We present a comprehensive end-to-end framework for simulating the real-time dynamics of chemical systems on a fault-tolerant quantum computer, incorporating both electronic and nuclear quantum degrees of freedom. An all-particle simulation is nominally efficient on a quantum computer, but practically infeasible. Hence, central to our approach is the construction of a first-quantized plane-wave algorithm making use of pseudoions. The latter consolidate chemically inactive electrons and the nucleus into a single effective dynamical ionic entity, extending the well-established concept of pseudopotentials in quantum chemistry to a two-body interaction. We explicitly describe efficient quantum circuits for initial state preparation across all degrees of freedom, as well as for block-encoding the Hamiltonian describing interacting pseudoions and chemically active electrons, by leveraging recent advances in quantum rejection sampling to optimize the implementations. To extract useful chemical information, we first design molecular fingerprints by combining density-functional calculations with machine learning techniques, and subsequently validate them through surrogate classical molecular dynamics simulations. These fingerprints are then coherently encoded on a quantum computer for efficient molecular identification via amplitude estimation. We provide an extensive analysis of the cost of running the algorithm on a fault-tolerant quantum computer for several chemically interesting systems. As an illustration, simulating the interaction between $\mathrm{NH_3}$ and $\mathrm{BF_3}$ (a 40-particle system) requires 808 logical qubits to encode the problem, and approximately $10^{11}$ Toffoli gates per femtosecond of time evolution. Our results establish a foundation for further quantum algorithm development targeting chemical and material dynamics.
Solid-state spin qubits are a promising platform for quantum computation and quantum networks. Recent experiments have demonstrated high-quality control over multi-qubit systems, elementary quantum algorithms and non-fault-tolerant error correction. Large-scale systems will require using error-corrected logical qubits that are operated fault-tolerantly, so that reliable computation is possible despite noisy operations. Overcoming imperfections in this way remains a major outstanding challenge for quantum science. Here, we demonstrate fault-tolerant operations on a logical qubit using spin qubi…
In the framework quotient algebra partition, a general methodology is introduced to construct fault tolerant encodes for an arbitrary action in an error-correcting code.
We present a quantum circuit synthesis algorithm for implementing universal fault-tolerant quantum computing based on concatenated codes. To realize fault-tolerant quantum computing, the fault-tolerant quantum protocols should be transformed into executable quantum circuits based on the nearest-neighbor interaction. Unlike topological codes that are defined based on local operations fundamentally, for the concatenated codes, it is possible to obtain the circuits composed of the local operations by applying the quantum circuit synthesis. However, by the existing quantum circuit synthesis develo…
I will give an overview of what I see as some of the most important future directions in the theory of fault-tolerant quantum computation. In particular, I will give a brief summary of the major problems that need to be solved in fault tolerance based on low-density parity check codes and in hardware-specific fault tolerance. I will then conclude with a discussion of a possible new paradigm for designing fault-tolerant protocols based on a space-time picture of quantum circuits.
As far as we know, a useful quantum computer will require fault-tolerant gates, and existing schemes demand a prohibitively large space and time overhead. We argue that a first generation quantum computer will be very valuable to design, test, and optimize fault-tolerant protocols tailored to the noise processes of the hardware. Our argument is essentially a critical analysis of the current methods envisioned to optimize fault-tolerant schemes, which rely on hardware characterization, noise modelling, and numerical simulations. We show that, even within a very restricted set of noise models, e…
A method for the implementation of a universal set of fault-tolerant logical gates is presented using homological product codes. In particular, it is shown that one can fault-tolerantly map between different encoded representations of a given logical state, enabling the application of different classes of transversal gates belonging to the underlying quantum codes. This allows for the circumvention of no-go results pertaining to universal sets of transversal gates and provides a general scheme for fault-tolerant computation while keeping the stabilizer generators of the code sparse.
