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arXiv 2409.03415cond-mat.mtrl-sci
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磁性隧道结中交变磁(altermagnetic)势垒的各向异性自旋过滤

Anisotropic spin filtering by an altermagnetic barrier in magnetic tunnel junctions

Boyuan Chi, Leina Jiang, Yu Zhu, Guoqiang Yu, Caihua Wan, Xiufeng Han

AI总结:

本文通过第一性原理计算揭示FeF$_2$的方向依赖自旋过滤效应,并据此设计两种ALM势垒MTJ,获得216%和3956%的TMR比。

摘要:

自旋过滤效应,即反向自旋极化电子在磁性势垒中经历不同衰减长度的现象,通常发生在铁磁(FM)绝缘体或半导体中。随着交变磁(ALM)材料的兴起——这类材料具有与铁磁体相似的电子自旋极化能力——ALM绝缘体或半导体是否也能充当自旋分裂效应的独特势垒,便成为一个自然的问题。本文通过第一性原理计算,研究了ALM绝缘体FeF$_2$的复能带结构,发现其具有各向异性自旋过滤效应:沿FeF$_2$的[001]方向,电流保持自旋中性,但在动量空间中具有局部非零的自旋极化;此外,沿FeF$_2$的[110]方向,反向自旋极化电子因不同的衰减长度而使电流发生全局自旋极化。利用这种各向异性自旋过滤效应,我们设计了两类以ALM为势垒的MTJ:ALM电极/ALM绝缘势垒/非磁(NM)电极,以及FM电极/ALM绝缘势垒/NM电极,并分别以RuO$_2$(001)/FeF$_2$/IrO$_2$和CrO$_2$(110)/FeF$_2$/IrO$_2$作为相应原型。我们发现,通过在动量空间中匹配电极的导电通道与势垒的自旋分辨最低衰减率,所提出的两种MTJ分别表现出216%和3956%的隧道磁电阻(TMR)比。本工作深化并推广了对新兴ALM绝缘体和半导体中自旋过滤效应的理解,并拓宽了AFM自旋电子学的应用。

英文摘要:

The spin filtering effect, distinct decaying lengths experienced by oppositely spin-polarized electrons in a magnetic barrier, generally occurs in ferromagnetic (FM) insulators or semiconductors. With the rise of altermagnetic (ALM) materials which exhibit similar capability of spin-polarizing electrons with ferromagnets, it is a nature question whether the ALM insulators or semiconductors can also act as unique barriers for the spin splitting effect. Here, through first-principles calculations, we investigated the complex band structure of the ALM insulator FeF$_2$ and found that it possesses an anisotropic spin filtering effect: along the [001] direction of FeF$_2$, a current remains spin-neutral but has locally nonvanishing spin polarizations in the momentum space; moreover, along the [110] direction of FeF$_2$, a current will be globally spin-polarized by different attenuation lengths of oppositely spin-polarized electrons. Leveraging this anisotropic spin filtering effect, we designed two types of MTJs with the ALM barrier: ALM electrode/ALM insulator barrier/non-magnetic (NM) electrode and FM electrode/ALM insulator barrier/NM electrode, using RuO$_2$(001)/FeF$_2$/IrO$_2$ and CrO$_2$(110)/FeF$_2$/IrO$_2$ as the corresponding prototypes, respectively. We found that these two proposed MTJs exhibited the tunneling magnetoresistance (TMR) ratios of 216\% and 3956\%, by matching the conduction channels of the electrodes and the spin-resolved lowest decay rate of the barrier in the momentum space. Our work deepens and generalizes understanding toward the spin filtering effect for the rising ALM insulators and semiconductors, and broadens applications of the AFM spintronics.

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