Nonperturbative Nonlinear Transport in a Floquet-Weyl Semimetal
Matthew W. Day, Kateryna Kusyak, Felix Sturm, Juan I. Aranzadi, Hope M. Bretscher, Michael Fechner, Toru Matsuyama, Marios H. Michael, Benedikt F. Schulte, Xiny… 展开作者
Matthew W. Day, Kateryna Kusyak, Felix Sturm, Juan I. Aranzadi, Hope M. Bretscher, Michael Fechner, Toru Matsuyama, Marios H. Michael, Benedikt F. Schulte, Xinyu Li, Jesse Hagelstein, Dorothee Herrmann, Gunda Kipp, Alex M. Potts, Jonathan M. DeStefano, Chaowei Hu, Yunfei Huang, Takashi Taniguchi, Kenji Watanabe, Guido Meier, Dongbin Shin, Angel Rubio, Jiun-Haw Chu, Dante M. Kennes, Michael A. Sentef, James W. McIver
Periodic laser driving, known as Floquet engineering, is a powerful tool to manipulate the properties of quantum materials. Using circularly polarized light, artificial magnetic fields, called Berry curvature, can be created in the photon-dressed Floquet-Bloch states that form. This mechanism, when applied to 3D Dirac and Weyl systems, is predicted to lead to photon-dressed movement of Weyl nodes which should be detectable in the transport sector. The transport response of such a topological light-matter hybrid, however, remains experimentally unknown. Here, we report on the transport properties of the type-II Weyl semimetal T$\mathrm{_d}$-MoTe$_\mathrm{2}$ illuminated by a femtosecond pulse of circularly polarized light. Using an ultrafast optoelectronic device architecture, we observed injection currents and a helicity-dependent anomalous Hall effect whose scaling with laser field strongly deviate from the perturbative laws of nonlinear optics. We show using Floquet theory that this discovery corresponds to the formation of a magnetic Floquet-Weyl semimetal state. Numerical ab initio simulations support this interpretation, indicating that the light-induced motion of the Weyl nodes contributes substantially to the measured transport signals. This work demonstrates the ability to generate large effective magnetic fields ($>$ 30T) with light, which can be used to manipulate the magnetic and topological properties of a range of quantum materials.
We propose that a Floquet Weyl semimetal state can be induced in three-dimensional topological insulators, either nonmagnetic or magnetic, by the application of off-resonant light. The virtual photon processes play a critical role in renormalizing the Dirac mass and so resulting in a topological semimetal with vanishing gap at Weyl points. The present mechanism via off-resonant light is quite different from that via on-resonant light, the latter being recently suggested to give rise to a Floquet topological state in ordinary band insulators.
We study the photoresponse of two-dimensional semi-Dirac semimetals and three-dimensional Dirac semimetals to off-resonant circularly polarized light. For two-dimensional semi-Dirac semimetals we find that incident light does not open a gap in the spectrum, in contrast to the case of purely linear dispersion. For the three-dimensional case we find that applying a circularly polarized light, one can tune from a trivial insulator to three-dimensional Dirac semimetal with an inverted gap. We propose and show that application of light leads to an intriguing platform for generation, motion and merg…
Weyl points with monopole charge $\pm 1$ have been extensively studied, however, real materials of multi-Weyl points, whose monopole charges are higher than $1$, have yet to be found. In this Rapid Communication, we show that nodal-line semimetals with nontrivial line connectivity provide natural platforms for realizing Floquet multi-Weyl points. In particular, we show that driving crossing nodal lines by circularly polarized light generates double-Weyl points. Furthermore, we show that monopole combination and annihilation can be observed in crossing-nodal-line semimetals and nodal-chain semi…
Floquet engineering, the concept of tailoring a system by a periodic drive, is increasingly exploited to design and manipulate topological phases of matter. In this work, we study periodically driven higher-order topological Dirac semimetals associated with a $k$-dependent quantized quadrupole moment by applying circularly polarized light. The undriven Dirac semimetals feature gapless higher-order hinge Fermi arc states which are the consequence of the higher-order topology of the Dirac nodes. Floquet Weyl semimetal phases with hybrid-order topology, characterized by both a $k$-dependent quant…
When a Dirac semimetal is subject to a circularly polarized laser, it is predicted that the Dirac cone splits into two Weyl nodes and a nonequilibrium transient state called the Floquet Weyl semimetal is realized. We focus on the previously unexplored low-frequency regime, where the upper and lower Dirac bands resonantly couple with each other through multi-photon processes, which is a realistic situation in solid state ultrafast pump-probe experiments. We find a series of new Weyl nodes emerging in pairs when the Floquet replica bands hybridize with each other. The nature of the Floquet Weyl …
