stated that coherent states remain coherent under certain circ…
We present an algorithm to simulate genuine, measurement-conditioned quantum trajectories for a class of non-Markovian systems, using a collision model for the environment. We derive two versions of the algorithm, the first corresponding to photodetection and the second to homodyne detection with a finite local oscillator amplitude. We use the algorithm to simulate trajectories for a system with delayed coherent feedback, as well as a system with a continuous memory.
Manipulation of a quantum system requires the knowledge of how it evolves. To impose that the dynamics of a system becomes a particular target operation (for any preparation of the system), it may be more useful to have an equation of motion for the dynamics itself--rather than the state. Here we develop a Markovian master equation for the process matrix of an open system, which resembles the Lindblad Markovian master equation. We employ this equation to introduce a scheme for optimal local coherent process control at target times, and extend the Krotov technique to obtain optimal control. We …
We investigate the quantum coherent dynamics of an externally driven effective two-level system subjected to a slow Ohmic environment characteristic of biomolecular protein-solvent reservoirs in photosynthetic light harvesting complexes. By means of the numerically exact quasi adiabatic propagator path integral (QUAPI) method we are able to include non-Markovian features of the environment and show the dependence of the quantum coherence on the characteristic bath cut-off frequency omega_c as well as on the driving frequency omega_l and the field amplitude A. Our calculations extend from the w…
We develop a formalism for modelling exact time dynamics in waveguide quantum electrodynamics (QED) using the real-space approach. The formalism does not assume any specific configuration of emitters and allows the study of Markovian dynamics fully analytically and non-Markovian dynamics semi-analytically with a simple numerical integration step. We use the formalism to study subradiance, superradiance and bound states in continuum. We discuss new phenomena such as subdivision of collective decay rates into symmetric and anti-symmetric subsets and non-Markovian superradiance effects that can l…
We study the dynamics of an open quantum system interacting with a non-thermal bath. Here, "non-thermal" means that the bath modes do not need to have the same temperature, but they have an effective temperature distribution. We find that, when a quantum system is interacting with such a non-thermal bath far from thermal equilibrium, it is no longer proper to use any coarse-grained Markovian description for the system, even when their coupling strength is quite weak. Especially, when there is coherent transition with strong interference strength in the quantum system, the Markovian master equa…
Resonance fluorescence of an artificial atom with a time-delayed coherent feedback
National Tsing Hua University（国立清华大学）；Queen’s University（女王大学）；University of Ottawa（渥太华大学）；ShanghaiTech University（上海科技大学）；National Chung Cheng University（国立中正大学）；Center for Quantum Technology, National Tsing Hua University（国立清华大学量子科技中心）；RIKEN（理化学研究所）；University of Michigan（密歇根大学）
We find the conditions under which a quantum regression theorem can be assumed valid for non-Markovian master equations consisting in Lindblad superoperators with memory kernels. Our considerations are based on a generalized Born-Markov approximation, which allows us to obtain our results from an underlying Hamiltonian description. We demonstrate that a non-Markovian quantum regression theorem can only be granted in a stationary regime if the dynamics satisfies a quantum detailed balance condition. As an example we study the correlations of a two level system embedded in a complex structured r…
The study of open quantum systems is important for fundamental issues of quantum physics as well as for technological applications such as quantum information processing. The interaction of a quantum system with it's environment is usually detrimental for the quantum properties of the system and leads to decoherence. However, sometimes a coherent partial exchange of information takes place between the system and the environment and the dynamics of the open system becomes non-Markovian. In this article we study discrete open quantum system dynamics where single evolution step consist of local u…
We study the collective radiative decay of a system of two two-level emitters coupled to a one-dimensional waveguide in a regime where their separation is comparable to the coherence length of a spontaneously emitted photon. The electromagnetic field propagating in the cavity-like geometry formed by the emitters exerts a retarded backaction on the system leading to strongly non-Markovian dynamics. The collective spontaneous emission rate of the emitters exhibits an enhancement or inhibition beyond the usual Dicke super- and sub-radiance due to a self-consistent coherent time-delayed feedback.
