arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2407.14481cond-mat.mes-hallcond-mat.mtrl-sci
收藏

EuZn2Sb2中顺磁自旋简并解除的观测

Observation of paramagnetic spin-degeneracy lifting in EuZn2Sb2

Milo X. Sprague, Sabin Regmi, Barun Ghosh, Anup Pradhan Sakhya, Mazharul Islam Mondal, Iftakhar Bin Elius, Nathan Valadez, Bahadur Singh, Tetiana Romanova, Dari… 展开作者

Milo X. Sprague, Sabin Regmi, Barun Ghosh, Anup Pradhan Sakhya, Mazharul Islam Mondal, Iftakhar Bin Elius, Nathan Valadez, Bahadur Singh, Tetiana Romanova, Dariusz Kaczorowski, Arun Bansil, Madhab Neupane

AI总结:

本研究结合高分辨率角分辨光电子能谱和第一性原理计算,在EuZn2Sb2中观测到顺磁相的自旋简并解除,并预测其产生一对Weyl节点,为无长程磁序下时间反演对称破缺物理提供关键进展。

摘要:

时间反演和空间反演对称性共同对晶体中的电子态施加了两重自旋简并。在中心对称材料中,这种简并可以通过引入磁性(无论是通过外部施加的场还是通过内部磁化)来解除。然而,即使在顺磁相中,自旋的相关排列也能解除电子态的自旋简并。在此,我们通过高分辨率角分辨光电子能谱测量与第一性原理计算的结合,报告了对Eu三元磷族化合物EuZn2Sb2电子能带结构的深入研究。对入射光子能量和样品温度范围内光电子线形的分析显示,在顺磁相中存在能带自旋简并解除。我们的ARPES结果与理论铁磁相计算吻合良好,这表明了系统中铁磁涨落的重要性。通过我们的计算,我们预测EuZn2Sb2中的自旋极化能带产生一对Weyl节点。我们在EuZn2Sb2中观测到的能带分裂为实现无长程磁序的时间反演对称破缺物理提供了关键一步。

英文摘要:

Taken together, time-reversal and spatial inversion symmetries impose a two-fold spin degeneracy of the electronic states in crystals. In centrosymmetric materials, this degeneracy can be lifted by introducing magnetism, either via an externally applied field or through internal magnetization. However, a correlated alignment of spins, even in the paramagnetic phase, can lift the spin degeneracy of electronic states. Here, we report an in-depth study of the electronic band structure of the Eu-ternary pnictide EuZn2Sb2 through a combination of high-resolution angle-resolved photoemission spectroscopy measurements and first principles calculations. An analysis of the photoemission lineshapes over a range of incident photon energies and sample temperatures is shown to reveal the presence of band spin degeneracy-lifting in the paramagnetic phase. Our ARPES results are in good agreement with theoretical ferromagnetic-phase calculations, which indicates the importance of ferromagnetic fluctuations in the system. Through our calculations, we predict that spin-polarized bands in EuZn2Sb2 generate a single pair of Weyl nodes. Our observation of band-splitting in EuZn2Sb2 provides a key step toward realizing time-reversal symmetry breaking physics in the absence of long-range magnetic order.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