Learning rheological parameters of non-Newtonian fluids from velocimetry data
Engineering Department, University of Cambridge（剑桥大学工程系）；Materials Science and Engineering Department, University of Sheffield（谢菲尔德大学材料科学与工程系）；School of Medicine and Population Health, Faculty of Health, University of Sheffield（谢菲尔德大学医学院与人口健康学院）；Mechanical & Aerospace Engineering Department, University of Manchester（曼彻斯特大学机械与航空航天工程系）
Alexandros Kontogiannis, Richard Hodgkinson, Emily L. Manchester
We solve a Bayesian inverse Navier-Stokes (N-S) problem that assimilates velocimetry data in order to jointly reconstruct the flow field and learn the unknown N-S parameters. By incorporating a Carreau shear-thinning viscosity model into the N-S problem, we devise an algorithm that learns the most likely Carreau parameters of a shear-thinning fluid, and estimates their uncertainties, from velocimetry data alone. We then conduct a flow-MRI experiment to obtain velocimetry data of an axisymmetric laminar jet through an idealised medical device (FDA nozzle) for a blood analogue fluid. We show that the algorithm can successfully reconstruct the flow field by learning the most likely Carreau parameters, and that the learned parameters are in very good agreement with rheometry measurements. The algorithm accepts any algebraic effective viscosity model, as long as the model is differentiable, and it can be extended to more complicated non-Newtonian fluids (e.g. Oldroyd-B fluid) if a viscoelastic model is incorporated into the N-S problem.
X-ray particle tracking velocimetry for steady-state rheological characterization: Case study of a complex polymer melt flow in material extrusion additive manufacturing
University of Stuttgart（斯图加特大学）；University of Milan（米兰大学）；CNR – Consiglio Nazionale delle Ricerche, Istituto di Chimica della Materia Condensata e di Tecnologie per l’Energia（意大利国家研究委员会凝聚态材料与能源技术研究所）
An Insight into Parameter Identifiability Issues in the Carreau-Yasuda Model: a More Consistent Rheological Formulation for Shear-thinning non-Newtonian Inelastic Fluids
Correlations of friction factors are presented for the general case of purely viscous non-Newtonian fluids without requiring a priori the adoption of a rheological model. They are based on an empirical estimate of the shift in the wall layer edge and the Kolmogorov point. The predictions of friction factors have the same level of accuracy as those of the Dodge-Metzner correlation but the visualisation is more compatible with measured velocity profiles. The general correlations obtained can be used to easily retrieve correlations for specific rheological models.
We propose a unifying mechanism based on the Stribeck curve for the coefficient of friction between the particles to capture the shear thinning - Newtonian plateau - shear thickening - shear thinning rheological behavior at low - intermediate - beyond critical - high shear rates, respectively, for a typical dense non-Brownian suspension. We establish the accuracy of the proposed model by comparing the numerical results with experimental data. The presence of non-DLVO (Derjaguin and Landau, Verwey and Overbeek) forces and a coefficient of friction reducing with asperity deformation explain the …
We investigate through Direct Numerical Simulations (DNS) the statistical properties of turbulent flows in the inertial subrange for non-Newtonian power-law fluids. The structural invariance found for the vortex size distribution is achieved through a self-organized mechanism at the microscopic scale of the turbulent motion that adjusts, according to the rheological properties of the fluid, the ratio between the viscous dissipations inside and outside the vortices. Moreover, the deviations from the K41 theory of the structure functions' exponents reveal that the anomalous scaling exhibits a sy…
Blood is a complex suspension that demonstrates several non-Newtonian rheological characteristics such as deformation-rate dependency, viscoelasticity and yield stress. In this paper we outline some issues related to the non-Newtonian effects in blood circulation system and present modeling approaches based mostly on the past work in this field.
