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arXiv 2406.18896cond-mat.supr-concond-mat.mtrl-sci
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二维超导体NbSe$_2$的电子与磁输运各向异性

Anisotropy in Electronic and Magneto-transport of 2D superconductor NbSe$_2$

N. K. Karn, M. M. Sharma, I. Felner, V. P. S. Awana

AI总结:

本文成功合成单晶二维NbSe2薄片,通过实验观测到其在7.3K下的超导转变及随磁场方向变化的电子与磁输运各向异性,并结合DFT计算揭示了其单层存在的带隙特征。

摘要:

本文报道了单晶二维NbSe$_2$薄片的成功合成。生长晶体的XRD图谱确保其结晶为单相六方结构。EDAX证实了生长样品的化学计量比。为研究振动模式,记录了拉曼光谱,其展现出预期的四个拉曼活性模式。电阻随温度的测量显示出在7.3 K下明确的超导转变(Tc)。针对面内和面外H方向,进行了ZFC(零场冷却)和FC(场冷却)磁化曲线以及等温MH(磁化强度随磁场变化)测量。在磁化和磁输运测量中均观察到随磁场方向变化的明显各向异性,导致不同的临界场(Hc)。面外磁输运数据暗示了丝状态的存在。使用密度泛函理论(DFT)研究了NbSe$_2$的能带结构。尽管体态能带结构证实了金属性,但在GGA+U框架下NbSe$_2$单层的能带结构显示出1.17eV的带隙。本文探讨了二维超导体NbSe$_2$在电子和磁输运方面的各向异性。

英文摘要:

This article reports the successful synthesis of single crystalline two-dimensional thin flakes of NbSe$_2$. The XRD pattern of the grown crystal ensured its crystallization in a single phase with a hexagonal structure. The EDAX endorsed the stoichiometry of the as grown sample. To study the vibrational modes, the Raman spectra were recorded, which exhibited the expected four Raman active modes. The resistance vs temperature measurement showed a well-established superconducting transition (Tc) at 7.3 K. The ZFC (Zero-Field Cooled) & FC (Field Cooled) magnetization curves, as well as the isothermal MH (Magnetization vs. field) measurements, have been performed for both in plane and out-of-plane H directions. Distinct anisotropy is observed in both magnetization and magneto-transport measurements with field direction, leading to different critical fields (Hc). Out-of-plane magneto-transport data hints towards the existence of a filamentary state. The density functional theory (DFT) has been used to study the band structure of NbSe$_2$. Although the bulk band structure confirmed metallic behavior, the same for mono-layers of NbSe$_2$ within the GGA+U framework showed a band gap of 1.17eV. The article addresses the anisotropy in the electronic and magneto-transport of 2D superconductor NbSe$_2$.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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