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arXiv 2406.04440cond-mat.mes-hall

范德瓦尔斯异质结中间接激子的长距离无衰减自旋输运

Long-distance decay-less spin transport in indirect excitons in a van der Waals heterostructure

Zhiwen Zhou, E. A. Szwed, D. J. Choksy, L. H. Fowler-Gerace, L. V. Butov

AI总结:

本研究以范德瓦尔斯异质结中的空间间接激子为自旋载体,观测到衰减距离超100μm的无衰减长距离自旋输运,其随密度变化的局域化-输运-再局域化行为符合Bose-Hubbard理论,为自旋电子器件提供了新平台。

摘要:

除了基础研究意义外,自旋损耗被抑制的长距离自旋输运对自旋电子器件至关重要。然而,由携带自旋的粒子散射引起的自旋弛豫限制了自旋输运。我们研究了由原子级薄的过渡金属二硫化物(TMD)层构成的范德瓦尔斯异质结(HS)中的空间间接激子(IXs,也称为层间激子),将其作为自旋载体。TMD HS还提供了自旋与能谷输运的耦合。我们观测到了长距离自旋输运,其衰减距离超过100μm且呈发散趋势,因此自旋流在该异质结中没有衰减。随着IX密度的增加,我们观测到自旋局域化、随后的长距离自旋输运以及再入型自旋局域化,这与Bose-Hubbard理论对莫尔超晶格产生的周期势中超流相和绝缘相的预测一致。激子超流中的散射抑制作用减弱了自旋弛豫,从而实现了长距离自旋输运。这种抵御自旋弛豫的机制使IXs成为实现长距离无衰减自旋输运的平台。

英文摘要:

In addition to its fundamental interest, the long-distance spin transport with suppressed spin losses is essential for spintronic devices. However, the spin relaxation caused by scattering of the particles carrying the spin, limits the spin transport. We explored spatially indirect excitons (IXs), also known as interlayer excitons, in van der Waals heterostructures (HS) composed of atomically thin layers of transition-metal dichalcogenides (TMD) as spin carries. TMD HS also offer coupling of spin and valley transport. We observed the long-distance spin transport with the decay distances exceeding 100~$μ$m and diverging so spin currents show no decay in the HS. With increasing IX density, we observed spin localization, then long-distance spin transport, and then reentrant spin localization, in agreement with the Bose-Hubbard theory prediction for superfluid and insulating phases in periodic potentials due to moiré superlattices. The suppression of scattering in exciton superfluid suppresses the spin relaxation and enables the long-distance spin transport. This mechanism of protection against the spin relaxation makes IXs a platform for the realization of long-distance decay-less spin transport.

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