The dynamics of thin films on a horizontal solid substrate is investigated in the case of non-Newtonian fluids exhibiting normal stress differences, the rheology of which is strongly non-linear. Two coupled equations of evolution for the thickness of the film and the shear rate are proposed within the lubrication approximation. This framework is applied to the motion of an advancing contact line. The apparent dynamic contact angle is found to depend logarithmically on a lengthscale determined solely by the rheological properties of the fluid and the velocity of the contact line.
Fluid mechanical peristaltic transport through esophagus has been of concern in the paper. A mathematical model has been developed with an aim to study the peristaltic transport of a rheological fluid for arbitrary wave shapes and tube lengths. The Ostwald-de Waele power law of viscous fluid is considered here to depict the non-Newtonian behaviour of the fluid. The model is formulated and analyzed with the specific aim of exploring some important information concerning the movement of food bolus through the esophagus. The analysis has been carried out by using lubrication theory. The study is …
In the present work a simple kinetic model based on the Enskog equation is solved to get the rheological properties of a hard-disk fluid under shear far from equilibrium, as functions of the density and shear rate. Comparison with Monte Carlo simulations of the Enskog equation show excellent agreement.
This study presents a detailed investigation of how the rheological behaviour of fluid could influence the electrokinetic instability (EKI) phenomenon in a microfluidic T-junction. The non-Newtonian power-law model with different values of the power-law index (n) is used to obtain fluids of different rheological behaviours. We find that as the fluid rheological behaviour changes from shear-thickening (n > 1) to shear-thinning (n < 1) via the Newtonian (n = 1) one, the EKI phenomenon is significantly influenced under the same conditions. In particular, the intensity of this EKI phenomenon is fo…
This work discusses the rheology of several vitreous humour (VH) substitutes used in eye surgery (perfluorocarbons and silicone oils) and their flow behaviour when subjected to saccadic eye movements. Shear rheology experiments revealed that all fluids tested exhibit a constant shear viscosity, while extensional rheological experiments showed that Siluron 2000 is the only fluid tested that exhibits a measurable elasticity. To characterise the dynamics during saccadic eye movements, numerical simulations of all the VH substitutes under study were performed with the open source software OpenFOAM…
In this paper we analyse a problem of a hydraulic fracture driven by a non-Newtonian shear-thinning fluid. For the PKN fracture geometry we consider three different rheological models of fluid: i) the Carreau fluid, ii) the truncated power-law fluid, iii) the power-law fluid. For each of these models a number of simulations are performed. The results are post-processed and compared with each other in order to find decisive factors for similarities/dissimilarities. It is shown that under certain conditions even the basic power-law rheology can be a good substitute for the Carreau characteristic…
We continue our investigation to the use of the variational method to derive flow relations for generalized Newtonian fluids in confined geometries. While in the previous investigations we used the straight circular tube geometry with eight fluid rheological models to demonstrate and establish the variational method, the focus here is on the plane long thin slit geometry using those eight rheological models, namely: Newtonian, power law, Ree-Eyring, Carreau, Cross, Casson, Bingham and Herschel-Bulkley. We demonstrate how the variational principle based on minimizing the total stress in the flo…
Predictive constitutive equations that connect easy-to-measure transport properties (e.g., viscosity and conductivity) with system performance variables (e.g., power consumption and efficiency) are needed to design advanced thermal and electrical systems. In this work, we explore the use of fluorescent particle-streak analysis to directly measure the local velocity field of a pressure-driven flow, introducing a new Python package (FSVPy) to perform the analysis. Fluorescent streak velocimetry (FSV) combines high-speed imaging with highly fluorescent particles to produce images that contain flu…
The present work focuses on the study of mixed convection of a purely viscous shear-thinning fluid in a horizontal annular eccentric duct. The inner and outer cylinders are heated with constant and uniform heat flux densities. The objective of this work is to study the effect of the variation of eccentricity, rheological behavior of the fluid as well as the thermodependency of the rheological parameters on the reorganization of the flow and thermal stratification caused by the buoyancy forces. At the entrance of the heating zone, the dynamic regime is assumed to be established and the temperat…