We study the behavior of non-Markovianity with respect to the localization of the initial environmental state. The "amount" of non-Markovianity is measured using divisibility and distinguishability as indicators, employing several schemes to construct the measures. The system used is a qubit coupled to an environment modeled by an Ising spin chain kicked by ultra-short pulses of a magnetic field. In the integrable regime, non-Markovianity and localization do not have a simple relation, but as the chaotic regime is approached, simple relations emerge, which we explore in detail. We also study t…
The squeezing dynamics of a damped harmonic oscillator are studied for different types of environment without making the Markovian approximation. The squeezing dynamics of a coherent state depend on the reservoir spectrum in a unique way that can, in the weak coupling approximation, be analyzed analytically. Comparison of squeezing dynamics for Ohmic, sub-Ohmic and super-Ohmic environments is done showing a clear connection between the squeezing--non-squeezing oscillations and reservoir structure. Understanding the effects occurring due to structured reservoirs is important both from a purely …
We investigate memory effects in the spin-boson model using a recently proposed measure for non-Markovian behavior based on the information exchange between an open system and its environment. Employing the numerical exact multilayer multiconfguration time-dependent Hartree approach, we simulate the dynamics of the spin-boson model at zero temperature for a broad range of parameters. For a fast bath, i.e. in the scaling limit, we find non-Markovian dynamics for a coherently decaying spin at weak system-bath coupling, whereas memory effects are absent for stronger coupling in the regimes of inc…
We propose a systematic scheme to engineer quantum states of a quantum system governed by a time-convolutionless non-Markovian master equation. According to the idea of reverse engineering, the general algebraic equation to determine the control parameters, such as coherent and incoherent control fields, is presented. Without artificially engineering the time-dependent decay rates and retaining the environment-induced Lamb shifts, the quantum state can still be transferred into the target state in a finite period of time along an arbitrary designed trajectory strictly in Hilbert space. As an a…
We explore the nonunital non-Markovian dynamics of a qubit immersed in a spin bath. The nonunital environmental effects on the precisions of quantum parameter estimation are investigated. The time-dependent transfer matrix and inhomogeneity vector are obtained for the description of the open dynamical process. The evolution of the coherent vectors for a qubit is studied so as to geometrically demonstrate the nonunital non-Markovian effects. The revivals of angles for the fidelity between a maximal mixed state and an arbitrary trajectory state are presented in the nonunital non-Markovian dynami…
We analyze precision bounds for a local phase estimation in the presence of general, non-Markovian phase noise. We demonstrate that the metrological equivalence of product and maximally entangled states that holds under strictly Markovian dephasing fails in the non-Markovian case. Using an exactly solvable model of a physically realistic finite bandwidth dephasing environment, we demonstrate that the ensuing non-Markovian dynamics enables quantum correlated states to outperform metrological strategies based on uncorrelated states using otherwise identical resources. We show that this conclusio…
In this work we develop a numerical framework to investigate the renormalization of the non-Markovian dynamics of an open quantum system to which dynamical decoupling is applied. We utilize a non-Markovian master equation which is derived from the non-Markovian quantum trajectories formalism. It contains incoherent Markovian dynamics and coherent Schrödinger dynamics as its limiting cases and is capable of capture the transition between them. We have performed comprehensive simulations for the cases in which the system is either driven by the Ornstein-Uhlenbeck noise or or is described by the …
One long-standing difficult problem in quantum dissipative dynamics is to solve the spin-boson model in a non-Markovian regime where a tractable systematic master equation does not exist. The spin-boson model is particularly important due to its crucial applications in quantum noise control and manipulation as well as its central role in developing quantum theories of open systems. Here we solve this important model by developing a non-Markovian quantum Langevin approach. By projecting the quantum Langevin equation onto the coherent states of the bath, we can derivie a set of non-Markovian qua…
In the context of a charge qubit under continuous monitoring by a single electron transistor, we propose an unraveling of the generalized quantum Markovian master equation into an ensemble of individual quantum trajectories for stochastic point process. A suboptimal feedback algorism is implemented into individual quantum trajectories to protect a desired pure state. Coherent oscillations of the charge qubit could be maintained in principle for an arbitrarily long time in case of sufficient feedback strength. The effectiveness of the feedback control is also reflected in the detector's noise s…
Quantum technologies rely on the ability to coherently manipulate, process and transfer information, encoded in quantum states, along quantum channels. Decoherence induced by the environment introduces errors, thus setting limits on the efficiency of any quantum-enhanced protocol or device. A fundamental bound on the ability of a noisy quantum channel to transmit quantum (classical) information is given by its quantum (classical) capacity. Generally, the longer is a quantum channel the more are the introduced errors, and hence the worse is its capacity. In this Letter we show that for non-Mark…
We investigate the dynamical information exchange between a two-state system and its environment which is measured by von Neumann entropy. It is found that in the underdamping regime, the entropy dynamics exhibits an extremely non-Markovian oscillation-hump feature, in which oscillations manifest quantum coherence and a hump of envelop demonstrates temporal memory of bath. It indicates that the process of entropy exchange is bidirectional. When the coupling strength increases a certain threshold, the hump along with ripple disappears, which is indicative of the coherent-incoherent dynamical cr…
Quantum memory effects can be qualitatively understood as a consequence of an environment-to-system backflow of information. Here, we analyze and compare how this concept is interpreted and implemented in different approaches to quantum non-Markovianity. We study a non-operational approach, defined by the istinguishability between two system states characterized by different initial conditions, and an operational approach, which is defined by the correlation between different outcomes associated to successive measurement processes performed over the system of interest. The differences, limitat…
A complete treatment of the entanglement of two-level systems, which evolves through the contact with a thermal bath, must include the fact that the system and the bath are not fully separable. Therefore, quantum coherent superpositions of system and bath states, which are almost never fully included in theoretical models, are invariably present when an entangled state is prepared experimentally. We show their importance for the time evolution of the entanglement of two qubits coupled to independent baths. In addition, our treatment is able to handle slow and low-temperature thermal baths.
We introduce a non-Markovianity measure for continuous variable open quantum systems based on the idea put forward in H.-P. Breuer et al., Phys. Rev. Lett.\textbf{103}, 210401 (2009), i.e., by quantifying the flow of information from the environment back to the open system. Instead of the trace distance we use here the fidelity to assess distinguishability of quantum states. We employ our measure to evaluate non-Markovianity of two paradigmatic Gaussian channels: the purely damping channel and the quantum Brownian motion channel with Ohmic environment. We consider different classes of Gaussian…
