Dielectric metasurfaces operating at quasi-bound states in the continuum (qBICs) can achieve exceptionally high radiative quality ($\textit{Q}$) factors by introducing small asymmetries into their unit cells. However, fabrication imperfections often impose major limitations on the experimentally observed $\textit{Q}$ factors. In this study, we experimentally demonstrate BIC metasurfaces with a record-high $\textit{Q}$ factor of 101,486 under normal excitation of light in the telecom wavelength range achieved by employing low-contrast silicon pairs. Our findings show that such ultrahigh-$\textit{Q}$ factors can be attained by leveraging both the high radiative $\textit{Q}$ factors of higher-order qBIC modes and reduced scattering losses in shallow-etched designs. Additionally, we demonstrate stable sub-picometer-level wavelength fluctuations in water, with a limit of detection of $10^{-5}$ for environmental refractive index changes. The proposed approach can be extended to BIC metasurfaces with many other configurations and operating wavelengths for ultrahigh-$\textit{Q}$ applications in both fundamental physics and advanced devices.
Bound states in the continuum (BICs) have attracted much attention in recent years due to the infinite quality factor (Q-factor) resonance and extremely localized field. In this study, BICs have been demonstrated by dielectric metasurfaces with hybrid surface lattice resonance (SLR) in the experiment. By breaking the symmetry of geometry, SLR can be easily switched between BICs and quasi-BICs. Comparing with literature, switching between BICs and quasi-BICs is usually accompanied by wavelength shift. Here, a design rule is proposed to prevent the wavelength shift when the Q-factor is changing.…
We demonstrate that rotationally symmetric chiral metasurfaces can support arbitrarily sharp resonances with the maximum optical chirality determined by precise shaping of bound states in the continuum (BICs). Being uncoupled from one circular polarisation of light and resonantly coupled to its counterpart, a metasurface hosting the chiral BIC resonance exhibits a narrow peak in the circular dichroism spectrum. We propose a realization of such chiral BIC metasurfaces based on pairs of dielectric bars and validate the concept of maximum chirality by numerical simulations
In this paper, we present a Bound states in the continuum (BIC) metamaterial in heterogeneous structures based on the universal coupled mode theory. We find the more general physical parameters to represent BIC, which are the resonant frequencies and corresponding phases of metamaterial structures. Therefore, BIC metamaterial comes from the equal value of the resonant frequencies and phases of metamaterial structures which are not only for homogeneous structures. Meanwhile if slightly vary one of metamaterial structure's resonant frequency and phase by varying geometry, we can obtain the quasi…
Bound states in the continuum (BICs) emerge throughout Physics as leaky/resonant modes that remain however highly localized. They have attracted much attention in Optics and Photonics, and especially in metasurfaces, i.e. planar arrays of sub-wavelength meta-atoms. One of their most outstanding feature is the arbitrarily large Q-factors they induce upon approaching the BIC condition, which we exploit here to achieve a narrow transparency band. We first show how to shift a canonical BIC in an all-dielectric metasurface, consisting of high-refractive disks exhibiting in- and out-of-plane magneti…
Fano resonance has raised great attention in nanophotonics attributing to its unique properties.In this work, we study the imaging function of Fano-resonant silicon metasurfece governed by quasi-bound states in the continuum (BICs). First, by breaking the in-plane symmetry of nanodisks, a symmetry-protected quasi-BIC is excited with the emergence of a sharp Fano resonance. The near field distributions, multipole contributions and radiation patterns of the metasurface are performed to uncover the mechanism and characteristics of this resonance. In addition, we investigate the imaging function o…
Metasurface-mediated bound states in the continuum (BIC) provides a versatile platform for light manipulation at subwavelength dimension with diverging radiative quality factor and extreme optical localization. In this work, we employ magnetic dipole quasi-BIC resonance in asymmetric silicon nanobar metasurfaces to realize giant Goos-Hänchen (GH) shift enhancement by more than three orders of wavelength. In sharp contrast to GH shift based on the Brewster dip or transmission-type resonance, the maximum GH shift here is located at the reflection peak with unity reflectance, which can be conveni…