The aim of this paper is to present a modeling for the rheological behavior of simple liquids as a function of the amplitude of the imposed shear stress or strain. The elastic mode theory (Ref. 6) is first generalized to take into account the fact that during a flow experiment, mechanical energy is injected in a system initially at thermodynamic equilibrium. This generalized theory can be seen as a particular aspect of the general problem of perturbation by the measurement, associated with that of the coupling between fluctuation and dissipation. This generalization leads to a "finitary" chara…
This paper reports experiments on the shear transient response of concentrated non-Brownian suspensions. The shear viscosity of the suspensions is measured using a wide-gap Couette rheometer equipped with a Particle Image Velocimetry (PIV) device that allows measuring the velocity field. The suspensions made of PMMA particles (31$μ$m in diameter) suspended in a Newtonian index- and density-matched liquid are transparent enough to allow an accurate measurement of the local velocity for particle concentrations as high as 50%. In the wide-gap Couette cell, the shear induced particle migration is …
We investigate the possibility that the spatial dependency of stress in generalized Newtonian flow systems is a function of the applied pressure field and the conduit geometry but not of the fluid rheology. This possibility is well established for the case of a one-dimensional flow through simply connected regions, specifically tubes of circular uniform cross sections and plane thin slits. If it can also be established for the more general case of generalized Newtonian flow through non-circular or multiply connected geometries, such as the two-dimensional flow through conduits of rectangular o…
We study the flow of a generalized Newtonian fluid, characterized by a power-law model, through a channel consisting of a wall with a flexible membrane under longitudinal tension. It is assumed that at steady state the flow through the channel admits a constant flux unidirectional flow profile, while for the unsteady case, we employ the long wave approximation and use a set of reduced equations to describe the variation of the shape of the membrane (assumed to be massless and elastic) and the variation of the fluid-flux. By means of asymptotic expansion, multiscale analysis and full numerical …
We analyse a problem of a hydraulic fracture driven by a non-Newtonian shear-thinning fluid. Fluid viscosity is described by the four-parameter truncated power-law model. By varying the parameters of the rheological model we investigate spatial and temporal evolution of fluid flow inside the crack and the resulting fracture geometry. A detailed quantitative and qualitative analysis of the underlying physical phenomena is delivered. The results demonstrate that rheological properties of fluids significantly affect the process of hydraulic fracture not only by the values of viscosity, but also b…
Linear stability of horizontal and inclined stratified channel flows of Newtonian/non-Newtonian shear-thinning fluids is investigated with respect to all wavelength perturbations. The Carreau model has been chosen for the modeling of the rheology of a shear-thinning fluid, owing to its capability to describe properly the constant viscosity limits (Newtonian behavior) at low and high shear rates. The results are presented in the form of stability boundaries on flow pattern maps (with the phases' superficial velocities as coordinates) for several practically important gas-liquid and liquid-liqui…
We investigate the rheological characteristics of human blood plasma in shear and elongational flows. While we can confirm a Newtonian behavior in shear flow within experimental resolution, we find a viscoelastic behavior of blood plasma in the pure extensional flow of a capillary break-up rheometer. The influence of the viscoelasticity of blood plasma on capillary blood flow is tested in a microfluidic device with a contraction-expansion geometry. Differential pressure measurements revealed that the plasma has a pronounced flow resistance compared to that of pure water. Supplementary measurem…
Many microorganisms swim in fluids with complex rheological properties. Although much is now understood about motion of these swimmers in Newtonian fluids, the understanding is still developing in non-Newtonian fluids --- this understanding is crucial for various biomimetic and biomedical applications. Here we study a common model for microswimmers, the squirmer model, in two common viscoelastic fluid models, the Giesekus fluid model and fluids of differential type (grade three), at zero Reynolds number. Through this article we address a recent commentary that discussed suitable values of para…