A Flexible GKP-State-Embedded Fault-Tolerant Quantum Computation Configuration Based on a Three-Dimensional Cluster State
Shanxi University（山西大学）；State Key Laboratory of Quantum Optics Technologies and Devices, Shanxi University（量子光学技术和器件国家重点实验室，山西大学）；College of Physics and Electronic Engineering, Shanxi University（山西大学物理电子工程学院）；Collaborative Innovation Center of Extreme Optics, Shanxi University（山西大学极端光学协同创新中心）
This paper aims to determine the fault tolerant quantum filter and fault detection equation for a class of open quantum systems coupled to a laser field that is subject to stochastic faults. In order to analyze this class of open quantum systems, we propose a quantum-classical Bayesian inference method based on the definition of a so-called quantum-classical conditional expectation. It is shown that the proposed Bayesian inference approach provides a convenient tool to simultaneously derive the fault tolerant quantum filter and the fault detection equation for this class of open quantum system…
Comment on "Resilient Quantum Computation in Correlated Environments: A Quantum Phase Transition Perspective" and "Fault-tolerant Quantum Computation with Longe-range Correlated Noise"
Quantum error correction protects fragile quantum information by encoding it into a larger quantum system. These extra degrees of freedom enable the detection and correction of errors, but also increase the operational complexity of the encoded logical qubit. Fault-tolerant circuits contain the spread of errors while operating the logical qubit, and are essential for realizing error suppression in practice. While fault-tolerant design works in principle, it has not previously been demonstrated in an error-corrected physical system with native noise characteristics. In this work, we experimenta…
Flag qubits have recently been proposed in syndrome extraction circuits to detect high-weight errors arising from fewer faults. The use of flag qubits allows the construction of fault-tolerant protocols with the fewest number of ancillas known to-date. In this work, we prove some critical properties of CSS codes constructed from classical cyclic codes that enable the construction of a flag fault-tolerant error correction scheme. We then develop fault-tolerant protocols as well as a family of circuits for flag fault-tolerant error correction and operator measurement, requiring only four ancilla…
A major challenge in practical quantum computation is the ineludible errors caused by the interaction of quantum systems with their environment. Fault-tolerant schemes, in which logical qubits are encoded by several physical qubits, enable correct output of logical qubits under the presence of errors. However, strict requirements to encode qubits and operators render the implementation of a full fault-tolerant computation challenging even for the achievable noisy intermediate-scale quantum technology. Here, we experimentally demonstrate the existence of the threshold in a special fault-toleran…
Constant-space-overhead fault-tolerant quantum input/output and communication
Institute for Quantum Computing and Department of Combinatorics and Optimization, University of Waterloo（滑铁卢大学量子计算研究所与组合优化系）；Department of Computer Science, Graduate School of Information Science and Technology, The University of Tokyo（东京大学信息理工学研究科计算机科学系）
We study fault-tolerant error correction in a quantum memory constructed as a two-dimensional model of Fibonacci anyons on a torus, in the presence of thermal noise represented by pair-creation processes and measurement errors. The correction procedure is based on the cellular automaton decoders originating in the works of Gács and Harrington. Through numerical simulations, we observe that this code behaves fault-tolerantly and that threshold behavior is likely present. Hence, we provide strong evidence for the existence of a fault-tolerant universal non-Abelian topological quantum computer.
An important approach to the fault-tolerant quantum computation is protecting the logical information using the quantum error correction. Usually, the logical information is in the form of logical qubits, which are encoded in physical qubits using quantum error correction codes. Compared with the qubit quantum computation, the fermionic quantum computation has advantages in quantum simulations of fermionic systems, e.g. molecules. In this paper, we show that the fermionic quantum computation can be universal and fault-tolerant if we encode logical Majorana fermions in physical Majorana fermion…
A Three-Layer Architecture for Fault-Tolerant Quantum Computing
Center on Frontiers of Computing Studies, Peking University（前沿计算研究中心，北京大学）；School of Computer Science, Peking University（计算机学院，北京大学）；Graduate School of China Academy of Engineering Physics（中国工程物理研究院研究生院）
The purpose of this paper is to solve a fault tolerant filtering and fault detection problem for a class of open quantum systems driven by a continuous-mode bosonic input field in single photon states when the systems are subject to stochastic faults. Optimal estimates of both the system observables and the fault process are simultaneously calculated and characterized by a set of coupled recursive quantum stochastic differential equations.
Robust quantum computation requires encoding delicate quantum information into degrees of freedom that are hard for the environment to change. Quantum encodings have been demonstrated in many physical systems by observing and correcting storage errors, but applications require not just storing information; we must accurately compute even with faulty operations. The theory of fault-tolerant quantum computing illuminates a way forward by providing a foundation and collection of techniques for limiting the spread of errors. Here we implement one of the smallest quantum codes in a five-qubit super…
The quantum logic gates used in the design of a quantum computer should be both universal, meaning arbitrary quantum computations can be performed, and fault-tolerant, meaning the gates keep errors from cascading out of control. A number of no-go theorems constrain the ways in which a set of fault-tolerant logic gates can be universal. These theorems are very restrictive, and conventional wisdom holds that a universal fault-tolerant logic gate set cannot be implemented natively, requiring us to use costly distillation procedures for quantum computation. Here, we present a general framework for…