Exotic topological states of matter such as Floquet topological insulator or Floquet Weyl semimetal can be induced by periodic driving. This work proposes a Floquet semimetal with Floquet-band holonomy. That is, the system is gapless, but as a periodic parameter viewed as quasimomentum of a synthetic dimension completes an adiabatic cycle, each Floquet band as a whole exchanges with other Floquet bands. The dynamical manifestations of such Floquet-band holonomy are studied. Under open boundary conditions, we discover anomalous chiral edge modes localized only at one edge, winding around the en…
Type-II Weyl semimetals have recently attracted intensive research interest because they host Lorentz-violating massless fermions as quasiparticles. The discovery of type-II Weyl semimetals evokes the study of type-II line-node semimetals (LNSMs) whose linear dispersion is strongly tilted near the nodal ring. We present here a study on the circularly polarized light-induced Floquet states in type-II LNSMs, as well as those in hybrid LNSMs that have a partially over-tilted linear dispersion in the vicinity of the nodal ring. We illustrate that two distinct types of Floquet Weyl semimetal (WSM) …
The Weyl semimetal exhibits various interesting physical phenomena because of the Weyl points, i.e., linear band-crossings. We show by Floquet theory that a linearly polarized light applied to a band insulator can induce controllable Weyl points. In a tight-binding model, we classify different types of photoinduced Weyl points that lead to a rich phase diagram characterized by the Chern number defined on each momentum slices of the bulk states. Taking account of the nonequilibrium electron distribution, we calculate and explain the nonmonotonous anomalous Hall conductivity in terms of the ligh…
It is generally believed that non-Hermiticity can transform Weyl semimetals into Weyl-exceptional-ring semimetals. However, this belief is from the systems without skin effect. We investigate the non-Hermitian Weyl semimental and its Floquet engineering in a system with skin effect, which breaks the bulk-boundary correspondence in its Hermitian counterpart. It is found in both the static and periodically driven cases that the skin effect makes this general belief no longer valid. We discover that exotic non-Hermitian topological matters, e.g., a composite phase of Weyl semimetal and topologica…
We consider tunneling of quasiparticles through a rectangular quantum well, subject to periodic driving. The quasiparticles are the itinerant charges in two-dimensional and three-dimensional semimetals having a quadratic band-touching (QBT) point in the Brillouin zone. In order to analyze the time-periodic Hamiltonian, we assume a non-adiabatic limit, where the Floquet theorem is applicable. By deriving the Floquet scattering matrices, we chalk out the transmission and shot noise spectra of the QBT semimetals. The spectra show Fano resonances, which we identify with the (quasi)bound states of …
We investigate the effects of periodic fields and disorder on topological properties of a Weyl-semimetal thin film. The two periodic fields, i.e., a periodic magnetic field and elliptically polarized light, are discussed respectively. By use of the Floquet theory, we find that both the two periodic drives can resonantly induce the topological transitions from normal insulator (NI) phases to Floquet topological insulator (FTI) phases. The Floquet topological transitions are characterized by variation of Chern number. Moreover, we show that the Floquet topological transitions can be explained by…
Weyl semimetals and nodal line semimetals are characterized by linear electronic bands touching at zero-dimensional points and one-dimensional lines, respectively. Recently, it has been predicted that nodal line semimetals can be driven into tunable Floquet-Weyl semimetals by circularly polarized light. Here, we study the occurrence of interface states between two regions of a nodal line semimetal shined by two beams of light with opposite circular polarizations. Within a minimal model, we find remarkable modifications of the energy structure by tuning the polarized light, such as the possible…
This work reports the general design and characterization of two exotic, anomalous nonequilibrium topological phases. In equilibrium systems, the Weyl nodes or the crossing points of nodal lines may become the transition points between higher-order and first-order topological phases defined on two-dimensional slices, thus featuring both hinge Fermi arc and surface Fermi arc. We advance this concept by presenting a strategy to obtain, using time-sequenced normal insulator phases only, Floquet higher-order Weyl semimetals and Floquet higher-order nexus semimetals, where the concerned topological…
Band crossings observed in a wide range of condensed matter systems are recognized as a key to understand low-energy fermionic excitations that behave as massless Dirac particles. Despite rapid progress in this field, the exploration of non-equilibrium topological states remains scarce and it has potential ability of providing a new platform to create unexpected massless Dirac states. Here we show that in a semiconductor quantum-well driven by a cw-laser with linear polarization, the optical Stark effect conducts bulk-band crossing, and the resulting Floquet-Dirac semimetallic phase supports a…