The motion of a long gas bubble in a confined capillary tube is ubiquitous in a wide range of engineering and biological applications. While the understanding of the deposited thin viscous film near the tube wall in Newtonian fluids is well developed, the deposition dynamics in commonly encountered non-Newtonian fluids remains much less studied. Here, we investigate the dynamics of a confined bubble moving in shear-thinning fluids with systematic experiments, varying the zero-shear-rate capillary number $Ca_0$ in the range of $O(10^{-3}-10^2)$ considering the zero-shear-rate viscosity. The thi…
We present the dynamic velocity profiles of a Newtonian fluid (glycerol) and a viscoelastic Maxwell fluid (CPyCl/NaSal in water) driven by an oscillating pressure gradient in a vertical cylindrical pipe. The frequency range explored has been chosen to include the first three resonance peaks of the dynamic permeability of the viscoelastic fluid / pipe system. Three different optical measurement techniques have been employed. Laser Doppler Anemometry has been used to measure the magnitude of the velocity at the centre of the liquid column. Particle Image Velocimetry and Optical Deflectometry are…
We discuss experimental investigations on steady streaming flows of dilute and semi-dilute polymer solutions in microfluidic devices. The effect of non-Newtonian behavior on steady streaming for different model fluids is determined by characterizing the evolution of the inner streaming layer as a function of oscillation frequency using particle tracking velocimetry. We find that steady streaming velocity profiles in constant-viscosity elastic liquids are qualitatively similar to those in Newtonian liquids. Steady streaming velocity profiles in elastic liquids with strong shear thinning, howeve…
We investigate the effects of helical swimmer shape (i.e., helical pitch angle and tail thickness) on swimming dynamics in a constant viscosity viscoelastic (Boger) fluid via a combination of particle tracking velocimetry, particle image velocimetry and 3D simulations of the FENE-P model. The 3D printed helical swimmer is actuated in a magnetic field using a custom-built rotating Helmholtz coil. Our results indicate that increasing the swimmer tail thickness and pitch angle enhances the normalized swimming speed (i.e., ratio of swimming speed in the Boger fluid to that of the Newtonian fluid).…
Dense suspensions are non-Newtonian fluids which exhibit strong shear thickening and normal stress differences. Using numerical simulation of extensional and shear flows, we investigate how rheological properties are determined by the microstructure which is built under flows and by the interactions between particles. By imposing extensional and shear flows, we can assess the degree of flow-type dependence in regimes below and above thickening. Even when the flow-type dependence is hindered, nondissipative responses, such as normal stress differences, are present and characterise the non-Newto…
We investigate the flow of various non-Newtonian fluids through three-dimensional disordered porous media by direct numerical simulation of momentum transport and continuity equations. Remarkably, our results for power-law (PL) fluids indicate that the flow, when quantified in terms of a properly modified permeability-like index and Reynolds number, can be successfully described by a single (universal) curve over a broad range of Reynolds conditions and power-law exponents. We also study the flow behavior of Bingham fluids described in terms of the Herschel-Bulkley model. In this case, our sim…
Longstanding problems regarding the causality of the diffusion equation are resolved through a class of exact solutions. A universal differential solution for diffusive processes is derived that is causal and exact at any analytic point in the data, albeit infinite order in spatial derivatives. This is true for systems both relativistic and nonrelativistic and shows that the hyperbolic and other relativistic extensions of the heat equation are not valid. A similar effect is demonstrated for flow enhanced mixing of solutions but with a new nonanalytic feature. Viscous hydrodynamics of liquids h…
A large eddy simulation (LES) with an extended Smagorinsky model has been carried to investigate numerically the fully developed turbulent flow of a shear thinning fluid (n=0.75) in a stationary pipe at a simulation's Reynolds number equals to 4000 with a grid resolution of 65 3 gridpoints in axial, radial and circumferential directions and a domain length of 20R. The present study set out to critically evaluate the influence of the Non-Newtonian rheological and hydrodynamic behaviour on the turbulence main features, as well as to ascertain the accuracy and reliability of the laboratory code p…