Dielectric metasurfaces supporting quasi-bound states in the continuum (quasi-BICs) exhibit very high quality factor resonances and electric field confinement. However, accessing the high-Q end of the quasi-BIC regime usually requires marginally distorting the metasurface design from a BIC condition, pushing the needed nanoscale fabrication precision to the limit. This work introduces a novel concept for generating high-Q quasi-BICs, which strongly relaxes this requirement by incorporating a relatively large perturbative element close to high-symmetry points of an undistorted BIC metasurface, …
Broad-angle photon-pair generation from flatband quasi-BIC resonant 3R-MoS$_{2}$ metasurfaces
Nanchang University（南昌大学）；Institute for Advanced Study, Nanchang University（南昌大学高等研究院）；National Laboratory of Solid-State Microstructures and College of Engineering and Applied Sciences, Nanjing University（南京大学固体微结构物理国家级实验室与工程应用学院）
We use numerical simulations to demonstrate third-harmonic generation with near-unity nonlinear circular dichroism (CD) and high conversion efficiency ($ 10^{-2}\ \text{W}^{-2}$) in asymmetric Si-on-SiO$_2$ metasurfaces. The working principle relies on the selective excitation of a quasi-bound state in the continuum, characterized by a very high ($>10^5$) quality-factor. By tuning multi-mode interference with the variation of the metasurface geometrical parameters, we show the possibility of independent control of linear CD and nonlinear CD. Our results pave the way for the development of all-…
Fingerprint spectral response of several materials with terahertz electromagnetic radiation indicates that terahertz technology is an effective tool for sensing applications. However, sensing few nanometer thin-film of dielectrics with much longer terahertz waves (1 THz = 0.3 mm) is challenging. Here, we demonstrate a quasi-bound state in the continuum (BIC) resonance for sensing of nanometer scale thin analyte deposited on a flexible metasurface. The large sensitivity originates from strong local field confinement of the quasi-BIC Fano resonance state and extremely low absorption loss of a lo…
The concept of optical bound states in the continuum (BICs) underpins the existence of strongly localized waves embedded into the radiation spectrum that can enhance the electromagnetic fields in subwavelength photonic structures. Early studies of optical BICs in waveguides and photonic crystals uncovered their topological properties, and the concept of quasi-BIC metasurfaces facilitated applications of strong light-matter interactions to biosensing, lasing, and low-order nonlinear processes. Here we employ BIC-empowered dielectric metasurfaces to generate efficiently high optical harmonics up…
Substrate-engineered tunable bound states in the continuum and directional radiation in dielectric metasurfaces
Neijiang Normal University（内江师范学院）；Neijiang Optoelectronic Devices Engineering Research Center（内江光电器件工程研究中心）；Shenzhen University（深圳大学）；Great Bay University（大湾区大学）；Chongqing University（重庆大学）
Terahertz (THz) chirality pursues customizable manipulation from narrowband to broadband. While conventional THz chirality is restricted by non-negligible linewidth and unable to handle narrowband well. Recently, the concept "quasi bound states in continuum" (quasi-BIC) is introduced to optics resonance system whose the quality factor can be extremely high with the ultra-low radiative loss, thus providing a conceptual feasibility for wave control with ultra-narrow linewidth. Herein, we construct quasi-BIC in a planar all-silicon THz metasurface with in-plane C2 and mirror symmetries breaking. …
The emerging all-dielectric platform exhibits high-quality ($Q$) resonances governed by the physics of bound states in the continuum (BIC) that drives highly efficient nonlinear optical processes. Here we demonstrate the robust enhancement of third-(THG) and fifth-harmonic generation (FHG) from all-dielectric metasurfaces composed of four silicon nanodisks. Through the symmetry breaking, the genuine BIC transforms into the high-$Q$ quasi-BIC resonance with tight field confinement for record high THG efficiency of $3.9\times10^{-4}$ W$^{-2}$ and FHG efficiency of $4.8\times10^{-10}$ W$^{-4}$ us…
Exciton-polaritons are mixed light-matter excitations that result from the strong coupling regime between an active excitonic material and photonic resonances. Harnessing these hybrid excitations provides a rich playground to explore fascinating fundamental features, such as out-of-equilibrium Bose-Einstein condensation and quantum fluids of light, as well as novel mechanisms to be exploited in optoelectronic devices. Here, we investigate experimentally the formation of exciton-polaritons arising from the mixing between hybrid inorganic-organic perovskite excitons and an optical Bound state In…