Multi-Weyl semimetals(m-WSMS) are characterized by anisotropic non-linear energy dispersion along 2-D plane and a linear dispersion in orthogonal direction. They have topological charge J and are realized when two or multiple Weyl nodes with nonzero net monopole charge bring together onto a high-symmetry point. The model Hamiltonians of such systems show various phases such as trivial normal insulators (NIs), WSMs and quantum anomalous Hall(QAH) states depending on the model parameters. We study a periodic driving of such Hamiltonians in trivial NI phase by circularly polarized light and shows…
Floquet states can be realized in quantum systems driven by continuous time-periodic perturbations. It is known that a state known as the Floquet Weyl semimetal can be realized when free Dirac fermions are placed in a rotating electric field. What will happen if strong interaction is introduced to this system? Will the interaction wash out the characteristic features of Weyl semimetals such as the Hall response? Is there a steady state and what is its thermodynamic behavior? We answer these questions using AdS/CFT correspondence in the $\mathcal{N}=2$ supersymmetric massless QCD in a rotating …
In mesoscopic physics, the application of a time-periodic drive leads to novel transport behaviour, which is absent in the static regimes. Here we consider a quantum pumping protocol, such that the quasiparticles of Weyl/multi-Weyl and nodal-line semimetals are subjected to a time-periodic rectangular potential well. The presence of an oscillating potential of frequency $ω$ creates equispaced Floquet side-bands with spacing $\hbar ω$. As a result, a Fano resonance is observed when the difference in the Fermi energy (i.e., the energy of the incident quasiparticle), and the energy of one of the …
Due to studies in nonequilibrium (periodically-driven) topological matter, it is now understood that some topological invariants used to classify equilibrium states of matter do not suffice to describe their nonequilibrium counterparts. Indeed, in Floquet systems the additional gap arising from the periodicity of the quasienergy Brillouin zone often leads to unique topological phenomena without equilibrium analogues. In the context of Floquet Weyl semimetal, Weyl points may be induced at both quasienergy zero and $π/T$ ($T$ being the driving period) and these two types of Weyl points can be ve…
Recent discoveries on topological characterization of gapless systems have attracted interest in both theoretical studies and experimental realizations. Examples of such gapless topological phases are Weyl semimetals, which exhibit 3D Dirac cones (Weyl points), and nodal line semimetals, which are characterized by line nodes (two bands touching along a line). Inspired by our previous discoveries that the kicked Harper model exhibits many fascinating features of Floquet topological phases, in this manuscript we consider a generalization of the model, where two additional periodic system paramet…
Weyl semimetal, a three-dimensional electronic system with relativistic linear energy dispersion around gapless points carrying nontrivial Berry charge, is predicted to exhibit a wealth of unique response and transport properties.A crucial question is whether those properties are robust against disorder and whether Anderson localization occurs.In this work, the effects of nonperturbative topological (vortex loop) excitations and Berry phase in disordered time-reversal invariant 3d Weyl semimetal are studied.It is shown that the chiral symmetry is restored in the nonlinear sigma model describin…
Simulating multi-node Weyl semimetals in a Mixed Floquet lattice
Indian Institute of Science Education and Research (IISER) Tirupati（印度科学教育研究所提鲁帕蒂分校）；Indian Institute of Science Education and Research Bhopal（印度科学教育研究所博帕尔分校）
Valence and conduction bands in nodal loop semimetals (NLSMs) touch along closed loops in momentum space. If such loops can proliferate and link intricately, NLSMs become exotic topological phases with unconventional topological characteristics and potentially peculiar transport properties. In conventional quantum materials or cold atom systems alike, such exotic phases necessarily require non-local hopping and are therefore intrinsically unrealistic. In this work, we show how this hurdle can be surmounted through an experimentally feasible periodic driving scheme. In particular, by tuning the…
In this paper, we discuss the effect of a periodically driving circularly polarized laser beam in the high frequency limit, on the band structure and thermal transport properties of type-I and type-II Weyl semimetals (WSMs). We develop the notion of an effective Fermi surface stemming from the time-averaged Floquet Hamiltonian and discuss its effects on the steady-state occupation numbers of electrons and holes in the linearized model. In order to compute the transport coefficients averaged over a period of the incident laser source, we employ the Kubo formalism for Floquet states and show tha…