The problem of buckling and coiling of jets of viscous, Newtonian liquids has received a substantial level of attention over the past two decades, both from experimental and theoretical points of view. Nevertheless, many industrial fluids and consumer products are non-Newtonian, and their rheological properties affect their flow behavior. The present work aims at studying the dynamics of cylindrical jets of a viscoelastic, shear-thinning solution of cetylpyridinium salt (CPyCl). In concentrated solutions, CPyCl surfactant molecules have been shown to assemble in long wormlike micellar structur…
Collinear Swimming of a Squirmer Pair in Newtonian and Shear-Thinning Fluids
Santa Clara University（圣克拉拉大学）；University of Illinois Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；Towson University（陶森大学）；New Jersey Institute of Technology（新泽理工学院）；Texas A&M University–Corpus Christi（德克萨斯农工大学科珀斯克里斯蒂分校）
We experimentally investigate the influence of finite-size spherical particles in turbulent flows of a Newtonian and a drag reducing viscoelastic fluid at varying particle volume fractions and fixed Reynolds number. Experiments are performed in a square duct at a Reynolds number $Re_{2H}$ of nearly $1.1\times10^4$, Weissenberg number $Wi$ for single-phase flow is between 1-2 and results in a drag-reduction of 43% compared to a Newtonian flow (at the same $Re_{2H}$). Particles are almost neutrally-buoyant hydrogel spheres having a density ratio of 1.0035$\pm$0.0003 and a duct height ${2H}$ to p…
We use a generic and general numerical method to obtain solutions for the flow of generalized Newtonian fluids through circular pipes and plane slits. The method, which is simple and robust can produce highly accurate solutions which virtually match any analytical solutions. The method is based on employing the stress, as a function of the pipe radius or slit thickness dimension, combined with the rate of strain function as represented by the fluid rheological constitutive relation that correlates the rate of strain to stress. Nine types of generalized Newtonian fluids are tested in this inves…
Many biological fluids have polymeric microstructures and display non-Newtonian rheology. We take advantage of such nonlinear fluid behavior and combine it with geometrical symmetry-breaking to design a novel small-scale propeller able to move only in complex fluids. Its propulsion characteristics are explored numerically in an Oldroyd-B fluid for finite Deborah numbers while the small Deborah number limit is investigated analytically using a second-order fluid model. We then derive expressions relating the propulsion speed to the rheological properties of the complex fluid, allowing thus to i…
The dynamics of a quasi two-dimensional isotropic droplet in a cholesteric liquid crystal medium under symmetric shear flow is studied by lattice Boltzmann simulations. We consider a geometry in which the flow direction is along the axis of the cholesteric, as this setup exhibits a significant viscoelastic response to external stress. We find that the dynamics depends upon the magnitude of the shear rate, the anchoring strength of the liquid crystal at the droplet interface and the chirality. While for low shear rate and weak interface anchoring the system shows a non-Newtonian behavior, a New…
We study fluid-structure interactions (FSIs) in a long and shallow microchannel, conveying a non-Newtonian fluid, at steady state. The microchannel has a linearly elastic and compliant top wall, while its three other walls are rigid. The fluid flowing inside the microchannel has a shear-dependent viscosity described by the power-law rheological model. We employ lubrication theory to solve for the flow problem inside the long and shallow microchannel. For the structural problem, we employ two plate theories, namely Kirchhoff-Love theory of thin plates and Reissner-Mindlin first-order shear defo…
Many microorganisms find themselves immersed in fluids displaying non-Newtonian rheological properties such as viscoelasticity and shear-thinning viscosity. The effects of viscoelasticity on swimming at low Reynolds numbers have already received considerable attention, but much less is known about swimming in shear-thinning fluids. A general understanding of the fundamental question of how shear-thinning rheology influences swimming still remains elusive. To probe this question further, we study a spherical squirmer in a shear-thinning fluid using a combination of asymptotic analysis and numer…