Bound states in the continuum (BICs) have exhibited extraordinary properties in photonics for enhanced light-matter interactions that enable appealing applications in nonlinear optics, biosensors, and ultrafast optical switches. The most common strategy to apply BICs in a metasurface is by breaking symmetry of resonators in the uniform array that leaks the otherwise uncoupled mode to free space and exhibits an inverse quadratic relationship between quality factor (Q) and asymmetry. Here, we propose a scheme to further reduce scattering losses and improve the robustness of symmetry-protected BI…
Dynamically reconfigurable metasurfaces promise compact and lightweight spatial light modulation for many applications, including LiDAR, AR/VR, and LiFi systems. Here, we design and computationally investigate high quality factor silicon-on-lithium niobate metasurfaces with electrically-driven, independent control of its constituent nanobars for full phase tunability with high tuning efficiency. Free-space light couples to guided modes within each nanobar via periodic perturbations, generating quality factors exceeding 30,000, while maintaining bar spacing <$λ$/1.5. We achieve nearly 2$π$ phas…
Nonlinear metasurface holography shows the great potential of metasurfaces to control the phase, amplitude, and polarization of light while simultaneously converting the frequency of the light. The possibility of tailoring the scattering properties of a coherent beam, as well as the scattering properties of nonlinear signals originating from the meta-atoms facilitates a huge degree of freedom in beam shaping application. Recently, several approaches showed that virtual objects or any kind of optical information can be generated at a wavelength different from the laser input beam. Here, we demo…
We discuss the recent advances in meta-optics and nanophotonics associated with the physics of bound states in the continuum (BICs). Such resonant states appear due to a strong coupling between leaky modes in optical guiding structures being supported by subwavelength high-index dielectric Mie-resonant nanoantennas or all-dielectric metasurfaces. First, we review briefly very recent developments in the BIC physics in application to isolated subwavelength particles. We pay a special attention to novel opportunities for nonlinear nanophotonics due to the large field enhancement inside the partic…
Recent progress in nanophotonics is driven by the desire to engineer light-matter interaction in two-dimensional (2D) materials using high-quality resonances in plasmonic and dielectric structures. Here, we demonstrate a link between the radiation control at critical coupling and the metasurface-based bound states in the continuum (BIC) physics, and develop a generalized theory to engineer light absorption of 2D materials in coupling resonance metasurfaces. In a typical example of hybrid graphene-dielectric metasurfaces, we present the manipulation of absorption bandwidth by more than one orde…
We present nonlinear optical four-wave mixing in a silicon nanodisk dimer metasurface. Under the oblique incident plane waves, the designed metasurface exhibits a multi-resonant feature with simultaneous excitations of three quasi-bound states in the continuum (BIC). Through employing these quasi-BICs with maximizing electric field energy at the input bump wavelengths, significant enhancement of third-order nonlinear processes including third-harmonic generation, degenerate and non-degenerate four-wave mixing are demonstrated, giving rise to ten new frequencies in the visible wavelengths. This…
Optical metasurfaces with high-Q chiral resonances can boost light-matter interaction for various applications of chiral response for ultrathin, active, and nonlinear metadevices. Usually, such metasurfaces require sophisticated depth-resolved nanofabrication to realize subwavelength stereo-nanostructures, posing overwhelming challenges, especially in the short-wavelength range. Here, we suggest a novel planar design for chiral metasurfaces supporting bound states in the continuum (BICs) and demonstrate experimentally chiroptical responses with record-high Q-factors (Q=390) and near-perfect ci…
Tailoring optical nonlinear effects (e.g. harmonic generation, sum-frequency mixing, etc.) in the recently emerging all-dielectric platform is important for both the fundamental science and industrial development of high-efficiency, ultrafast, and miniaturized photonic devices. In this work, we propose a novel paradigm for dynamically switchable high-harmonic generation in Silicon nanodimer metasurfaces by exploiting polarization-controlled dual bound states in the continuum (BIC). Owing to the high-quality factor of BIC resonances, efficient harmonic signals including the third-harmonic gener…