We discuss the circularly polarized light (of amplitude $A_0$ and frequency $ω$) driven thermo-electric transport properties of type-I and type-II multi-Weyl semimetals (mWSMs) in the high frequency limit. Considering the low energy model, we employ the Floquet-Kubo formalism to compute the thermal Hall and Nernst conductivities for both types of mWSMs. We show that the anisotropic nature of the dispersion for arbitrary integer monopole charge $n>1$ plays an important role in determining the effective Fermi surface behavior; interestingly, one can observe momentum dependent corrections in Floq…
We study non-perturbatively the anomalous Hall current and its high harmonics generated in Weyl and Dirac semimetals by strong elliptically polarized laser fields, in the context of kinetic theory. We find a novel crossover between perturbative and non-perturbative regimes characterized by the electric field strength $\mathcal{E}^{*}= \frac{μω}{ 2 e v_F}$ ($ω$: laser frequency, $μ$: Fermi energy, $v_F$: Fermi velocity). In the perturbative regime, the anomalous Hall current quadratically depends on the field strength ($\mathcal{E}$), whereas the higher order corrections, as well as high harmon…
We show that Floquet engineering using bicircular light (BCL) is a versatile way to control magnetic symmetries and topology in materials. The electric field of BCL, which is a superposition of two circularly polarized light waves with frequencies that are integer multiples of each other, traces out a rose pattern in the polarization plane that can be chosen to break selective symmetries, including spatial inversion. Using a realistic low-energy model, we theoretically demonstrate that the three-dimensional Dirac semimetal Cd$_3$As$_2$ is a promising platform for BCL Floquet engineering. Witho…
Creating and manipulating topological states is a key goal of condensed matter physics. Periodic driving offers a powerful method to manipulate electronic states, and even to create topological states in solids. Here, we investigate the tunable Floquet states in a periodically driven higher-order nodal line semimetal with both spatial inversion and time-reversal symmetries. We found that the Floquet Weyl semimetal states, which support both one-dimensional hinge Fermi arc and two-dimensional surface Fermi arc states, can be induced in the higher-order nodal-line semimetal by shining circularly…
Using the Landau-Zener-Stückelberg-Majorana-type (LZSM) semiclassical approach, we study both graphene and a thin film of a Weyl semimetal subjected to a strong AC electromagnetic field. The spectrum of quasi energies in the Weyl semimetal turns out to be similar to that of a graphene sheet. Earlier it has been predicted qualitatively that the transport properties of strongly-irradiated graphene oscillate as a function of the radiation intensity [S.V. Syzranov et al., Phys. Rev. B 88, 241112 (2013)]. Here we obtain rigorous quantitative results for a driven linear conductance of graphene and a…
Weyl semimetals and nodal line semimetals are characterized by linear band touching at zero-dimensional points and one-dimensional lines, respectively. We predict that a circularly polarized light drives nodal line semimetals into Weyl semimetals. The Floquet Weyl points thus obtained are tunable by the incident light, which enables investigations of them in a highly controllable manner. The transition from nodal line semimetals to Weyl semimetals is accompanied by the emergence of a large and tunable anomalous Hall conductivity. Our predictions are experimentally testable by transport measure…
We study the stroboscopic dynamics of hinge modes of a second-order topological material modeled by a tight-binding free fermion Hamiltonian on a cubic lattice in the intermediate drive frequency regime for both discrete (square pulse) and continuous (cosine) periodic drive protocols. We analyze the Floquet phases of this system and show that its quasienergy spectrum becomes almost gapless in the large drive amplitude regime at special drive frequencies. Away from these frequencies, the gapped quasienergy spectrum supports weakly dispersing Floquet hinge modes. Near them, these hinge modes pen…
Semimetals exhibiting nodal lines or nodal surfaces represent a novel class of topological states of matter. While conventional Weyl semimetals exhibit momentum-space Dirac monopoles, these more exotic semimetals can feature unusual topological defects that are analogous to extended monopoles. In this work, we describe a scheme by which nodal rings and nodal spheres can be realized in synthetic quantum matter through well-defined periodic-driving protocols. As a central result of our work, we characterize these nodal defects through the quantum metric, which is a gauge-invariant quantity assoc…
We theoretically study the circularly polarized light-induced Floquet state in line-node semimetals with time-reversal symmetry and inversion symmetry. It is found that the Floquet state can show the photovoltaic anomalous Hall effect when an applied circularly polarized light gaps out the line node in the bulk and leave Weyl point nodes. The Hall conductivity is sensitive to the location of Fermi level: When the Fermi level locates at the node, the Hall conductivity depends on the radius of line node and is nearly independent of the intensity of light. Away from the line node, the Hall conduc…
Graphene exhibits extremely strong optical nonlinearity when a strong perpendicular magnetic field is applied, the response current shows strong field dependence even for moderate light intensity, and the perturbation theory fails. We nonperturbatively calculate full optical conductivities induced by a periodic field in an equation-of-motion framework based on the Floquet theorem, with the scattering described phenomenologically. The nonlinear response at high fields is understood in terms of the dressed electronic states, or Floquet states, which is further characterized by the optical conduc…
Time-periodic driving in the form of coherent radiation provides powerful tool for the manipulation of topological materials or synthetic quantum matter. In this paper we propose a scheme to realize non-Hermitian semimetals exhibiting exceptional rings in the spectra through Floquet engineering. A transition from a concentric pair of the rings to a dipolar pair is observed. The concentric pair carries only a quantized Berry phase while the dipolar pair possesses opposite Chern numbers in addition, signaling a topological Lifshitz transition of the Fermi surface. The transport properties of the…
We study the interaction between elliptically polarized light and a three-dimensional Luttinger semimetal with quadratic band touching using Floquet theory. In the absence of light, the touching bands can have the same or the opposite signs of the curvature; in each case, we show that simply tuning the light parameters allows us to create a zoo of Weyl semimetallic phases. In particular, we find that double and single Weyl points can coexist at different energies, and they can be tuned to be type I or type II. We also find an unusual phase transition, in which a pair of Weyl nodes form at fini…
Periodically driven systems provide tunable platforms to realize interesting Floquet topological phases and phase transitions. In electronic systems with Weyl dispersions, the band crossings are topologically protected even in the presence of time-periodic perturbations. This robustness permits various routes to shift and tilt the Weyl spectra in the momentum and energy space using circularly polarized light of sufficient intensity. We show that type-II Weyl fermions, in which the Weyl dispersions are tilted with the appearance of pocket-like Fermi surfaces, can be induced in driven Dirac semi…
We investigate the development of novel surface states when 3D Dirac or Weyl semimetals are placed under circularly polarized electromagnetic radiation. We find that the hybridization between inverted Floquet bands opens in general a gap, which closes at so-called exceptional points found for complex values of the momentum. This corresponds to the appearance of midgap surface states in the form of evanescent waves decaying from the surface exposed to the radiation. We observe a phenomenon reminiscent of Landau quantization by which the midgap surface states get a large degeneracy proportional …
We study the topological properties of 3D Floquet bandstructures, which are defined using unitary evolution matrices rather than Hamiltonians. Previously, 2D bandstructures of this sort have been shown to exhibit anomalous topological behaviors, such as topologically-nontrivial zero-Chern-number phases. We show that the bandstructure of a 3D network model can exhibit Weyl phases, which feature "Fermi arc" surface states like those found in Weyl semimetals. Tuning the network's coupling parameters can induce transitions between Weyl phases and various topologically distinct gapped phases. We id…
The Floquet spectrum in an anisotropic tilted Dirac semimetal modulated by linearly polarized light is addressed through the solution of the time-dependent Schrödinger equation for the two-dimensional Dirac Hamiltonian via the Floquet theorem. The time-dependent wave functions and the quasienergy spectrum of the two-dimensional Dirac Hamiltonian under the normal incidence of linearly polarized waves are obtained for an arbitrarily intense electromagnetic radiation. We applied a set of unitary transformations to reduce the Schrödinger equation to an ordinary second-order differential Hill equat…
By making use of a low-energy effective model of Weyl semimetals, we show that the Fermi arc transport is dissipative. The origin of the dissipation is the scattering of the surface Fermi arc states into the bulk of the semimetal. It is noticeable that corresponding scattering rate is nonzero and can be estimated even in a perturbative theory, although in general the reliable calculations of transport properties necessitate a nonperturbative approach. Nondecoupling of the surface and bulk sectors in the low-energy theory of Weyl semimetals invalidates the usual argument of a nondissipative tra…
